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Journal articles on the topic 'Heterometallic Coordination Architectures'

Author: Grafiati

Published: 4 June 2021

Last updated: 6 September 2023

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1

Saloutin, Viktor I., Yulia O. Edilova, Yulia S. Kudyakova, Yanina V. Burgart та Denis N. Bazhin. "Heterometallic Molecular Architectures Based on Fluorinated β-Diketone Ligands". Molecules 27, № 22 (2022): 7894. http://dx.doi.org/10.3390/molecules27227894.

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This review summarizes the data on the synthesis of coordination compounds containing two or more different metal ions based on fluorinated β-diketonates. Heterometallic systems are of high interest in terms of their potential use in catalysis, medicine and diagnostics, as well as in the development of effective sensor devices and functional materials. Having a rich history in coordination chemistry, fluorinated β-diketones are well-known ligands generating a wide variety of heterometallic complexes. In this context, we focused on both the synthetic approaches to β-dicarbonyl ligands with addi

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2

Andruh, Marius. "Binuclear complexes as tectons in designing supramolecular solid-state architectures." Pure and Applied Chemistry 77, no. 10 (2005): 1685–706. http://dx.doi.org/10.1351/pac200577101685.

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Oligonuclear complexes as well as coordination polymers with various network topologies can be obtained by using homo- or heterobinuclear complexes as starting materials. These building blocks are stable complexes, where the metal ions are held together by compartmental ligands, or alkoxo-bridged Cu(II) species. The binuclear nodes can be connected through appropriate exo-dentate ligands, or through metal-containing anions (e.g., [M(CN)6]3-, M = CrIII, FeIII, CoIII). A rich variety of 3d-3d and 3d-4f heterometallic complexes, with interesting architectures and topologies of the spin carriers,

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3

Zigon, Nicolas, Nathalie Kyritsakas, and Mir Wais Hosseini. "Molecular tectonics: heterometallic coordination networks based on a Pt(ii) organometallic metallatecton." Dalton Transactions 44, no. 32 (2015): 14204–7. http://dx.doi.org/10.1039/c5dt02404h.

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4

Kang, Yi-Fan, Ping Liu, Chao Yuan, Lin Cui, Yang Liu, and Yao-Yu Wang. "An intriguing 4d–4f heterometallic coordination polymer with 1D pseudo-nanotube architectures." Inorganic Chemistry Communications 36 (October 2013): 4–7. http://dx.doi.org/10.1016/j.inoche.2013.07.006.

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5

Han, Lizhi, Longyi Jin, Enbo Wang, and Zhongmin Su. "Synthesis and characterization of two isostructural 3d–4f coordination compounds based on pyridine-2,6-dicarboxylic acid and 4,4′-bipyridine." Acta Crystallographica Section C Structural Chemistry 75, no. 6 (2019): 723–27. http://dx.doi.org/10.1107/s2053229619006004.

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The design and synthesis of 3d–4f heterometallic coordination polymers have attracted much interest due to the intriguing diversity of their architectures and topologies. Pyridine-2,6-dicarboxylic acid (H2pydc) has a versatile coordination mode and has been used to construct multinuclear and heterometallic compounds. Two isostructural centrosymmetric 3d–4f coordination compounds constructed from pyridine-2,6-dicarboxylic acid and 4,4′-bipyridine (bpy), namely 4,4′-bipyridine-1,1′-diium diaquabis(μ2-pyridine-2,6-dicarboxylato)tetrakis(pyridine-2,6-dicarboxylato)bis[4-(pyridin-4-yl)pyridinium]co

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6

Xu, Bo, Senwen Yuan, Xiutao Zhang, and Cuncheng Li. "A Yb(III)–Zn(II) heterometallic coordination polymer with interesting three-fold 1D pseudo-nanotube architectures." Journal of Molecular Structure 1068 (June 2014): 53–57. http://dx.doi.org/10.1016/j.molstruc.2014.03.058.

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7

Zhao, Jiong-Peng, Bo-Wen Hu, Xiao-Feng Zhang, et al. "One Pot Synthesis of Heterometallic 3d−3d Azide Coordination Architectures: Effect of the Single-Ion Anisotropy." Inorganic Chemistry 49, no. 24 (2010): 11325–32. http://dx.doi.org/10.1021/ic101089n.

