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Journal articles on the topic 'Gas-phase basicity'

Author: Grafiati

Published: 4 June 2021

Last updated: 1 February 2022

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1

Desaphy, Sylvain, Christian Malosse, and Guy Bouchoux. "Gas-phase basicity of methionine." Journal of Mass Spectrometry 43, no. 1 (2007): 116–25. http://dx.doi.org/10.1002/jms.1289.

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2

Ricci, Andreina, Simona Piccolella, Federico Pepi, et al. "Gas-phase basicity of 2-furaldehyde." Journal of Mass Spectrometry 47, no. 11 (2012): 1488–94. http://dx.doi.org/10.1002/jms.3058.

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3

Marcuzzi, Franco, Giorgio Modena, and Cristina Paradisi. "Gas-phase basicity of ring-substituted phenylacetylenes." Journal of Organic Chemistry 50, no. 24 (1985): 4973–75. http://dx.doi.org/10.1021/jo00224a068.

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4

Audier, H. E., J. Fossey, J. P. Denhez, J. P. Jacquet, and P. Mourgues. "Gas phase basicity of silanaldehydes and silanones." International Journal of Mass Spectrometry 227, no. 3 (2003): 381–89. http://dx.doi.org/10.1016/s1387-3806(03)00089-7.

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5

Do, Khanh, Timothy P. Klein, Cynthia Ann Pommerening, Steven M. Bachrach, and Lee S. Sunderlin. "The Gas-Phase Basicity of Sulfuric Acid." Journal of the American Chemical Society 120, no. 24 (1998): 6093–96. http://dx.doi.org/10.1021/ja970415t.

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6

Riffet, Vanessa, Sophie Bourcier, and Guy Bouchoux. "Gas-phase basicity and acidity of tryptophan." International Journal of Mass Spectrometry 316-318 (April 2012): 47–56. http://dx.doi.org/10.1016/j.ijms.2011.12.014.

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7

Dávalos, Juan Z., Javier González, Rocío Ramos, Andrés Guerrero, and Alexsandre F. Lago. "Intrinsic (gas-phase) acidity and basicity of paracetamol." Arkivoc 2014, no. 2 (2013): 150–60. http://dx.doi.org/10.3998/ark.5550190.p008.249.

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8

Wang, Feng, Shuguang Ma, Duxi Zhang, and R. Graham Cooks. "Proton Affinity and Gas-Phase Basicity of Urea." Journal of Physical Chemistry A 102, no. 17 (1998): 2988–94. http://dx.doi.org/10.1021/jp9804493.

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9

Kaljurand, Ivari, Ilmar A. Koppel, Agnes Kütt, et al. "Experimental Gas-Phase Basicity Scale of Superbasic Phosphazenes." Journal of Physical Chemistry A 111, no. 7 (2007): 1245–50. http://dx.doi.org/10.1021/jp066182m.

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10

Decouzon, Michele, Otto Exner, Jean Francois Gal, and Pierre Charles Maria. "The gas-phase basicity of hydroxamic acid derivatives." Journal of Organic Chemistry 57, no. 5 (1992): 1621–22. http://dx.doi.org/10.1021/jo00031a059.

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11

Carlos, Luis R., Héctor Loro, Alexsandre F. Lago, and Juan Z. Dávalos. "Gas-phase proton affinity and basicity of hydroxybenzophenones." Chemical Physics Letters 713 (December 2018): 132–36. http://dx.doi.org/10.1016/j.cplett.2018.10.033.

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12

Lin, Ziqing, Lei Tan, Yang Yang, et al. "Gas-phase reactions of cyclopropenylidene with protonated alkyl amines." Analyst 141, no. 8 (2016): 2412–17. http://dx.doi.org/10.1039/c6an00235h.

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13

Mayeux, Charly, Peeter Burk, Jean-Francois Gal, et al. "Gas-Phase Lithium Cation Basicity: Revisiting the High Basicity Range by Experiment and Theory." Journal of The American Society for Mass Spectrometry 25, no. 11 (2014): 1962–73. http://dx.doi.org/10.1007/s13361-014-0970-4.

