Thematische Bibliographien / Nucleophilic reactions. Organic compounds

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Auswahl der wissenschaftlichen Literatur zum Thema „Nucleophilic reactions. Organic compounds“

Autor: Grafiati

Veröffentlicht am 4. Juni 2021

Zuletzt aktualisiert am 13. Februar 2022

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Zeitschriftenartikel zum Thema "Nucleophilic reactions. Organic compounds"

Vilotijevic, Ivan, Markus Lange, and You Zi. "Latent (Pro)Nucleophiles in Enantioselective Lewis Base Catalyzed Allylic Substitutions." Synlett 31, no. 13 (2020): 1237–43. http://dx.doi.org/10.1055/s-0040-1707130.

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The use of latent nucleophiles, which are molecules that are not nucleophilic but can be activated to act as a nucleophile at an opportune time during the reaction, expands the scope of Lewis base catalyzed reactions. Here, we provide an overview of the concept and show examples of applications to N- and C-centered nucleophiles in allylic substitutions. N- and C-silyl compounds are superior latent (pro)nucleophiles in Lewis base catalyzed reactions with allylic fluorides in which the formation of the strong Si–F bond serves as the driving force for the reactions. The latent (pro)nucleophiles e

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Tong, Shuo, and Mei-Xiang Wang. "Domino Reactions of Tertiary Enamides in Organic Synthesis." Synlett 32, no. 14 (2021): 1419–27. http://dx.doi.org/10.1055/a-1352-6358.

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AbstractStudies in recent decade have shown that tertiary enamides, once thought of as unreactive and marginally useful enamine variants, are shelf-stable yet versatile nucleophilic intermediates in organic synthesis. Many compounds, especially N-heterocycles, have been synthesized by monofunctionalization reactions of tertiary enamides. By taking advantage of intramolecular and intermolecular interception of the putative acyliminium intermediates formed by the initial nucleophilic reactions of tertiary enamides, we have established several novel difunctionalization reaction methods for constr

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Christoffers, Jens, and David Kieslich. "Cyanide Anions as Nucleophilic Catalysts in Organic Synthesis." Synthesis 53, no. 19 (2021): 3485–96. http://dx.doi.org/10.1055/a-1499-8943.

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AbstractThe nucleophilic addition of a cyanide anion to a carbonyl group is the basis for several cyanide-catalyzed organic reactions, which are summarized in this review. Since cyanide is also a good leaving group, it is an excellent catalyst for transacylation reactions. As an electron-withdrawing group, it also stabilizes a negative charge in its α-position, thus allowing the umpolung of aldehydes to formyl anion equivalents. The two leading examples are the benzoin condensation and the Michael–Stetter reaction furnishing α-hydroxy ketones and 1,4-dicarbonyl compounds, which are both cataly

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Dolliver, Debra D., David B. Delatte, Derek B. Linder, James E. Johnson, Diana C. Canesco, and Jeffrey E. Rowe. "Nucleophilic substitution reactions of N-alkoxyimidoyl fluorides by carbon nucleophiles." Canadian Journal of Chemistry 85, no. 11 (2007): 913–22. http://dx.doi.org/10.1139/v07-097.

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Nucleophilic substitutions of N-alkoxybenzoimidoyl fluorides [p-ClArC(F)=NOR; R = CH3, i-Pr] by enolate-type ions have been performed to produce compounds that can exist in two tautomeric forms: the imine form{p-ClArC(Y)=NOR [Y = CH(CN)2, CH(CN)(CO2Et), CH(CO2Et)2]}or the enamine form {p-ClArC(NHOR)=C(R1)(R2) [R1, R2 = CN, CO2Et]}. These compounds display varying ratios of imine–enamine tautomerizm in chloroform: the diester compound exists almost solely in the imine form, the dicyano compound exists solely in the enamine form, and the cyano-ester compound exists in both tautomeric forms. Comp

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Birdsall, A. W., C. R. Miner, L. E. Mael, and M. J. Elrod. "Mechanistic study of secondary organic aerosol components formed from nucleophilic addition reactions of methacrylic acid epoxide." Atmospheric Chemistry and Physics Discussions 14, no. 14 (2014): 19917–54. http://dx.doi.org/10.5194/acpd-14-19917-2014.

