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Artykuły w czasopismach na temat „Hybrid solid electrolyte”

Autor: Grafiati

Data publikacji: 5 października 2024

Data aktualizacji: 31 lipca 2025

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1

Kanai, Yamato, Koji Hiraoka, Mutsuhiro Matsuyama, and Shiro Seki. "Chemically and Physically Cross-Linked Inorganic–Polymer Hybrid Solvent-Free Electrolytes." Batteries 9, no. 10 (2023): 492. http://dx.doi.org/10.3390/batteries9100492.

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Safe, self-standing, all-solid-state batteries with improved solid electrolytes that have adequate mechanical strength, ionic conductivity, and electrochemical stability are strongly desired. Hybrid electrolytes comprising flexible polymers and highly conductive inorganic electrolytes must be compatible with soft thin films with high ionic conductivity. Herein, we propose a new type of solid electrolyte hybrid comprising a glass–ceramic inorganic electrolyte powder (Li1+x+yAlxTi2−xSiyP3−yO12; LICGC) in a poly(ethylene)oxide (PEO)-based polymer electrolyte that prevents decreases in ionic condu

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2

Lee, Wang-Geun. "Hybrid Electrolyte Strategies for High-Energy Sodium-Based Batteries." ECS Meeting Abstracts MA2024-02, no. 9 (2024): 1303. https://doi.org/10.1149/ma2024-0291303mtgabs.

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Sodium-based batteries are emerging as a promising and crucial technology for sustainable energy storage due to the abundance and cost-effectiveness of sodium compared to lithium. While these batteries offer an attractive option for large-scale applications, they face challenges such as lower voltage and energy density. To overcome these limitations and enhance high-energy sodium-based battery performance, researchers are exploring innovative hybrid electrolyte strategies. Hybrid electrolytes, which combine solid and liquid systems, provide improvements in safety, efficiency, and performance.

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3

Lv, Wenjing, Kaidong Zhan, Xuecheng Ren, Lu Chen, and Fan Wu. "Comparing Charge Dynamics in Organo-Inorganic Halide Perovskite: Solid-State versus Solid-Liquid Junctions." Journal of Nanoelectronics and Optoelectronics 19, no. 2 (2024): 121–28. http://dx.doi.org/10.1166/jno.2024.3556.

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In this study, we explore the dynamics of a perovskite-electrolyte photoelectrochemical cell, pivotal for advancing electrolyte-gated field effect transistors, water-splitting photoelectrochemical and photocatalytic cells, supercapacitors, and CO2 capture and reduction technologies. The instability of hybrid perovskite materials in aqueous electrolytes presents a significant challenge, yet recent breakthroughs have been achieved in stabilizing organo-inorganic halide perovskite films. This stabilization is facilitated by employing liquid electrolytes, specifically those formed by dissolving te

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4

Choi, Kyoung Hwan, Eunjeong Yi, Kyeong Joon Kim, et al. "(Invited) Pragmatic Approach and Challenges of All Solid State Batteries: Hybrid Solid Electrolyte for Technical Innovation." ECS Meeting Abstracts MA2023-01, no. 6 (2023): 988. http://dx.doi.org/10.1149/ma2023-016988mtgabs.

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For the growth of electric vehicle market, lithium-ion batteries (LIBS) used in the EVs still requires safety and reliability. Unfortunately, large-scale application of the LIBs is being challenged due to the fact that the use of flammable liquid electrolytes has caused safety issues such as leakage and fire explosion. In this respect, all-solid-state batteries (ASSBs) have been intensively studied to ensure the safety and mileage that are superior to the current LIBs. In terms of solid electrolytes, oxide electrolytes not only shows high ionic conductivity (10-4 ~ 10-3 S/cm) but also high mec

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5

Liao, Cheng Hung, Chia-Chin Chen, Ru-Jong Jeng, and Nae-Lih (Nick) Wu. "Application of Artificial Interphase on Ni-Rich Cathode Materials Via Hybrid Ceramic-Polymer Electrolyte in All Solid State Batteries." ECS Meeting Abstracts MA2023-01, no. 6 (2023): 1050. http://dx.doi.org/10.1149/ma2023-0161050mtgabs.

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Among many cathode materials, nickel-rich LiNi0.83Co0.12Mn0.05O2 (NCM 831205) has been spotlighted as one of the most feasible candidates for next-generation LIBs because of its high discharge capacity (~200 mAh/g). However, NCM 831205 shows significant performance degradation, which is mostly attributed to cation mixing, surface side reactions, and intrinsic structural instability originating from the large volume changes during repeated cycling. Conventional lithium ion batteries (LIB) normally use flammable nonaqueous liquid electrolytes, resulting in a serious safety issue in use. In this

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6

LI, X. D., X. J. YIN, C. F. LIN, et al. "INFLUENCE OF I2 CONCENTRATION AND CATIONS ON THE PERFORMANCE OF QUASI-SOLID-STATE DYE-SENSITIZED SOLAR CELLS WITH THERMOSETTING POLYMER GEL ELECTROLYTE." International Journal of Nanoscience 09, no. 04 (2010): 295–99. http://dx.doi.org/10.1142/s0219581x10006831.

