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1
Olofsson, Karl-Johan. „Black-box optimization of simulated light extraction efficiency from quantum dots in pyramidal gallium nitride structures“. Thesis, Linköpings universitet, Matematiska institutionen, 2019. http://urn.kb.se/resolve?urn=urn:nbn:se:liu:diva-162235.
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Microsized hexagonal gallium nitride pyramids show promise as next generation Light Emitting Diodes (LEDs) due to certain quantum properties within the pyramids. One metric for evaluating the efficiency of a LED device is by studying its Light Extraction Efficiency (LEE). To calculate the LEE for different pyramid designs, simulations can be performed using the FDTD method. Maximizing the LEE is treated as a black-box optimization problem with an interpolation method that utilizes radial basis functions. A simple heuristic is implemented and tested for various pyramid parameters. The LEE is shown to be highly dependent on the pyramid size, the source position and the polarization. Under certain circumstances, a LEE over 17% is found above the pyramid. The results are however in some situations very sensitive to the simulation parameters, leading to results not converging properly. Establishing convergence for all simulation evaluations must be done with further care. The results imply a high LEE for the pyramids is possible, which motivates the need for further research.
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Huang, Sa. „GaN-Based and High-Speed Metal-Semiconductor-Metal Photodetector: Growth and Device Structures for Integration“. Diss., Available online, Georgia Institute of Technology, 2003:, 2003. http://etd.gatech.edu/theses/available/etd-11242003-173234/unrestricted/huang%5Fsa%5F200312%5Fphd.pdf.
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Thesis (Ph. D.)--Electrical and Computer Engineering, Georgia Institute of Technology, 2004.Ferguson, Ian T., Committee Member ; Rhodes, William T., Committee Member ; Wang, Zhonglin, Committee Member ; Brown, April S., Committee Chair ; Jokerst, Nan M., Committee Co-Chair ; Doolittle, W. Alan, Committee Member. Vita. Includes bibliographical references.
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Pan, Guiquan. „Colloidal gallium nitride quantum dots (GaN QDs) : synthesis and characterization /“. View abstract, 2006. http://gateway.proquest.com/openurl?url_ver=Z39.88-2004&res_dat=xri:pqdiss&rft_val_fmt=info:ofi/fmt:kev:mtx:dissertation&rft_dat=xri:pqdiss:3248456.
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Wang, Yingjuan. „Comprehensive optical spectroscopic investigations of GaN epilayers and InGaN/GaN quantum structures“. Click to view the E-thesis via HKUTO, 2006. http://sunzi.lib.hku.hk/hkuto/record/B37090343.
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5
Bychkov, Andrey. „Quantum effects in artificial atoms“. Thesis, University of Oxford, 2003. http://ora.ox.ac.uk/objects/uuid:93a68cff-9823-47d7-9505-b63806f1bbd4.
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This thesis contains a theoretical and experimental investigation of semiconductor quantum dots (artificial atoms). The first part presents a numerical study of spin effects in GaAs/AlAs modulation-doped quantum dots containing 0 to 50 electrons. A theoretical model is developed to calculate confinement potentials and ground-state electron density distributions using the Kohn-Sham local spin-density approximation. Spin polarization, defined as the difference between the up- and down-spin electron densities, is predicted to occur spontaneously in symmetric quantum dots and in quantum point contacts in the lowdensity regime as a result of electron exchange interactions. This spontaneous magnetization can be controlled by an applied gate voltage, which opens up applications in spintronics and provides a possible explanation for the non-integer quantization of the quantum point contact conductance. The second part describes experimental techniques to investigate photon-exciton coupling in InAs/GaAs self-assembled quantum dots. Two experiments on resonant excitation of a single quantum dot are proposed, whereby the quantum-dot emission is distinguished from resonant pump light by either photon bunching of collected photons with reference photons, or Michelson interferometry. The feasibility study of the proposed experiments shows that the photon-exciton coupling efficiency must be dramatically increased by putting the quantum dot inside an optical microcavity. Novel types of high-quality, low mode-volume semiconductor microcavities containing quantum dots are designed, fabricated, and studied on a newly built setup. We present the first results of photoluminescence studies of InAs quantum dots inside both GaAs single-defect square-lattice photonic-crystal slabs and GaAs/AlAs micropillars, and InAs artificial molecules formed by vertically coupled strain-assisted quantum dots. The results indicate the potential of these nanostructures for implementing resonant transfer of quantum information, developing quantum repeaters and entangled-photon sources, and studying QED effects in the strong-coupling regime.
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Wen, Yuan, und 文苑. „Theoretical and experimental studies of electronic states in InAs/GaAsself-assembled quantum dots“. Thesis, The University of Hong Kong (Pokfulam, Hong Kong), 2009. http://hub.hku.hk/bib/B43224003.
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Wang, Yingjuan, und 王穎娟. „Comprehensive optical spectroscopic investigations of GaN epilayers and InGaN/GaN quantum structures“. Thesis, The University of Hong Kong (Pokfulam, Hong Kong), 2006. http://hub.hku.hk/bib/B37090343.
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Wen, Yuan. „Theoretical and experimental studies of electronic states in InAs/GaAs self-assembled quantum dots“. Click to view the E-thesis via HKUTO, 2009. http://sunzi.lib.hku.hk/hkuto/record/B43224003.
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Park, Gyoungwon. „GaAs-based long-wavelength quantum dot lasers /“. Digital version, 2001. http://wwwlib.umi.com/cr/utexas/fullcit?p3008414.