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Abstract. Recently, methacrylic acid epoxide (MAE) has been proposed as a precursor to an important class of isoprene-derived compounds found in secondary organic aerosol (SOA): 2-methylglyceric acid (2-MG) and a set of oligomers, nitric acid esters and sulfuric acid esters related to 2-MG. However, the specific chemical mechanisms by which MAE could form these compounds have not been previously studied. In order to determine the relevance of these processes to atmospheric aerosol, MAE and 2-MG have been synthesized and a series of bulk solution-phase experiments aimed at studying the reactivi

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Birdsall, A. W., C. R. Miner, L. E. Mael, and M. J. Elrod. "Mechanistic study of secondary organic aerosol components formed from nucleophilic addition reactions of methacrylic acid epoxide." Atmospheric Chemistry and Physics 14, no. 23 (2014): 12951–64. http://dx.doi.org/10.5194/acp-14-12951-2014.

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Abstract. Recently, methacrylic acid epoxide (MAE) has been proposed as a precursor to an important class of isoprene-derived compounds found in secondary organic aerosol (SOA): 2-methylglyceric acid (2-MG) and a set of oligomers, nitric acid esters, and sulfuric acid esters related to 2-MG. However, the specific chemical mechanisms by which MAE could form these compounds have not been previously studied with experimental methods. In order to determine the relevance of these processes to atmospheric aerosol, MAE and 2-MG have been synthesized and a series of bulk solution-phase experiments aim

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Shcherbakov, Konstantin V., Yanina V. Burgart, Victor I. Saloutin, and Oleg N. Chupakhin. "Modification of Polyfluoro-Containing 3-(Ethoxycarbonyl)flavones by Biogenic Amines and Amino Acids." Current Organic Synthesis 15, no. 5 (2018): 707–14. http://dx.doi.org/10.2174/1570179415666180405120706.

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Aim and Objective: The objective of our work was to study the peculiarities of transformations of fluorine-containing flavone-3-carboxylates with N-nucleophiles, including biogenic amines and amino acids. Materials and Methods: 6,7,8-Trifluoro and 5,6,7,8-tetrafluoroflavone-3-carboxylates were involved in interactions with a number of N-nucleophiles, such as pyrrolidine, morpholine, proline, arginine, gammaaminobutyric acid, beta-alanine, histamine, dopamine and amantadine under different reaction conditions. All synthesized compounds were characterized by NMR 1H, 19F, (NMR 13C for some compou

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Jin, Fengyan, Tao Yang, Xian-Rong Song, et al. "TMSBr-Promoted Cascade Cyclization of ortho-Propynol Phenyl Azides for the Synthesis of 4-Bromo Quinolines and Its Applications." Molecules 24, no. 21 (2019): 3999. http://dx.doi.org/10.3390/molecules24213999.

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Difficult-to-access 4-bromo quinolines are constructed directly from easily prepared ortho-propynol phenyl azides using TMSBr as acid-promoter. The cascade transformation performs smoothly to generate desired products in moderate to excellent yields with good functional groups compatibility. Notably, TMSBr not only acted as an acid-promoter to initiate the reaction, and also as a nucleophile. In addition, 4-bromo quinolines as key intermediates could further undergo the coupling reactions or nucleophilic reactions to provide a variety of functionalized compounds with molecular diversity at C4

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Singh, Rajendra P., and Jean'ne M. Shreeve. "Nucleophilic Trifluoromethylation Reactions of Organic Compounds with (Trifluoromethyl)trimethylsilane." Tetrahedron 56, no. 39 (2000): 7613–32. http://dx.doi.org/10.1016/s0040-4020(00)00550-0.

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Zaki, Remon M., Adel M. Kamal El-Dean, Shaban M. Radwan, and Ahmed F. Saber. "Efficient synthesis, reactions and spectral characterization of pyrazolo[4’,3’:4,5]thieno[3,2-d] pyrimidines and related heterocycles." Heterocyclic Communications 25, no. 1 (2019): 39–46. http://dx.doi.org/10.1515/hc-2019-0004.