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Thermosetting polymer gel electrolytes (TPGEs) based on poly(acrylic acid)-poly(ethylene glycol) (PAA-PEG) hybrid were prepared and applied to fabricate dye-sensitized solar cells (DSCs). N-methylpyrrolidone (NMP) and γ-butyrolactone (GBL) were used as solvents for liquid electrolytes and LiI and KI as iodide source, separately. The microstructure of PAA-PEG shows a well swelling ability in liquid electrolyte and excellent stability of the swollen hybrid. The TPGE was optimized in terms of the liquid electrolyte absorbency and ionic conductivity photovoltaic performance. Quasi-solid-state DSCs

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7

Zahiri, Beniamin, Chadd Kiggins, Dijo Damien, et al. "Hybrid Halide Solid Electrolytes and Bottom-up Cell Assembly Enable High Voltage Solid-State Lithium Batteries." ECS Meeting Abstracts MA2022-01, no. 2 (2022): 327. http://dx.doi.org/10.1149/ma2022-012327mtgabs.

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Interface between halide based solid electrolytes and layered transition metal oxide cathodes has been found to be electro-chemically stable due to stability of chloride compounds, in particular, at >4V range. The extent of interfacial stability is correlated with the type of cationic and anionic species in the solid electrolyte compound, a fact supported by theoretical prediction and yet, not accurately measured in composite cathode mixtures. By altering the architecture of cathode into a dense additive-free structure, we have identified differences in interfacial stability of chloride com

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8

Zhai, Yanfang, Wangshu Hou, Zongyuan Chen, et al. "A hybrid solid electrolyte for high-energy solid-state sodium metal batteries." Applied Physics Letters 120, no. 25 (2022): 253902. http://dx.doi.org/10.1063/5.0095923.

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Exploring solid electrolytes with promising electrical properties and desirable compatibility toward electrodes for safe and high-energy sodium metal batteries remains a challenge. In this work, these issues are addressed via an in situ hybrid strategy, viz., highly conductive and thermally stable 1-ethyl-3-methylimidazolium bis(fluorosulfonyl)imide is immobilized in nanoscale silica skeletons to form ionogel via a non-hydrolytic sol-gel route, followed by hybridizing with polymeric poly(ethylene oxide) and inorganic conductor Na3Zr2Si2PO12. Such hybrid design yields the required solid electro

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9

Zaman, Wahid, Nicholas Hortance, Marm B. Dixit, Vincent De Andrade, and Kelsey B. Hatzell. "Visualizing percolation and ion transport in hybrid solid electrolytes for Li–metal batteries." Journal of Materials Chemistry A 7, no. 41 (2019): 23914–21. http://dx.doi.org/10.1039/c9ta05118j.

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10

Mohanty, Debabrata, Shu-Yu Chen, and I.-Ming Hung. "Effect of Lithium Salt Concentration on Materials Characteristics and Electrochemical Performance of Hybrid Inorganic/Polymer Solid Electrolyte for Solid-State Lithium-Ion Batteries." Batteries 8, no. 10 (2022): 173. http://dx.doi.org/10.3390/batteries8100173.

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Lithium-ion batteries are popular energy storage devices due to their high energy density. Solid electrolytes appear to be a potential replacement for flammable liquid electrolytes in lithium batteries. This inorganic/hybrid solid electrolyte is a composite of lithium bis(trifluoromethanesulfonyl)imide (LiTFSI) salt, (poly(vinylidene fluoride-hexafluoro propylene) (PVDF-HFP) polymer and sodium superionic conductor (NASICON)-type Li1+xAlxTi2−x(PO4)3 (LATP) ceramic powder. The structure, morphology, mechanical behavior, and electrochemical performance of this composite solid electrolyte, based o

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11

Vargas-Barbosa, Nella Marie, Sebastian Puls, and Henry Michael Woolley. "Hybrid Material Concepts for Thiophosphate-Based Solid-State Batteries." ECS Meeting Abstracts MA2023-01, no. 6 (2023): 984. http://dx.doi.org/10.1149/ma2023-016984mtgabs.

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Solid-state batteries (SSBs) could replace conventional lithium-ion batteries due to the possibility of increasing the energy density of the cells by using lithium metal as the anode material.[1] Among the many electrolyte candidates for lithium SSBs, the lithium thiophosphates are particularly interesting due to their high ionic conductivities at room temperature (>1 mS/cm). However, the (electro)chemical stability of these solid electrolytes is limited and not fully compatible with state-of-the-art high-potential cathode active materials[2] or the lithium metal anode.[3] At the cell level

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12

Villaluenga, Irune, Kevin H. Wujcik, Wei Tong, et al. "Compliant glass–polymer hybrid single ion-conducting electrolytes for lithium batteries." Proceedings of the National Academy of Sciences 113, no. 1 (2015): 52–57. http://dx.doi.org/10.1073/pnas.1520394112.