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Wang, Hongjiang, und 王泓江. „Spectroscopic investigation of optical properties of GaN epilayers andInGaN/GaN quantum wells“. Thesis, The University of Hong Kong (Pokfulam, Hong Kong), 2002. http://hub.hku.hk/bib/B29779911.
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Dufåker, Daniel, L. O. Mereni, Fredrik K. Karlsson, V. Dimastrodonato, G. Juska, Per-Olof Holtz und E. Pelucchi. „Exciton-phonon coupling in single quantum dots with different barriers“. Linköpings universitet, Halvledarmaterial, 2011. http://urn.kb.se/resolve?urn=urn:nbn:se:liu:diva-67198.
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The coupling between longitudinal-optical (LO) phonons and neutral excitons in two different kinds of InGaAs pyramidal quantum dots embedded in either AlGaAs or GaAs barriers is experimentally examined. We find a slightly weaker exciton-LO-phonon coupling and increased linewidth of the phonon replicas for the quantum dots with GaAs barriers compared to the ones with AlGaAs barriers. These results, combined with the fact that the LO-phonon energy of the exciton is the same for both kinds of dots, are taken as evidence that the excitons mainly couple to LO-phonons within the QDs.Original Publication:Daniel Dufåker, L. O. Mereni, Fredrik K. Karlsson, V. Dimastrodonato, G. Juska, Per-Olof Holtz and E. Pelucchi, Exciton-phonon coupling in single quantum dots with different barriers, 2011, Applied Physics Letters, (98), 25, 251911.http://dx.doi.org/10.1063/1.3600781Copyright: American Institute of Physicshttp://www.aip.org/
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Auzelle, Thomas. „Nanofils de GaN/AlN : nucléation, polarité et hétérostructures quantiques“. Thesis, Université Grenoble Alpes (ComUE), 2015. http://www.theses.fr/2015GREAY057/document.
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Usant de certaines conditions, la croissance épitaxiale de GaN sur un large panel de substrats donne lieu à une assemblée de nanofils. Cette géométrie filaire peut permettre la croissance d'hétérostructures libres de tous défauts cristallins étendus, ce qui les rendent attractives pour créer des dispositifs de hautes performances. En premier lieu, mon travail de thèse a visé à clarifier le mécanisme de nucléation auto-organisé des nanofils de GaN sur substrat de silicium. Dans ce but, une étude approfondie de la couche tampon d'AlN, déposée préalablement à la nucléation des nanofils, a été réalisée, mettant en évidence une inattendue forte réactivité de l'Al avec le substrat. La nécessité de la polarité azote pour la croissance des nanofils de GaN a été mise en lumière, bien que des nanofils contenant dans leur cœur un domaine de polarité Ga ont également été observés. Dans ces nanofils, une paroi d'inversion de domaine est présente et a été démontrée être optiquement active, exhibant une photoluminescence à 3.45 eV. Ensuite des hétérostuctures filaires GaN/AlN ont été synthétisée pour des caractérisations structurales et optiques. Il a été montré que le mode de croissance de l'hétérostructure peut être changé en fonction du diamètre du nanofil. En dernier lieu, en prenant avantage de la géométrie cylindrique des nanofils, des mesures de diffusion de porteurs de charge ont été réalisées dans des nanofils de GaN et d'AlNUsing specific conditions, GaN can be epitaxially grown on a large variety of substrates as a nanowire (NW) array. This geometry allows the subsequent growth of wire-like heterostructures likely free of extended defects, which makes them promising for increasing device controllability and performance. First, my PhD work has been devoted to the understanding of self-organized nucleation of GaN NWs on silicon substrates. For this purpose, a deep characterization of the growth mechanism of the AlN buffer deposited prior to NW nucleation has been done, emphasizing an unexpected large reactivity of Al with the substrate. The requirement of the N polarity to nucleate GaN NWs has been evidenced, although the possible existence of NWs hosting a Ga polar core has been observed as well. In these NWs, an inversion domain boundary is present and has been demonstrated to be optically active, having a photoluminescence signature at 3.45 eV. Next, GaN/AlN wire heterostructures have been grown for structural and optical characterization. It has been shown that by changing the wire diameter, different growth mode for the heterostructure could be reached.At last, thanks to the cylindrical geometry of NWs, the measurement of diffusion length for charge carriers in GaN and AlN NWs have been performed
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Davies, Matthew John. „Optical studies of InGaN/GaN quantum well structures“. Thesis, University of Manchester, 2014. https://www.research.manchester.ac.uk/portal/en/theses/optical-studies-of-ingangan-quantum-well-structures(f6c6e59b-8366-44aa-b149-9338d3f03dc0).html.