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AbstractNew pyrazolothienopyrimidines were synthesized. The key intermediate 4-aminothieno[2,3-c]pyrazole-5-carbonitrile 1 was converted to the chloroacetyl amino derivative 2 followed by nucleophilic substitution and Dimorth rearrangement upon treatment with nitrogen nucleophiles to give the pyrimidinones 3a-c. Treatment of 3a with formaldehyde and with triethyl orthoformate afforded the respective tetracyclic derivatives 4 and 5. Condensation of the amino group in the o-aminocarbonitrile 1 with triethyl orthoformate followed by cycloaddition reaction with hydrazine led to the formation of py

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Dissertationen zum Thema "Nucleophilic reactions. Organic compounds"

Diep, Nhut Kiet. "Studies of nucleophile ring opening of oxabicyclic systems in highly polar media application to a total synthesis of antitumor agent, (-)-epothilone B /." Diss., Montana State University, 2006. http://etd.lib.montana.edu/etd/2006/diep/DiepN0806.pdf.

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Polyketides constitute an important family of natural products, having a broad spectrum of biological activity such as antitumor, antibiotic, antifungal, or immunomodulatory action.Â¹ Many of these compounds possess polypropionates (units with alternating hydroxyl and methyl groups), reflecting their common biosynthesis that is found within nature. Their structural complexity and importance of these compounds as therapeutical agents have made them attractive targets for synthetic organic chemists.Â¹ Excellent chiral propionate reagents have been developed over the years,

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Dehestani, Ahmad. "Exploring reactivities of oxo and nitrido ligands on high valent osmium with electrophiles, nucleophiles, alkenes, hydrogen, and methane. /." Thesis, Connect to this title online; UW restricted, 2004. http://hdl.handle.net/1773/8626.

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Cheong, Yuen-Ki. "Studies of the reactions of nucleophilic organophosphorus species with organic cabonyl-coataining compounds." Thesis, Queen Mary, University of London, 2007. http://ethos.bl.uk/OrderDetails.do?uin=uk.bl.ethos.582586.

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The majority of this project is to discover novel mechanistic pathways for a wide range of organic reactions involving different carbonyl compounds with trivalent phosphorus compounds. The first part of our research involved the one-pot intra-molecular cyclisation reaction of the different 2-substituted benzoylphosphonates in the presence of triniethyl phosphite. The mechanistic pathway of these reactions was found to intra-molecular insert to the electrophilic carbonyl centre in the substituent via the initially formed carbanionic intermediate. The subsequently formed tricyclic phospholane in

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Moagi, Kgotso Herbet. "Reaction Mechanism of 2-monosubstituted Quinoxalines with Organolithium Compounds : a Theoretical Study." Diss., University of Pretoria, 2020. http://hdl.handle.net/2263/75182.

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This dissertation describes the density functional theory (DFT) computational modelling of reactions between organolithium nucleophiles and various substituted quinoxalines. These reactions result in the functionalisation of the C (sp2)–H bond, thus substituting the sigma-hydrogen. The reactions are known as nucleophilic substitution of hydrogen (SNH) and are used by experimental chemists to form new C–C bonds. The SNH reactions are very important in various industries, e.g. in designing and manufacturing of pharmaceuticals. Quinoxaline is widely used in medicinal chemistry due to its various

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HADDAD-FAHED, OMAIMA. "Catalyse micellaire de reactions de substitution nucleophile aromatique comportant des reactifs electriquement charges." Paris 6, 1987. http://www.theses.fr/1987PA066419.

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Fejfar, José Luiz. "Resolução cinética em reações de substituição nucleofílica mediadas por catalisadores por transferência de fase derivados da efedrina, cinchonidina e quinina." Universidade de São Paulo, 2001. http://www.teses.usp.br/teses/disponiveis/46/46135/tde-29112018-120557/.

