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Dissertations / Theses on the topic 'CO2-sorbent'

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1

Benedetti, Alberto. "Microstructural Characterization of CaO-based Sorbents During CO2 Capture and Sorbent Regeneration." Doctoral thesis, Università degli studi di Padova, 2018. http://hdl.handle.net/11577/3424687.

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This work of thesis deals with the micro-textural properties characterization of calcium oxide as CO2 capture solid sorbent, that strongly influence the carbonation reaction step performances. The investigation of the sorbent micro-structure was carried out by means of both in-situ and ex-situ techniques, varying the precursor (CaCO3) activation conditions and sintering effects on the final sorbent pore network. X-ray diffraction and N2-adsorption techniques were used to identify correlations between the sorbent micro-textural properties and the average sorbent crystallite size, by considerin
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2

Butler, James. "Limestone as a sorbent for CO2 capture and its application in enhanced biomass gasification." Thesis, University of British Columbia, 2013. http://hdl.handle.net/2429/45680.

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Global greenhouse gas emissions continue to increase despite the knowledge that the rise in atmospheric concentrations will have devastating effects on climate and human lives. Carbon dioxide capture and storage can be a stop-gap measure to mitigate CO₂ emissions from existing fossil fuel facilities during their gradual replacement by low-carbon alternatives such as biomass. Calcium oxide-based CO₂ capture is a relatively mature technology, ready for implementation. Limestone CaO precursor is relatively low-cost and readily available. A thorough understanding of the CaO-CO₂ reaction and its re
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3

Isenberg, Mathew. "Development of Solid Amine Immobilized Silica Sorbent and Gram Scale Process for CO2 Capture." University of Akron / OhioLINK, 2010. http://rave.ohiolink.edu/etdc/view?acc_num=akron1282936403.

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4

Tanthana, Jak. "In Situ Infrared and Mass Spectroscopic Study on Amine-Immobilized Silica for CO2 Capture: Investigation of Mechanisms and Degradation." University of Akron / OhioLINK, 2011. http://rave.ohiolink.edu/etdc/view?acc_num=akron1302287239.

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5

Yu, Mingzhao. "Model Reduction and Nonlinear Model Predictive Control of Large-Scale Distributed Parameter Systems with Applications in Solid Sorbent-Based CO2 Capture." Research Showcase @ CMU, 2017. http://repository.cmu.edu/dissertations/887.

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This dissertation deals with some computational and analytic challenges for dynamic process operations using first-principles models. For processes with significant spatial variations, spatially distributed first-principles models can provide accurate physical descriptions, which are crucial for offline dynamic simulation and optimization. However, the large amount of time required to solve these detailed models limits their use for online applications such as nonlinear model predictive control (NMPC). To cope with the computational challenge, we develop computationally efficient and accurate
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6

Wilfong, Walter Christopher. "In Situ FTIR and Tubular Reactor Studies for CO2 Capture of Immobilized Amine Sorbents and Liquid Amine Films." University of Akron / OhioLINK, 2014. http://rave.ohiolink.edu/etdc/view?acc_num=akron1403704363.

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7

Hills, Thomas Peter. "Investigations of the use of spent sorbent from the Ca looping process in cement manufacture and investigation of long-term CO2 uptake in cement and concrete." Thesis, Imperial College London, 2016. http://hdl.handle.net/10044/1/39286.

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This thesis comes in three distinct parts: an evaluation of concrete carbonation to improve accuracy of lifecycle carbon emissions of concrete; a detailed rationale outlining the importance of carbon capture and storage (CCS) for Portland cement and discussing viable technology deployment trajectories for the UK; and experimental investigation of one of the most promising carbon capture technology for the industry. Using a data set of around 2000 points from the literature, two regression models using common predictor variables were generated using multilevel modelling. One of these was used t
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8

Wang, Alan Yao. "Clean Coal Chemical Looping Technology: the Influence of Metal Oxide on the Thermoplasticity of Bituminous Coal and the Steam Reactivation of Metal Oxide Sorbent for CO2 Capture." The Ohio State University, 2016. http://rave.ohiolink.edu/etdc/view?acc_num=osu1467162960.

