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1
Li, Chong, Jing Li, Oleg Dubovik, Zhao-Cheng Zeng, and Yuk L. Yung. "Impact of Aerosol Vertical Distribution on Aerosol Optical Depth Retrieval from Passive Satellite Sensors." Remote Sensing 12, no. 9 (2020): 1524. http://dx.doi.org/10.3390/rs12091524.
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When retrieving Aerosol Optical Depth (AOD) from passive satellite sensors, the vertical distribution of aerosols usually needs to be assumed, potentially causing uncertainties in the retrievals. In this study, we use the Moderate Resolution Spectroradiometer (MODIS) and Visible Infrared Imaging Radiometer Suite (VIIRS) sensors as examples to investigate the impact of aerosol vertical distribution on AOD retrievals. A series of sensitivity experiments was conducted using radiative transfer models with different aerosol profiles and surface conditions. Assuming a 0.2 AOD, we found that the AOD retrieval error is the most sensitive to the vertical distribution of absorbing aerosols; a −1 km error in aerosol scale height can lead to a ~30% AOD retrieval error. Moreover, for this aerosol type, ignoring the existence of the boundary layer can further result in a ~10% AOD retrieval error. The differences in the vertical distribution of scattering and absorbing aerosols within the same column may also cause −15% (scattering aerosols above absorbing aerosols) to 15% (scattering aerosols below absorbing aerosols) errors. Surface reflectance also plays an important role in affecting the AOD retrieval error, with higher errors over brighter surfaces in general. The physical mechanism associated with the AOD retrieval errors is also discussed. Finally, by replacing the default exponential profile with the observed aerosol vertical profile by a micro-pulse lidar at the Beijing-PKU site in the VIIRS retrieval algorithm, the retrieved AOD shows a much better agreement with surface observations, with the correlation coefficient increased from 0.63 to 0.83 and bias decreased from 0.15 to 0.03. Our study highlights the importance of aerosol vertical profile assumption in satellite AOD retrievals, and indicates that considering more realistic profiles can help reduce the uncertainties.
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Loughman, Robert, Pawan K. Bhartia, Zhong Chen, Philippe Xu, Ernest Nyaku, and Ghassan Taha. "The Ozone Mapping and Profiler Suite (OMPS) Limb Profiler (LP) Version 1 aerosol extinction retrieval algorithm: theoretical basis." Atmospheric Measurement Techniques 11, no. 5 (2018): 2633–51. http://dx.doi.org/10.5194/amt-11-2633-2018.
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Abstract. The theoretical basis of the Ozone Mapping and Profiler Suite (OMPS) Limb Profiler (LP) Version 1 aerosol extinction retrieval algorithm is presented. The algorithm uses an assumed bimodal lognormal aerosol size distribution to retrieve aerosol extinction profiles at 675 nm from OMPS LP radiance measurements. A first-guess aerosol extinction profile is updated by iteration using the Chahine nonlinear relaxation method, based on comparisons between the measured radiance profile at 675 nm and the radiance profile calculated by the Gauss–Seidel limb-scattering (GSLS) radiative transfer model for a spherical-shell atmosphere. This algorithm is discussed in the context of previous limb-scattering aerosol extinction retrieval algorithms, and the most significant error sources are enumerated. The retrieval algorithm is limited primarily by uncertainty about the aerosol phase function. Horizontal variations in aerosol extinction, which violate the spherical-shell atmosphere assumed in the version 1 algorithm, may also limit the quality of the retrieved aerosol extinction profiles significantly.
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Taha, G., D. F. Rault, R. P. Loughman, A. E. Bourassa, and C. von Savigny. "SCIAMACHY stratospheric aerosol extinction profile retrieval." Atmospheric Measurement Techniques Discussions 3, no. 6 (2010): 5343–74. http://dx.doi.org/10.5194/amtd-3-5343-2010.
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Abstract. The Ozone Mapper and Profiler Suite Limp Profiler (OMPS/LP) algorithm is used to retrieve ozone and aerosol profiles using a series of 120 SCIAMACHY limb measurements collocated with SAGE II solar occultation events. The primary goal of the study is to ascertain the capability of the OMPS/LP retrieval algorithm to accurately retrieve the vertical distribution of stratospheric aerosol extinction coefficient so as to better account for aerosol effects in the ozone profiling retrieval process. Using simulated radiances, we show that the aerosol extinction coefficient can be retrieved from limb scatter measurements within 5% and a standard deviation better than 15%, which is more than sufficient to improve the OMPS/LP ozone products to be used as Environmental Data Records. We also illustrate the ability of SCIAMACHY limb measurements to retrieve stratospheric aerosol profiles with accuracy comparable to other instruments. The retrieved aerosol profiles agree with collocated SAGE II measurements on average to within 25%, with a standard deviation of 35%.
4
Geddes, A., and H. Bösch. "Aerosol profile information from high resolution oxygen A-Band measurements from space." Atmospheric Measurement Techniques Discussions 7, no. 6 (2014): 6021–63. http://dx.doi.org/10.5194/amtd-7-6021-2014.
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Abstract. Aerosols are an important factor of the Earth climatic system and they play a key role for air quality and public health. Observations of the oxygen A-Band at 760 nm can provide information on the vertical distribution of aerosols from passive satellite sensors, that can be of great interest for operational monitoring applications with high coverage if the aerosol information is obtained with sufficient precision, accuracy and vertical resolution. To address this issue, retrieval simulations of the aerosol vertical profile retrieval from O2 A Band observations by GOSAT, the upcoming OCO-2 and Sentinel 5-P mission and the proposed CarbonSat mission have been carried out. Precise retrievals of AOD within the boundary layer were found to favour low resolution, high SNR instruments such as Sentinel-5 P, whereas higher resolution instruments such as OCO-2 showed greater performance at higher altitudes and in information content above the boundary layer. Accurate retrievals of the AOD in the 0–2 km range appears difficult from all studied instruments and the retrieval errors typically exceed a value of 0.05. Constraining the surface albedo is a promising and effective way of improving the retrieval of aerosol, but the required level of a priori knowledge is very high. Due to the limited information content of the aerosol profile retrieval, the use of a parameterised aerosol distribution has been assessed and we show that the AOD and height of an aerosol layer can be retrieved well if the aerosol layer is uplifted to the free troposphere but errors are often large for aerosol layers in the boundary layer. Additional errors will be introduced by incorrect assumptions on surface pressure and aerosol type which can both bias retrieved AOD and height by up to 40%. We conclude the aerosol profile retrievals from O2 A Band using existing or upcoming satellite sensors will only provide limited information on aerosols in the boundary layer but such observations can be of great value for observing and mapping aerosol plumes in the free troposphere.
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Geddes, A., and H. Bösch. "Tropospheric aerosol profile information from high-resolution oxygen A-band measurements from space." Atmospheric Measurement Techniques 8, no. 2 (2015): 859–74. http://dx.doi.org/10.5194/amt-8-859-2015.
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Abstract. Aerosols are an important factor in the Earth climatic system and they play a key role in air quality and public health. Observations of the oxygen A-band at 760 nm can provide information on the vertical distribution of aerosols from passive satellite sensors that can be of great interest for operational monitoring applications with high spatial coverage if the aerosol information is obtained with sufficient precision, accuracy and vertical resolution. To address this issue, retrieval simulations of the aerosol vertical profile retrieval from O2 A-band observations by GOSAT, the upcoming Orbiting Carbon Observatory-2 (OCO-2) and Sentinel 5-P missions, and the proposed CarbonSat mission have been carried out. Precise retrievals of aerosol optical depth (AOD) within the boundary layer were found to favour low-resolution, high signal-to-noise instruments such as Sentinel-5 P, whereas higher-resolution instruments such as OCO-2 showed greater performance at higher altitudes and in information content above the boundary layer. Retrieval of the AOD in the 0–2 km range with precision appears difficult from all studied instruments and the retrieval errors typically exceed a value of 0.05 for AODs up to 0.3. Constraining the surface albedo is a promising and effective way of improving the retrieval of aerosol, but the accuracy of the required prior knowledge is very high. Due to the limited information content of the aerosol profile retrieval, the use of a parameterised aerosol distribution is assessed, and we show that the AOD and height of an aerosol layer can be retrieved well if the aerosol layer is uplifted to the free troposphere; however, errors are often large for aerosol layers in the boundary layer. Additional errors are introduced by incorrect assumptions on surface pressure and aerosol mixture, which can both bias retrieved AOD and height by up to 45%. In addition, assumptions of the boundary layer temperature are found to yield an additional error of up to 8%. We conclude that the aerosol profile retrievals from O2 A-band using existing or upcoming satellite sensors will only provide limited information on aerosols in the boundary layer but such observations can be of great value for observing and mapping aerosol plumes in the free troposphere.
6
Lin, J. T., R. V. Martin, K. F. Boersma, et al. "Retrieving tropospheric nitrogen dioxide over China from the Ozone Monitoring Instrument: effects of aerosols, surface reflectance anisotropy and vertical profile of nitrogen dioxide." Atmospheric Chemistry and Physics Discussions 13, no. 8 (2013): 21203–57. http://dx.doi.org/10.5194/acpd-13-21203-2013.
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Abstract. Retrievals of tropospheric nitrogen dioxide (NO2) from the Ozone Monitoring Instrument (OMI) are subject to errors in the treatments of aerosols, surface reflectance anisotropy, and vertical profile of NO2. Here we quantify the influences over China via an improved retrieval process. We explicitly account for aerosol optical effects (simulated by nested GEOS-Chem at 0.667° lon × 0.5° lat and constrained by aerosol measurements), surface reflectance anisotropy, and high-resolution vertical profiles of NO2 (simulated by GEOS-Chem). Prior to the NO2 retrieval, we derive the cloud information using consistent ancillary assumptions. We compare our retrieval to the widely used DOMINO v2 product, using as reference MAX-DOAS measurements at three urban/suburban sites in East China and focusing the analysis on the 127 OMI pixels (in 30 days) closest to the MAX-DOAS sites. We find that our retrieval reduces the interference of aerosols on the retrieved cloud properties, thus enhancing the number of valid OMI pixels by about 25%. Compared to DOMINO v2, our retrieval improves the correlation with the MAX-DOAS data in the day-to-day variability of NO2 (R2 = 0.96 vs. 0.72). Our retrieved NO2 columns are about 50% of the MAX-DOAS data on average. This reflects the inevitable spatial inconsistency between the two types of measurement, uncertainties in MAX-DOAS data, and residual uncertainties in our OMI retrievals related to aerosols and vertical profile of NO2. Through a series of tests, we find that excluding aerosol scattering/absorption can either increase or decrease the retrieved NO2, with a mean absolute difference by about 20%. Concentrating aerosols at the boundary layer top enhances the retrieved NO2 by 8% on average with a mean absolute difference by 23%. The aerosol perturbations also affect nonlinearly the retrieved cloud fraction and particularly cloud pressure. Employing various surface albedo datasets alters the retrieved NO2 by 0–7% on average. The retrieved NO2 columns increase when the NO2 profiles are taken from MAX-DOAS retrievals (by 20% on average) or TM4 simulations (by 10%) instead of GEOS-Chem simulations. Our findings are also relevant to retrievals of other pollutants (e.g., sulfur dioxide, formaldehyde, glyoxal) from UV-vis backscatter satellite instruments.
7
Lin, J. T., R. V. Martin, K. F. Boersma, et al. "Retrieving tropospheric nitrogen dioxide from the Ozone Monitoring Instrument: effects of aerosols, surface reflectance anisotropy, and vertical profile of nitrogen dioxide." Atmospheric Chemistry and Physics 14, no. 3 (2014): 1441–61. http://dx.doi.org/10.5194/acp-14-1441-2014.
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Abstract. Retrievals of tropospheric nitrogen dioxide (NO2) from the Ozone Monitoring Instrument (OMI) are subject to errors in the treatments of aerosols, surface reflectance anisotropy, and vertical profile of NO2. Here we quantify the influences over China via an improved retrieval process. We explicitly account for aerosol optical effects (simulated by nested GEOS-Chem at 0.667° long. × 0.5° lat. and constrained by aerosol measurements), surface reflectance anisotropy, and high-resolution vertical profiles of NO2 (simulated by GEOS-Chem). Prior to the NO2 retrieval, we derive the cloud information using consistent ancillary assumptions. We compare our retrieval to the widely used DOMINO v2 product, using MAX-DOAS measurements at three urban/suburban sites in East China as reference and focusing the analysis on the 127 OMI pixels (in 30 days) closest to the MAX-DOAS sites. We find that our retrieval reduces the interference of aerosols on the retrieved cloud properties, thus enhancing the number of valid OMI pixels by about 25%. Compared to DOMINO v2, our retrieval better captures the day-to-day variability in MAX-DOAS NO2 data (R2 = 0.96 versus 0.72), due to pixel-specific radiative transfer calculations rather than the use of a look-up table, explicit inclusion of aerosols, and consideration of surface reflectance anisotropy. Our retrieved NO2 columns are 54% of the MAX-DOAS data on average, reflecting the inevitable spatial inconsistency between the two types of measurement, errors in MAX-DOAS data, and uncertainties in our OMI retrieval related to aerosols and vertical profile of NO2. Sensitivity tests show that excluding aerosol optical effects can either increase or decrease the retrieved NO2 for individual OMI pixels with an average increase by 14%. Excluding aerosols also complexly affects the retrievals of cloud fraction and particularly cloud pressure. Employing various surface albedo data sets slightly affects the retrieved NO2 on average (within 10%). The retrieved NO2 columns increase when the NO2 profiles are taken from MAX-DOAS retrievals (by 19% on average) or TM4 simulations (by 13%) instead of GEOS-Chem simulations. Our findings are also relevant to retrievals of other pollutants (e.g., sulfur dioxide, ormaldehyde, glyoxal) from UV–visible backscatter satellite instruments.