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Despite high ionic conductivities, current inorganic solid electrolytes cannot be used in lithium batteries because of a lack of compliance and adhesion to active particles in battery electrodes as they are discharged and charged. We have successfully developed a compliant, nonflammable, hybrid single ion-conducting electrolyte comprising inorganic sulfide glass particles covalently bonded to a perfluoropolyether polymer. The hybrid with 23 wt% perfluoropolyether exhibits low shear modulus relative to neat glass electrolytes, ionic conductivity of 10−4 S/cm at room temperature, a cation transf

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13

Spencer Jolly, Dominic, Dominic L. R. Melvin, Isabella D. R. Stephens, et al. "Interfaces between Ceramic and Polymer Electrolytes: A Comparison of Oxide and Sulfide Solid Electrolytes for Hybrid Solid-State Batteries." Inorganics 10, no. 5 (2022): 60. http://dx.doi.org/10.3390/inorganics10050060.

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Hybrid solid-state batteries using a bilayer of ceramic and solid polymer electrolytes may offer advantages over using a single type of solid electrolyte alone. However, the impedance to Li+ transport across interfaces between different electrolytes can be high. It is important to determine the resistance to Li+ transport across these heteroionic interfaces, as well as to understand the underlying causes of these resistances; in particular, whether chemical interphase formation contributes to giving high resistances, as in the case of ceramic/liquid electrolyte interfaces. In this work, two ce

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14

Spencer Jolly, Dominic, Dominic L. R. Melvin, Isabella D. R. Stephens, et al. "Interfaces between Ceramic and Polymer Electrolytes: A Comparison of Oxide and Sulfide Solid Electrolytes for Hybrid Solid-State Batteries." Inorganics 10, no. 5 (2022): 60. http://dx.doi.org/10.3390/inorganics10050060.

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Hybrid solid-state batteries using a bilayer of ceramic and solid polymer electrolytes may offer advantages over using a single type of solid electrolyte alone. However, the impedance to Li+ transport across interfaces between different electrolytes can be high. It is important to determine the resistance to Li+ transport across these heteroionic interfaces, as well as to understand the underlying causes of these resistances; in particular, whether chemical interphase formation contributes to giving high resistances, as in the case of ceramic/liquid electrolyte interfaces. In this work, two ce

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15

Gu, Sui, Xiao Huang, Qing Wang, et al. "A hybrid electrolyte for long-life semi-solid-state lithium sulfur batteries." Journal of Materials Chemistry A 5, no. 27 (2017): 13971–75. http://dx.doi.org/10.1039/c7ta04017b.

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16

Lim, Seung, Juyoung Moon, Uoon Baek, Jae Lee, Youngjin Chae, and Jung Park. "Shape-Controlled TiO2 Nanomaterials-Based Hybrid Solid-State Electrolytes for Solar Energy Conversion with a Mesoporous Carbon Electrocatalyst." Nanomaterials 11, no. 4 (2021): 913. http://dx.doi.org/10.3390/nano11040913.

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One-dimensional (1D) titanium dioxide (TiO2) is prepared by hydrothermal method and incorporated as nanofiller into a hybrid polymer matrix of polyethylene glycol (PEG) and employed as a solid-electrolyte in dye-sensitized solar cells (DSSCs). Mesoporous carbon electrocatalyst with a high surface area is obtained by the carbonization of the PVDC-g-POEM double comb copolymer. The 1D TiO2 nanofiller is found to increase the photoelectrochemical performance. As a result, for the mesoporous carbon-based DSSCs, 1D TiO2 hybrid solid-state electrolyte yielded the highest efficiencies, with 6.1% under

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17

Woolley, Henry Michael, and Nella Vargas-Barbosa. "Electrochemical Characterization of Thiophosphate- Ionic Liquid Hybrid Lithium Electrolytes Against Li Metal." ECS Meeting Abstracts MA2023-01, no. 6 (2023): 986. http://dx.doi.org/10.1149/ma2023-016986mtgabs.

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(Almost) solid-state batteries that utilize thiophosphate solid electrolytes (SE) are an exciting technology emerging as a potential alternative to lithium-ion batteries. When used alongside a lithium metal anode they can offer the high energy densities [1] required to meet the increasing demand for energy storage. However, they suffer from numerous issues which predominately occur at the cathode- or anode-SE interface. Issues include dendrite propagation through gaps, pores and grain boundaries of the solid electrolyte which can eventually puncture electrolyte crystallites and lead to cell fa

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18

CHENG, Xiong, Man LI, Yang Li, Seunghyun Song, Sowjanya Vallem, and Joonho Bae. "Novel DNA-Based Polymer Solid Electrolytes for Lithium-Ion Batteries." ECS Meeting Abstracts MA2024-01, no. 2 (2024): 350. http://dx.doi.org/10.1149/ma2024-012350mtgabs.