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14

Gorman, Greg S., and I. Jonathan Amster. "Gas-phase basicity measurements of dipeptides that contain valine." Journal of the American Chemical Society 115, no. 13 (1993): 5729–35. http://dx.doi.org/10.1021/ja00066a044.

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15

Borgarello, M., R. Houriet, E. D. Raczynska, and T. Drapala. "Gas-phase basicity of N1,N1-dimethyl-N2-phenylformamidines." Journal of Organic Chemistry 55, no. 1 (1990): 38–42. http://dx.doi.org/10.1021/jo00288a008.

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16

Decouzon, Mich�le, Otto Exner, Jean-fran�ois Gal, Pierre-Charles Maria, and Karel Waisser. "Acidity and basicity of thiocarboxamides in the gas phase." Journal of Physical Organic Chemistry 7, no. 9 (1994): 511–17. http://dx.doi.org/10.1002/poc.610070907.

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17

Bouchoux, Guy, and Danielle Leblanc. "Gas-Phase Basicity of Formaldehyde by the Thermokinetic Method." European Journal of Mass Spectrometry 6, no. 2 (2000): 109–12. http://dx.doi.org/10.1255/ejms.318.

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A series of proton transfer reactions monitored in a Fourier transform ion cyclotron resonance (FT-ICR) mass spectrometer allows the determination of the gas-phase basicity ( GB) and the proton affinity ( PA) of formaldehyde. The values determined by the thermokinetic method, GB(CH2O) = 681.5 ± 0.7 kJ mol−1 and PA(CH2O) = 711.5 ± 2.1 kJ mol−1 are in excellent agreement with data originating from proton transfer equilibrium constant determinations or from G2 calculations.

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18

Bouchoux, G., I. Hanna, R. Houriet, and E. Rolli. "Gas phase basicity of dihydropyran and dihydro-1,4-dioxin." Canadian Journal of Chemistry 64, no. 7 (1986): 1295–97. http://dx.doi.org/10.1139/v86-222.

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The gas phase basicity (GB) of dihydropyran 1 and dihydro-1,4-dioxin 2 is measured in equilibrium proton transfer reactions conducted in an ion cyclotron resonance spectrometer. GB(1) is found to be greater than GB(2) by 37 kJ mol−1, this difference parallels the lower reactivity of 2 observed in solution under acidic condition. Conclusion as to the favoured protonation of the C—C double bond, giving rise for both 1 and 2 to oxycarbonium cations, is drawn from comparison with analogous compounds and substantiated by molecular orbital calculations (MNDO) on the protonated structures.

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19

Liu, Chao, Yue Kang, Yuzhu Zhang, and Hongwei Xing. "Granulation Effect Analysis of Gas Quenching Blast Furnace Slag with Different Basicities." Coatings 10, no. 4 (2020): 372. http://dx.doi.org/10.3390/coatings10040372.

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High content amorphous phase blast furnace slag beads were prepared by gas quenching blast furnace slag (BFS), which could not only avoid a series of environmental problems caused by traditional water quenching methods, but also significantly increase the added value of BFS subsequent products. In this paper, the granulation mechanism of BFS and the amorphous phase formation mechanism of slag beads were studied by combining the physical properties of BFS and the granulation effect. The results showed that the viscosity of BFS decreased with the increase of basicity; the bigger the basicity, th

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20

Raczyńska, Ewa D., Jean-François Gal, Pierre-Charles Maria та Hamid Saeidian. "Push–Pull Effect on the Gas-Phase Basicity of Nitriles: Transmission of the Resonance Effects by Methylenecyclopropene and Cyclopropenimine π-Systems Substituted by Two Identically Strong Electron Donors". Symmetry 13, № 9 (2021): 1554. http://dx.doi.org/10.3390/sym13091554.