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8

Moutier, F., A. M. Khalil, S. A. Baudron, and C. Lescop. "Gleaned snapshots on the road to coordination polymers: heterometallic architectures based on Cu(i) metallaclips and 2,2′-bis-dipyrrin metalloligands." Chemical Communications 56, no. 72 (2020): 10501–4. http://dx.doi.org/10.1039/d0cc04862c.

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The assembly of binuclear Cu(i) metallaclips with 2,2′-bis-dipyrrin based metalloligands affords recurrent π-stacked compact tetranuclear metallacycles organizing into discrete or infinite architectures.

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9

Santanni, Fabio, Laura Chelazzi, Lorenzo Sorace, Grigore A. Timco, and Roberta Sessoli. "Structural and Magnetic Properties of the {Cr(pybd)3[Cu(cyclen)]2}(BF4)4 Heteronuclear Complex." Crystals 13, no. 6 (2023): 901. http://dx.doi.org/10.3390/cryst13060901.

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Heterotopic ligands containing chemically different binding centers are appealing candidates for obtaining heteronuclear metal complexes. By exploiting this strategy, it is possible to introduce different paramagnetic centers characterized by specific anisotropic magnetic properties that make them distinguishable when weakly magnetically coupled. This molecular approach has great potential to yield multi-spin adducts capable of mimicking logical architectures necessary for quantum information processing (QIP), i.e., quantum logic gates. A possible route for including a single-ion magnetic cent

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10

Artizzu, Flavia, Luca Pilia, Angela Serpe, et al. "Anion-Induced Structural Diversity and Optical Chromism in a Series of Cyano-Bridged Heterometallic 3d-4f Coordination Polymers." Molecules 28, no. 6 (2023): 2871. http://dx.doi.org/10.3390/molecules28062871.

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The self-assembly reaction of the neutral dicyano-bis(1,10-phenanthroline) iron(II) complex with lanthanide ions (Ln = Eu(III), Gd(III), Er(III)) provided two different classes of heterometallic cyano-bridged 3d-4f architectures depending on the nature of the counteranion, irrespective of the size of the 4f metal ion. Tetranuclear oligomers with a squared Fe2Ln2 core were isolated when using nitrate salts, whereas unusual 1D polymeric chains were obtained when resorting to triflate salts under the same synthetic conditions. It is shown that the different structural motifs have a remarkable imp

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11

Vega, Andres, Bianca Baldo, Veronica Paredes-García, Evgenia Spodine, and Diego Venegas-Yazigi. "General Synthetic Route and Structural Characterization of New 3d-4f Materials." Acta Crystallographica Section A Foundations and Advances 70, a1 (2014): C1775. http://dx.doi.org/10.1107/s2053273314082242.

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Within the field of coordination chemistry, the crystal engineering has been applied mainly through the design and synthesis of Metal-Organic Materials (MOMs), which are attractive not only by the wide variety of architectures and topologies that they present, but also by the potential applications in catalysis, ion exchange, molecular adsorption, fluorescence, nonlinear optics, and magnetism. From a structural and synthetic point of view, the literature shows that a wide variety of MOMs ranging from 0D to 3D structures have been rationally designed and synthesized by the appropriate selection

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12

Chowdhury, Habibar, and Chandan Adhikary. "Copper(II)-Nickel(II) Induced Cyanide Bridged 2D Heterometallic Coordination Polymer: Synthesis, X-ray Structure and Magnetic Study." Asian Journal of Chemistry 34, no. 6 (2022): 1472–76. http://dx.doi.org/10.14233/ajchem.2022.23678.

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One new two-dimensional heterometallic coordination polymer [Cu3Ni(L)2(CN)6]n (1) [L = 2-methylethylenediamine, CN– = cyanide ion] was synthesized and characterized by X-ray crystallography. Compound 1 crystallizes in the monoclinic C2/c space group. The single crystal X-ray structure of compound 1 indicated that it is a 2D coordination polymer with three copper(II) ion embedded with [Ni(CN)4]2- molecular ion in architecture through μ-CN/μ-NC bridges results heterometallic polymer. In compound 1, each Cu1 center with a CuN5 chromophore is encompassed by four N atoms of the two different bident

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13

Guo, Pei-Ying, De-Yun Ma, and Hai-Fu Guo. "A twofold interpenetrating three-dimensional heterometallic metal–organic framework with pcu topology based on 2-methylbiphenyl-4,4′-dicarboxylic acid." Acta Crystallographica Section C Structural Chemistry 73, no. 6 (2017): 470–75. http://dx.doi.org/10.1107/s2053229617006829.