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Solid electrolytes are becoming increasingly popular due to their safety [1], and the application of organic biomolecules in electrochemical devices is also an important strategy for sustainable development [2]. Recently, we have studied the application of DNA in electrochemical energy storage devices [3]. A novel PVDF@DNA solid polymer electrolyte was designed in this work, we studied the effect of different DNA addition amounts on polymer solid electrolytes. DNA as a plasticizer-like additive, reduces the crystallinity of the polymer solid electrolyte and improves its ionic conductivity [4].

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19

Song, Shufeng, Masashi Kotobuki, Feng Zheng, et al. "Al conductive hybrid solid polymer electrolyte." Solid State Ionics 300 (February 2017): 165–68. http://dx.doi.org/10.1016/j.ssi.2016.12.023.

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20

Kim, Jae-Kwang, Young Jun Lim, Hyojin Kim, Gyu-Bong Cho, and Youngsik Kim. "A hybrid solid electrolyte for flexible solid-state sodium batteries." Energy & Environmental Science 8, no. 12 (2015): 3589–96. http://dx.doi.org/10.1039/c5ee01941a.

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21

Devaux, Didier, Natalia Stankiewicz, Thomas Boulmier, et al. "PEO Electrolyte As Interlayer for Li Metal Battery Comprising an Halide Based Hybrid Electrolyte." ECS Meeting Abstracts MA2024-02, no. 7 (2024): 777. https://doi.org/10.1149/ma2024-027777mtgabs.

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In the context of the energetic transition, lithium (Li) metal is considered as the most promising material for battery anode electrodes regarding its physico-chemical and electrochemical properties with its high capacity leading to high energy density of the device. However, safety issues, such as the well-known dendrites causing short-circuits, limits its use. Solid-state-electrolytes1 such as hybrid electrolyte based on halides2 that are designed to generate synergy between an organic and inorganic phase is foreseen as promising contenders to overcome the current Li-ion limitations. Despite

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22

Méry, Adrien, Steeve Rousselot, David Lepage, David Aymé-Perrot, and Mickael Dollé. "Limiting Factors Affecting the Ionic Conductivities of LATP/Polymer Hybrid Electrolytes." Batteries 9, no. 2 (2023): 87. http://dx.doi.org/10.3390/batteries9020087.

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All-Solid-State Lithium Batteries (ASSLB) are promising candidates for next generation lithium battery systems due to their increased safety, stability, and energy density. Ceramic and solid composite electrolytes (SCE), which consist of dispersed ceramic particles within a polymeric host, are among the preferred technologies for use as electrolytes in ASSLB systems. Synergetic effects between ceramic and polymer electrolyte components are usually reported in SCE. Herein, we report a case study on the lithium conductivity of ceramic and SCE comprised of Li1.4Al0.4Ti1.6(PO4)3 (LATP), a NASICON-

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Shah, Rajesh, Vikram Mittal, and Angelina Mae Precilla. "Challenges and Advancements in All-Solid-State Battery Technology for Electric Vehicles." J 7, no. 3 (2024): 204–17. http://dx.doi.org/10.3390/j7030012.

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Recent advances in all-solid-state battery (ASSB) research have significantly addressed key obstacles hindering their widespread adoption in electric vehicles (EVs). This review highlights major innovations, including ultrathin electrolyte membranes, nanomaterials for enhanced conductivity, and novel manufacturing techniques, all contributing to improved ASSB performance, safety, and scalability. These developments effectively tackle the limitations of traditional lithium-ion batteries, such as safety issues, limited energy density, and a reduced cycle life. Noteworthy achievements include fre

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24

Thangadurai, Venkataraman. "(Invited) Garnet Solid Electrolytes for Advanced All-Solid-State Li Metal Batteries." ECS Meeting Abstracts MA2022-02, no. 47 (2022): 1759. http://dx.doi.org/10.1149/ma2022-02471759mtgabs.

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These days, Li metal anode-based battery has been arisen as one of the key energy storage technologies due to its high theoretical energy density compared to conventional lithium and sodium ion-based batteries. The present Li-S batteries suffer due to Li dendrite formation and capacity decay due to polysulfide dissolution effect, because of organic electrolytes used in the current research. Solid state (ceramic) electrolytes are promising to prevent Li dendrite growth and polysulfide dissolution. Among different ceramic electrolytes garnet-type structure solid inorganic electrolytes are very p

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Giffin, Guinevere A., Mara Goettlinger, Hendrik Bohn, et al. "Development of a Polymer-Based Silicon-NMC Solid-State Cell." ECS Meeting Abstracts MA2023-02, no. 2 (2023): 373. http://dx.doi.org/10.1149/ma2023-022373mtgabs.