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The gas-phase basicity of nitriles can be enhanced by a push–pull effect. The role of the intercalated scaffold between the pushing group (electron-donor) and the pulling (electron-acceptor) nitrile group is crucial in the basicity enhancement, simultaneously having a transmission function and an intrinsic contribution to the basicity. In this study, we examine the methylenecyclopropene and the N-analog, cyclopropenimine, as the smallest cyclic π systems that can be considered for resonance propagation in a push–pull system, as well as their derivatives possessing two strong pushing groups (X)

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21

Bouchoux, G., F. Djazi, R. Houriet, and E. Rolli. "Gas-phase basicity of olefinic C5 and C6 carbonyl compounds." Journal of Organic Chemistry 53, no. 15 (1988): 3498–501. http://dx.doi.org/10.1021/jo00250a016.

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22

Lamsabhi, M., M. Esseffar, W. Bouab, et al. "Gas-Phase Basicity of 2,7-Dimethyl-[1,2,4]-Triazepine Thio Derivatives." Journal of Physical Chemistry A 106, no. 32 (2002): 7383–89. http://dx.doi.org/10.1021/jp0207782.

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23

Cauletti, C., G. Cerichelli, F. Grandinetti, L. Luchetti, and M. Speranza. "Gas-phase basicity and ionization energies in some N-arylazacycloalkanes." Journal of Physical Chemistry 92, no. 10 (1988): 2751–53. http://dx.doi.org/10.1021/j100321a011.

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24

You, H., G. E. Kim, C. H. Na, et al. "An empirical model for gas phase acidity and basicity estimation." SAR and QSAR in Environmental Research 25, no. 2 (2014): 91–115. http://dx.doi.org/10.1080/1062936x.2013.864997.

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25

Zhang, Kui, and Alice Chung-Phillips. "Gas-Phase Basicity of Glycine: A Comprehensive ab Initio Study." Journal of Physical Chemistry A 102, no. 20 (1998): 3625–34. http://dx.doi.org/10.1021/jp981405x.

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26

Bouchoux, G., and J. Y. Salpin. "Gas-Phase Basicity and Heat of Formation of Sulfine CH2SO." Journal of the American Chemical Society 118, no. 27 (1996): 6516–17. http://dx.doi.org/10.1021/ja9610601.

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27

Díaz, David D., M. G. Finn, and Masaaki Mishima. "Substituent Effects on the Gas-Phase Basicity of Formamidine Ureas." European Journal of Organic Chemistry 2006, no. 1 (2006): 235–40. http://dx.doi.org/10.1002/ejoc.200500516.

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28

de Petris, Giulia, Antonella Cartoni, Marzio Rosi, Vincenzo Barone, Cristina Puzzarini, and Anna Troiani. "The Proton Affinity and Gas-Phase Basicity of Sulfur Dioxide." ChemPhysChem 12, no. 1 (2010): 112–15. http://dx.doi.org/10.1002/cphc.201000920.

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29

Remko, Milan, Paul D. Lyne, and W. Graham Richards. "Molecular structure, gas-phase acidity and basicity of N-hydroxyurea." Physical Chemistry Chemical Physics 1, no. 23 (1999): 5353–57. http://dx.doi.org/10.1039/a906667e.

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30

Srivastava, Ambrish Kumar, and Neeraj Misra. "Superalkali-hydroxides as strong bases and superbases." New Journal of Chemistry 39, no. 9 (2015): 6787–90. http://dx.doi.org/10.1039/c5nj01259g.

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31

Decouzon, M., J. F. Gal, J. C. Guillemin, and P. C. Maria. "The gas-phase basicity of ethyl-, ethenyl- and ethynylphosphines and arsines." International Journal of Mass Spectrometry and Ion Processes 175, no. 1-2 (1998): 27–33. http://dx.doi.org/10.1016/s0168-1176(98)00108-6.

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32

Raczyńska, Ewa D., Jean-François Gal, and Pierre-Charles Maria. "Enhanced Basicity of Push–Pull Nitrogen Bases in the Gas Phase." Chemical Reviews 116, no. 22 (2016): 13454–511. http://dx.doi.org/10.1021/acs.chemrev.6b00224.