8
Ernst, F., C. von Savigny, A. Rozanov, et al. "Global stratospheric aerosol extinction profile retrievals from SCIAMACHY limb-scatter observations." Atmospheric Measurement Techniques Discussions 5, no. 4 (2012): 5993–6035. http://dx.doi.org/10.5194/amtd-5-5993-2012.
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Abstract. Stratospheric aerosol extinction profiles are retrieved from SCIAMACHY/Envisat limb-scatter observations in the visible spectral range. The retrieval algorithm is based on a colour-index approach using the normalized limb-radiance profiles at 470 nm and 750 nm wavelength. The optimal estimation approach in combination with the radiative transfer model SCIATRAN is employed for the retrievals. This study presents a detailed description of the retrieval algorithm, and a sensitivity analysis investigating the impact of the most important parameters that affect the aerosol extinction profile retrieval accuracy. It is found that the parameter with the largest impact is surface albedo, particularly for SCIAMACHY observations in the Southern Hemisphere where the error in stratospheric aerosol extinction can be up to 50% if the surface albedo is not well known. The effect of errors in the assumed ozone and neutral density profiles on the aerosol profile retrievals is with generally less than 6% relatively small. The aerosol extinction profiles retrieved from SCIAMACHY are compared with co-located SAGE II solar occultation measurements of stratospheric aerosol extinction during the period 2003–2005. The mean aerosol extinction profiles averaged over all co-locations agree to within 20% between 15 and 35 km altitude. However, larger differences are observed at specific latitudes.
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Taha, G., D. F. Rault, R. P. Loughman, A. E. Bourassa, and C. von Savigny. "SCIAMACHY stratospheric aerosol extinction profile retrieval using the OMPS/LP algorithm." Atmospheric Measurement Techniques 4, no. 3 (2011): 547–56. http://dx.doi.org/10.5194/amt-4-547-2011.
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Abstract. The Ozone Mapper and Profiler Suite, Limp Profiler (OMPS/LP) algorithm is used to retrieve ozone concentration and aerosol extinction profiles using a series of 120 SCIAMACHY limb measurements collocated with SAGE II solar occultation events. The primary goal of the study is to ascertain the capability of the OMPS/LP retrieval algorithm to accurately retrieve the vertical distribution of stratospheric aerosol extinction coefficient so as to better account for aerosol effects in the ozone profiling retrieval process. Using simulated radiances, we show that the aerosol extinction coefficient can be retrieved from limb scatter measurements within 5% and a standard deviation better than 15%, which is more than sufficient to improve the OMPS/LP ozone products to be used as Environmental Data Records. We also illustrate the ability of SCIAMACHY limb measurements to retrieve stratospheric aerosol extinction profiles with accuracy comparable to other instruments. The retrieved aerosol extinction profiles agree with collocated SAGE II measurements on average to within 25%, with a standard deviation of 35%.
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Sanders, A. F. J., J. F. de Haan, M. Sneep, et al. "Evaluation of the operational Aerosol Layer Height retrieval algorithm for Sentinel-5 Precursor: application to O<sub>2</sub> A band observations from GOME-2A." Atmospheric Measurement Techniques 8, no. 11 (2015): 4947–77. http://dx.doi.org/10.5194/amt-8-4947-2015.
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Abstract. An algorithm setup for the operational Aerosol Layer Height product for TROPOMI on the Sentinel-5 Precursor mission is described and discussed, applied to GOME-2A data, and evaluated with lidar measurements. The algorithm makes a spectral fit of reflectance at the O2 A band in the near-infrared and the fit window runs from 758 to 770 nm. The aerosol profile is parameterised by a scattering layer with constant aerosol volume extinction coefficient and aerosol single scattering albedo and with a fixed pressure thickness. The algorithm's target parameter is the height of this layer. In this paper, we apply the algorithm to observations from GOME-2A in a number of systematic and extensive case studies, and we compare retrieved aerosol layer heights with lidar measurements. Aerosol scenes cover various aerosol types, both elevated and boundary layer aerosols, and land and sea surfaces. The aerosol optical thicknesses for these scenes are relatively moderate. Retrieval experiments with GOME-2A spectra are used to investigate various sensitivities, in which particular attention is given to the role of the surface albedo. From retrieval simulations with the single-layer model, we learn that the surface albedo should be a fit parameter when retrieving aerosol layer height from the O2 A band. Current uncertainties in surface albedo climatologies cause biases and non-convergences when the surface albedo is fixed in the retrieval. Biases disappear and convergence improves when the surface albedo is fitted, while precision of retrieved aerosol layer pressure is still largely within requirement levels. Moreover, we show that fitting the surface albedo helps to ameliorate biases in retrieved aerosol layer height when the assumed aerosol model is inaccurate. Subsequent retrievals with GOME-2A spectra confirm that convergence is better when the surface albedo is retrieved simultaneously with aerosol parameters. However, retrieved aerosol layer pressures are systematically low (i.e., layer high in the atmosphere) to the extent that retrieved values no longer realistically represent actual extinction profiles. When the surface albedo is fixed in retrievals with GOME-2A spectra, convergence deteriorates as expected, but retrieved aerosol layer pressures become much higher (i.e., layer lower in atmosphere). The comparison with lidar measurements indicates that retrieved aerosol layer heights are indeed representative of the underlying profile in that case. Finally, subsequent retrieval simulations with two-layer aerosol profiles show that a model error in the assumed profile (two layers in the simulation but only one in the retrieval) is partly absorbed by the surface albedo when this parameter is fitted. This is expected in view of the correlations between errors in fit parameters and the effect is relatively small for elevated layers (less than 100 hPa). If one of the scattering layers is near the surface (boundary layer aerosols), the effect becomes surprisingly large, in such a way that the retrieved height of the single layer is above the two-layer profile. Furthermore, we find that the retrieval solution, once retrieval converges, hardly depends on the starting values for the fit. Sensitivity experiments with GOME-2A spectra also show that aerosol layer height is indeed relatively robust against inaccuracies in the assumed aerosol model, even when the surface albedo is not fitted. We show spectral fit residuals, which can be used for further investigations. Fit residuals may be partly explained by spectroscopic uncertainties, which is suggested by an experiment showing the improvement of convergence when the absorption cross section is scaled in agreement with Butz et al. (2013) and Crisp et al. (2012), and a temperature offset to the a priori ECMWF temperature profile is fitted. Retrieved temperature offsets are always negative and quite large (ranging between −4 and −8 K), which is not expected if temperature offsets absorb remaining inaccuracies in meteorological data. Other sensitivity experiments investigate fitting of stray light and fluorescence emissions. We find negative radiance offsets and negative fluorescence emissions, also for non-vegetated areas, but from the results it is not clear whether fitting these parameters improves the retrieval. Based on the present results, the operational baseline for the Aerosol Layer Height product currently will not fit the surface albedo. The product will be particularly suited for elevated, optically thick aerosol layers. In addition to its scientific value in climate research, anticipated applications of the product for TROPOMI are providing aerosol height information for aviation safety and improving interpretation of the Absorbing Aerosol Index.
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Sanders, A. F. J., J. F. de Haan, M. Sneep, et al. "Evaluation of the operational Aerosol Layer Height retrieval algorithm for Sentinel-5 Precursor: application to O<sub>2</sub> A band observations from GOME-2A." Atmospheric Measurement Techniques Discussions 8, no. 6 (2015): 6045–118. http://dx.doi.org/10.5194/amtd-8-6045-2015.
Full textAbstract:
Abstract. An algorithm setup for the operational Aerosol Layer Height product for TROPOMI on the Sentinel-5 Precursor mission is described and discussed, applied to GOME-2A data, and evaluated with lidar measurements. The algorithm makes a spectral fit of reflectance at the O2 A band in the near-infrared and the fit window runs from 758 to 770 nm. The aerosol profile is parameterized by a scattering layer with constant aerosol volume extinction coefficient and aerosol single scattering albedo and with a fixed pressure thickness. The algorithm's target parameter is the height of this layer. In this paper, we apply the algorithm to observations from GOME-2A in a number of systematic and extensive case studies and we compare retrieved aerosol layer heights with lidar measurements. Aerosol scenes cover various aerosol types, both elevated and boundary layer aerosols, and land and sea surfaces. The aerosol optical thicknesses for these scenes are relatively moderate. Retrieval experiments with GOME-2A spectra are used to investigate various sensitivities, in which particular attention is given to the role of the surface albedo. From retrieval simulations with the single-layer model, we learn that the surface albedo should be a fit parameter when retrieving aerosol layer height from the O2 A band. Current uncertainties in surface albedo climatologies cause biases and non-convergences when the surface albedo is fixed in the retrieval. Biases disappear and convergence improves when the surface albedo is fitted, while precision of retrieved aerosol layer pressure is still largely within requirement levels. Moreover, we show that fitting the surface albedo helps to ameliorate biases in retrieved aerosol layer height when the assumed aerosol model is inaccurate. Subsequent retrievals with GOME-2A spectra confirm that convergence is better when the surface albedo is retrieved simultaneously with aerosol parameters. However, retrieved aerosol layer pressures are systematically low (i.e., layer high in the atmosphere) to the extent that retrieved values are not realistically representing actual extinction profiles anymore. When the surface albedo is fixed in retrievals with GOME-2A spectra, convergence deteriorates as expected, but retrieved aerosol layer pressures become much higher (i.e., layer lower in atmosphere). The comparison with lidar measurements indicates that retrieved aerosol layer heights are indeed representative of the underlying profile in that case. Finally, subsequent retrieval simulations with two-layer aerosol profiles show that a model error in the assumed profile (two layers in the simulation but only one in the retrieval) is partly absorbed by the surface albedo when this parameter is fitted. This is expected in view of the correlations between errors in fit parameters and the effect is relatively small for elevated layers (less than 100 hPa). In case one of the scattering layers is near the surface (boundary layer aerosols), the effect becomes surprisingly large such that the retrieved height of the single layer is above the two-layer profile. Furthermore, we find that the retrieval solution, once retrieval converges, hardly depends on the starting values for the fit. Sensitivity experiments with GOME-2A spectra also show that aerosol layer height is indeed relatively robust against inaccuracies in the assumed aerosol model, even when the surface albedo is not fitted. We show spectral fit residuals, which can be used for further investigations. Fit residuals may be partly explained by spectroscopic uncertainties, which is suggested by an experiment showing the improvement of convergence when the absorption cross section is scaled in agreement with Butz et al. (2012) and Crisp et al. (2012) and a temperature offset to the a priori ECMWF temperature profile is fitted. Retrieved temperature offsets are always negative and quite large (ranging between −4 and −8 K), which is not expected if temperature offsets absorb remaining inaccuracies in meteorological data. Other sensitivity experiments investigate fitting of stray light and fluorescence emissions. We find negative radiance offsets and negative fluorescence emissions, also for non-vegetated areas, but from the results it is not clear whether fitting these parameters improves the retrieval. Based on the present results, the operational baseline for the Aerosol Layer Height product currently will not fit the surface albedo. The product will be particularly suited for elevated, optically thick aerosol layers. In addition to its scientific value in climate research, anticipated applications of the product for TROPOMI are providing aerosol height information for aviation safety and improving interpretation of the Absorbing Aerosol Index.
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Tian, Xin, Yang Wang, Steffen Beirle, et al. "Technical note: Evaluation of profile retrievals of aerosols and trace gases for MAX-DOAS measurements under different aerosol scenarios based on radiative transfer simulations." Atmospheric Chemistry and Physics 21, no. 17 (2021): 12867–94. http://dx.doi.org/10.5194/acp-21-12867-2021.
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Abstract. Ground-based Multi-AXis Differential Optical Absorption Spectroscopy (MAX-DOAS) is a state-of-the-art remote sensing technique for deriving vertical profiles of trace gases and aerosols. However, MAX-DOAS profile inversions under aerosol pollution scenarios are challenging because of the complex radiative transfer and limited information content of the measurements. In this study, the performances of two inversion algorithms were evaluated for various aerosol pollution scenarios based on synthetic slant column densities (SCDs) derived from radiative transfer simulations. Compared to previous studies, in our study, much larger ranges of aerosol optical depth (AOD) and NO2 vertical column densities (VCDs) are covered. One inversion algorithm is based on optimal estimation; the other uses a parameterized approach. In this analysis, three types of profile shapes for aerosols and NO2 were considered: exponential, Boltzmann, and Gaussian. First, the systematic deviations of the retrieved aerosol profiles from the input profiles were investigated. For most cases, the AODs of the retrieved profiles were found to be systematically lower than the input values, and the deviations increased with increasing AOD. In particular for the optimal estimation algorithm and for high AOD, these findings are consistent with the results in previous studies. The assumed single scattering albedo (SSA) and asymmetry parameter (AP) have a systematic influence on the aerosol retrieval. However, for most cases the influence of the assumed SSA and AP on the retrieval results are rather small (compared to other uncertainties). For the optimal estimation algorithm, the agreement with the input values can be improved by optimizing the covariance matrix of the a priori uncertainties. Second, the aerosol effects on the NO2 profile retrieval were tested. Here, especially for the optimal estimation algorithm, a systematic dependence on the NO2 VCD was found, with a strong relative overestimation of the retrieved results for low NO2 VCDs and an underestimation for high NO2 VCDs. In contrast, the dependence on the aerosol profiles was found to be rather low. Interestingly, the results for both investigated wavelengths (360 and 477 nm) were found to be rather similar, indicating that the differences in the radiative transfer between both wavelengths have no strong effect. In general, both inversion schemes can retrieve the near-surface values of aerosol extinction and trace gas concentrations well.