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Solid-state batteries are seen as the next generation of battery technology with the promise of high energy density and improved safety as compared to conventional lithium-ion batteries. To achieve these goals, high-capacity negative electrodes, e.g., silicon or lithium, need to be combined with high capacity and high voltage positive electrodes, e.g., Ni-rich NMC. This combination of active materials provides a number of significant challenges for the solid-state electrolyte. If silicon is used as the anode active material, significant volume changes during lithiation/delithiation occur. Thes

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Ryu, Kun, Kyungbin Lee, Hyun Ju, Jinho Park, Ilan Stern, and Seung Woo Lee. "Ceramic/Polymer Hybrid Electrolyte with Enhanced Interfacial Contact for All-Solid-State Lithium Batteries." ECS Meeting Abstracts MA2022-02, no. 7 (2022): 2621. http://dx.doi.org/10.1149/ma2022-0272621mtgabs.

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All solid-state lithium batteries (ASSLBs) with a high energy density are challenging, yet desired by the rising energy demands. Its intrinsic safety of solid-state electrolytes (SSEs) compared to flammable liquid electrolytes makes ASSLBs a modern-day necessity. NASICON-type Li1.5Al0.5Ge1.5P3O12 (LAGP) has high ionic conductivity, high stability against air and water, and a wide electrochemical window. However, the application of LAGP is significantly hindered by its slow interfacial kinetics and brittle nature. In addition, the ionic conductivity of LAGP is relatively low at room temperature

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SHIMANO, Satoshi, and Itaru HONMA. "Organic-Inorganic Nano-Hybrid Solid-State-Electrolyte." Kobunshi 56, no. 3 (2007): 141. http://dx.doi.org/10.1295/kobunshi.56.141.

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Kim, Ji Sook, Sun Hwa Lee, and Dong Wook Shin. "Fabrication of Hybrid Solid Electrolyte by LiPF₆ Liquid Electrolyte Infiltration into Nano-Porous Na₂O-SiO₂-B₂O₃ Glass Membrane." Solid State Phenomena 124-126 (June 2007): 1027–30. http://dx.doi.org/10.4028/www.scientific.net/ssp.124-126.1027.

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To improve ion mobility in solid inorganic electrolyte for lithium ion battery, the hybrid electrolytes were developed in the form of the organic-inorganic meso-scale hybridization by the infiltration of liquid electrolyte into meso-porous inorganic glass membrane. Glass electrolyte membranes with nanopores were prepared by spinodal decomposition and subsequent acid leaching. The most suitable glass electrolyte membranes could be fabricated from the 7.5Na2O-46.25B2O3 -46.25SiO2 (mol%). The effect of leaching temperature, leaching time and leaching acids on the preparation of the membranes were

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Thangadurai, Venkataraman. "(Invited) Lithium – Sulfur Batteries." ECS Meeting Abstracts MA2022-02, no. 4 (2022): 545. http://dx.doi.org/10.1149/ma2022-024545mtgabs.

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These days, Li-S battery has been arisen as one of the key energy storage technologies due to its high theoretical energy density compared to conventional lithium and sodium ion-based batteries. The present Li-S batteries suffer due to Li dendrite formation and capacity decay due to polysulfide dissolution effect, due to organic electrolytes used in the current research. Solid state (ceramic) electrolytes are promising to prevent Li dendrite growth and polysulfide dissolution. Among different ceramic electrolytes garnet-type structure solid inorganic electrolytes are very promising because of

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Jiang, Wen, Lingling Dong, Shuanghui Liu, et al. "Improvement of the Interface between the Lithium Anode and a Garnet-Type Solid Electrolyte of Lithium Batteries Using an Aluminum-Nitride Layer." Nanomaterials 12, no. 12 (2022): 2023. http://dx.doi.org/10.3390/nano12122023.

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The next generation of all-solid-state batteries can feature battery safety that is unparalleled among conventional liquid batteries. The garnet-type solid-state electrolyte Li7La3Zr2O12 (LLZO), in particular, is widely studied because of its high Li-ion conductivity and stability in air. However, the poor interface-contact between Li and the electrolyte (garnet) severely limits the development of solid electrolytes. In this study, we synthesize cubic phase Li6.4La3Zr1.4Ta0.6O12 (LLZTO) using a secondary sintering method. In addition, a thin aluminum nitride (AlN) layer is introduced between t

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Ji, Xiaoyu, Yiruo Zhang, Mengxue Cao, et al. "Advanced inorganic/polymer hybrid electrolytes for all-solid-state lithium batteries." Journal of Advanced Ceramics 11, no. 6 (2022): 835–61. http://dx.doi.org/10.1007/s40145-022-0580-8.