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In this thesis I present and discuss the results of optical spectroscopy performed on InGaN/GaN single and multiple quantum well (QW) structures. I report on the optical properties of InGaN/GaN single and multiple QW structures, measured at high excitation power densities. I show a correlation exists between the reduction in PL efficiency at high excitation power densities, the phenomenon so-called ``efficiency-droop'', and a broadening of the PL spectra. I also show a distinct change in recombination dynamics, measured by time-resolved photoluminescence (PL), which occurs at the excitation power densities for which efficiency droop is measured. The broadening of the PL spectra at high excitation power densities is shown to occur due to a rapidly redshifting, short-lived high energy emission band. The high energy emission band is proposed to be due to the recombination of weakly localised/delocalised carriers occurring as a consequence of the progressive saturation of the local potential fluctuations responsible for carrier localisation, at high excitation power densities. I report on the effects of varying threading dislocation (TD) density on the optical properties of InGaN/GaN multiple QW structures. No systematic relationship exists between the room temperature internal quantum efficiency (IQE) and the TD density, in a series of nominally identical InGaN/GaN multiple QWs deposited on GaN templates of varying TD density. I also show the excitation power density dependence of the PL efficiency, at room temperatures, is unaffected for variation in the TD density between 2 x107 and 5 x109 cm-2. The independence of the optical properties to TD density is proposed to be a consequence of the strong carrier localisation, and hence short carrier diffusion lengths. I report on the effects of including an InGaN underlayer on the optical and microstructural properties of InGaN/GaN multiple QW structures. I show an increase in the room temperature IQE occurs for the structure containing the InGaN underlayer, compared to the reference. I show using PL excitation spectroscopy that an additional carrier transfer and recombination process occurs on the high energy side of the PL spectrum associated with the InGaN underlayer. Using PL decay time measurements I show the additional recombination process for carriers excited in the underlayer occurs on a faster timescale than the recombination at the peak of the PL spectrum. The additional contribution to the spectrum from the faster recombination process is proposed as responsible for the increase in room temperature IQE.
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Ibrahim, Saber. „Synthesis of Functional Block Copolymers for use in Nano-hybrids“. Doctoral thesis, Saechsische Landesbibliothek- Staats- und Universitaetsbibliothek Dresden, 2011. http://nbn-resolving.de/urn:nbn:de:bsz:14-qucosa-67435.
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Polystyrene block polyethyleneimine (PS-b-PEI) copolymer prepared by combining PS and poly(2-methyl-2-oxazoline) (PMeOx) segments together through two strategies. Furthermore, PMeOx block was hydrolysis to produce PEI block which linked with PS block.
Macroinitiator route is one of these two ways to prepare PS-b-PEI copolymer. Polystyrene macroinitiator or poly(2-methyl-2-oxazoline) macroinitiator prepared through Nitroxide Mediate Radical Polymerization (NMRP) or Cationic Ring Opening Polymerization (CROP) respectively. Each macroinitiator has active initiated terminal group toward another block monomer. Second strategy based on coupling of PS segment with PMeOx block through “click” coupling chemistry. Polystyrene modified with terminal azide moiety are combined with PMeOx functionalized with alkyne group via 1,3 dipolar cycloaddition reaction “click reaction”.
PS-b-PMeOx was hydrolysis in alkaline medium to produce amphiphilic PS-b-PEI copolymer. A set of block copolymer with different block ratios was prepared and investigated to select suitable block copolymer for further applications. Stichiometric PS-b-PEI copolymer selected to stabilize gold nanoparticle (Au NPs) in polymer matrix. PEI segment work as reducing and stabilizing agent of gold precursor in aqueous solution. Various concentrations of gold precursor were loaded and its effect on UVVIS absorbance, particle size and particle distribution studied. In addition, reduction efficiency of PEI block was determined from XPS measurements. The thickness of Au NPs/PS-b-PEI thin film was determined with a novel model for composite system. On the other hand, Gallium nitride quantum dots (GaN QDs) stabilized in PS-b-PEI copolymer after annealing. Our amphiphilic block copolymer exhibit nice thermal stability under annealing conditions. GaN QDs prepared in narrow nano-size with fine particle distribution. Blue ray was observed as an indication to emission activity of GaN crystal. Over all, PS-b-PEI copolymer synthesized through macroinitiator and click coupling methods. It was successfully stabilized Au NPs and GaN QDs in polymer matrix with controlled particle size which can be post applied in tremendous industrial and researcher fields.
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Zallo, Eugenio. „Control of electronic and optical properties of single and double quantum dots via electroelastic fields“. Doctoral thesis, Universitätsbibliothek Chemnitz, 2015. http://nbn-resolving.de/urn:nbn:de:bsz:ch1-qucosa-162870.
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Semiconductor quantum dots (QDs) are fascinating systems for potential applications in quantum information processing and communication, since they can emit single photons and polarisation entangled photons pairs on demand. The asymmetry and inhomogeneity of real QDs has driven the development of a universal and fine post-growth tuning technique. In parallel, new growth methods are desired to create QDs with high emission efficiency and to control combinations of closely-spaced QDs, so-called "QD molecules" (QDMs). These systems are crucial for the realisation of a scalable information processing device after a tuning of their interaction energies.
In this work, GaAs/AlGaAs QDs with low surface densities, high optical quality and widely tuneable emission wavelength are demonstrated, by infilling nanoholes fabricated by droplet etching epitaxy with different GaAs amounts. A tuning over a spectral range exceeding 10 meV is obtained by inducing strain in the dot layer. These results allow a fine tuning of the QD emission to the rubidium absorption lines, increasing the yield of single photons that can be used as hybrid semiconductor-atomic-interface.
By embedding InGaAs/GaAs QDs into diode-like nanomembranes integrated onto piezoelectric actuators, the first device allowing the QD emission properties to be engineered by large electroelastic fields is presented. The two external fields reshape the QD electronic properties and allow the universal recovery of the QD symmetry and the generation of entangled photons, featuring the highest degree of entanglement reported to date for QD-based photon sources.
