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Journal articles on the topic 'Concerted mechanism'

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Published: 4 June 2021
Last updated: 1 February 2022

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1

Yonetani, Takashi. "Allosteric Mechanism of Hemoglobin: Concerted Mechanisms or Graded Mechanisms." Biophysical Journal 96, no. 3 (February 2009): 438a. http://dx.doi.org/10.1016/j.bpj.2008.12.2244.

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2

Miura, Retsu, and Yoshihiro Miyake. "The reaction mechanism of d-amino acid oxidase: Concerted or not concerted?" Bioorganic Chemistry 16, no. 1 (March 1988): 97–110. http://dx.doi.org/10.1016/0045-2068(88)90039-9.

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3

Liao, Daiqing. "Concerted Evolution: Molecular Mechanism and Biological Implications." American Journal of Human Genetics 64, no. 1 (January 1999): 24–30. http://dx.doi.org/10.1086/302221.

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4

Winkler, Andreas, Andrzej Łyskowski, Sabrina Riedl, Martin Puhl, Toni M. Kutchan, Peter Macheroux, and Karl Gruber. "A concerted mechanism for berberine bridge enzyme." Nature Chemical Biology 4, no. 12 (October 26, 2008): 739–41. http://dx.doi.org/10.1038/nchembio.123.

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5

Iguchi-Ariga, Sanae M. M., and Hiroyoshi Ariga. "Concerted mechanism of DNA replication and transcription." Cell Structure and Function 14, no. 6 (1989): 649–51. http://dx.doi.org/10.1247/csf.14.649.

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6

Islam, Zahidul, Timothy S. Strutzenberg, Ilya Gurevic, and Amnon Kohen. "Concerted versus Stepwise Mechanism in Thymidylate Synthase." Journal of the American Chemical Society 136, no. 28 (July 2014): 9850–53. http://dx.doi.org/10.1021/ja504341g.

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7

Cremer, Dieter, Elfi Kraka, Ramon Crehuet, Josep Anglada, and Jürgen Gräfenstein. "The ozone–acetylene reaction: concerted or non-concerted reaction mechanism? A quantum chemical investigation." Chemical Physics Letters 347, no. 1-3 (October 2001): 268–76. http://dx.doi.org/10.1016/s0009-2614(01)01032-6.

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8

Borisenko, Konstantin B., Yixin Chen, Se Ahn Song, Duc Nguyen-Manh, and David J. H. Cockayne. "A concerted rational crystallization/amorphization mechanism of Ge2Sb2Te5." Journal of Non-Crystalline Solids 355, no. 43-44 (October 2009): 2122–26. http://dx.doi.org/10.1016/j.jnoncrysol.2009.06.029.

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9

Jay, Eleanor E., Michael J. D. Rushton, and Robin W. Grimes. "Migration of fluorine in fluorapatite – a concerted mechanism." Journal of Materials Chemistry 22, no. 13 (2012): 6097. http://dx.doi.org/10.1039/c2jm16235k.

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10

Jackson, M. L., E. E. Jay, M. J. D. Rushton, and R. W. Grimes. "A concerted mechanism for Cl−migration in chlorapatite." J. Mater. Chem. A 2, no. 38 (August 6, 2014): 16157–64. http://dx.doi.org/10.1039/c4ta03275f.

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11

ARIGA, Takayuki. "Concerted Mechanism of Rotary Motor F1, Using Hybrid Enzymes." Seibutsu Butsuri 49, no. 2 (2009): 080–83. http://dx.doi.org/10.2142/biophys.49.080.

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12

Janotti, A., A. Fazzio, R. Mota, and P. Piquini. "Concerted-exchange mechanism for antistructure pair defects in GaAs." Solid State Communications 110, no. 8 (April 1999): 457–61. http://dx.doi.org/10.1016/s0038-1098(98)00606-1.

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13

Drain, Peter, Xuehui Geng, and Lehong Li. "Concerted Gating Mechanism Underlying KATP Channel Inhibition by ATP." Biophysical Journal 86, no. 4 (April 2004): 2101–12. http://dx.doi.org/10.1016/s0006-3495(04)74269-1.

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14

Chen, Wei-Hao, Xuejiao J. Gao, and Xingfa Gao. "Methanol-Assisted Phthalimide Ring Opening: Concerted or Stepwise Mechanism?" Journal of Physical Chemistry A 122, no. 12 (March 7, 2018): 3115–19. http://dx.doi.org/10.1021/acs.jpca.7b11347.