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AbstractSolid-state batteries have become a frontrunner in humankind’s pursuit of safe and stable energy storage systems with high energy and power density. Electrolyte materials, currently, seem to be the Achilles’ heel of solid-state batteries due to the slow kinetics and poor interfacial wetting. Combining the merits of solid inorganic electrolytes (SIEs) and solid polymer electrolytes (SPEs), inorganic/polymer hybrid electrolytes (IPHEs) integrate improved ionic conductivity, great interfacial compatibility, wide electrochemical stability window, and high mechanical toughness and flexibili

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Teshima, Katsuya, Hajime Wagata, and Shuji Oishi. "All-Crystal-State Lithium-Ion Batteries: Innovation Inspired by Novel Flux Coating Method." Additional Conferences (Device Packaging, HiTEC, HiTEN, and CICMT) 2013, CICMT (2013): 000187–91. http://dx.doi.org/10.4071/cicmt-wp41.

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All-solid-state lithium-ion rechargeable batteries (LIBs) consisting of solid electrolyte materials have attracted a number of research interests because no use of organic liquid electrolyte increases packaging density and intrinsic safety of LIB, which contribute the development on environmentally-friendly automobiles such as electric vehicle (EV), hybrid vehicle (HV), and plug-in hybrid vehicle (HEV), in addition to efficient utilization of electric energy in smart grid. Among various solid electrolytes, inorganic electrolyte materials have achieved relatively high lithium-ion conductivity a

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Tronstad, Zachary, and Bryan D. McCloskey. "Exploring the Interaction between EC and Ta-Doped LLZO." ECS Meeting Abstracts MA2024-02, no. 8 (2024): 1227. https://doi.org/10.1149/ma2024-0281227mtgabs.

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Solid-state electrolytes are a primary strategy for unlocking the use of lithium metal anodes and enabling batteries with higher energy density.1 Garnet-type Li7La3Zr2O12 (LLZO) is a leading candidate among ceramic-type materials due to its high ionic conductivity and kinetic stability against lithium metal.2 However, LLZO is air sensitive, spontaneously reacting with CO2 in ambient air to form lithium carbonate layers.3–6 Additionally, we have recently collected evidence, as described below, that suggests that LLZO may even be reactive towards ethylene carbonate (EC), a key liquid electrolyte

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Peng, Shihao, Jiakun Luo, Wenwen Liu, Xiaolong He, and Fang Xie. "Enhanced Capacity Retention of Li3V2(PO4)3-Cathode-Based Lithium Metal Battery Using SiO2-Scaffold-Confined Ionic Liquid as Hybrid Solid-State Electrolyte." Molecules 28, no. 13 (2023): 4896. http://dx.doi.org/10.3390/molecules28134896.

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Li3V2(PO4)3 (LVP) is one of the candidates for high-energy-density cathode materials matching lithium metal batteries due to its high operating voltage and theoretical capacity. However, the inevitable side reactions of LVP with a traditional liquid-state electrolyte under high voltage, as well as the uncontrollable growth of lithium dendrites, worsen the cycling performance. Herein, a hybrid solid-state electrolyte is prepared by the confinement of a lithium-containing ionic liquid with a mesoporous SiO2 scaffold, and used for a LVP-cathode-based lithium metal battery. The solid-state electro

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Kirchberger, Anna Maria, Patrick Walke, and Tom Nilges. "Effect of Nanostructured Inorganic Ceramic Filler on Poly(ethylene oxide)-Based Solid Polymer Electrolytes." ECS Meeting Abstracts MA2023-01, no. 6 (2023): 991. http://dx.doi.org/10.1149/ma2023-016991mtgabs.

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In view of the ongoing changes in energy science and technology, the possibilities of energy storage are getting increasingly important. In particular, storing electrical energy is more complex than with fossil fuels. Lithium-Ion batteries are the most commonly used media for energy storage, but they also have some safety-related problems: toxic decomposition products can leak out and the devices can catch fire. Research is underway to find alternatives to minimize this potential hazards. Great improvements in safety matters can be achieved by replacing liquid electrolytes with ceramic/polymer

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Wang, Linsheng. "Development of Novel High Li-Ion Conductivity Hybrid Electrolytes of Li10GeP2S12 (LGPS) and Li6.6La3Zr1.6Sb0.4O12 (LLZSO) for Advanced All-Solid-State Batteries." Oxygen 1, no. 1 (2021): 16–21. http://dx.doi.org/10.3390/oxygen1010003.

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A lithium superionic conductor of Li10GeP2S12 that exhibits the highest lithium ionic conductivity among the sulfide electrolytes and the most promising oxide electrolytes, namely, Li6.6La3Sr0.06Zr1.6Sb0.4O12 and Li6.6La3Zr1.6Sb0.4O12, are successfully synthesized. Novel hybrid electrolytes with a weight ratio of Li6.6La3Zr1.6Sb0.4O12 to Li10GeP2S12 from 1/1 to 1/3 with the higher Li-ion conductivity than that of the pure Li10GeP2S12 electrolyte are developed for the fabrication of the advanced all-solid-state Li batteries.

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Muñoz, Bianca K., Jorge Lozano, María Sánchez, and Alejandro Ureña. "Hybrid Solid Polymer Electrolytes Based on Epoxy Resins, Ionic Liquid, and Ceramic Nanoparticles for Structural Applications." Polymers 16, no. 14 (2024): 2048. http://dx.doi.org/10.3390/polym16142048.