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Li, Dingdong, Yonghua Wu, Barry Gross, and Fred Moshary. "Capabilities of an Automatic Lidar Ceilometer to Retrieve Aerosol Characteristics within the Planetary Boundary Layer." Remote Sensing 13, no. 18 (2021): 3626. http://dx.doi.org/10.3390/rs13183626.
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Continuous observation and quantitative retrieval of aerosol backscatter coefficients are important in the study of air quality and climate in metropolitan areas such as New York City. Ceilometers are ideal for this application, but aerosol backscatter coefficient retrievals from ceilometers are challenging and require proper calibration. In this study, we calibrate the ceilometer (Lufft CHM15k, 1064 nm) system constant with the molecular backscatter coefficient and evaluate the calibrated profiles with other independent methods, including the water-phase cloud method and comparison with the NASA Cloud-Aerosol Lidar and Infrared Pathfinder Satellite Observation (CALIPSO) attenuated backscatter coefficient profile. Multiple-day calibration results show a stable system constant with a relative uncertainty of about 7%. We also evaluate the overlap correction for the CHM15k ceilometer (provided by Lufft) with a Vaisala CL-31 ceilometer, and the results show good consistency between two ceilometers’ range-corrected signal (RCS) profiles above 200 m. Next, we implement a forward iterative method to retrieve aerosol backscatter coefficients from continuous ceilometer measurements. In the retrieval, the lidar ratio is constrained by the co-located NASA AERONET radiometer aerosol optical depth (AOD) retrieval and agrees with the AERONET lidar-ratio products, derived from aerosol microphysical parameters. The aerosol backscatter coefficient retrievals are validated with co-located elastic-Raman lidar retrievals and indicate a good correlation (R2≥0.95) in the planetary boundary layer (PBL). Furthermore, a case study shows that the ceilometer retrieved aerosol extinction coefficient profiles can be used to estimate the AOD of the PBL and the aloft plumes. Finally, simulations of the uncertainty of aerosol backscatter coefficient retrieval show that a calibration error of 10% results in 10–20% of relative error in the aerosol backscatter coefficient retrievals, while relative error caused by a lidar-ratio error of 10% is less than 4% in the PBL.
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Friedrich, Martina Michaela, Claudia Rivera, Wolfgang Stremme, et al. "NO<sub>2</sub> vertical profiles and column densities from MAX-DOAS measurements in Mexico City." Atmospheric Measurement Techniques 12, no. 4 (2019): 2545–65. http://dx.doi.org/10.5194/amt-12-2545-2019.
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Abstract. We present a new numerical code, Mexican MAX-DOAS Fit (MMF), developed to retrieve profiles of different trace gases from the network of MAX-DOAS instruments operated in Mexico City. MMF uses differential slant column densities (dSCDs) retrieved with the QDOAS (Danckaert et al., 2013) software. The retrieval is comprised of two steps, an aerosol retrieval and a trace gas retrieval that uses the retrieved aerosol profile in the forward model for the trace gas. For forward model simulations, VLIDORT is used (e.g., Spurr et al., 2001; Spurr, 2006, 2013). Both steps use constrained least-square fitting, but the aerosol retrieval uses Tikhonov regularization and the trace gas retrieval optimal estimation. Aerosol optical depth and scattering properties from the AERONET database, averaged ceilometer data, WRF-Chem model data, and temperature and pressure sounding data are used for different steps in the retrieval chain. The MMF code was applied to retrieve NO2 profiles with 2 degrees of freedom (DOF = 2) from spectra of the MAX-DOAS instrument located at the Universidad Nacional Autónoma de México (UNAM) campus. We describe the full error analysis of the retrievals and include a sensitivity exercise to quantify the contribution of the uncertainties in the aerosol extinction profiles to the total error. A data set comprised of measurements from January 2015 to July 2016 was processed and the results compared to independent surface measurements. We concentrate on the analysis of four single days and additionally present diurnal and annual variabilities from averaging the 1.5 years of data. The total error, depending on the exact counting, is 14 %–20 % and this work provides new and relevant information about NO2 in the boundary layer of Mexico City.
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Vlemmix, T., F. Hendrick, G. Pinardi, et al. "MAX-DOAS observations of aerosols, formaldehyde and nitrogen dioxide in the Beijing area: comparison of two profile retrieval approaches." Atmospheric Measurement Techniques Discussions 7, no. 9 (2014): 9673–731. http://dx.doi.org/10.5194/amtd-7-9673-2014.
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Abstract. A four year data set of MAX-DOAS observations in the Beijing area (2008–2012) is analysed with a focus on NO2, HCHO, and aerosols. Two very different retrieval methods are applied. Method A describes the tropospheric profile with 13 layers and makes use of the optimal estimation method. Method B uses 2–4 parameters to describe the tropospheric profile and an inversion based on a least-squares fit. For each constituent (NO2, HCHO and aerosols) the retrieval outcomes are compared in terms of tropospheric columns, surface concentrations, and "characteristic profile heights" (i.e. the height below which 75% of the vertically integrated tropospheric column resides). We find best agreement between the two methods for tropospheric NO2 columns, with a standard deviation of relative differences below 10%, a correlation of 0.99 and a linear regression with a slope of 1.03. For tropospheric HCHO columns we find a similar slope, but also a systematic bias of almost 10% which is likely related to differences in profile height. Aerosol optical depths (AODs) retrieved with method B are 20% high compared to method A. They are more in agreement with AERONET measurements, which are on average only 5% lower, however with considerable relative differences (standard deviation ~25%). With respect to near surface volume mixing ratios and aerosol extinction we find considerably larger relative differences: 10 ± 30%, −23 ± 28% and −8 ± 33% for aerosols, HCHO and NO2 respectively. The frequency distributions of these near-surface concentrations show however a quite good agreement, and this indicates that near-surface concentrations derived from MAX-DOAS are certainly useful in a climatological sense. A major difference between the two methods is the dynamic range of retrieved characteristic profile heights which is larger for method B than for method A. This effect is most pronounced for HCHO, where retrieved profile shapes with method A are very close to the a priori, and moderate for NO2 and aerosols which on average show quite good agreement for characteristic profile heights below 1.5 km. One of the main advantages of method A is the stability, even under suboptimal conditions (e.g., in the presence of clouds). Method B is generally more unstable and this explains probably a substantial part of the quite large relative differences between the two methods. However, despite a relatively low precision for individual profile retrievals it appears as if seasonally averaged profile heights retrieved with method B are less biased towards a priori assumptions than those retrieved with method A. This gives confidence in the result obtained with method B, namely that aerosol profiles tend on average to be higher than NO2 profiles in spring and summer, whereas they seem on average to be of the same height in winter, a result which is especially relevant in relation to the validation of satellite retrievals.
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Vlemmix, T., F. Hendrick, G. Pinardi, et al. "MAX-DOAS observations of aerosols, formaldehyde and nitrogen dioxide in the Beijing area: comparison of two profile retrieval approaches." Atmospheric Measurement Techniques 8, no. 2 (2015): 941–63. http://dx.doi.org/10.5194/amt-8-941-2015.
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Abstract. A 4-year data set of MAX-DOAS observations in the Beijing area (2008–2012) is analysed with a focus on NO2, HCHO and aerosols. Two very different retrieval methods are applied. Method A describes the tropospheric profile with 13 layers and makes use of the optimal estimation method. Method B uses 2–4 parameters to describe the tropospheric profile and an inversion based on a least-squares fit. For each constituent (NO2, HCHO and aerosols) the retrieval outcomes are compared in terms of tropospheric column densities, surface concentrations and "characteristic profile heights" (i.e. the height below which 75% of the vertically integrated tropospheric column density resides). We find best agreement between the two methods for tropospheric NO2 column densities, with a standard deviation of relative differences below 10%, a correlation of 0.99 and a linear regression with a slope of 1.03. For tropospheric HCHO column densities we find a similar slope, but also a systematic bias of almost 10% which is likely related to differences in profile height. Aerosol optical depths (AODs) retrieved with method B are 20% high compared to method A. They are more in agreement with AERONET measurements, which are on average only 5% lower, however with considerable relative differences (standard deviation ~ 25%). With respect to near-surface volume mixing ratios and aerosol extinction we find considerably larger relative differences: 10 ± 30, −23 ± 28 and −8 ± 33% for aerosols, HCHO and NO2 respectively. The frequency distributions of these near-surface concentrations show however a quite good agreement, and this indicates that near-surface concentrations derived from MAX-DOAS are certainly useful in a climatological sense. A major difference between the two methods is the dynamic range of retrieved characteristic profile heights which is larger for method B than for method A. This effect is most pronounced for HCHO, where retrieved profile shapes with method A are very close to the a priori, and moderate for NO2 and aerosol extinction which on average show quite good agreement for characteristic profile heights below 1.5 km. One of the main advantages of method A is the stability, even under suboptimal conditions (e.g. in the presence of clouds). Method B is generally more unstable and this explains probably a substantial part of the quite large relative differences between the two methods. However, despite a relatively low precision for individual profile retrievals it appears as if seasonally averaged profile heights retrieved with method B are less biased towards a priori assumptions than those retrieved with method A. This gives confidence in the result obtained with method B, namely that aerosol extinction profiles tend on average to be higher than NO2 profiles in spring and summer, whereas they seem on average to be of the same height in winter, a result which is especially relevant in relation to the validation of satellite retrievals.
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Wang, Zhuoru, Ka Lok Chan, Klaus-Peter Heue, et al. "A multi-axis differential optical absorption spectroscopy aerosol profile retrieval algorithm for high-altitude measurements: application to measurements at Schneefernerhaus (UFS), Germany." Atmospheric Measurement Techniques 13, no. 4 (2020): 1835–66. http://dx.doi.org/10.5194/amt-13-1835-2020.
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Abstract. We present a new aerosol extinction profile retrieval algorithm for multi-axis differential optical absorption spectrometer (MAX-DOAS) measurements at high-altitude sites. The algorithm is based on the lookup table method. It is applied to retrieve aerosol extinction profiles from the long-term MAX-DOAS measurements (February 2012 to February 2016) at the Environmental Research Station Schneefernerhaus (UFS), Germany (47.417∘ N, 10.980∘ E), which is located near the summit of Zugspitze at an altitude of 2650 m. The lookup table consists of simulated O4 differential slant column densities (DSCDs) corresponding to numerous possible aerosol extinction profiles. The sensitivities of O4 absorption to several parameters were investigated for the design and parameterization of the lookup table. In the retrieval, simulated O4 DSCDs for each possible profile are derived by interpolating the lookup table to the observation geometries. The cost functions are calculated for each aerosol profile in the lookup table based on the simulated O4 DSCDs, the O4 DSCD observations, and the measurement uncertainties. Valid profiles are selected from all the possible profiles according to the cost function, and the optimal solution is defined as the weighted mean of all the valid profiles. A comprehensive error analysis is performed to better estimate the total uncertainty. Based on the assumption that the lookup table covers all possible profiles under clear-sky conditions, we determined a set of O4 DSCD scaling factors for different elevation angles and wavelengths. The profiles retrieved from synthetic measurement data can reproduce the synthetic profile. The results also show that the retrieval is insensitive to measurement noise, indicating the retrieval is robust and stable. The aerosol optical depths (AODs) retrieved from the long-term measurements were compared to coinciding and co-located sun photometer observations. High correlation coefficients (R) of 0.733 and 0.798 are found for measurements at 360 and 477 nm, respectively. However, especially in summer, the sun photometer AODs are systematically higher than the MAX-DOAS retrievals by a factor of ∼2. The discrepancy might be related to the limited measurement range of the MAX-DOAS and is probably also related to the decreased sensitivity of the MAX-DOAS measurements at higher altitudes. The MAX-DOAS measurements indicate the aerosol extinction decreases with increasing altitude during all seasons, which agrees with the co-located ceilometer measurements. Our results also show maximum AOD and maximum Ångström exponent in summer, which is consistent with observations at an AERONET station located ∼43 km from the UFS.
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Young, Stuart A., Mark A. Vaughan, Ralph E. Kuehn, and David M. Winker. "The Retrieval of Profiles of Particulate Extinction from Cloud–Aerosol Lidar and Infrared Pathfinder Satellite Observations (CALIPSO) Data: Uncertainty and Error Sensitivity Analyses." Journal of Atmospheric and Oceanic Technology 30, no. 3 (2013): 395–428. http://dx.doi.org/10.1175/jtech-d-12-00046.1.