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15

Smith, William B. "Ethylene glycol to acetaldehyde-dehydration or a concerted mechanism." Tetrahedron 58, no. 11 (March 2002): 2091–94. http://dx.doi.org/10.1016/s0040-4020(02)00103-5.

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16

Zhang, X., and T. C. Bruice. "Reaction mechanism of guanidinoacetate methyltransferase, concerted or step-wise." Proceedings of the National Academy of Sciences 103, no. 44 (October 19, 2006): 16141–46. http://dx.doi.org/10.1073/pnas.0607503103.

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17

Wang, Jun, and Weitao Yang. "Concerted Proton Transfer Mechanism ofClostridium thermocellumRibose-5-phosphate Isomerase." Journal of Physical Chemistry B 117, no. 32 (August 2, 2013): 9354–61. http://dx.doi.org/10.1021/jp404948c.

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18

Bhak, Ghi-Bom, Young-Jun Choe, and Seung-R. Paik. "Mechanism of amyloidogenesis: nucleation-dependent fibrillation versus double-concerted fibrillation." BMB Reports 42, no. 9 (September 30, 2009): 541–51. http://dx.doi.org/10.5483/bmbrep.2009.42.9.541.

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19

Eberson, Lennart, Mark W. Lehmann, Armin Burghart, R. Daniel Little, Giuseppe Silvestri, André Tallec, Tatsuya Shono, and H. Toftlund. "Problems and Prospects of the Concerted Dissociative Electron Transfer Mechanism." Acta Chemica Scandinavica 53 (1999): 751–64. http://dx.doi.org/10.3891/acta.chem.scand.53-0751.

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20

Gridnev, Ilya D., Aleksey V. Shastin, and Elisabeth S. Balenkova. "The concerted mechanism of acylamidation. Syn-stereospecificity of the reaction." Tetrahedron 47, no. 29 (July 1991): 5577–84. http://dx.doi.org/10.1016/s0040-4020(01)80989-3.

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21

Wang, Li, and Ming Wah Wong. "Mechanism of halogen-catalyzed Mukaiyama aldol reactions: concerted or stepwise?" Tetrahedron Letters 49, no. 24 (June 2008): 3916–20. http://dx.doi.org/10.1016/j.tetlet.2008.04.054.

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22

Sun, Huabin, Chengbu Liu, Liming Zhao, and Lu Deng. "Mechanism of the concerted ring expansion of singlet cyclopropyl nitrene." Chemical Physics Letters 228, no. 1-3 (September 1994): 268–72. http://dx.doi.org/10.1016/0009-2614(94)00921-x.

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23

Newcomb, Martin, Marie-Helene Le Tadic-Biadatti, Daryl L. Chestney, Elizabeth S. Roberts, and Paul F. Hollenberg. "A nonsynchronous concerted mechanism for cytochrome P-450 catalyzed hydroxylation." Journal of the American Chemical Society 117, no. 49 (December 1995): 12085–91. http://dx.doi.org/10.1021/ja00154a008.

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24

Pandey, K. C. "Diffusion without Vacancies or Interstitials: A New Concerted Exchange Mechanism." Physical Review Letters 57, no. 18 (November 3, 1986): 2287–90. http://dx.doi.org/10.1103/physrevlett.57.2287.

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25

Bachrach, Steven M., and John C. Gilbert. "The Reaction of Cyclopentyne with Ethene: Concerted vs Stepwise Mechanism?" Journal of Organic Chemistry 69, no. 19 (September 2004): 6357–64. http://dx.doi.org/10.1021/jo0492970.

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26

Koleva, Gergana, Boris Galabov, Jing Kong, Henry F. Schaefer, and Paul von R. Schleyer. "Electrophilic Aromatic Sulfonation with SO3: Concerted or Classic SEAr Mechanism?" Journal of the American Chemical Society 133, no. 47 (November 30, 2011): 19094–101. http://dx.doi.org/10.1021/ja201866h.

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27

Sowa, Gwendolyn A., Alvan C. Hengge, and W. W. Cleland. "18O Isotope Effects Support a Concerted Mechanism for Ribonuclease A." Journal of the American Chemical Society 119, no. 9 (March 1997): 2319–20. http://dx.doi.org/10.1021/ja963974t.

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28

Pandey, K. "Diffusion without Vacancies or Interstitials: A New Concerted Exchange Mechanism." Materials Science Forum 10-12 (January 1986): 121–26. http://dx.doi.org/10.4028/www.scientific.net/msf.10-12.121.