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Solid polymer electrolytes (SPE) and composite polymer electrolytes (CPE) serve as crucial components in all-solid-state energy storage devices. Structural batteries and supercapacitors present a promising alternative for electric vehicles, integrating structural functionality with energy storage capability. However, despite their potential, these applications are hampered by various challenges, particularly in the realm of developing new solid polymer electrolytes that require more investigation. In this study, novel solid polymer electrolytes and composite polymer electrolytes were synthesiz

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Gerstenberg, Jessica, Dominik Steckermeier, Arno Kwade, and Peter Michalowski. "Effect of Mixing Intensity on Electrochemical Performance of Oxide/Sulfide Composite Electrolytes." Batteries 10, no. 3 (2024): 95. http://dx.doi.org/10.3390/batteries10030095.

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Despite the variety of solid electrolytes available, no single solid electrolyte has been found that meets all the requirements of the successor technology of lithium-ion batteries in an optimum way. However, composite hybrid electrolytes that combine the desired properties such as high ionic conductivity or stability against lithium are promising. The addition of conductive oxide fillers to sulfide solid electrolytes has been reported to increase ionic conductivity and improve stability relative to the individual electrolytes, but the influence of the mixing process to create composite electr

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Zhang, L. X., Y. Z. Li, L. W. Shi, et al. "Electrospun Polyethylene Oxide (PEO)-Based Composite polymeric nanofiber electrolyte for Li-Metal Battery." Journal of Physics: Conference Series 2353, no. 1 (2022): 012004. http://dx.doi.org/10.1088/1742-6596/2353/1/012004.

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Abstract Composite polymer electrolytes (CPEs) based on polyethylene oxide (PEO) offer manufacturing feasibility and outstanding mechanical flexibility. However, the low ionic conductivity of the CPEs at room temperature, as well as the poor mechanical properties, have hindered their commercialization. In this work, Solid-state electrolytes based on polyethylene oxide (PEO) with and without fumed SiO2 (FS) nanoparticles are prepared by electrostatic spinning process. The as-spun PEO hybrid nanofiber electrolyte with 6.85 wt% FS has a relatively high lithium ion conductivity and electrochemical

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Foran, Gabrielle, Nina Verdier, David Lepage, Cédric Malveau, Nicolas Dupré, and Mickaël Dollé. "Use of Solid-State NMR Spectroscopy for the Characterization of Molecular Structure and Dynamics in Solid Polymer and Hybrid Electrolytes." Polymers 13, no. 8 (2021): 1207. http://dx.doi.org/10.3390/polym13081207.

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Solid-state NMR spectroscopy is an established experimental technique which is used for the characterization of structural and dynamic properties of materials in their native state. Many types of solid-state NMR experiments have been used to characterize both lithium-based and sodium-based solid polymer and polymer–ceramic hybrid electrolyte materials. This review describes several solid-state NMR experiments that are commonly employed in the analysis of these systems: pulse field gradient NMR, electrophoretic NMR, variable temperature T1 relaxation, T2 relaxation and linewidth analysis, excha

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Zhang, Mi, A.-Man Zhang, Yifa Chen, et al. "Polyoxovanadate-polymer hybrid electrolyte in solid state batteries." Energy Storage Materials 29 (August 2020): 172–81. http://dx.doi.org/10.1016/j.ensm.2020.04.017.

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Shah, Vaidik, and Yong Lak Joo. "Rationally Designed in-Situ Gelled Polymer-Ceramic Hybrid Electrolyte Enables Superior Performance and Stability in Quasi-Solid-State Lithium-Sulfur Batteries." ECS Meeting Abstracts MA2023-02, no. 4 (2023): 535. http://dx.doi.org/10.1149/ma2023-024535mtgabs.

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Despite boasting giant leaps in performance improvement over the years, the current commercial standard, Li-ion batteries, are fast approaching their theoretical limits. Meanwhile, Lithium-Sulfur (Li-S) batteries offering ultra-high theoretical energy density (～2600 Whkg-1), cost-effectiveness, and nontoxicity are being seen as promising alternatives. Despite their plentiful advantages, the practicality of Li-S batteries has been largely stymied by several challenges: a) deleterious polysulfide dissolution and ‘shuttle effect’, b) significant volume change of S cathodes during cycling, c) safe

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Okos, Alexandru, Cristina Florentina Ciobota, Adrian Mihail Motoc, and Radu-Robert Piticescu. "Review on Synthesis and Properties of Lithium Lanthanum Titanate." Materials 16, no. 22 (2023): 7088. http://dx.doi.org/10.3390/ma16227088.