A method for controlling the lateral QDM formation over randomly distributed nanoholes, created by droplet etching epitaxy, is demonstrated by depositing a thin GaAs buffer over the nanoholes. The effect on the nanohole occupancy of the growth parameters, such as InAs amount, substrate temperature and arsenic overpressure, is investigated as well. The QD pairs show good optical quality and selective etching post-growth is used for a better characterisation of the system.
For the first time, the active tuning of the hole tunnelling rates in vertically aligned InGaAs/GaAs QDM is demonstrated, by the simultaneous application of electric and strain fields, optimising the device concept developed for the single QDs. This result is relevant for the creation and control of entangled states in optically active QDs. The modification of the electronic properties of QDMs, obtained by the combination of the two external fields, may enable controlled quantum operations.
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Arlery, Magali. „Etude par microscopie électronique à transmission de couches et structures semi-conductrices GaN/AlxGa(1-x)N“. Université Joseph Fourier (Grenoble), 1998. http://www.theses.fr/1998GRE10047.
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Nous presentons une etude structurale de depots epais de gan sur alumine et d'heterostructures gan / al#xga#1#-#xn de basse dimensionnalite. Les systemes etudies ont ete elabores par epitaxie par jet moleculaire (mbe) ou par depot en phase vapeur d'organo-metalliques (mocvd). La technique d'investigation est la microscopie electronique a transmission, utilisee en modes conventionnel, haute resolution et faisceau convergent. La premiere partie de l'etude traite de la croissance optimisee de couches de gan sur substrat d'alumine. La polarite des depots est le parametre clef de cette croissance. En effet, la presence de domaines d'inversion de polarite ga dans une matrice a polarite n provoque une croissance sous forme d'ilots hexagonaux, tandis qu'une matrice a polarite ga assure une surface de croissance lisse. Les depots realises contiennent tous des dislocations en grande densite (10#+#1#0/cm#2), dont les vecteurs de burgers sont egaux a 1/3 <2,1,1,0>, 1/3 <2,1,1,3> et 0001. Des nanotubes sont formes par l'ouverture locale du coeur de dislocations 0001. Des defauts prismatiques 2,1,1,0 et 0,1,1,0 ont aussi ete observes. Les derniers forment les parois des domaines d'inversion de polarite et introduisent une translation de 1/20001 entre les cristaux de polarites opposees. Dans une seconde partie, differentes heterostructures gan / al#xga#1#-#xn (puits, super-reseaux et boites quantiques) sont etudiees a l'echelle atomique par analyse quantitative des images haute resolution. L'epitaxie de gan sur al#. #1#5ga#. #8#5n reste coherente pour 16 monocouches deposees. Par contre, une relaxation partielle apparait dans un super-reseau gan / aln dont les couches ont une epaisseur superieure a 11 monocouches. Les heterostructures aln / gan sont caracterisees par une faible miscibilite et des interfaces relativement abruptes. Selon la temperature, les couches de gan deposees sur aln adoptent un mode de croissance bidimensionnel ou de type stranski-krastanov. Ce dernier mode de croissance permet le confinement d'ilots de gan dans aln et ouvre la voie a la realisation de boites quantiques.
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Widmann, Frédéric. „Epitaxie par jets moléculaires de GaN, AlN, InN et leurs alliages : physique de la croissance et réalisation de nanostructures“. Université Joseph Fourier (Grenoble), 1998. http://www.theses.fr/1998GRE10234.
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Ce travail a porte sur la croissance epitaxiale des nitrures d'elements iii gan, aln, et inn, en utilisant l'epitaxie par jets moleculaires assistee par plasma d'azote. Nous avons optimise les premiers stades de la croissance de gan ou aln sur substrat al#2o#3 (0001). Le processus utilise consiste a nitrurer la surface du substrat a l'aide du plasma d'azote, afin de la transformer en aln, puis a faire croitre une couche tampon d'aln ou de gan a basse temperature, avant de reprendre la croissance de gan ou aln a haute temperature (680 a 750c). Nous avons en particulier etudie les proprietes d'une couche de gan en fonction de la temperature a laquelle est realisee l'etape de nitruration. Lorsque les conditions de demarrage de la croissance sont optimisees, nous avons pu observer des oscillations de rheed pendant la croissance de la couche de gan. Nous avons etudie l'effet du rapport v/iii sur la morphologie de surface et les proprietes optiques et structurales de cette couche. Nous avons propose l'utilisation de l'indium en tant que surfactant pour ameliorer ces proprietes. Nous avons ensuite aborde la realisation de superreseaux gan/aln dont nous avons optimise les interfaces. Les mecanismes de relaxation des contraintes de aln sur gan et gan sur aln ont ete etudies. Nous avons egalement elabore les alliages algan et ingan, comme barrieres quantiques dans les heterostructures. Nous avons montre que la relaxation elastique des contraintes de gan en epitaxie sur aln donne lieu a la formation d'ilots de tailles nanometriques, qui se comportent comme des boites quantiques. Leur densite et leur taille dependent de la temperature de croissance, et des conditions de murissement apres croissance. Les proprietes optiques de ces ilots sont gouvernees a la fois par les effets de confinement quantique et par le fort champ piezo-electrique induit par la contrainte dans les ilots.
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Tremblay, Ronan. „Propriétés structurales, optiques et électriques de nanostructures et alliages à base de GaP pour la photonique intégrée sur silicium“. Thesis, Rennes, INSA, 2018. http://www.theses.fr/2018ISAR0026/document.