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The 2-methylbiphenyl-4,4′-dicarboxylate (mbpdc2−) ligand has versatile coordination modes and can be used to construct multinuclear structures. Despite this, reports of the synthesis of coordination complexes involving this ligand are scarce. The title compound, poly[[triaquadi-μ3-hydroxido-hexakis(μ4-2-methylbiphenyl-4,4′-dicarboxylato)calcium(II)hexazinc(II)] monohydrate], {[CaZn6(C15H10O4)6(OH)2(H2O)3]·H2O} n , has been prepared by the hydrothermal assembly of Zn(NO3)2·6H2O, CaCl2 and 2-methylbiphenyl-4,4′-dicarboxylic acid. Two ZnII atoms adopt a four-coordinated distorted tetrahedral geom

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14

Wytrych, Patrycja, Józef Utko, Tadeusz Lis, and Łukasz John. "Polyoxometalate-like structure of new potassium triphenylsiloxides: [K6(OSiPh3)6(C3H7OH)(H2O)]·2C6H5CH3 and [K6(OSiPh3)6(H2O)2]." Acta Crystallographica Section C Structural Chemistry 77, no. 9 (2021): 522–28. http://dx.doi.org/10.1107/s2053229621008160.

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The synthesis and structural characterization of two new potassium triphenylsiloxides, namely, aqua(propan-2-ol)hexakis(triphenylsilanolato)hexapotassium toluene disolvate, [K6(C18H15OSi)6(C3H8O)(H2O)]·2C7H8, and diaquahexakis(triphenylsilanolato)hexapotassium, [K6(C18H15OSi)6(H2O)2], are reported. Both compounds crystallize in the triclinic space group P-1. The structure in each case resembles an alkali metal polyoxometalate-like structure, in which electrostatic interactions are observed in the metal–oxygen core. Furthermore, both compounds also resemble a reverse micelles-like architecture,

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15

Ghosh, Soumavo, Sanjib Giri, and Ashutosh Ghosh. "An adaptable heterometallic trinuclear coordination cluster in the synthesis of tailored one-dimensional architecture: Structural characterization, magnetic analysis and theoretical calculations." Polyhedron 102 (December 2015): 366–74. http://dx.doi.org/10.1016/j.poly.2015.10.014.

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16

Kalinowska, Monika, Ewelina Gołębiewska, Liliana Mazur, et al. "Crystal Structure, Spectroscopic Characterization, Antioxidant and Cytotoxic Activity of New Mg(II) and Mn(II)/Na(I) Complexes of Isoferulic Acid." Materials 14, no. 12 (2021): 3236. http://dx.doi.org/10.3390/ma14123236.

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The Mg(II) and heterometallic Mn(II)/Na(I) complexes of isoferulic acid (3-hydroxy-4-methoxycinnamic acid, IFA) were synthesized and characterized by infrared spectroscopy FT-IR, FT-Raman, electronic absorption spectroscopy UV/VIS, and single-crystal X-ray diffraction. The reaction of MgCl2 with isoferulic acid in the aqueous solutions of NaOH resulted in synthesis of the complex salt of the general formula of [Mg(H2O)6]⋅(C10H9O4)2⋅6H2O. The crystal structure of this compound consists of discrete octahedral [Mg(H2O)6]2+ cations, isoferulic acid anions and solvent water molecules. The hydrated

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17

Song, Xue-Qin, Xue-Li Xia, Fu-Qiang Song, Guo-Hua Liu, and Li Wang. "Tuning the coordination behavior of an unexplored asymmetric multidentate ligand for developing diverse heterometallic architectures with luminescent and magnetic properties." CrystEngComm, 2021. http://dx.doi.org/10.1039/d0ce01298j.

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18

Viau, Lydie, Michael Knorr, Lena Knauer, Lukas Brieger, and Carsten Strohman. "2,2’-Ethylenebis(1,3-dithiane) as polydentate m2-, m4- and m5-assembling ligand for the construction of sulphur-rich Cu(I), Hg(II) and heterometallic Cu(I)/Hg(II) coordination polymers featuring uncommon network architectures." Dalton Transactions, 2022. http://dx.doi.org/10.1039/d2dt00800a.

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With the aim to elaborate novel and inexpensive sulphur-rich materials featuring unusual network architectures, the coordination chemistry of the tetradentate thiaheterocycle 1,2-di(1,3-dithian-2-yl)ethane L1 ligand toward CuX and HgX2 salts was...

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