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9

Fisher, James C. II. "The Reduction of CO2 Emissions Via CO2 Capture and Solid Oxide Fuel Cells." University of Akron / OhioLINK, 2009. http://rave.ohiolink.edu/etdc/view?acc_num=akron1247250147.

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10

Iyer, Mahesh Venkataraman. "High temperature reactive separation process for combined carbon dioxide and sulfur dioxide capture from flue gas and enhanced hydrogen production with in-situ carbon dioxide capture using high reactivity calcium and biomineral sorbents." The Ohio State University, 2006. http://rave.ohiolink.edu/etdc/view?acc_num=osu1135961929.

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11

Di, Giuliano Andrea. "Synthesis, characterization and industrial applicability of combined sorbent-catalyst materials for sorption enhanced steam methane reforming." Thesis, Strasbourg, 2017. http://www.theses.fr/2017STRAF065/document.

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SESMR (Sorption Enhanced Steam Methane Reforming), SMR (Steam Methane Reforming) avec capture de CO2 in situ par un adsorbant solide, peut amener à une exploitation durable du gaz naturel pour la production de H2. La thèse, partie du projet de recherche ASCENT (Advanced Solid Cycles with Efficient Novel Technologies), concerne le développement de matériaux combinés adsorbants catalyseurs Ni-CaO-mayenite pour le SESMR, aux fins d’étudier les influences dues à la fraction de Ni, aux sels précurseurs du Ni (Ni acétate ou Ni nitrate), et à la fraction de CaO disponible. Les techniques ICP AES, XRD
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12

Silva, Mojica Ernesto. "Polymer-silica Hybrids for Separation of CO2 and Catalysis of Organic Reactions." University of Akron / OhioLINK, 2014. http://rave.ohiolink.edu/etdc/view?acc_num=akron1398439043.

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13

Wu, Di. "A Novel Method to Prepare Silica Based Carbon Dioxide Capture Sorbent." University of Akron / OhioLINK, 2008. http://rave.ohiolink.edu/etdc/view?acc_num=akron1215095709.

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14

Hsiao, Wei-yuan, and 蕭惟元. "The effects of Ca-based sorbent on CO2 retention in multiple CO2 capture cycles." Thesis, 2010. http://ndltd.ncl.edu.tw/handle/63659924414391748838.

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碩士<br>國立聯合大學<br>環境與安全衛生工程學系碩士班<br>98<br>The calcium-based adsorbent wasused to capture CO2 in a fixed bed reactor in this study. The carbonation of Ca-based sorbent can adsorbtion CO2, then it can be regenerated by a reverse calcination reaction. The high concentration CO2 which is produced in the calcination reaction can be recycled and reused. This process is called the multiple CO2 capture cycles. Limestone and dolomite are the typically-used natural Ca-based sorbent. In this study, the effects of the compositions of various sorbents, the various operating temperature, the pretreatment proc
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15

Huang, Jun-Qiang, and 黃俊強. "Preparation of CO2 adsorption sorbent by reutilizing waste oyster shell." Thesis, 2014. http://ndltd.ncl.edu.tw/handle/48310814213578503647.

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碩士<br>國立清華大學<br>生醫工程與環境科學系<br>102<br>In this study, we demonstrate a means of simultaneously solving two serious environmental issues by reutilization of pulverized waste oyster shells to prepare CaO-based sorbents for CO2 capture. First, waste oyster shell are calcined with poly(methyl methacrylate) (PMMA) nanospheres. Here, a highly surface area and pore volume “three-dimensionally ordered macroporous (3DOM)” structures are formed. After 10 cycles of isothermal carbonation/calcination at 750 °C, the greatest CO2 uptake (0.19 g CO2/g sorbent) is that for the sorbent featuring 70 wt% of PMMA,
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16

Jian-Syun-Li and 李建勳. "Post-combustion CO2 capture in a dry sorbent injection system." Thesis, 2015. http://ndltd.ncl.edu.tw/handle/24235645898048680655.