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Ce travail de thèse porte sur les propriétés structurales, optiques et électriques de nanostructures et alliages à base de GaP pour la photonique intégrée sur silicium. Parmi les méthodes d’intégration des semi-conducteurs III-V sur Si, l’intérêt de l’approche GaP/Si est tout d’abord discuté. Une étude de la croissance et du dopage de l’AlGaP est présentée afin d’assurer le confinement optique et l’injection électrique dans les structures lasers GaP. Les difficultés d’activation des dopants n sont mises en évidence. Ensuite, les propriétés de photoluminescence des boites quantiques InGaAs/GaP sont étudiées en fonction de la température et de la densité d’excitation. Les transitions optiques mises en jeu sont identifiées comme étant des transitions indirectes de type-I avec les électrons dans les niveaux Xxy et les trous dans les niveaux HH des boites quantiques InGaAs et de type-II avec les électrons dans les niveaux Xz du GaP contraint. Malgré une modification notable de la structure électronique de ces émetteurs, une transition optique directe et type I n’est pas obtenue ce qui reste le verrou majeur pour la promotion d’émetteurs GaP sur Si. La maitrise de l’interface GaP/Si et de l’injection électrique est par ailleurs validée par la démonstration de l’électroluminescence à température ambiante d’une LED GaPN sur Si. Si l’effet laser n’est pas obtenu dans les structures lasers rubans GaP, un possible début de remplissage de la bande Гdans les QDs est discuté. Enfin, l’adéquation des lasers à l’état de l’art avec les critères d’interconnections optiques sur puce est discutéeThis PhD work focuses on the structural, optical, electrical properties of GaP-based nanostructures and alloys for integrated photonics on silicon. Amongst the integration approaches of III-V on Si, the interest of GaP/Si is firstly discussed. A study of the growth and the doping of AlGaP used as laser cladding layers (optical confinement and electrical injection) is presented. The activation complexity of n-dopants is highlighted. Then, the photoluminescence properties of InGaAs/GaP quantum dots are investigated as a function of temperature and optical density. The origin of the optical transitions involved are identified as (i) indirect type-I transition between electrons in Xxy states and holes in HH states of quantum dots InGaAs and (ii) indirect type-II with electrons in Xz states of strained GaP. Despite an effective modification in the electronic structure of these emitters, a direct type I optical transition is not demonstrated. This is the major bottleneck in the promotion of GaP based emitters on Si. This said, the control of the GaP/Si interface and electrical injection are confirmed by the demonstration of electroluminescence at room temperature on Si. If no laser effect is obtained in rib laser architectures, a possible beginning of Г band filling in QDs is discussed. Finally, the adequacy of state of the art integrated lasers with the development of on-chip optical interconnects is discussed
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Girardi, Tiago Illipronti 1986. „Efeito de interface nas propriedades ópticas de pontos quânticos de InP/GaAs“. [s.n.], 2012. http://repositorio.unicamp.br/jspui/handle/REPOSIP/277762.
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Orientador: Fernando IikawaDissertação (mestrado) - Universidade Estadual de Campinas, Instituto de Física Gleb Wataghin
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Resumo: Neste trabalho, estudamos o efeito de diferentes condições de interface de InP/GaAs nas propriedades ópticas de pontos quânticos auto-organizados, crescidos por epitaxia de feixe químico, no modo Stranskii-Krastanov. Espera-se que os pontos quânticos de InP/GaAs apresentem alinhamento de bandas do tipo II, e somente os elétrons ficam confinados, enquanto os buracos ficam localizados nas camadas de GaAs em volta do ponto quântico, atraídos pelo elétron. No entanto, devido ao efeito de mistura de átomos nas interfaces o perfil de potencial nas interfaces pode ser alterado significativamente, afetando, com isso, as propriedades ópticas dos pontos quânticos. Foram estudadas amostras com as seguintes condições de interface entre a camada de InP e as camadas de GaAs: inclusão ou não de uma camada de InGaP em uma ou nas duas interfaces. O InGaP gera uma barreira para ambos os tipos de portadores de carga em uma junção tanto com o GaAs como InP e evita a difusa de As das camadas de GaAs para a de InP. Através de medidas de fotoluminescência resolvida no tempo, observamos a variação do tempo de decaimento da emissão óptica associada aos pontos quânticos de acordo com as diferentes condições de interface. Foi observado um tempo curto de decaimento em amostras sem a inclusão de InGaP e com a inclusão apenas na interface superior, enquanto foi observado um tempo longo quando incluímos camadas de InGaP em ambas as interfaces. O tempo de decaimento curto é incompatível com o alinhamento de bandas do tipo II, que deveria separar espacialmente o elétron do buraco. A partir desses resultados e estudos anteriores a esse trabalho, pudemos concluir que o tempo curto se deve à mistura de átomos nas regiões de ambas as interfaces, gerando ligas que localizam os portadores próximos um ao outro. O tempo longo na amostra contendo InGaP nas duas interfaces é atribuído à separação espacial do elétron e do buraco. O efeito de mistura de átomos nas interfaces, neste caso, não forma uma liga na interface que localize os dois tipos de portadores próximos um ao outro. Isso pode ser uma alternativa de preparação de pontos quânticos de InP/GaAs onde se mantém separados espacialmente o elétron e o buraco
Abstract: We studied the effect of different interface conditions on the optical properties of InP/GaAs self-assembled quantum dots grown by chemical beam epitaxy in the Stranskii-Krastanov mode. InP/GaAs quantum dots is expected to present type II band alignment, and only electrons are confined, whereas the holes are localized in the GaAs layers around the quantum dot, attracted by the electron. However, due to the atomic intermixing effect in the interface the potential profile can be strongly changed, affecting the optical properties of the quantum dots. We studied samples with the following conditions at the interfaces between the InP layer and GaAs layers: the inclusion, or the lack of, a InGaP layer at one of or both interfaces. InGaP generates a barrier for both types of carriers in a junction with GaAs and InP, and avoid the diffusion of As from the GaAs layers to the InP one. Using time-resolved photo-luminescence, we observed a change of the optical emission decay times associated to the quantum dots as the interface condition is changed. We observed a short decay lifetime in samples without InGaP layers and with the inclusion in the top interface only, whereas we observed a long decay time when we included InGaP layers in both interfaces. The short decay lifetime is incompatible with the type II band alignment, where the electron and the hole should be spatially separated. Using these and other previous results, we concluded that the short decay lifetime is due to the atomic intermixing in both interfaces regions, forming alloys that localize the carriers near each other. The long lifetime observed for sample containing InGaP in both interfaces is attributed to the large electron-hole spatial separation. In this case intermixing effects at the interfaces do not form a potential well to localize the carries near each other
Mestrado
Física
Mestre em Física
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Mahesh, Kumar *. „Group III-Nitride Epi And Nanostructures On Si(111) By Molecular Beam Epitaxy“. Thesis, 2011. http://hdl.handle.net/2005/2408.