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Abstract Profiles of atmospheric cloud and aerosol extinction coefficients are retrieved on a global scale from measurements made by the lidar on board the Cloud–Aerosol Lidar and Infrared Pathfinder Satellite Observations (CALIPSO) mission since mid-June 2006. This paper presents an analysis of how the uncertainties in the inputs to the extinction retrieval algorithm propagate as the retrieval proceeds downward to lower levels of the atmosphere. The mathematical analyses, which are being used to calculate the uncertainties reported in the current (version 3) data release, are supported by figures illustrating the retrieval uncertainties in both simulated and actual data. Equations are also derived that describe the sensitivity of the extinction retrieval algorithm to errors in profile calibration and in the lidar ratios used in the retrievals. Biases that could potentially result from low signal-to-noise ratios in the data are also examined. Using simulated data, the propagation of bias errors resulting from errors in profile calibration and lidar ratios is illustrated.
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Frieß, U., H. Klein Baltink, S. Beirle, et al. "Intercomparison of aerosol extinction profiles retrieved from MAX-DOAS measurements." Atmospheric Measurement Techniques 9, no. 7 (2016): 3205–22. http://dx.doi.org/10.5194/amt-9-3205-2016.
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Abstract. A first direct intercomparison of aerosol vertical profiles from Multi-Axis Differential Optical Absorption Spectroscopy (MAX-DOAS) observations, performed during the Cabauw Intercomparison Campaign of Nitrogen Dioxide measuring Instruments (CINDI) in summer 2009, is presented. Five out of 14 participants of the CINDI campaign reported aerosol extinction profiles and aerosol optical thickness (AOT) as deduced from observations of differential slant column densities of the oxygen collision complex (O4) at different elevation angles. Aerosol extinction vertical profiles and AOT are compared to backscatter profiles from a ceilometer instrument and to sun photometer measurements, respectively. Furthermore, the near-surface aerosol extinction coefficient is compared to in situ measurements of a humidity-controlled nephelometer and dry aerosol absorption measurements. The participants of this intercomparison exercise use different approaches for the retrieval of aerosol information, including the retrieval of the full vertical profile using optimal estimation and a parametrised approach with a prescribed profile shape. Despite these large conceptual differences, and also differences in the wavelength of the observed O4 absorption band, good agreement in terms of the vertical structure of aerosols within the boundary layer is achieved between the aerosol extinction profiles retrieved by the different groups and the backscatter profiles observed by the ceilometer instrument. AOTs from MAX-DOAS and sun photometer show a good correlation (R>0.8), but all participants systematically underestimate the AOT. Substantial differences between the near-surface aerosol extinction from MAX-DOAS and from the humidified nephelometer remain largely unresolved.
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Bourassa, A. E., D. A. Degenstein, and E. J. Llewellyn. "Retrieval of stratospheric aerosol size information from OSIRIS limb scattered sunlight spectra." Atmospheric Chemistry and Physics Discussions 8, no. 1 (2008): 4001–16. http://dx.doi.org/10.5194/acpd-8-4001-2008.
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Abstract. Recent work has shown that the retrieval of stratospheric aerosol vertical profiles is possible using limb scattered sunlight measurements at optical wavelengths. The aerosol number density profile is retrieved for an assumed particle size distribution and composition. This result can be used to derive the extinction at the measured wavelength. However, large systematic error can result from the uncertainty in the assumed size distribution when the result is used to estimate the extinction at other wavelengths. It is shown in this work that the addition of information obtained from the near infrared limb radiance profile at 1530 nm measured by the imaging module of the OSIRIS instrument yields an indication of the aerosol size distribution profile that can be used to improve the fidelity of the retrievals. A comparison of the estimated extinction profile at 1020 nm with coincident occultation measurements demonstrates agreement to within approximately 15% from 12 to 27 km altitude.
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Bourassa, A. E., D. A. Degenstein, and E. J. Llewellyn. "Retrieval of stratospheric aerosol size information from OSIRIS limb scattered sunlight spectra." Atmospheric Chemistry and Physics 8, no. 21 (2008): 6375–80. http://dx.doi.org/10.5194/acp-8-6375-2008.
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Abstract. Recent work has shown that the retrieval of stratospheric aerosol vertical profiles is possible using limb scattered sunlight measurements at optical wavelengths. The aerosol number density profile is retrieved for an assumed particle size distribution and composition. This result can be used to derive the extinction at the measured wavelength. However, large systematic error can result from the uncertainty in the assumed size distribution when the result is used to estimate the extinction at other wavelengths. It is shown in this work that the addition of information obtained from the near infrared limb radiance profile at 1530 nm measured by the imaging module of the OSIRIS instrument yields an indication of the aerosol size distribution profile that can be used to improve the fidelity of the retrievals. A comparison of the estimated extinction profile at 1020 nm with two coincident occultation measurements demonstrates agreement to within approximately 15% from 12 to 27 km altitude.
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Chen, Xi, Yi Liu, Dongxu Yang, Zhaonan Cai, Hongbin Chen, and Maohua Wang. "A Theoretical Analysis for Improving Aerosol-Induced CO2 Retrieval Uncertainties Over Land Based on TanSat Nadir Observations Under Clear Sky Conditions." Remote Sensing 11, no. 9 (2019): 1061. http://dx.doi.org/10.3390/rs11091061.
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Aerosols significantly affect carbon dioxide (CO2) retrieval accuracy and precision by modifying the light path. Hyperspectral measurements in the near infrared and shortwave infrared (NIR/SWIR) bands from the generation of new greenhouse gas satellites (e.g., the Chinese Global Carbon Dioxide Monitoring Scientific Experimental Satellite, TanSat) contain aerosol information for correction of scattering effects in the retrieval. Herein, a new approach is proposed for optimizing the aerosol model used in the TanSat CO2 retrieval algorithm to reduce CO2 uncertainties associated with aerosols. The weighting functions of hyperspectral observations with respect to elements in the state vector are simulated by a forward radiative transfer model. Using the optimal estimation method (OEM), the information content and each component of the CO2 column-averaged dry-air mole fraction (XCO2) retrieval errors from the TanSat simulations are calculated for typical aerosols which are described by Aerosol Robotic Network (AERONET) inversion products at selected sites based on the a priori and measurement assumptions. The results indicate that the size distribution parameters (reff, veff), real refractive index coefficient of fine mode (arf) and fine mode fraction (fmf) dominate the interference errors, with each causing 0.2–0.8 ppm of XCO2 errors. Given that only 4–7 degrees of freedom for signal (DFS) of aerosols can be obtained simultaneously and CO2 information decreases as more aerosol parameters are retrieved, four to seven aerosol parameters are suggested as the most appropriate for inclusion in CO2 retrieval. Focusing on only aerosol-induced XCO2 errors, forward model parameter errors, rather than interference errors, are dominant. A comparison of these errors across different aerosol parameter combination groups reveals that fewer aerosol-induced XCO2 errors are found when retrieving seven aerosol parameters. Therefore, the model selected as the optimal aerosol model includes aerosol optical depth (AOD), peak height of aerosol profile (Hp), width of aerosol profile (Hw), effective variance of fine mode aerosol (vefff), effective radius of coarse mode aerosol (reffc), coefficient a of the real part of the refractive index for the fine mode and coarse mode (arf and arc), with the lowest error of less than 1.7 ppm for all aerosol and surface types. For marine aerosols, only five parameters (AOD, Hp, Hw, reffc and arc) are recommended for the low aerosol information. This optimal aerosol model therefore offers a theoretical foundation for improving CO2 retrieval precision from real TanSat observations in the future.
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Bourassa, A. E., L. A. Rieger, N. D. Lloyd, and D. A. Degenstein. "Odin-OSIRIS stratospheric aerosol data product and SAGE III intercomparison." Atmospheric Chemistry and Physics 12, no. 1 (2012): 605–14. http://dx.doi.org/10.5194/acp-12-605-2012.
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Abstract. The scattered sunlight measurements made by the Optical Spectrograph and InfraRed Imaging System (OSIRIS) on the Odin spacecraft are used to retrieve vertical profiles of stratospheric aerosol extinction at 750 nm. The recently released OSIRIS Version 5 data product contains the first publicly released stratospheric aerosol extinction retrievals, and these are now available for the entire Odin mission, which extends from the present day back to launch in 2001. A proof-of-concept study for the retrieval of stratospheric aerosol extinction from limb scatter measurements was previously published and the Version 5 data product retrievals are based on this work, but incorporate several important improvements to the algorithm. One of the primary changes is the use of a new retrieval vector that greatly improves the sensitivity to aerosol scattering by incorporating a forward modeled calculation of the radiance from a Rayleigh atmosphere. Additional improvements include a coupled retrieval of the effective albedo, a new method for normalization of the retrieval vector to improve signal-to-noise, and the use of an initial guess that is representative of very low background aerosol loading conditions, which allows for maximal retrieval range. Furthermore, the Version 5 data set is compared to Stratospheric Aerosol and Gas Experiment (SAGE) III 755 nm extinction profiles during the almost four years of mission overlap from 2002 to late 2005. The vertical structure in coincident profile measurements is well correlated and the statistics on a relatively large set of tight coincident measurements show agreement between the measurements from the two instruments to within approximately 10% throughout the 15 to 25 km altitude range, which covers the bulk of the stratospheric aerosol layer for the mid and high latitude cases studied here.
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Callewaert, Sieglinde, Sophie Vandenbussche, Nicolas Kumps, et al. "The Mineral Aerosol Profiling from Infrared Radiances (MAPIR) algorithm: version 4.1 description and evaluation." Atmospheric Measurement Techniques 12, no. 7 (2019): 3673–98. http://dx.doi.org/10.5194/amt-12-3673-2019.
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Abstract. The Mineral Aerosol Profiling from Infrared Radiances (MAPIR) algorithm retrieves vertical dust concentration profiles from cloud-free Infrared Atmospheric Sounding Interferometer (IASI) thermal infrared (TIR) radiances using Rodgers' optimal estimation method (OEM). We describe the new version 4.1 and evaluation results. Main differences with respect to previous versions are the Levenberg–Marquardt modification of the OEM, the use of the logarithm of the concentration in the retrieval and the use of Radiative Transfer for TOVS (RTTOV) for in-line radiative transfer calculations. The dust aerosol concentrations are retrieved in seven 1 km thick layers centered at 0.5 to 6.5 km. A global data set of the daily dust distribution was generated with MAPIR v4.1 covering September 2007 to June 2018, with further extensions planned every 6 months. The post-retrieval quality filters reject about 16 % of the retrievals, a huge improvement with respect to the previous versions in which up to 40 % of the retrievals were of bad quality. The median difference between the observed and fitted spectra of the good-quality retrievals is 0.32 K, with lower values over oceans. The information content of the retrieved profiles shows a dependence on the total aerosol load due to the assumption of a lognormal state vector. The median degrees of freedom in dusty scenes (min 10 µm AOD of 0.5) is 1.4. An evaluation of the aerosol optical depth (AOD) obtained from the integrated MAPIR v4.1 profiles was performed against 72 AErosol RObotic NETwork (AERONET) stations. The MAPIR AOD correlates well with the ground-based data, with a mean correlation coefficient of 0.66 and values as high as 0.88. Overall, there is a mean AOD (550 nm) positive bias of only 0.04 with respect to AERONET, which is an extremely good result. The previous versions of MAPIR were known to largely overestimate AOD (about 0.28 for v3). A second evaluation exercise was performed comparing the mean aerosol layer altitude from MAPIR with the mean dust altitude from Cloud–Aerosol LIdar with Orthogonal Polarization (CALIOP). A small underestimation was found, with a mean difference of about 350 m (standard deviation of about 1 km) with respect to the CALIOP cumulative extinction altitude, which is again considered very good as the vertical resolution of MAPIR is 1 km. In the comparisons against AERONET and CALIOP, a dependence of MAPIR on the quality of the temperature profiles used in the retrieval is observed. Finally, a qualitative comparison of dust aerosol concentration profiles was done against lidar measurements from two ground-based stations (M'Bour and Al Dhaid) and from the Cloud–Aerosol Transport System (CATS) instrument on board the International Space Station (ISS). MAPIR v4.1 showed the ability to detect dust plumes at the same time and with a similar extent as the lidar instruments. This new MAPIR version shows a great improvement of the accuracy of the aerosol profile retrievals with respect to previous versions, especially so for the integrated AOD. It now offers a unique 3-D dust data set, which can be used to gain more insight into the transport and emission processes of mineral dust aerosols.
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Bourassa, A. E., L. A. Rieger, N. D. Lloyd, and D. A. Degenstein. "Odin-OSIRIS stratospheric aerosol data product and SAGE III intercomparison." Atmospheric Chemistry and Physics Discussions 11, no. 9 (2011): 25785–811. http://dx.doi.org/10.5194/acpd-11-25785-2011.