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33

Xu, Jiahui, Joel Mieres-Perez, Elsa Sanchez-Garcia, and Jeehiun K. Lee. "Gas-Phase Deprotonation of Benzhydryl Cations: Carbene Basicity, Multiplicity, and Rearrangements." Journal of Organic Chemistry 84, no. 12 (2019): 7685–93. http://dx.doi.org/10.1021/acs.joc.9b00496.

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34

Mishima, Masaaki, Takahiro Terasaki, Mizue Fujio, Yuho Tsuno, Yoshio Takai, and Masami Sawada. "Substituent Effect on the Gas Phase Basicity of Pyridine N-Oxide." Chemistry Letters 21, no. 6 (1992): 1081–84. http://dx.doi.org/10.1246/cl.1992.1081.

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35

Meng, Lingbiao, Zhuo Wang, Jicheng Zhang, Minjie Zhou, and Weidong Wu. "Low Energy Conformations and Gas-Phase Acidity and Basicity of Pyrrolysine." Journal of Physical Chemistry A 118, no. 34 (2014): 7085–95. http://dx.doi.org/10.1021/jp503444h.

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36

Mayhan, Collin M., Harshita Kumari, Elizabeth M. McClure, Joel F. Liebman, and Carol A. Deakyne. "Proton affinity and gas-phase basicity of hydroxyquinol: A computational study." Journal of Chemical Thermodynamics 73 (June 2014): 171–77. http://dx.doi.org/10.1016/j.jct.2013.12.015.

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37

Cacace, Fulvio, M. Elisa Crestoni, Giulia De Petris, Simonetta Fornarini, and Felice Grandinetti. "A comparative study of gas phase aromatic desilylation and detertbutylation by charged electrophiles." Canadian Journal of Chemistry 66, no. 12 (1988): 3099–107. http://dx.doi.org/10.1139/v88-478.

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Aromatic desilylation and detertbutylation by CH5+, C2H5+, i-C3H7+, and t-C4H9+ ions have been studied in the gas phase by mass spectrometric and radiolytic techniques. The higher rate of desilylation than of dealkylation is traced to the step involving the formation of ipso arenium ions, protonated at the ring carbon bearing the SiMe3 or the CMe3 substituent. The latter has been shown by ab initio calculations at the SCF STO-3G level to selectively depress the basicity of the ipso position, hence the stability of the corresponding arenium ion relative to its protomers, e.g. the basicity of th

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38

Grimm, Deborah Thomas, and John E. Bartmess. "Intrinsic (gas-phase) basicity of some anionic bases commonly used in condensed-phase synthesis." Journal of the American Chemical Society 114, no. 4 (1992): 1227–31. http://dx.doi.org/10.1021/ja00030a016.

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39

Witt, Matthias, and Hans-Friedrich Grützmacher. "Proton-bound dimers of aliphatic carboxamides: gas-phase basicity and dissociation energy." International Journal of Mass Spectrometry and Ion Processes 165-166 (November 1997): 49–62. http://dx.doi.org/10.1016/s0168-1176(97)00152-3.

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40

Fabian, Walter. "Gas Phase Basicity of Substituted Benzaldehydes and Methylbenzoates.A Semiempirical Molecular Orbital Study." Zeitschrift für Naturforschung A 43, no. 1 (1988): 85–90. http://dx.doi.org/10.1515/zna-1988-0113.

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AbstractThe semiempirical AM1 method is used to calculate relative proton affinities of a series of meta-and para-substituted benzaldehydes and methylbenzoates. Close agreement between the results of these calculations and experimental relative gas phase basicities could be obtained. The influence of a substituent on the stability of both neutral as well as protonated forms is estimated via isodesmic reactions. In any case the influence of a substituent is most pronounced in the protonated carbonyl compound. The contribution of the inductive/field effect of a substituent is approximated by the

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41

Böhm, Stanislav, Jean-François Gal, Pierre-Charles Maria, Jiří Kulhánek, and Otto Exner. "Steric Effects in Isolated Molecules: Gas-Phase Basicity of Methyl-Substituted Acetophenones." European Journal of Organic Chemistry 2005, no. 12 (2005): 2580–88. http://dx.doi.org/10.1002/ejoc.200400837.