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The present work has been focused on the growth of Group III-nitride epitaxial layers and nanostructures on Si (111) substrates by plasma-assisted molecular beam epitaxy. Silicon is regarded as a promising substrate for III-nitrides, since it is available in large quantity, at low cost and compatible to microelectronics device processing. However, three-dimensional island growth is unavoidable for the direct growth of GaN on Si (111) because of the extreme lattice and thermal expansion coefficient mismatch. To overcome these difficulties, by introducing β-Si3N4 buffer layer, the yellow luminescence free GaN can be grow on Si (111) substrate. The overall research work carried out in the present study comprises of five main parts. In the first part, high quality, crack free and smooth surface of GaN and InN epilayers were grown on Si(111) substrate using the substrate nitridation process. Crystalline quality and surface roughness of the GaN and InN layers are extremely sensitive to nitridation conditions such as nitridation temperature and time. Raman and PL studies indicate that the GaN film obtained by the nitridation sequences has less tensile stress and optically good. The optical band gaps of InN are obtained between ~0.73 to 0.78 eV and the blueshift of absorption edge can be induced by background electron concentration. The higher electron concentration brings in the larger blueshift, due to a possible Burstein–Moss effect. InN epilayers were also grown on GaN/Si(111) substrate by varying the growth parameters such as indium flux, substrate temperature and RF power.
In the second part, InGaN/Si, GaN/Si3N4/n-Si and InN/Si3N4/n-Si heterostructures were fabricated and temperature dependent electrical transport behaviors were studied. Current density-voltage plots (J-V-T) of InGaN/Si heterostructure revealed that the ideality factor and Schottky barrier height are temperature dependent and the incorrect values of the Richardson’s constant produced, suggests an inhomogeneous barrier at the heterostructure interface. The higher value of the ideality factor compared to the ideal value and its temperature dependence suggest that the current transport is primarily dominated by thermionic field emission rather than thermionic emission. The valence band offset of GaN/β-Si3N4/Si and InGaN/Si heterojunctions were determined by X-ray photoemission spectroscopy. InN QDs on Si(111) substrate by droplet epitaxy and S-K growth method were grown in the third part. Single-crystalline structure of InN QDs (droplet epitaxy) was verified by TEM and the chemical bonding configurations of InN QDs were examined by XPS. The interdigitated electrode pattern was created and (I-V) characteristics of InN QDs were studied in a metal–semiconductor–metal configuration in the temperature range of 80–300 K. The I-V characteristics of lateral grown InN QDs were explained by using the trap model. A systematic manipulation of the morphology, optical emission and structural properties of InN/Si (111) QDs (S-K method) is demonstrated by changing the growth kinetics parameters such as flux rate and growth time. The growth kinetics of the QDs has been studied through the scaling method and observed that the distribution of dot sizes, for samples grown under varying conditions, has followed the scaling function.
In the fourth part, InN nanorods (NRs) were grown on Si(111) and current transport properties of NRs/Si heterojunctions were studied. The rapid rise and decay of infrared on/off characteristics of InN NRs/Si heterojunction indicate that the device is highly sensitive to the IR light. Self-aligned GaN nanodots were grown on semi-insulating Si(111) substrate. The interdigitated electrode pattern was created on nanodots using photolithography and dark as well as UV photocurrent were studied. Surface band gaps of InN QDs were estimated from scanning tunneling spectroscopy (STS) I-V curves in the last part. It is found that band gap is strongly dependent on the size of InN QDs. The observed size-dependent STS band gap energy blueshifts as the QD’s diameter or height was reduced.
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Cao, Chuanshun Deppe Dennis G. „Carrier dynamics in quantum dot and GaAs-based quantum dot cascade laser“. 2004. http://wwwlib.umi.com/cr/utexas/fullcit?p3143662.
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Cao, Chuanshun 1972. „Carrier dynamics in quantum dot and GaAs-based quantum dot cascade laser“. 2004. http://hdl.handle.net/2152/12750.