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Abstract. The scattered sunlight measurements made by the Optical Spectrograph and InfraRed Imaging System (OSIRIS) on the Odin spacecraft are used to retrieve vertical profiles of stratospheric aerosol extinction at 750 nm. The recently released OSIRIS Version 5 data product contains the first publicly released stratospheric aerosol extinction retrievals, and these are now available for the entire Odin mission, which extends from the present day back to launch in 2001. A proof-of-concept study for the retrieval of stratospheric aerosol extinction from limb scatter measurements was previously published and the Version 5 data product retrievals are based on this work, but incorporate several important improvements to the algorithm. One of the primary changes is the use of a new retrieval vector that greatly improves the sensitivity to aerosol scattering by incorporating a forward modeled calculation of the radiance from a Rayleigh atmosphere. Additional improvements include a coupled retrieval of the effective albedo, a new method for normalization of the measurement vector to improve signal-to-noise, and the use of an initial guess that is representative of very low background aerosol loading conditions, which allows for maximal retrieval range. Furthermore, the Version 5 data set is compared to SAGE III 755 nm extinction profiles during the almost four years of mission overlap from 2002 to late 2005. The vertical structure in coincident profile measurements is well correlated and the statistics on a relatively large set of tight coincident measurements show agreement between the measurements from the two instruments to within approximately 10 % throughout the 15 to 25 km altitude range, which covers the bulk of the stratospheric aerosol layer for the mid and high latitude cases studied here.
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Tirpitz, Jan-Lukas, Udo Frieß, Robert Spurr, and Ulrich Platt. "Enhancing MAX-DOAS atmospheric state retrievals by multispectral polarimetry – studies using synthetic data." Atmospheric Measurement Techniques 15, no. 7 (2022): 2077–98. http://dx.doi.org/10.5194/amt-15-2077-2022.
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Abstract. Ground-based multi-axis differential optical absorption spectroscopy (MAX-DOAS) is a widely used measurement technique for the remote detection of atmospheric aerosol and trace gases. The technique relies on the analysis of ultra-violet and visible radiation spectra of scattered sunlight (skylight) to obtain information on different atmospheric parameters. From an appropriate set of spectra recorded under different viewing directions (typically a group of observations at different elevation angles) the retrieval of aerosol and trace gas vertical distributions is achieved through numerical inversion methods. It is well known that the polarisation state of skylight is particularly sensitive to atmospheric aerosol content as well as aerosol properties and that polarimetric measurements could therefore provide additional information for MAX-DOAS profile retrievals; however, such measurements have not yet been used for this purpose. To address this issue, we have developed the RAPSODI (Retrieval of Atmospheric Parameters from Spectroscopic Observations using DOAS Instruments) algorithm. In contrast to existing MAX-DOAS algorithms, it can process polarimetric information, and it can retrieve simultaneously profiles of aerosols and various trace gases at multiple wavelengths in a single retrieval step; a further advantage is that it contains a Mie scattering model, allowing for the retrieval of aerosol microphysical properties. The forward-model component in RAPSODI is based on a linearised vector radiative transfer model with Jacobian facilities, and we have used this model to create a database of synthetic measurements in order to carry out sensitivity analyses aimed at assessing the potential of polarimetric MAX-DOAS observations. We find that multispectral polarimetry significantly enhances the sensitivity, particularly to aerosol-related quantities. Assuming typical viewing geometries, the degrees of freedom for signal (DOFS) increase by about 50 % and 70 % for aerosol vertical distributions and aerosol properties, respectively, and by approximately 10 % for trace gas vertical profiles. For an idealised scenario with a horizontally homogeneous atmosphere, our findings predict an improvement in the inversion results' accuracy (root-mean-square deviations to the true values) of about 60 % for aerosol vertical column densities (VCDs) as well as for aerosol surface concentrations and by 40 % for aerosol properties. For trace gas VCDs, very little improvement is apparent, although the accuracy of trace gas surface concentrations improves by about 50 %.
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Kudo, Rei, Tomoaki Nishizawa, and Toshinori Aoyagi. "Vertical profiles of aerosol optical properties and the solar heating rate estimated by combining sky radiometer and lidar measurements." Atmospheric Measurement Techniques 9, no. 7 (2016): 3223–43. http://dx.doi.org/10.5194/amt-9-3223-2016.
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Abstract. The SKYLIDAR algorithm was developed to estimate vertical profiles of aerosol optical properties from sky radiometer (SKYNET) and lidar (AD-Net) measurements. The solar heating rate was also estimated from the SKYLIDAR retrievals. The algorithm consists of two retrieval steps: (1) columnar properties are retrieved from the sky radiometer measurements and the vertically mean depolarization ratio obtained from the lidar measurements and (2) vertical profiles are retrieved from the lidar measurements and the results of the first step. The derived parameters are the vertical profiles of the size distribution, refractive index (real and imaginary parts), extinction coefficient, single-scattering albedo, and asymmetry factor. Sensitivity tests were conducted by applying the SKYLIDAR algorithm to the simulated sky radiometer and lidar data for vertical profiles of three different aerosols, continental average, transported dust, and pollution aerosols. The vertical profiles of the size distribution, extinction coefficient, and asymmetry factor were well estimated in all cases. The vertical profiles of the refractive index and single-scattering albedo of transported dust, but not those of transported pollution aerosol, were well estimated. To demonstrate the performance and validity of the SKYLIDAR algorithm, we applied the SKYLIDAR algorithm to the actual measurements at Tsukuba, Japan. The detailed vertical structures of the aerosol optical properties and solar heating rate of transported dust and smoke were investigated. Examination of the relationship between the solar heating rate and the aerosol optical properties showed that the vertical profile of the asymmetry factor played an important role in creating vertical variation in the solar heating rate. We then compared the columnar optical properties retrieved with the SKYLIDAR algorithm to those produced with the more established scheme SKYRAD.PACK, and the surface solar irradiance calculated from the SKYLIDAR retrievals was compared with pyranometer measurement. The results showed good agreements: the columnar values of the SKYLIDAR retrievals agreed with reliable SKYRAD.PACK retrievals, and the SKYLIDAR retrievals were sufficiently accurate to evaluate the surface solar irradiance.
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Zhu, Fang, Fuqi Si, Haijin Zhou, Ke Dou, Minjie Zhao, and Quan Zhang. "Sensitivity Analysis of Ozone Profiles Retrieved from SCIAMACHY Limb Radiance Based on the Weighted Multiplicative Algebraic Reconstruction Technique." Remote Sensing 14, no. 16 (2022): 3954. http://dx.doi.org/10.3390/rs14163954.
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A detailed sensitivity analysis of ozone density profile retrieval was applied to scattering solar radiance spectra measured with the SCanning Imaging Absorption spectroMeter for Atmospheric CHartographY (SCIAMACHY) instrument aboard the ENVIronmental SATellite (ENVISAT). The vertical density distribution of ozone between 10 and 69 km was obtained using the weighted multiplicative algebraic reconstruction technique and the radiative transfer model for SCIAMACHY. This study investigates the error sources for the retrieved ozone profiles, which are relevant to explain the difference between two independent instruments. The numerical simulation method was adapted to quantify the impact of various error sources on the retrieval accuracy of ozone profiles. First, the tangent height (TH) registration was found to be the largest error source. Assuming an aerosol-free atmosphere, under the condition of background aerosol, the ozone profile showed a negative deviation of ~2–10% below 40 km. With an incorrect a priori profile, ozone estimates may result in a 5–10% average error at the upper and lower boundaries. The ozone retrieval error caused by the uncertainty of surface albedo, ozone absorption cross-section, temperature, pressure profile, and low clouds was relatively small. The random error caused by the disturbance of the measurement vector obeying a Gaussian distribution did not exceed 5%. Second, the estimation of various error sources for different solar zenith angles was investigated. The error sources most strongly dependent on SZAs were aerosols, surface albedo, and clouds. Finally, the error estimation of the ozone retrieval between the northern hemisphere (NH) and the southern hemisphere (SH) was investigated, revealing that there were no strong interhemispheric differences, except for cloud height. These results can be used for interpretation of instrumental comparisons and validation of SCIAMACHY ozone profiles retrieved from different algorithms in a rigorous manner.
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Peers, Fanny, Peter Francis, Cathryn Fox, et al. "Observation of absorbing aerosols above clouds over the south-east Atlantic Ocean from the geostationary satellite SEVIRI – Part 1: Method description and sensitivity." Atmospheric Chemistry and Physics 19, no. 14 (2019): 9595–611. http://dx.doi.org/10.5194/acp-19-9595-2019.
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Abstract. High-temporal-resolution observations from satellites have a great potential for studying the impact of biomass burning aerosols and clouds over the south-east Atlantic Ocean (SEAO). This paper presents a method developed to simultaneously retrieve aerosol and cloud properties in aerosol above-cloud conditions from the geostationary instrument Meteosat Second Generation/Spinning Enhanced Visible and Infrared Imager (MSG/SEVIRI). The above-cloud aerosol optical thickness (AOT), the cloud optical thickness (COT) and the cloud droplet effective radius (CER) are derived from the spectral contrast and the magnitude of the signal measured in three channels in the visible to shortwave infrared region. The impact of the absorption from atmospheric gases on the satellite signal is corrected by applying transmittances calculated using the water vapour profiles from a Met Office forecast model. The sensitivity analysis shows that a 10 % error on the humidity profile leads to an 18.5 % bias on the above-cloud AOT, which highlights the importance of an accurate atmospheric correction scheme. In situ measurements from the CLARIFY-2017 airborne field campaign are used to constrain the aerosol size distribution and refractive index that is assumed for the aforementioned retrieval algorithm. The sensitivities in the retrieved AOT, COT and CER to the aerosol model assumptions are assessed. Between 09:00 and 15:00 UTC, an uncertainty of 40 % is estimated on the above-cloud AOT, which is dominated by the sensitivity of the retrieval to the single-scattering albedo. The absorption AOT is less sensitive to the aerosol assumptions with an uncertainty generally lower than 17 % between 09:00 and 15:00 UTC. Outside of that time range, as the scattering angle decreases, the sensitivity of the AOT and the absorption AOT to the aerosol model increases. The retrieved cloud properties are only weakly sensitive to the aerosol model assumptions throughout the day, with biases lower than 6 % on the COT and 3 % on the CER. The stability of the retrieval over time is analysed. For observations outside of the backscattering glory region, the time series of the aerosol and cloud properties are physically consistent, which confirms the ability of the retrieval to monitor the temporal evolution of aerosol above-cloud events over the SEAO.
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Bösch, Tim, Vladimir Rozanov, Andreas Richter, et al. "BOREAS – a new MAX-DOAS profile retrieval algorithm for aerosols and trace gases." Atmospheric Measurement Techniques 11, no. 12 (2018): 6833–59. http://dx.doi.org/10.5194/amt-11-6833-2018.
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Abstract. We present a new MAX-DOAS profiling algorithm for aerosols and trace gases, BOREAS, which utilizes an iterative solution method including Tikhonov regularization and the optimal estimation technique. The aerosol profile retrieval is based on a novel approach in which the absorption depth of O4 is directly used in order to retrieve extinction coefficient profiles instead of the commonly used perturbation theory method. The retrieval of trace gases is done with the frequently used optimal estimation method but significant improvements are presented on how to deal with wrongly weighted a priori constraints and for scenarios in which the a priori profile is inaccurate. Performance tests are separated into two parts. First, we address the general sensitivity of the retrieval to the example of synthetic data calculated with the radiative transfer model SCIATRAN. In the second part of the study, we demonstrate BOREAS profiling accuracy by validating the results with the help of ancillary measurements carried out during the CINDI-2 campaign in Cabauw, the Netherlands, in 2016. The synthetic sensitivity tests indicate that the regularization between measurement and a priori constraints is insufficient when knowledge of the true state of the atmosphere is poor. We demonstrate a priori pre-scaling and extensive regularization tests as a tool for the optimization of retrieved profiles. The comparison of retrieval results with in situ, ceilometer, NO2 lidar, sonde and long-path DOAS measurements during the CINDI-2 campaign always shows high correlations with coefficients greater than 0.75. The largest differences can be found in the morning hours, when the planetary boundary layer is not yet fully developed and the concentration of trace gases and aerosol, as a result of a low night-time boundary layer having formed, is focused in a shallow, near-surface layer.
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Seo, Jongjin, Haklim Choi, and Youngsuk Oh. "Potential of AOD Retrieval Using Atmospheric Emitted Radiance Interferometer (AERI)." Remote Sensing 14, no. 2 (2022): 407. http://dx.doi.org/10.3390/rs14020407.
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Aerosols in the atmosphere play an essential role in the radiative transfer process due to their scattering, absorption, and emission. Moreover, they interrupt the retrieval of atmospheric properties from ground-based and satellite remote sensing. Thus, accurate aerosol information needs to be obtained. Herein, we developed an optimal-estimation-based aerosol optical depth (AOD) retrieval algorithm using the hyperspectral infrared downwelling emitted radiance of the Atmospheric Emitted Radiance Interferometer (AERI). The proposed algorithm is based on the phenomena that the thermal infrared radiance measured by a ground-based remote sensor is sensitive to the thermodynamic profile and degree of the turbid aerosol in the atmosphere. To assess the performance of algorithm, AERI observations, measured throughout the day on 21 October 2010 at Anmyeon, South Korea, were used. The derived thermodynamic profiles and AODs were compared with those of the European center for a reanalysis of medium-range weather forecasts version 5 and global atmosphere watch precision-filter radiometer (GAW-PFR), respectively. The radiances simulated with aerosol information were more suitable for the AERI-observed radiance than those without aerosol (i.e., clear sky). The temporal variation trend of the retrieved AOD matched that of GAW-PFR well, although small discrepancies were present at high aerosol concentrations. This provides a potential possibility for the retrieval of nighttime AOD.