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Neste trabalho foram estudadas reações de substituição nucleofílica alifática de seis substratos halogenados, na presença de sais quaternários de amônio quirais (catalisadores por transferência de fase), derivados de alcalóides naturais. O sistema usado durante os trabalhos foi o sólido-líquido, sendo utilizado o tolueno como solvente do substrato halogenado. Os eletrófilos escolhidos para este trabalho foram, em sua grande maioria, compostos halogenados na posição alfa à carbonila e o nucleófilo foi o fenilmercapteto de sódio. A estrutura do substratos, as condições de reação e o tipo de cata

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Martin, Peter Arnold. "Nucleophilic substitution reactions of some polyhalogenated compounds." Thesis, Durham University, 1987. http://etheses.dur.ac.uk/6876/.

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Rate measurements for the reactions of a series of polyfluoro - and polychloro - pyridines with aniline and ammonia in 60/40 dioxan/water at 25ºC has shown that chlorine, when ortho and para to the position of attack, is activating with respect to fluorine, but at the position meta to the point of attack, chlorine and fluorine are virtually equivalent in their effect on reaction rate. The trifluoromethyl and nitrile groups were found to be activating relative to fluorine when ortho and para to the position of substitution and the nitrile group was thus found to be ortho/para directing. The ort

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Kim, Jong Chul. "Nucleophilic Addition Reactions to Carbonyl Compounds under High Pressure Environment." Kyoto University, 2003. http://hdl.handle.net/2433/148945.

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Kyoto University (京都大学) 0048 新制・課程博士 博士(人間・環境学) 甲第10308号 人博第195号 14||159(吉田南総合図書館) 新制||人||48(附属図書館) UT51-2003-H729 京都大学大学院人間・環境学研究科人間・環境学専攻 (主査)教授松本澄, 教授山内淳, 教授山口良平 学位規則第4条第1項該当

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Drew, S. M. "Photochemical nucleophilic substitution reactions of quinones and related systems." Thesis, University of Leeds, 1986. http://ethos.bl.uk/OrderDetails.do?uin=uk.bl.ethos.374182.

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Stevens, James Andrew. "Structure-reactivity patterns in nucleophilic addition to activated aromatic compounds." Thesis, Durham University, 1990. http://etheses.dur.ac.uk/6217/.

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Kinetic and equilibrium data for the reactions of some aromatic nitro compounds with nucleophiles have been investigated using various spectrophotometric techniques (UV/visible, stopped-flow and temperature jump) and nmr spectroscopy. Kinetic and equilibrium data are reported for the formation of 1:1 and 1:2 adducts in aqueous solutions from 1,3,5-trinitrobenzene (TNB) and 2,4,6-trinitro- toluene (TNT) with thiolate ions derived from thioglycolic acid, thiomalic acid and glutathione. The results are used to determine intrinsic reactivities, kg, for the thiolate ions in adduct-forming reactions

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Bücher zum Thema "Nucleophilic reactions. Organic compounds"

Perlmutter, P. Conjugate addition reactions in organic synthesis. Pergamon, 1992.

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N, Charushin Valery, and Plas, H. C. van der., eds. Nucleophilic aromatic substitution of hydrogen. Academic Press, 1994.

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G, Morrell Dennis, Organic Reactions Catalysis Society, and North American Catalysis Society, eds. Catalysis of organic reactions. Marcel Dekker, 2003.

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R, Sowa John, ed. Catalysis of organic reactions. Taylor & Francis, 2005.

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Hassner, Alfred. Organic syntheses based on name reactions and unnamed reactions. Pergamon, 1994.

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Conference on the Catalysis of Organic Reactions (22nd 2008 Richmond, Virginia). Catalysis of organic reactions. Edited by Prunier Michael L. Taylor & Francis, 2008.

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Voronkov, M. G., N. S. Vyazankin, E. N. Deryagina, A. S. Nakhmanovich, and V. A. Usov. Reactions of Sulfur with Organic Compounds. Edited by J. S. Pizey. Springer US, 1987. http://dx.doi.org/10.1007/978-1-4684-0679-5.

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Radical reactions in organic synthesis. Oxford University Press, 2003.