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Inciong, Michelle R., und 蜜雪兒. „Improved Optical Properties in PAMAM Dendrimers and Gallium Nitride Using Graphene Quantum Dots“. Thesis, 2016. http://ndltd.ncl.edu.tw/handle/53483310406877742655.
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碩士中原大學
物理研究所
104
Graphene is a novel 2D material composed of carbon molecules with strong mechanical features, remarkable thermal conductivity, and outstanding electrical properties. The excellent properties of graphene makes it a very powerful material that has been used and applied into numerous various applications. A 0D version of graphene called graphene quantum dots (GQDs) expands the application of graphene into a nanodimensional aspect. GQDs possess unique optical, electrical, and chemical properties attributed to their major structural components, which is the quantum confinement and surface effects. Numerous fabrication techniques have been used to synthesize GQDs and tune its photoluminescence (PL). This study implicates the synthesis of GQDs with tunable PL and optical applications of other materias by using GQDs. Herein, we present the use of pulsed laser ablation (PLA) as a means to synthesize a tunable luminescent GQDs in ethanol solvent. With regards to the applications of GQDs, a drop-cast method was used to incorporate the GQDs on different materials. Through this method, photoinduced carrier transfer from GQDs to poly(amido amine) (PAMAM) dendrimers was observed in the GQD/PAMAM composite, resulting to an enhanced PL intensity with a factor of 10.9 at 0.9 mg/ml GQD concentration. The mechanism of photoinduced carrier transfer was confirmed by the steady-state and time-resolved PL, and Kelvin probe measurements. Also, a drop-cast method demonstrate the photoinduced carrier transfer which modulates the electrical properties and enhances the photoconductivity of GaN epilayers. At a GQD concentration of 0.9 mg/ml, a 23-fold photocurrent enhancement was observed in the GQD-doped GaN epilayers. Such carrier transfer which occurred in PAMAM dendrimers (GaN epilayers) through the incorporation of GQDs is deduced to be the work function difference between PAMAM dendrimers (GaN) and GQDs. The enhanced electrical and optical properties from photoinduced carrier transfer are very potential for the applications of GQD in GaN-based devices, solar cell, and other devices.
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El, Afandy Rami. „Optical and Micro-Structural Characterization of MBE Grown Indium Gallium Nitride Polar Quantum Dots“. Thesis, 2011. http://hdl.handle.net/10754/205810.
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Gallium nitride and related materials have ushered in scientific and technological breakthrough for lighting, mass data storage and high power electronic applications. These III-nitride materials have found their niche in blue light emitting diodes and blue laser diodes. Despite the current development, there are still technological problems that still impede the performance of such devices. Three-dimensional nanostructures are proposed to improve the electrical and thermal properties of III-nitride optical devices. This thesis consolidates the characterization results and unveils the unique physical properties of polar indium gallium nitride quantum dots grown by molecular beam epitaxy technique.
In this thesis, a theoretical overview of the physical, structural and optical properties of polar III-nitrides quantum dots will be presented. Particular emphasis will be given to properties that distinguish truncated-pyramidal III-nitride quantum dots from other III-V semiconductor based quantum dots. The optical properties of indium gallium nitride quantum dots are mainly dominated by large polarization fields, as well as quantum confinement effects. Hence, the experimental investigations for such quantum dots require performing bandgap calculations taking into account the internal strain fields, polarization fields and confinement effects. The experiments conducted in this investigation involved the transmission electron microscopy and x-ray diffraction as well as photoluminescence spectroscopy.
The analysis of the temperature dependence and excitation power dependence of the PL spectra sheds light on the carrier dynamics within the quantum dots, and its underlying wetting layer. A further analysis shows that indium gallium nitride quantum dots through three-dimensional confinements are able to prevent the electronic carriers from getting thermalized into defects which grants III-nitrides quantum dot based light emitting diodes superior thermally induced optical properties compared to other nanostructures. Excitation power dependent PL measurements reveal an increase in the excitonic confinements and hence higher quantum efficiencies compared to lower dimensional nanostructures. Finally it is argued that such characteristics allows quantum dots based InGaN structures to become potentially a strong candidate for high quantum efficiency white solid-state light emitting diodes and ultra-violet/blue laser diode operating at room temperature.
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Huang, Hua Deppe Dennis G. „Theoretical study of GaAs-based quantum dot lasers and microcavity light emitting diodes“. 2004. http://repositories.lib.utexas.edu/bitstream/handle/2152/2019/huangh042.pdf.
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Huang, Hua. „Theoretical study of GaAs-based quantum dot lasers and microcavity light emitting diodes“. Thesis, 2004. http://hdl.handle.net/2152/2019.
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Shetty, Arjun. „Device Applications of Epitaxial III-Nitride Semiconductors“. Thesis, 2015. http://etd.iisc.ernet.in/2005/3530.
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Through the history of mankind, novel materials have played a key role in techno- logical progress. As we approach the limits of scaling it becomes difficult to squeeze out any more extensions to Moore’s law by just reducing device feature sizes. It is important to look for an alternate semiconductor to silicon in order to continue making the progress predicted by Moore’s law. Among the various semiconductor options being explored world-wide, the III-nitride semiconductor material system has certain unique characteristics that make it one of the leading contenders. We explore the III-nitride semiconductor material system for the unique advantages that it offers over the other alternatives available to us.