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Xing, Chengzhi, Cheng Liu, Shanshan Wang, et al. "Observations of the vertical distributions of summertime atmospheric pollutants and the corresponding ozone production in Shanghai, China." Atmospheric Chemistry and Physics 17, no. 23 (2017): 14275–89. http://dx.doi.org/10.5194/acp-17-14275-2017.
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Abstract. Ground-based multi-axis differential optical absorption spectroscopy (MAX-DOAS) and lidar measurements were performed in Shanghai, China, during May 2016 to investigate the vertical distribution of summertime atmospheric pollutants. In this study, vertical profiles of aerosol extinction coefficient, nitrogen dioxide (NO2) and formaldehyde (HCHO) concentrations were retrieved from MAX-DOAS measurements using the Heidelberg Profile (HEIPRO) algorithm, while vertical distribution of ozone (O3) was obtained from an ozone lidar. Sensitivity study of the MAX-DOAS aerosol profile retrieval shows that the a priori aerosol profile shape has significant influences on the aerosol profile retrieval. Aerosol profiles retrieved from MAX-DOAS measurements with Gaussian a priori profile demonstrate the best agreements with simultaneous lidar measurements and vehicle-based tethered-balloon observations among all a priori aerosol profiles. Tropospheric NO2 vertical column densities (VCDs) measured with MAX-DOAS show a good agreement with OMI satellite observations with a Pearson correlation coefficient (R) of 0.95. In addition, measurements of the O3 vertical distribution indicate that the ozone productions do not only occur at surface level but also at higher altitudes (about 1.1 km). Planetary boundary layer (PBL) height and horizontal and vertical wind field information were integrated to discuss the ozone formation at upper altitudes. The results reveal that enhanced ozone concentrations at ground level and upper altitudes are not directly related to horizontal and vertical transportation. Similar patterns of O3 and HCHO vertical distributions were observed during this campaign, which implies that the ozone productions near the surface and at higher altitudes are mainly influenced by the abundance of volatile organic compounds (VOCs) in the lower troposphere.
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Bousserez, N. "Space-based retrieval of NO<sub>2</sub> over biomass burning regions: quantifying and reducing uncertainties." Atmospheric Measurement Techniques Discussions 6, no. 4 (2013): 6645–84. http://dx.doi.org/10.5194/amtd-6-6645-2013.
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Abstract. The quality of space-based nitrogen dioxide (NO2) retrievals from solar backscatter depends on a priori knowledge of the vertical profiles of NO2 and aerosol optical properties. This information is contained in an air mass factor (AMF), which accounts for atmospheric scattering and is used to convert the measured line-of-sight "slant" columns into vertical columns. In this study we investigate the impact of biomass burning emissions on the AMF in order to quantify NO2 retrieval errors in the Ozone Monitoring Instrument (OMI) products over these sources. Sensitivity analyses are conducted using the Linearized Discrete Ordinate Radiative Transfer (LIDORT) model and the GEOS-Chem chemistry-transport model with an improved daily biomass burning emission inventory. Aircraft in situ data collected during two field campaigns, Arctic Research of the Composition of the Troposphere from Aircraft and Satellites (ARCTAS) and Dust and Biomass-burning Experiment (DABEX), are used to evaluate the modeled aerosol optical properties and NO2 profiles over Canadian boreal fires and western Africa savanna fires respectively. Biomass burning aerosols increase the AMF by 3 to 15% over boreal fires, while they decrease the AMF by −10 to −30% over savanna fires. The presence of an elevated aerosol layer over west Africa due to the Harmattan front explains the negative aerosol effect over this area. The impact of fires on the AMF is driven by the NO2 shape profile perturbations, which decrease the AMF by −10 to −60% over both regions. Aerosol and shape factor effects are most sensitive to surface reflectance and clouds. In particular, retrieval errors associated with shape factor uncertainties can increase by a factor of 2 due to the presence of clouds. In contrast with conclusions from previous studies, we demonstrate that in the presence of pre-existing clouds, the effect of aerosols on the AMF cannot be fully accounted for through the modified retrieved cloud parameters. Finally, a new method that uses slant column information to correct for shape factor error in the retrieval is proposed and tested over west African fires.
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Wang, Shanshan, Carlos A. Cuevas, Udo Frieß, and Alfonso Saiz-Lopez. "MAX-DOAS retrieval of aerosol extinction properties in Madrid, Spain." Atmospheric Measurement Techniques 9, no. 10 (2016): 5089–101. http://dx.doi.org/10.5194/amt-9-5089-2016.
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Abstract. Multi-axis differential optical absorption spectroscopy (MAX-DOAS) measurements were performed in the urban environment of Madrid, Spain, from March to September 2015. The O4 absorption in the ultraviolet (UV) spectral region was used to retrieve the aerosol extinction profile using an inversion algorithm. The results show a good agreement between the hourly retrieved aerosol optical depth (AOD) and the correlative Aerosol Robotic Network (AERONET) product, with a correlation coefficient of R = 0.87. Higher AODs are found in the summer season due to the more frequent occurrence of Saharan dust intrusions. The surface aerosol extinction coefficient as retrieved by the MAX-DOAS measurements was also compared to in situ PM2.5 concentrations. The level of agreement between both measurements indicates that the MAX-DOAS retrieval has the ability to characterize the extinction of aerosol particles near the surface. The retrieval algorithm was also used to study a case of severe dust intrusion on 12 May 2015. The capability of the MAX-DOAS retrieval to recognize the dust event including an elevated particle layer is investigated along with air mass back-trajectory analysis.
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Molero, Francisco, Manuel Pujadas, and Begoña Artíñano. "Study of the Effect of Aerosol Vertical Profile on Microphysical Properties Using GRASP Code with Sun/Sky Photometer and Multiwavelength Lidar Measurements." Remote Sensing 12, no. 24 (2020): 4072. http://dx.doi.org/10.3390/rs12244072.
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In this paper, we study the effect of the vertical distribution of aerosols on the inversion process to obtain microphysical properties of aerosols. The GRASP code is used to retrieve the aerosol size distribution from two different schemes. Firstly, only sun/sky photometer measurements of aerosol optical depth and sky radiances are used as input to the retrieval code, and then, both this information and the range-corrected signals from an advanced lidar system are provided to the code. Measurements taken at the Madrid EARLINET station, complemented with those from the nearby AERONET station, have been analyzed for the 2016–2019 time range. The effect found of the measured vertical profile on the inversion is a shift to smaller radius of the fine mode with average differences of 0.05 ± 0.02 µm, without noticeable effects for the coarse mode radius. This coarse mode is sometimes split into two modes, related to large AOD or elevated aerosol-rich layers. The first scheme´s retrieved size distributions are also compared with those provided by AERONET, observing the unusual persistence of a large mode centered at 5 µm. These changes in the size distributions affect slightly the radiative forcing calculated also by the GRASP code. A stronger forcing, dependent on the AOD, is observed in the second scheme. The shift in the fine mode and the effect on the radiative forcing indicate the importance of considering the vertical profile of aerosols on the retrieval of microphysical properties by remote sensing.
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Papayannis, A., R. E. Mamouri, V. Amiridis, et al. "Optical-microphysical properties of Saharan dust aerosols and composition relationship using a multi-wavelength Raman lidar, in situ sensors and modelling: a case study analysis." Atmospheric Chemistry and Physics Discussions 11, no. 9 (2011): 25473–516. http://dx.doi.org/10.5194/acpd-11-25473-2011.
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Abstract. A strong Saharan dust event occurred over the city of Athens, Greece (37.9° N, 23.6° E) between 27 March and 3 April 2009. The BSC-DREAM8b model was used to forecast the dust event and to provide the vertical profiles of the aerosol concentration. Due to mixture of dust particles with low clouds during most of the reported period, the dust event could be followed by the National Technical University of Athens (NTUA) 6-wavelength Raman lidar system only during the unclouded day of 2 April 2009. The lidar data obtained were used to retrieve the vertical profile of the optical (extinction and backscatter coefficients) properties of aerosols in the troposphere. Additionally, a retrieval technique representing dust as a mixture of spheres and spheroids was used to derive the mean aerosol dust microphysical properties (mean and effective radius, number, surface and volume density, and mean refractive index) in different layers between 1.8 and 3.5 km a.s.l. The final data set of the aerosol optical and microphysical properties along with the water vapor profiles obtained by Raman lidar were incorporated into the ISORROPIA II model to infer an in situ aerosol composition consistent with the retrieved refractive index values. PM10 concentrations levels, PM10 composition results and SEM-EDX (Scanning Electron Microscope-Energy Dispersive X-ray) analysis results on sizes and mineralogy of particles from samples during the Saharan dust transport event were used to evaluate the retrieval.
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Colosimo, Santo Fedele, Vijay Natraj, Stanley P. Sander, and Jochen Stutz. "A sensitivity study on the retrieval of aerosol vertical profiles using the oxygen A-band." Atmospheric Measurement Techniques 9, no. 4 (2016): 1889–905. http://dx.doi.org/10.5194/amt-9-1889-2016.
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Abstract. Atmospheric absorption in the O2 A-band (12 950–13 200 cm−1) offers a unique opportunity to retrieve aerosol extinction profiles from space-borne measurements due to the large dynamic range of optical thickness in that spectral region. Absorptions in strong O2 lines are saturated; therefore, any radiance measured in these lines originates from scattering in the upper part of the atmosphere. Outside of O2 lines, or in weak lines, the atmospheric column absorption is small, and light penetrates to lower atmospheric layers, allowing for the quantification of aerosols and other scatterers near the surface.While the principle of aerosol profile retrieval using O2 A-band absorption from space is well-known, a thorough quantification of the information content, i.e., the amount of vertical profile information that can be obtained, and the dependence of the information content on the spectral resolution of the measurements, has not been thoroughly conducted. Here, we use the linearized vector radiative transfer model VLIDORT to perform spectrally resolved simulations of atmospheric radiation in the O2 A-band for four different aerosol extinction profile scenarios: urban (urban–rural areas), highly polluted (megacity areas with large aerosol extinction), elevated layer (identifying elevated plumes, for example for biomass burning) and low extinction (representative of small aerosol extinction, such as vegetated, marine and arctic areas). The high-resolution radiances emerging from the top of the atmosphere measurements are degraded to different spectral resolutions, simulating spectrometers with different resolving powers. We use optimal estimation theory to quantify the information content in the aerosol profile retrieval with respect to different aerosol parameters and instrument spectral resolutions. The simulations show that better spectral resolution generally leads to an increase in the total amount of information that can be retrieved, with the number of degrees of freedom (DoF) varying between 0.34–2.01 at low resolution (5 cm−1) to 3.43–5.38 at high resolution (0.05 cm−1) among all the different cases. A particularly strong improvement was found in the retrieval of tropospheric aerosol extinction profiles in the lowest 5 km of the atmosphere. At high spectral resolutions (0.05 cm−1), 1.18–1.48 and 1.31–1.96 DoF can be obtained in the lower (0–2 km) and middle (2–5 km) troposphere, respectively, for the different cases. Consequently, a separation of lower and mid tropospheric aerosols is possible, implying the feasibility of identification of elevated biomass burning aerosol plumes (elevated layer scenario). We find that a higher single scattering albedo (SSA) allows for the retrieval of more aerosol information. However, the dependence on SSA is weaker at higher spectral resolutions. The vegetation (surface albedo 0.3), marine (surface albedo 0.05) and arctic (surface albedo 0.9) cases show that the dependence of DoF on the surface albedo decreases with higher resolution. At low resolution (5 cm−1), the DoF are 1.19 for the marine case, 0.73 for the vegetation case and 0.34 for the arctic case, but increase considerably at 0.05 cm−1 resolution to 3.84 (marine) and 3.43 (both vegetation and arctic), showing an improvement of a factor of 10 for the arctic case. Vegetation and arctic case also show the same DoF at higher resolution, showing that an increase of albedo beyond a certain value, i.e., 0.3 in our case, does not lead to a larger information content. The simulations also reveal a moderate dependence of information content on the integration time of the measurements, i.e., the noise of the spectra. However, our results indicate that a larger increase in DoF is obtained by an increase in spectral resolution despite lower signal-to-noise ratios.
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Sanghavi, S., J. V. Martonchik, J. Landgraf, and U. Platt. "Retrieval of aerosol optical depth and vertical distribution using O<sub>2</sub> A- and B-band SCIAMACHY observations over Kanpur: a case study." Atmospheric Measurement Techniques Discussions 4, no. 6 (2011): 6779–809. http://dx.doi.org/10.5194/amtd-4-6779-2011.