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碩士<br>國立中興大學<br>環境工程學系所<br>103<br>Powder 13X zeolite was employed as the adsorbent for CO2 capture from flue gas by the dry sorbent injection and the feasibility of this process was evaluated. Research results were divided into the following two phases.The first phase was the comparison of the efficiency of capturing carbon dioxide between concurrent and countercurrent dry sorbent injection with powder 13X zeolite. The results indicate that the best of adsorption capacity was obtained under 30°C with 15 vol% CO2 inlet using powder 13X zeolite by the countercurrent dry sorbent injection. The ad
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17

Chen, Jia-Xian, and 陳嘉賢. "Post-combustion CO2 capture in a Dry Sorbent Injection system." Thesis, 2016. http://ndltd.ncl.edu.tw/handle/85586514884678742723.

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碩士<br>國立中興大學<br>環境工程學系所<br>104<br>The aim of this research is to obtain a technique of carbon capture which has economical development, refering to air pollution equipment in existence, we aim to change DSI into a technique of carbon capture. We use commercial material, zeolite 13X, to capture carbon for CO2 capture from flue gas. We intend to reduce carbon release and condense concentration of CO2 efficiently to promote capture and reuse of carbon. Then, we evaluate the possibility of this method according to the result of the resarch. Research results were divided into the following: The f
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18

Huang, Wen-Cheng, and 黃文誠. "CO2 Capture from Flue Gases by Continuous Modular Dry Sorbent Injection System." Thesis, 2018. http://ndltd.ncl.edu.tw/handle/qryq2z.

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碩士<br>國立中興大學<br>環境工程學系所<br>106<br>The research chooses commercially available granular 13X zeolites to capture CO2 in dry sorbent injection system. The gas mixture will simulate post-combustion flue gas with 15% CO2 and then discuss with CO2 adsorption capacity, desorption and regeneration effects. The research includes two parts. The first part is the test of desorption conditions with different temperatures, times and pressures. The adsorption process is conducted on 25oC with 0 vol.% water content and solid gas feed ratio is 24 g/L. After that, the research will do cyclic experiments for 3
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19

Hsieh, Tsung Yu, and 謝宗育. "On uniform temperature design of scale-up CO2 capture sorbent in fixed bed regeneration reactors." Thesis, 2016. http://ndltd.ncl.edu.tw/handle/41620705133456405524.

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碩士<br>國立清華大學<br>動力機械工程學系<br>104<br>The aim of this study is to design a uniform temperature distribution in scale-up fixed bed reactors with inserting the internal heat conducting part and different heating methods by numerical simulation. The performance of sorbents, the relevant capture efficiency and the number of running cycles can be improved due to the absence of hot spots. The simulation results show that the performance of desorption is only 58 % at 850 ℃ for the original design as the diameter of the reaction tube is increased from 1 inch to 4 inches. The reactor can be effectively
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20

Wu, Bi-Ching, and 吳碧卿. "Experimental study of CO2 Adsorption / Desorption with Solid Polyaniline Sorbent and Concentrating High Purity CO2 from Syngas after Oxy-fuel Combustion by Pressure Swing Adsorption Process." Thesis, 2017. http://ndltd.ncl.edu.tw/handle/babf6j.

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碩士<br>國立中央大學<br>化學工程與材料工程學系<br>105<br>With technology development, the greenhouse effect is becoming more and more serious. Reducing greenhouse gas emissions has become an important issue. The first part of the study is the experimental study of CO2 adsorption / desorption with Solid Polyaniline Sorbent of Taiwan Power Company (Taipower). Changing the different conditions for the synthesis of solid polyaniline carbon dioxide sorbent and the preparation of pelletization procedures obtains the optimal condition for producing solid polyaniline sorbent. The effects of different factors such as syn
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21

Lin, Chieh-Yen, and 林杰燕. "Synthesis and Characterization of Novel Ca-Mg-Mixed Metal Organic Framework as Sorbent Precursor Material for Efficient High Temperature CO2 Capture." Thesis, 2015. http://ndltd.ncl.edu.tw/handle/qtyppr.

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