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42

Despotović, Ines. "Basicity of Some Pyridinophanes in Gas Phase and Acetonitrile – a DFT Study." ChemistrySelect 3, no. 27 (2018): 7718–31. http://dx.doi.org/10.1002/slct.201801449.

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43

Marino, T., N. Russo, E. Tocci, and M. Toscano. "Density functional computations of proton affinity and gas-phase basicity of proline." Journal of Mass Spectrometry 36, no. 3 (2001): 301–5. http://dx.doi.org/10.1002/jms.134.

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44

Kolomeitsev, Alexander A., Ilmar A. Koppel, Toomas Rodima, et al. "Guanidinophosphazenes: Design, Synthesis, and Basicity in THF and in the Gas Phase." Journal of the American Chemical Society 127, no. 50 (2005): 17656–66. http://dx.doi.org/10.1021/ja053543n.

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45

Decouzon, Michele, Jean Francois Gal, Pierre Charles Maria, and Ewa D. Raczynska. "Gas-phase basicity of N1,N1-dimethyl-N2-alkylformamidines: substituent polarizability effects." Journal of Organic Chemistry 56, no. 11 (1991): 3669–73. http://dx.doi.org/10.1021/jo00011a041.

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46

Glasovac, Zoran, and Mirjana Eckert-Maksić. "Effect of Intramolecular Hydrogen Bonds on the Gas-Phase Basicity of Guanidines." Australian Journal of Chemistry 67, no. 7 (2014): 1056. http://dx.doi.org/10.1071/ch14182.

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Three series of novel trisubstituted guanidines containing at least one hydrogen bond accepting (HBA) group were modelled using B3LYP/6–311+G(2df,p)//B3LYP/6–31G(d) calculations. Their structure was modified by incorporating a variety of different HBA groups covering a wide range of hydrogen bond strengths. Calculated gas-phase basicities (GBs) ranged from 1035 to 1181 kJ mol–1 depending on the nature of the substituent. To rationalise changes in the GB, a correlation of GB against two independent variables (pKHB and σ4B) was conducted where pKHB served as the descriptor of the hydrogen bond s

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47

Raczyńska, Ewa D., Jean-François Gal, and Pierre-Charles Maria. "Gas-phase basicity of aromatic azines: A short review on structural effects." International Journal of Mass Spectrometry 418 (July 2017): 130–39. http://dx.doi.org/10.1016/j.ijms.2016.10.016.

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48

Koppel, Ilmar A., Frederick Anvia, and Robert W. Taft. "Rechecking of the equilibrium gas-phase basicity scale for low-basicity compounds using fourier transform ion cyclotron resonance spectrometry." Journal of Physical Organic Chemistry 7, no. 12 (1994): 717–24. http://dx.doi.org/10.1002/poc.610071210.

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49

Raczynska, Ewa D., Pierre Charles Maria, Jean Francois Gal, and Michele Decouzon. "Gas-phase basicity of N1,N1-dimethylformamidines: substituent polarizability and field effects and comparison with Broensted basicity in solution." Journal of Organic Chemistry 57, no. 21 (1992): 5730–35. http://dx.doi.org/10.1021/jo00047a029.

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50

Benoit, Robert L., Monique Fréchette, and Diane Lefebvre. "2,6-Di-tert-butylpyridine: an unusually weak base in dimethylsulfoxide." Canadian Journal of Chemistry 66, no. 5 (1988): 1159–62. http://dx.doi.org/10.1139/v88-190.

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The ionization constants of the conjugate acids BH+ of pyridine, 2-picoline, 2,6-lutidine, and 2,6-di-tert-butylpyridine (DTBP) have been determined in Me2SO. The partition coefficients of the bases B between Me2SO and water, and the enthalpies of solution and protonation of B in Me2SO have also been obtained. In contrast to its high basicity in the gas phase, DTBP is an abnormally weak base in Me2SO (pK = 0.81). The factors responsible for this very low basicity are analyzed by considering correlations between the gas-phase, Me2SO, and aqueous basicities of B and by comparing the transfer par

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