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Abstract. The vertical profiles of aerosol often provide a clear picture of transport processes, and are an indicator of elevated secondary aerosol formation or primary aerosol sources close to the surface. The vertical extent of clouds and aerosols also governs the sign and magnitude of their net radiative forcing. Ground- and satellite-based lidar measurements presently provide much of this information, however their sampling of 3-D data is limited due to infrequent, sparce or uneven coverage. From a remote-sensing perspective, retrievals of many trace-gases suffer from uncertainties due to aerosol and would benefit from co-located information on the amount and vertical distribution of aerosol loading. This motivates the development of complementary methods to retrieve vertical information on aerosols using satellite data, which have the advantage of more frequent global coverage. SCIAMACHY onboard ENVISAT provides spectral data at moderate resolution in the UV/VIS including the O2 A- and B-bands, which contain vertical information due to the known vertical profile of O2. We make combined use of these bands in an optimal estimation based algorithm applicable both over bright and dark surfaces to retrieve the parametrized vertical profile of aerosol, in addition to the optical thickness from SCIAMACHY data. We present a case study over Kanpur, India, showing good agreement with coincident AERONET data, capturing seasonal cycles and a periodic wind-blown dust event over Kanpur.
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Morille, Y., M. Haeffelin, P. Drobinski, and J. Pelon. "STRAT: An Automated Algorithm to Retrieve the Vertical Structure of the Atmosphere from Single-Channel Lidar Data." Journal of Atmospheric and Oceanic Technology 24, no. 5 (2007): 761–75. http://dx.doi.org/10.1175/jtech2008.1.
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Abstract Today several lidar networks around the world provide large datasets that are extremely valuable for aerosol and cloud research. Retrieval of atmospheric constituent properties from lidar profiles requires detailed analysis of spatial and temporal variations of the signal. This paper presents an algorithm called Structure of the Atmosphere (STRAT), which is designed to retrieve the vertical distribution of cloud and aerosol layers in the boundary layer and through the free troposphere and to identify near-particle-free regions of the vertical profile and the range at which the lidar signal becomes too attenuated for exploitation, from a single lidar channel. The paper describes each detection method used in the STRAT algorithm and its application to a tropospheric backscatter lidar operated at the SIRTA observatory, in Palaiseau, 20 km south of Paris, France. STRAT retrievals are compared to other means of layer detection and classification; retrieval performances and uncertainties are discussed.
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Colosimo, S. F., V. Natraj, S. P. Sander, and J. Stutz. "A sensitivity study on the retrieval of aerosol vertical profiles using the oxygen A-band." Atmospheric Measurement Techniques Discussions 8, no. 11 (2015): 11853–91. http://dx.doi.org/10.5194/amtd-8-11853-2015.
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Abstract. Atmospheric absorption in the O2 A-band (12 950–13 200 cm−1) offers a unique opportunity to retrieve aerosol extinction profiles from space-borne measurements due to the large dynamic range of optical thickness in that spectral region. Absorptions in strong O2 lines are saturated; therefore, any radiance measured in these lines originates from scattering in the upper part of the atmosphere. Outside of O2 lines, or in weak lines, the atmospheric column absorption is small, and light penetrates to lower atmospheric layers, allowing for the quantification of aerosols and other scatterers near the surface. While the principle of aerosol profile retrieval using O2 A-band absorption from space is well known, a thorough quantification of the information content, i.e., the amount of vertical profile information that can be obtained, and the dependence of the information content on the spectral resolution of the measurements, has not been thoroughly conducted. Here, we use the linearized vector radiative transfer model VLIDORT to perform spectrally resolved simulations of atmospheric radiation in the O2 A-band in the presence of aerosol for four different generic scenarios: Urban, Highly polluted, Elevated layer, and Marine–Arctic. The high-resolution radiances emerging from the top of the atmosphere are degraded to different spectral resolutions, simulating spectrometers with different resolving powers. We use optimal estimation theory to quantify the information content in the aerosol profile retrieval with respect to different aerosol parameters and instrument spectral resolutions. The simulations show that better spectral resolution generally leads to an increase in the total amount of information that can be retrieved, with the number of degrees of freedom (DoF) varying between 0.34–2.11 at low resolution (5 cm−1) to 3.43–5.92 at high resolution (0.05 cm−1) for the four different cases. A particularly strong improvement was found in the retrieval of tropospheric aerosol extinction profiles in the lowest 5 km of the atmosphere. At high spectral resolutions (0.05 cm−1), 1.18–1.7 and 1.31–2.34 DoF can be obtained in the lower (0–2 km) and middle (2–5 km) troposphere, respectively, for the different cases. Consequently a separation of lower and mid tropospheric aerosols is possible, implying the feasibility of identification of elevated biomass burning aerosol plumes (Elevated layer scenario). We find that higher single scattering albedo (SSA) allows for the retrieval of more aerosol information. However, the dependence on SSA is weaker at higher spectral resolutions. The Marine (surface albedo 0.05) and Arctic (surface albedo 0.9) cases show that the dependence of DoF on the surface albedo decreases with higher resolution. While at low resolution (5 cm−1) the DoF is 1 for the Marine case and 0.34 for the Arctic case, the DoF considerably increase at 0.05 cm−1 resolution to 3.8 and 3.4, respectively. In the Arctic case this is an improvement of a factor of 10. The simulations also reveal a moderate dependence of information content on the integration time of the measurements, i.e., the noise of the spectra. However, our results indicate that a larger increase in DoF is obtained by an increase in spectral resolution despite lower signal-to-noise ratios.
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Iwasaki, Chisa, Ryoichi Imasu, Andrey Bril, et al. "Optimization of the Photon Path Length Probability Density Function-Simultaneous (PPDF-S) Method and Evaluation of CO2 Retrieval Performance Under Dense Aerosol Conditions." Sensors 19, no. 5 (2019): 1262. http://dx.doi.org/10.3390/s19051262.
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The photon path length probability density function-simultaneous (PPDF-S) algorithm is effective for retrieving column-averaged concentrations of carbon dioxide (XCO2) and methane (XCH4) from Greenhouse gases Observing Satellite (GOSAT) spectra in Short Wavelength InfraRed (SWIR). Using this method, light-path modification attributable to light reflection/scattering by atmospheric clouds/aerosols is represented by the modification of atmospheric transmittance according to PPDF parameters. We optimized PPDF parameters for a more accurate XCO2 retrieval under aerosol dense conditions based on simulation studies for various aerosol types and surface albedos. We found a more appropriate value of PPDF parameters referring to the vertical profile of CO2 concentration as a measure of a stable solution. The results show that the constraint condition of a PPDF parameter that represents the light reflectance effect by aerosols is sufficiently weak to affect XCO2 adversely. By optimizing the constraint, it was possible to obtain a stable solution of XCO2. The new optimization was applied to retrieval analysis of the GOSAT data measured in Western Siberia. First, we assumed clear sky conditions and retrieved XCO2 from GOSAT data obtained near Yekaterinburg in the target area. The retrieved XCO2 was validated through a comparison with ground-based Fourier Transform Spectrometer (FTS) measurements made at the Yekaterinburg observation site. The validation results showed that the retrieval accuracy was reasonable. Next, we applied the optimized method to dense aerosol conditions when biomass burning was active. The results demonstrated that optimization enabled retrieval, even under smoky conditions, and that the total number of retrieved data increased by about 70%. Furthermore, the results of the simulation studies and the GOSAT data analysis suggest that atmospheric aerosol types that affected CO2 analysis are identifiable by the PPDF parameter value. We expect that we will be able to suggest a further improved algorithm after the atmospheric aerosol types are identified.
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Toth, Travis D., James R. Campbell, Jeffrey S. Reid, et al. "Minimum aerosol layer detection sensitivities and their subsequent impacts on aerosol optical thickness retrievals in CALIPSO level 2 data products." Atmospheric Measurement Techniques 11, no. 1 (2018): 499–514. http://dx.doi.org/10.5194/amt-11-499-2018.
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Abstract. Due to instrument sensitivities and algorithm detection limits, level 2 (L2) Cloud-Aerosol Lidar with Orthogonal Polarization (CALIOP) 532 nm aerosol extinction profile retrievals are often populated with retrieval fill values (RFVs), which indicate the absence of detectable levels of aerosol within the profile. In this study, using 4 years (2007–2008 and 2010–2011) of CALIOP version 3 L2 aerosol data, the occurrence frequency of daytime CALIOP profiles containing all RFVs (all-RFV profiles) is studied. In the CALIOP data products, the aerosol optical thickness (AOT) of any all-RFV profile is reported as being zero, which may introduce a bias in CALIOP-based AOT climatologies. For this study, we derive revised estimates of AOT for all-RFV profiles using collocated Moderate Resolution Imaging Spectroradiometer (MODIS) Dark Target (DT) and, where available, AErosol RObotic NEtwork (AERONET) data. Globally, all-RFV profiles comprise roughly 71 % of all daytime CALIOP L2 aerosol profiles (i.e., including completely attenuated profiles), accounting for nearly half (45 %) of all daytime cloud-free L2 aerosol profiles. The mean collocated MODIS DT (AERONET) 550 nm AOT is found to be near 0.06 (0.08) for CALIOP all-RFV profiles. We further estimate a global mean aerosol extinction profile, a so-called “noise floor”, for CALIOP all-RFV profiles. The global mean CALIOP AOT is then recomputed by replacing RFV values with the derived noise-floor values for both all-RFV and non-all-RFV profiles. This process yields an improvement in the agreement of CALIOP and MODIS over-ocean AOT.
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Castellanos, P., K. F. Boersma, O. Torres, and J. F. de Haan. "OMI tropospheric NO<sub>2</sub> air mass factors over South America: effects of biomass burning aerosols." Atmospheric Measurement Techniques 8, no. 9 (2015): 3831–49. http://dx.doi.org/10.5194/amt-8-3831-2015.
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Abstract. Biomass burning is an important and uncertain source of aerosols and NOx (NO + NO2) to the atmosphere. Satellite observations of tropospheric NO2 are essential for characterizing this emissions source, but inaccuracies in the retrieval of NO2 tropospheric columns due to the radiative effects of aerosols, especially light-absorbing carbonaceous aerosols, are not well understood. It has been shown that the O2–O2 effective cloud fraction and pressure retrieval is sensitive to aerosol optical and physical properties, including aerosol optical depth (AOD). Aerosols implicitly influence the tropospheric air mass factor (AMF) calculations used in the NO2 retrieval through the effective cloud parameters used in the independent pixel approximation. In this work, we explicitly account for the effects of biomass burning aerosols in the Ozone Monitoring Instrument (OMI) tropospheric NO2 AMF calculation for cloud-free scenes. We do so by including collocated aerosol extinction vertical profile observations from the CALIOP instrument, and aerosol optical depth (AOD) and single scattering albedo (SSA) retrieved by the OMI near-UV aerosol algorithm (OMAERUV) in the DISAMAR radiative transfer model. Tropospheric AMFs calculated with DISAMAR were benchmarked against AMFs reported in the Dutch OMI NO2 (DOMINO) retrieval; the mean and standard deviation of the difference was 0.6 ± 8 %. Averaged over three successive South American biomass burning seasons (2006–2008), the spatial correlation in the 500 nm AOD retrieved by OMI and the 532 nm AOD retrieved by CALIOP was 0.6, and 68 % of the daily OMAERUV AOD observations were within 30 % of the CALIOP observations. Overall, tropospheric AMFs calculated with observed aerosol parameters were on average 10 % higher than AMFs calculated with effective cloud parameters. For effective cloud radiance fractions less than 30 %, or effective cloud pressures greater than 800 hPa, the difference between tropospheric AMFs based on implicit and explicit aerosol parameters is on average 6 and 3 %, respectively, which was the case for the majority of the pixels considered in our study; 70 % had cloud radiance fraction below 30 %, and 50 % had effective cloud pressure greater than 800 hPa. Pixels with effective cloud radiance fraction greater than 30 % or effective cloud pressure less than 800 hPa corresponded with stronger shielding in the implicit aerosol correction approach because the assumption of an opaque effective cloud underestimates the altitude-resolved AMF; tropospheric AMFs were on average 30–50 % larger when aerosol parameters were included, and for individual pixels tropospheric AMFs can differ by more than a factor of 2. The observation-based approach to correcting tropospheric AMF calculations for aerosol effects presented in this paper depicts a promising strategy for a globally consistent aerosol correction scheme for clear-sky pixels.
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Castellanos, P., K. F. Boersma, O. Torres, and J. F. de Haan. "OMI tropospheric NO<sub>2</sub> air mass factors over South America: effects of biomass burning aerosols." Atmospheric Measurement Techniques Discussions 8, no. 3 (2015): 2683–733. http://dx.doi.org/10.5194/amtd-8-2683-2015.