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C, Stumer, and Hassner Alfred 1930-, eds. Organic syntheses based on name reactions. 2nd ed. Pergamon, 2002.

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Mieczkowski, Józef Bogusław. Zastosowanie reakcji substytucji nukleofilowej do pełnych syntez wybranych alkaloidów i nowych układów heterocyklicznych. Wydawnictwa Uniwersytetu Warszawskiego, 1990.

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Buchteile zum Thema "Nucleophilic reactions. Organic compounds"

Went, Charles. "Nucleophilic Reactions of Carbonyl Compounds." In Ionic Organic Mechanisms. Macmillan Education UK, 1986. http://dx.doi.org/10.1007/978-1-349-07964-3_7.

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Ollevier, Thierry. "Bismuth-Catalyzed Addition of Silyl Nucleophiles to Carbonyl Compounds and Imines." In Bismuth-Mediated Organic Reactions. Springer Berlin Heidelberg, 2011. http://dx.doi.org/10.1007/128_2011_298.

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Ross, Sidney D. "Nucleophilic Aromatic Substitution Reactions." In Progress in Physical Organic Chemistry. John Wiley & Sons, Inc., 2007. http://dx.doi.org/10.1002/9780470171806.ch2.

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Went, Charles. "Nucleophilic Reactions of Carboxylic Acids and their Derivatives." In Ionic Organic Mechanisms. Macmillan Education UK, 1986. http://dx.doi.org/10.1007/978-1-349-07964-3_8.

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Carey, Francis A., and Richard J. Sundberg. "Reactions of Carbonyl Compounds." In Advanced Organic Chemistry. Springer US, 1990. http://dx.doi.org/10.1007/978-1-4613-9795-3_8.

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Best, Erich, Peter Kuhn, Wolfgang Kurtz, and Hildegard List. "Reactions with Organic Compounds." In W Tungsten. Springer Berlin Heidelberg, 1986. http://dx.doi.org/10.1007/978-3-662-08687-2_5.

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Hiyama, Tamejiro, and Hisashi Yamamoto. "Organic Reactions with Fluorinated Reagents." In Organofluorine Compounds. Springer Berlin Heidelberg, 2000. http://dx.doi.org/10.1007/978-3-662-04164-2_8.

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Shreeve, Jean'ne M. "Trifluoromethyl Compounds via Electrophilic and Nucleophilic Reactions." In Efficient Preparations of Fluorine Compounds. John Wiley & Sons, Inc., 2012. http://dx.doi.org/10.1002/9781118409466.ch21.

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Voronkov, M. G., N. S. Vyazankin, E. N. Deryagina, A. S. Nakhmanovich, and V. A. Usov. "Organic Sulfur Compounds." In Reactions of Sulfur with Organic Compounds. Springer US, 1987. http://dx.doi.org/10.1007/978-1-4684-0679-5_5.

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Minkin, Vladimir I., Boris Ya Simkin, and Ruslan M. Minyaev. "Pericyclic Reactions." In Quantum Chemistry of Organic Compounds. Springer Berlin Heidelberg, 1990. http://dx.doi.org/10.1007/978-3-642-75679-5_10.

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Konferenzberichte zum Thema "Nucleophilic reactions. Organic compounds"

Amaral, André Felipe C., Wender A. Silva, and Carlos Kleber Z. Andrade. "Microwave-assisted synthesis of fused tetrazoleketopiperazine compounds via Ugi reactions." In 15th Brazilian Meeting on Organic Synthesis. Editora Edgard Blücher, 2013. http://dx.doi.org/10.5151/chempro-15bmos-bmos2013_2013916112849.

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Ścianowski, Jacek, Anna Banach, and Agata Pacuła. "Synthesis and Reactions of New Tellurium-substituted Terpenyl Compounds." In The 17th International Electronic Conference on Synthetic Organic Chemistry. MDPI, 2013. http://dx.doi.org/10.3390/ecsoc-17-a001.

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Trzoss, Michael, and Stefan Bienz. "A Chiral Silyl Ether as Auxiliary for the Asymmetric Nucleophilic Addition to a- and b-Silyloxy Carbonyl Compounds." In The 4th International Electronic Conference on Synthetic Organic Chemistry. MDPI, 2000. http://dx.doi.org/10.3390/ecsoc-4-01865.