This thesis studies the device applications of epitaxial III-nitride films and nanos- tructures grown using plasma assisted molecular beam epitaxy (PAMBE)
The material characterisation of the PAMBE grown epitaxial III-nitrides was car- ried out using techniques like high resolution X-ray diffraction (HR-XRD), field emis- sion scanning electron microscopy (FESEM), room temperature photoluminescence (PL) and transmission electron microscopy (TEM). The epitaxial III-nitrides were then further processed to fabricate devices like Schottky diodes, photodetectors and surface acoustic wave (SAW) devices. The electrical charcterisation of the fabricated devices was carried out using techniques like Hall measurement, IV and CV measure- ments on a DC probe station and S-parameter measurements on a vector network analyser connected to an RF probe station.
We begin our work on Schottky diodes by explaining the motivation for adding an interfacial layer in a metal-semiconductor Schottky contact and how high-k di- electrics like HfO2 have been relatively unexplored in this application. We report the work carried out on the Pt/n-GaN metal-semiconductor (MS) Schottky and the Pt/HfO2/n-GaN metal-insulator-semiconductor (MIS) Schottky diode. We report an improvement in the diode parameters like barrier height (0.52 eV to 0.63 eV), ideality factor (2.1 to 1.3) and rectification ratio (35.9 to 98.9 @2V bias) after the introduction of 5 nm of HfO2 as the interfacial layer. Temperature dependent I-V measurements were done to gain a further understanding of the interface. We observe that the barrier height and ideality factor exhibit a temperature dependence. This was attributed to inhomogeneities at the interface and by assuming a Gaussian distribution of barrier heights.
UV and IR photodetectors using III-nitrides are then studied. Our work on UV photodetectors describes the growth of epitaxial GaN films. Au nanoparticles were fabricated on these films using thermal evaporation and annealing. Al nanostruc- tures were fabricated using nanosphere lithography. Plasmonic enhancement using these metallic nanostructures was explored by fabricating metal-semiconductor-metal (MSM) photodetectors. We observed plasmonic enhancement of photocurrent in both cases. To obtain greater improvement, we etched down on the GaN film using reac tive ion etching (RIE). This resulted in further increase in photocurrent along with a reduction in dark current which was attributed to creation of new trap states. IR photodetectors studied in this thesis are InN quantum dots whose density can be controlled by varying the indium flux during growth. We observe that increase in InN quantum dot density results in increase in photocurrent and decrease in dark current in the fabricated IR photodetectors.
We then explore the advantages that InGaN offers as a material that supports surface acoustic waves and fabricate InGaN based surface acoustic wave devices. We describe the growth of epitaxial In0.23 Ga0.77 N films on GaN template using molecular beam epitaxy. Material characterisation was carried out using HR-XRD, FESEM, PL and TEM. The composition was determined from HR-XRD and PL measurements and both results matched each other. This was followed by the fabrication of interdigited electrodes with finger spacing of 10 µm. S-parameter results showed a transmission
peak at 104 MHz with an insertion loss of 19 dB. To the best of our knowledge, this is the first demonstration of an InGaN based SAW device.
In summary, this thesis demonstrates the practical advantages of epitaxially grown film and nanostructured III-nitride materials such as GaN, InN and InGaN using plasma assisted molecular beam epitaxy for Schottky diodes, UV and IR photodetec- tors and surface acoustic wave devices.
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Zallo, Eugenio. „Control of electronic and optical properties of single and double quantum dots via electroelastic fields“. Doctoral thesis, 2014. https://monarch.qucosa.de/id/qucosa%3A20217.
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Semiconductor quantum dots (QDs) are fascinating systems for potential applications in quantum information processing and communication, since they can emit single photons and polarisation entangled photons pairs on demand. The asymmetry and inhomogeneity of real QDs has driven the development of a universal and fine post-growth tuning technique. In parallel, new growth methods are desired to create QDs with high emission efficiency and to control combinations of closely-spaced QDs, so-called "QD molecules" (QDMs). These systems are crucial for the realisation of a scalable information processing device after a tuning of their interaction energies.
In this work, GaAs/AlGaAs QDs with low surface densities, high optical quality and widely tuneable emission wavelength are demonstrated, by infilling nanoholes fabricated by droplet etching epitaxy with different GaAs amounts. A tuning over a spectral range exceeding 10 meV is obtained by inducing strain in the dot layer. These results allow a fine tuning of the QD emission to the rubidium absorption lines, increasing the yield of single photons that can be used as hybrid semiconductor-atomic-interface.
By embedding InGaAs/GaAs QDs into diode-like nanomembranes integrated onto piezoelectric actuators, the first device allowing the QD emission properties to be engineered by large electroelastic fields is presented. The two external fields reshape the QD electronic properties and allow the universal recovery of the QD symmetry and the generation of entangled photons, featuring the highest degree of entanglement reported to date for QD-based photon sources.
A method for controlling the lateral QDM formation over randomly distributed nanoholes, created by droplet etching epitaxy, is demonstrated by depositing a thin GaAs buffer over the nanoholes. The effect on the nanohole occupancy of the growth parameters, such as InAs amount, substrate temperature and arsenic overpressure, is investigated as well. The QD pairs show good optical quality and selective etching post-growth is used for a better characterisation of the system.
For the first time, the active tuning of the hole tunnelling rates in vertically aligned InGaAs/GaAs QDM is demonstrated, by the simultaneous application of electric and strain fields, optimising the device concept developed for the single QDs. This result is relevant for the creation and control of entangled states in optically active QDs. The modification of the electronic properties of QDMs, obtained by the combination of the two external fields, may enable controlled quantum operations.