Full textAbstract:
Abstract. Biomass burning is an important and uncertain source of aerosols and NOx (NO + NO2) to the atmosphere. OMI observations of tropospheric NO2 are essential for characterizing this emissions source, but inaccuracies in the retrieval of NO2 tropospheric columns due to the radiative effects of aerosols, especially light-absorbing carbonaceous aerosols, are not well understood. It has been shown that the O2–O2 effective cloud fraction and pressure retrieval is sensitive to aerosol optical and physical properties, including aerosol optical depth (AOD). Aerosols implicitly influence the tropospheric air mass factor (AMF) calculations used in the NO2 retrieval through the effective cloud parameters used in the independent pixel approximation. In this work, we explicitly account for the effects of biomass burning aerosols in the tropospheric NO2 AMF calculation by including collocated aerosol extinction vertical profile observations from the CALIOP instrument, and aerosol optical depth (AOD) and single scattering albedo (SSA) retrieved by the OMI near-UV aerosol algorithm (OMAERUV) in the DISAMAR radiative transfer model for cloud-free scenes. Tropospheric AMFs calculated with DISAMAR were benchmarked against AMFs reported in the Dutch OMI NO2 (DOMINO) retrieval; the mean and standard deviation (SD) of the difference was 0.6 ± 8%. Averaged over three successive South American biomass burning seasons (2006–2008), the spatial correlation in the 500 nm AOD retrieved by OMI and the 532 nm AOD retrieved by CALIOP was 0.6, and 72% of the daily OMAERUV AOD observations were within 0.3 of the CALIOP observations. Overall, tropospheric AMFs calculated with observed aerosol parameters were on average 10% higher than AMFs calculated with effective cloud parameters. For effective cloud radiance fractions less than 30%, or effective cloud pressures greater than 800 hPa, the difference between tropospheric AMFs based on implicit and explicit aerosol parameters is on average 6 and 3%, respectively, which was the case for the majority of the pixels considered in our study. Pixels with effective cloud radiance fraction greater than 30% or effective cloud pressure less than 800 hPa corresponded with stronger shielding in the implicit aerosol correction approach because the assumption of a opaque effective cloud underestimates the altitude resolved AMF; tropospheric AMFs were on average 30–50% larger when aerosol parameters were included, and for individual pixels tropospheric AMFs can differ by more than a factor of two. The observation-based approach to correcting tropospheric AMF calculations for aerosol effects presented in this paper depicts a promising strategy for a globally consistent aerosol correction scheme for clear sky pixels.
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Kumari, B. Padma, S. H. Kulkarni, D. B. Jadhav, A. L. Londhe, and H. K. Trimbake. "Exploring Atmospheric Aerosols by Twilight Photometry." Journal of Atmospheric and Oceanic Technology 25, no. 9 (2008): 1600–1607. http://dx.doi.org/10.1175/2008jtecha1090.1.
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Abstract The instrument twilight photometer was designed, developed, and installed at the Indian Institute of Tropical Meteorology (IITM), Pune, India (18°43′N, 73°51′E), to monitor the vertical distribution of atmospheric aerosols. The instrument, based on passive remote sensing technique, is simple and inexpensive. It is operated only during twilights, and the method of retrieval of aerosol profile is based on a simple twilight technique. It functions at a single wavelength (660 nm), and a photomultiplier tube is used as a detector. The amplifier, an important component of the system, was designed and developed by connecting 10 single integrated-circuit (IC) amplifiers in parallel so that the noise at the output is drastically reduced and the sensitivity of the system has been increased. As a result, the vertical profiles are retrieved to a maximum of 120 km. A brief description of the basic principle of twilight technique, the experimental setup, and the method of retrieval of aerosol profiles using the above photometer are detailed in this paper.
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Lopatin, A., O. Dubovik, A. Chaikovsky, et al. "Enhancement of aerosol characterization using synergy of lidar and sun-photometer coincident observations: the GARRLiC algorithm." Atmospheric Measurement Techniques 6, no. 8 (2013): 2065–88. http://dx.doi.org/10.5194/amt-6-2065-2013.
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Abstract. This paper presents the GARRLiC algorithm (Generalized Aerosol Retrieval from Radiometer and Lidar Combined data) that simultaneously inverts coincident lidar and radiometer observations and derives a united set of aerosol parameters. Such synergetic retrieval results in additional enhancements in derived aerosol properties because the back-scattering observations by lidar improve sensitivity to the columnar properties of aerosol, while radiometric observations provide sufficient constraints on aerosol amount and type that are generally missing in lidar signals. GARRLiC is based on the AERONET algorithm, improved to invert combined observations by radiometer and multi-wavelength elastic lidar observations. The algorithm is set to derive not only the vertical profile of total aerosol concentration but it also differentiates between the contributions of fine and coarse modes of aerosol. The detailed microphysical properties are assumed height independent and different for each mode and derived as a part of the retrieval. The GARRLiC inversion retrieves vertical distribution of both fine and coarse aerosol concentrations as well as the size distribution and complex refractive index for each mode. The potential and limitations of the method are demonstrated by the series of sensitivity tests. The effects of presence of lidar data and random noise on aerosol retrievals are studied. Limited sensitivity to the properties of the fine mode as well as dependence of retrieval accuracy on the aerosol optical thickness were found. The practical outcome of the approach is illustrated by applications of the algorithm to the real lidar and radiometer observations obtained over Minsk AERONET site.
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Irie, H., T. Nakayama, A. Shimizu, et al. "Evaluation of MAX-DOAS aerosol retrievals by coincident observations using CRDS, lidar, and sky radiometer inTsukuba, Japan." Atmospheric Measurement Techniques 8, no. 7 (2015): 2775–88. http://dx.doi.org/10.5194/amt-8-2775-2015.
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Abstract. Coincident aerosol observations of multi-axis differential optical absorption spectroscopy (MAX-DOAS), cavity ring-down spectroscopy (CRDS), lidar, and sky radiometer were conducted in Tsukuba, Japan, on 5–18 October 2010. MAX-DOAS aerosol retrieval (for aerosol extinction coefficient and aerosol optical depth at 476 nm) was evaluated from the viewpoint of the need for a correction factor for oxygen collision complexes (O4 or O2–O2) absorption. The present study strongly supports this need, as systematic residuals at relatively high elevation angles (20 and 30°) were evident in MAX-DOAS profile retrievals conducted without the correction. However, adopting a single number for the correction factor (fO4 = 1.25) for all of the elevation angles led to systematic overestimation of near-surface aerosol extinction coefficients, as reported in the literature. To achieve agreement with all three observations, we limited the set of elevation angles to ≤10° and adopted an elevation-angle-dependent correction factor for practical profile retrievals with scattered light observations by a ground-based MAX-DOAS. With these modifications, we expect to minimize the possible effects of temperature-dependent O4 absorption cross section and uncertainty in DOAS fit on an aerosol profile retrieval, although more efforts are encouraged to quantitatively identify a physical explanation for the need of a correction factor.
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Irie, H., T. Nakayama, A. Shimizu, et al. "Evaluation of MAX-DOAS aerosol retrievals by coincident observations using CRDS, lidar, and sky radiometer in Tsukuba, Japan." Atmospheric Measurement Techniques Discussions 8, no. 1 (2015): 1013–54. http://dx.doi.org/10.5194/amtd-8-1013-2015.
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Abstract. Coincident aerosol observations of Multi-Axis Differential Optical Absorption Spectroscopy (MAX-DOAS), Cavity Ring Down Spectroscopy (CRDS), lidar, and sky radiometer were conducted in Tsukuba, Japan on 5–18 October 2010. MAX-DOAS aerosol retrieval (for aerosol extinction coefficient and aerosol optical depth at 476 nm) was evaluated from the viewpoint of the need for a correction factor for oxygen collision complexes (O4 or O2-O2) absorption. The present study strongly supports this need, as systematic residuals at relatively high elevation angles (20 and 30°) were evident in MAX-DOAS profile retrievals conducted without the correction. However, adopting a single number for the correction factor (fO4 = 1.25) for all of the elevation angles led to systematic overestimation of near-surface aerosol extinction coefficients, as reported in the literature. To achieve agreement with all three observations, we limited the set of elevation angles to ≤ 10° and adopted an elevation-angle-dependent correction factor for practical profile retrievals with scattered light observations by a ground-based MAX-DOAS. With these modifications, we expect to minimize the possible effects of temperature-dependent O4 absorption cross section and uncertainty in DOAS fit on an aerosol profile retrieval, although more efforts are encouraged to quantitatively identify a physical explanation for the need of a correction factor.
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Sheridan, P. J., E. Andrews, J. A. Ogren, J. L. Tackett, and D. M. Winker. "Vertical profiles of aerosol optical properties over Central Illinois and comparison with surface and satellite measurements." Atmospheric Chemistry and Physics Discussions 12, no. 7 (2012): 17187–244. http://dx.doi.org/10.5194/acpd-12-17187-2012.
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Abstract. Between June 2006 and September 2009, an instrumented light aircraft measured over 400 vertical profiles of aerosol and trace gas properties over Eastern and Central Illinois. The primary objectives of this program were to (1) measure the in situ aerosol properties and determine their vertical and temporal variability and (2) relate these aircraft measurements to concurrent surface and satellite measurements. The primary profile location was within 10 km of the NOAA/ESRL surface aerosol monitoring station near Bondville, Illinois. Identical instruments at the surface and on the aircraft ensured that the data from both platforms would be directly comparable and permitted a determination of how representative surface aerosol properties were of the lower column. Aircraft profiles were also conducted occasionally at two other nearby locations to increase the frequency of A-Train satellite underflights for the purpose of comparing in situ and satellite-retrieved aerosol data. Measurements over the Bondville site compare well with the surface aerosol data and do not indicate any major sampling issues or that the aerosol is radically different at the surface compared with the lowest flyby altitude of ~240 m a.g.l. Statistical analyses of the in situ vertical profile data indicate that aerosol loading (e.g. light scattering and absorption) decreases substantially with increasing altitude. Parameters related to the nature of the aerosol (e.g. single-scattering albedo, Ångström exponent, etc.), however, are relatively constant throughout the mixed layer, and do not vary as much as the aerosol amount throughout the profile. While individual profiles often showed more variability, the median in situ single-scattering albedo was 0.93–0.95 for all sampled altitudes. Several parameters (e.g. submicrometer scattering fraction, hemispheric backscattering fraction, and scattering Ångström exponent) suggest that the fraction of smaller particles in the aerosol is larger near the surface than at high altitudes. The observed dependence of scattering on size, wavelength, angular integration range, and relative humidity, together with the spectral dependence of absorption, show that the aerosol at higher altitudes is larger, less hygroscopic, and more strongly absorbing at shorter wavelengths, suggesting an increased contribution from dust or organic aerosols. The aerosol profiles show significant differences among seasons. The largest amounts of aerosol (as determined by median light extinction profile measurements) throughout most of the sampled column were observed during summer, with the lowest amounts in the winter and intermediate values in the spring and fall. The highest three profile levels (3.1, 3.7, 4.6 km), however, showed larger median extinction values in the spring, which could reflect long-range transport of dust or smoke aerosols. The aerosols in the mixed layer were darkest (i.e. lowest single-scattering albedo) in the fall, in agreement with surface measurements at Bondville and other continental sites in the US. In-situ profiles of aerosol radiative forcing efficiency showed little seasonal or vertical variability. Underflights of the CALIPSO satellite show reasonable agreement for extinction at 532 nm for most comparison points in a majority of retrieved profiles, and suggest that routine aircraft profiling programs can be used to better understand and validate satellite retrieval algorithms. CALIPSO tended to overestimate the aerosol extinction at this location in some boundary layer flight segments when scattered or broken clouds were present, which could be related to problems with CALIPSO cloud screening methods. Our in situ aerosol data suggest extinction thresholds for the likelihood of aerosol layers being detected by the CALIOP lidar. In this study, aerosol layers with light extinction values >50 Mm−1 were detected by CALIPSO ~95% of the time, while aerosol layers with extinction values lower than 10 Mm−1 had a detection efficiency of <2%. For all collocated comparison cases, a 50% probability of detection falls at an in situ extinction level of 20–25 Mm−1. These statistical data offer guidance as to the likelihood of CALIPSO's ability to retrieve aerosol extinction at various locations around the globe.
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Frieß, Udo, Steffen Beirle, Leonardo Alvarado Bonilla, et al. "Intercomparison of MAX-DOAS vertical profile retrieval algorithms: studies using synthetic data." Atmospheric Measurement Techniques 12, no. 4 (2019): 2155–81. http://dx.doi.org/10.5194/amt-12-2155-2019.
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Abstract. Multi-axis differential optical absorption spectroscopy (MAX-DOAS) is a widely used measurement technique for the detection of a variety of atmospheric trace gases. Using inverse modelling, the observation of trace gas column densities along different lines of sight enables the retrieval of aerosol and trace gas vertical profiles in the atmospheric boundary layer using appropriate retrieval algorithms. In this study, the ability of eight profile retrieval algorithms to reconstruct vertical profiles is assessed on the basis of synthetic measurements. Five of the algorithms are based on the optimal estimation method, two on parametrised approaches, and one using an analytical approach without involving any radiative transfer modelling. The synthetic measurements consist of the median of simulated slant column densities of O4 at 360 and 477 nm, as well as of HCHO at 343 nm and NO2 at 477 nm, from seven datasets simulated by five different radiative transfer models. Simulations are performed for a combination of 10 trace gas and 11 aerosol profiles, as well as 11 elevation angles, three solar zenith, and three relative azimuth angles. Overall, the results from the different algorithms show moderate to good performance for the retrieval of vertical profiles, surface concentrations, and total columns. Except for some outliers, the root-mean-square difference between the true and retrieved state ranges between (0.05–0.1) km−1 for aerosol extinction and (2.5–5.0) ×1010 molec cm−3 for HCHO and NO2 concentrations.