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Plehovich, Sergey, Sergey Zelentsov, and Alexandre Plehovich. "Quantum-chemical Study of Mechanism of the Photochemical Reactions of Nitro Compounds with Sulfur - and Nitroso Containing Compounds." In The 16th International Electronic Conference on Synthetic Organic Chemistry. MDPI, 2012. http://dx.doi.org/10.3390/ecsoc-16-01048.

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Pilewski, John D., Shikha Sharma, and Vikas Agrawal. "ANALYSIS OF ORGANIC COMPOUNDS PRODUCED FROM HIGH TEMPERATURE AND PRESSURE FLUID-ROCK REACTIONS." In GSA Annual Meeting in Seattle, Washington, USA - 2017. Geological Society of America, 2017. http://dx.doi.org/10.1130/abs/2017am-306871.

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Gushchin, Alexey, Dmitry Moiseev, Vera Morugova, Julia Malysheva, and Victor Dodonov. "Use of Arylantimony(III,V), Bismuth(III) Compounds and Peroxides in Cross-Coupling Reactions with Alkenes." In The 8th International Electronic Conference on Synthetic Organic Chemistry. MDPI, 2004. http://dx.doi.org/10.3390/ecsoc-8-01964.

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Vinogradov, Andrey, and Vyacheslav Platonov. "Reactions of polyfluoroarylzinc compounds with Vilsmeier-Haack reagent; new synthesis of polyfluorinated aromatic aldehydes and acetales." In The 15th International Electronic Conference on Synthetic Organic Chemistry. MDPI, 2011. http://dx.doi.org/10.3390/ecsoc-15-00607.

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Plehovitch, Sergey, Sergei Zelentsov, Dmitry Fomichev, Sergey Zelentsov, and Dmitry Ovsyannikov. "Quantum-chemical calculations of the possible formation of nitroso oxides in the course of the photooxidation reactions by nitro compounds." In The 17th International Electronic Conference on Synthetic Organic Chemistry. MDPI, 2013. http://dx.doi.org/10.3390/ecsoc-17-e004.

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Chong, Hwansoo, Seung Yeon Yang, and Kyeong Ook Lee. "Accurate Measurements of Heat Release, Oxidation Rates, and Soluble Organic Compounds of Diesel Particulates through Thermal Reactions." In SAE 2010 World Congress & Exhibition. SAE International, 2010. http://dx.doi.org/10.4271/2010-01-0814.

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Beyke, Gregory, and Gregory J. Smith. "Advances in the Application of In Situ Electrical Resistance Heating." In The 11th International Conference on Environmental Remediation and Radioactive Waste Management. ASMEDC, 2007. http://dx.doi.org/10.1115/icem2007-7136.

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Electrical Resistance Heating (ERH) is an aggressive in situ thermal remediation technology that was developed by the U.S. Department of Energy from the original oil production technology to enhance vapor extraction remediation technologies in low permeability soils. Soil and groundwater are heated by the passage of electrical current through saturated and unsaturated soil between electrodes, not by the electrodes themselves. It is the resistance to the flow of electrical current that results in increased subsurface temperatures, and this is typically applied to the boiling point of water. It

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Berichte der Organisationen zum Thema "Nucleophilic reactions. Organic compounds"

Midey, Anthony. Ion-Molecular Reactions With Organic and Atmospheric Compounds from 150-1400K. Defense Technical Information Center, 2000. http://dx.doi.org/10.21236/ada405891.

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Suria, Sabartanty. Intermolecula transfer and elimination of molecular hydrogen in thermal reactions of unsaturated organic compounds. Office of Scientific and Technical Information (OSTI), 1995. http://dx.doi.org/10.2172/108159.

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Lunsford, J. H. The Adsorption and Reactions of Halogenated Volatile Organic Compounds (VOCs) on Metal Oxides - Final Report. Office of Scientific and Technical Information (OSTI), 2000. http://dx.doi.org/10.2172/775042.

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