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The rapid development of portable electronic devices and the efforts to find alternatives to fossil fuels have triggered the rapid development of battery technology. The conventional lithium-ion batteries have reached a high degree of sophistication. However, improvements related to specific capacity, charge rate, safety and sustainability are still required. Solid state batteries try to answer these demands by replacing the organic electrolyte of the standard battery with a solid (crystalline, but also polymer and hybrid) electrolyte. One of the most promising solid electrolytes is Li3xLa2/3−

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Lee, Yan Ying, and Andre Weber. "Harmonization of Testing Procedures for All Solid State Batteries." ECS Meeting Abstracts MA2023-02, no. 2 (2023): 340. http://dx.doi.org/10.1149/ma2023-022340mtgabs.

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All Solid State Batteries (ASSBs) with lithium-ion based conducting solid state electrolytes are considered the next generation high performance batteries. They enable high power densities due to their single ion conducting solid electrolyte, eliminating salt concentration gradients and related polarization losses in the cell, and ensuring an unrivalled level of safety due to their non-combustibility. Currently, a variety of ASSBs based on different solid state electrolytes such as polymers, thiophosphates, oxides and combinations thereof are being developed. One general problem with ASSBs is

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Yan, Shuo, Chae-Ho Yim, Ali Merati, Elena A. Baranova, Yaser Abu-Lebdeh, and Arnaud Weck. "Interfacial Challenge for Solid-State Lithium Batteries- Liquid Addition." ECS Meeting Abstracts MA2023-01, no. 6 (2023): 1010. http://dx.doi.org/10.1149/ma2023-0161010mtgabs.

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All solid-state lithium batteries with garnet electrolytes (Li7La3Zr2O12, LLZO) are promising energy storage devices that have gained increasing attention due to their huge potential towards non-flammability and higher energy density. However, reported solid-state lithium batteries cannot achieve the projected energy density (> 500 Wh/kg at the cell level) mainly due to insufficient contact and poor compatibility between LLZO and electrodes. The use of liquid electrolytes in small quantities has been suggested as a component in the quasi-solid hybrid electrolytes to address these two issues

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Kim, Jae-Kwang, Johan Scheers, Tae Joo Park, and Youngsik Kim. "Superior Ion-Conducting Hybrid Solid Electrolyte for All-Solid-State Batteries." ChemSusChem 8, no. 4 (2014): 636–41. http://dx.doi.org/10.1002/cssc.201402969.

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Tsurumaki, Akiko, Rossella Rettaroli, Lucia Mazzapioda, and Maria Assunta Navarra. "Inorganic–Organic Hybrid Electrolytes Based on Al-Doped Li7La3Zr2O12 and Ionic Liquids." Applied Sciences 12, no. 14 (2022): 7318. http://dx.doi.org/10.3390/app12147318.

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Organic–inorganic hybrid electrolytes based on Al-doped Li7La3Zr2O12 (LLZO) and two different ionic liquids (ILs), namely N-ethoxyethyl-N-methylpiperidinium bis(fluorosulfonyl)imide (FSI IL) and N-ethoxyethyl-N-methylpiperidinium difluoro(oxalato)borate (DFOB IL), were prepared with the aim of improvement of inherent flexibilities of inorganic solid electrolytes. The composites were evaluated in terms of thermal, spectroscopical, and electrochemical properties. In the impedance spectra of LLZO composites with 15 wt% ILs, a semi-circle due to grain boundary resistances was not observed. With th

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Kim, Hyun Woo, Palanisamy Manikandan, Young Jun Lim, Jin Hong Kim, Sang-cheol Nam, and Youngsik Kim. "Hybrid solid electrolyte with the combination of Li7La3Zr2O12 ceramic and ionic liquid for high voltage pseudo-solid-state Li-ion batteries." Journal of Materials Chemistry A 4, no. 43 (2016): 17025–32. http://dx.doi.org/10.1039/c6ta07268b.

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Concerning the safety aspects of high-voltage Li-ion batteries, a pelletized hybrid solid electrolyte (HSE) was prepared by blending Li<sub>7</sub>La<sub>3</sub>Zr<sub>2</sub>O<sub>12</sub> (LLZO) ceramic particles and an ionic liquid electrolyte (ILE) for use in pseudo-solid-state Li-ion batteries.

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Tang, Jiantao, Leidanyang Wang, Longzhen You, et al. "Effect of Organic Electrolyte on the Performance of Solid Electrolyte for Solid–Liquid Hybrid Lithium Batteries." ACS Applied Materials & Interfaces 13, no. 2 (2021): 2685–93. http://dx.doi.org/10.1021/acsami.0c19671.

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Luo, Wen-Bin, Shu-Lei Chou, Jia-Zhao Wang, Yong-Mook Kang, Yu-Chun Zhai, and Hua-Kun Liu. "A hybrid gel–solid-state polymer electrolyte for long-life lithium oxygen batteries." Chemical Communications 51, no. 39 (2015): 8269–72. http://dx.doi.org/10.1039/c5cc01857a.

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A gel–solid state polymer electrolyte has been used as the separator and an electrolyte for lithium oxygen batteries, which can not only avoid electrolyte evaporation but also protect the lithium metal anode during reactions over long-term cycling.

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