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Academic literature on the topic 'Catalytic conjunctive cross-coupling'
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Journal articles on the topic "Catalytic conjunctive cross-coupling"
Zhang, L., G. J. Lovinger, E. K. Edelstein, A. A. Szymaniak, M. P. Chierchia, and J. P. Morken. "Catalytic conjunctive cross-coupling enabled by metal-induced metallate rearrangement." Science 351, no. 6268 (December 31, 2015): 70–74. http://dx.doi.org/10.1126/science.aad6080.
Full textMeng, Yan, Ziyin Kong, and James P. Morken. "Catalytic Enantioselective Synthesis of anti ‐Vicinal Silylboronates by Conjunctive Cross‐Coupling." Angewandte Chemie International Edition 59, no. 22 (March 19, 2020): 8456–59. http://dx.doi.org/10.1002/anie.202000937.
Full textMeng, Yan, Ziyin Kong, and James P. Morken. "Catalytic Enantioselective Synthesis of anti ‐Vicinal Silylboronates by Conjunctive Cross‐Coupling." Angewandte Chemie 132, no. 22 (March 19, 2020): 8534–37. http://dx.doi.org/10.1002/ange.202000937.
Full textLaw, Chunyin, Elton Kativhu, Johnny Wang, and James P. Morken. "Diastereo‐ and Enantioselective 1,4‐Difunctionalization of Borylenynes by Catalytic Conjunctive Cross‐Coupling." Angewandte Chemie International Edition 59, no. 26 (April 15, 2020): 10311–15. http://dx.doi.org/10.1002/anie.202001580.
Full textLaw, Chunyin, Elton Kativhu, Johnny Wang, and James P. Morken. "Diastereo‐ and Enantioselective 1,4‐Difunctionalization of Borylenynes by Catalytic Conjunctive Cross‐Coupling." Angewandte Chemie 132, no. 26 (April 15, 2020): 10397–401. http://dx.doi.org/10.1002/ange.202001580.
Full textAparece, Mark D., Weipeng Hu, and James P. Morken. "Catalytic Enantioselective Synthesis of β-Allenyl Boronic Esters by Conjunctive Cross-Coupling with Propargylic Carbonates." ACS Catalysis 9, no. 12 (October 31, 2019): 11381–85. http://dx.doi.org/10.1021/acscatal.9b04453.
Full textTran, Van T., Zi‐Qi Li, Timothy J. Gallagher, Joseph Derosa, Peng Liu, and Keary M. Engle. "Integrating Allyl Electrophiles into Nickel‐Catalyzed Conjunctive Cross‐Coupling." Angewandte Chemie International Edition 59, no. 18 (March 13, 2020): 7029–34. http://dx.doi.org/10.1002/anie.201915454.
Full textMega, Riccardo S., Vincent K. Duong, Adam Noble, and Varinder K. Aggarwal. "Decarboxylative Conjunctive Cross‐coupling of Vinyl Boronic Esters using Metallaphotoredox Catalysis." Angewandte Chemie International Edition 59, no. 11 (February 3, 2020): 4375–79. http://dx.doi.org/10.1002/anie.201916340.
Full textMega, Riccardo S., Vincent K. Duong, Adam Noble, and Varinder K. Aggarwal. "Decarboxylative Conjunctive Cross‐coupling of Vinyl Boronic Esters using Metallaphotoredox Catalysis." Angewandte Chemie 132, no. 11 (March 9, 2020): 4405–9. http://dx.doi.org/10.1002/ange.201916340.
Full textMyhill, Jesse A., Christopher A. Wilhelmsen, Liang Zhang, and James P. Morken. "Diastereoselective and Enantioselective Conjunctive Cross-Coupling Enabled by Boron Ligand Design." Journal of the American Chemical Society 140, no. 45 (October 30, 2018): 15181–85. http://dx.doi.org/10.1021/jacs.8b09909.
Full textDissertations / Theses on the topic "Catalytic conjunctive cross-coupling"
Zhang, Liang. "Catalytic Conjunctive Cross-Coupling and Catalytic Diboration Reactions." Thesis, Boston College, 2017. http://hdl.handle.net/2345/bc-ir:107561.
Full textThis dissertation will present four main projects focused on stereoselective construction of borylated compounds as well as their applications in asymmetric syntheses. The first two projects describe the development of a catalytic conjunctive cross-coupling reaction. By merging three simple starting materials, an organolithium reagent, an organoboronate, and an organic electrophile, a synthetically valuable secondary boronate is furnished by the conjunctive cross-coupling in an efficient and enantioselective fashion. Next, this strategy is expanded to synthesize severely hindered tertiary boronates, a synthetic challenging but powerful building block to access a variety of quaternary stereocenters. The third project presents a platinum-catalyzed enantioselective diboration of alkenyl boronates to furnish a broad range of 1,1,2-tris(boronates) products. A deborylative alkylation of the 1,1,2-tris(boronates) leads to a variety of internal vicinal bis(boronates) with high diastereoselectivity. In the final chapter, a general and practical synthesis of alkenyl boronates via the boron-Wittig reaction is disclosed. Utilizing readily accessible geminal bis(boronates) and aldehydes, a broad range of disubstituted and trisubstituted alkenyl boronates are afforded with good yield and stereoselectivity
Thesis (PhD) — Boston College, 2017
Submitted to: Boston College. Graduate School of Arts and Sciences
Discipline: Chemistry
Myhill, Jesse Alexander. "Development of Catalytic Conjunctive Cross-Coupling Reactions and Progress Towards the Total Synthesis of the Sarcodictyins:." Thesis, Boston College, 2020. http://hdl.handle.net/2345/bc-ir:108724.
Full textThis dissertation describes the development of a method for the stereoselective synthesis of organoboronates and the applications of these products to target-oriented synthesis. The first chapter discusses an investigation of the palladium-catalyzed conjunctive cross-coupling reaction by kinetic analysis. This reaction enables the asymmetric synthesis of organoboronates by utilizing the 1,2-metallate rearrangement of borates as a mechanistic step in a cross-coupling reaction. The second chapter describes the application of the conjunctive cross-coupling reaction to the asymmetric synthesis of tertiary boronic esters. In chapter three, the conjunctive cross-coupling reaction of 1,2-disubstituted alkenyl boronates is presented. Such a substrate class is susceptible to the undesired Suzuki-Miyaura cross-coupling reaction, and this challenge led to the development of a novel diol ligand for boron as an effective solution. The final chapter details the progress toward the total synthesis of the sarcodictyin natural products, which display promising anti-cancer activity. The synthetic route utilizes reactions of organoboronates for powerful C–C bond formations; the construction of a fully-cyclyzed advanced intermediate is achieved in eight steps
Thesis (PhD) — Boston College, 2020
Submitted to: Boston College. Graduate School of Arts and Sciences
Discipline: Chemistry