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29

Singleton, Daniel A., and Brian E. Schulmeier. "Evidence for a Concerted Mechanism in a Palladium Trimethylenemethane Cycloaddition." Journal of the American Chemical Society 121, no. 40 (October 1999): 9313–17. http://dx.doi.org/10.1021/ja9919229.

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30

Cornaton, Yann, and Jean-Pierre Djukic. "A noncovalent interaction insight onto the concerted metallation deprotonation mechanism." Physical Chemistry Chemical Physics 21, no. 36 (2019): 20486–98. http://dx.doi.org/10.1039/c9cp03650d.

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31

Liu, Xiandong, and Evert Jan Meijer. "Mechanism of Base-Promoted Dehydrochlorination of Pentachloroethane: Concerted or Stepwise?" Journal of Physical Chemistry A 113, no. 15 (April 16, 2009): 3542–44. http://dx.doi.org/10.1021/jp900944g.

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32

Pratiwi, Indah, Bambang Cahyono, and Parsaoran Siahaan. "Ab-Initio Computational Study : The Activation Energy Changes and Steric Effects In Peptide Synthesis Of Ac-AA-NH2 and Ac-AP-NH2." Molekul 16, no. 2 (July 20, 2021): 137. http://dx.doi.org/10.20884/1.jm.2021.16.2.723.

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Ab-Initio computational method can be used for simulating reaction mechanisms, such as concerted reaction mechanism on peptide synthesis. The concerted reaction is one of many possible pathways on how peptide can be synthesized. The purpose of this study are probing the concerted reaction mechanism and comparing the steric effect to the reaction, given by different side-chain of alanine (A) and proline (P). Two dipeptides formed from alanine and proline were computed at HF-SCF/6-31G** theory level: Ac-AA-NH2 and Ac-AP-NH2. The res.lts show the activation energy of Ac-AA-NH2 and Ac-AP-NH2 forming via concerted pathway are 167.541 kJ/mol and 161.044 kJ/mol, respectively. The steric difference in side-chain affects the dihedral angle of the structure, and also gives difference to the entropy value of reaction.
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33

YU, LINGJUAN, DACHENG FENG, MAOXIA HE, RUI LI, and ZHENGTING CAI. "THEORETICAL STUDY ON HYDROLYSIS MECHANISM OF β-PHOSPHOLACTAMS." Journal of Theoretical and Computational Chemistry 05, spec01 (January 2006): 421–31. http://dx.doi.org/10.1142/s0219633606002362.

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The neutral hydrolysis mechanisms of a simple β-phospholactam with and without water-assisted reaction have been studied by using quantum chemical method at HF/6-31G**, MP2/6-31G** and B3LYP/6-31G** levels, respectively. The reaction can proceed by two different mechanisms: concerted and stepwise. There are two pathways in stepwise, i.e. pathway a and b, and the energy barriers of them are close. The energy barriers of water-assisted hydrolysis of β-phospholactam are obviously lower than those of no-water-assisted hydrolysis system. The energy barriers of stepwise mechanism are much lower than those of the concerted pathway in both cases. The solvent effects have been considered by means of a polarizable continuum model. The hydrolysis mechanism of β-phospholactam with that of the β-lactam and β-sultam was compared.
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34

Siadati, Seyyed Amir. "Beyond the Alternatives that Switch the Mechanism of the 1,3-Dipolar CyCloadditions from Concerted to Stepwise or Vice Versa: A Literature Review." Progress in Reaction Kinetics and Mechanism 41, no. 4 (November 2016): 331–44. http://dx.doi.org/10.3184/146867816x14719552202168.

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For several decades, the concerted or stepwise character of the mechanism of the 1,3-dipolar cycloaddition reaction has been one of the most debated issues in the field of organic chemistry. The significance of this problem is due to the fact that in a catalyst-free 1,3-dipolar cycloaddition, when the mechanism switches from concerted to stepwise, the stereospecificity is lost and thus unwanted stereoisomers may emerge. The first proposals about the mechanism of the 1,3-dipolar reaction were due to Huisgen (concerted model) and subsequently by Firestone (two-step diradical channel) in the 1960s. After a decade of debate, most researchers accepted the concerted model for the reaction, but during these years, researchers reported some examples of the stepwise mechanism for catalyst-free 1,3-dipolar cycloadditions. This review attempts to find a number of factors that could influence the reaction channels and switch the mechanism from concerted to stepwise, or vice versa.
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35

Tepper, Harald L., and Gregory A. Voth. "Protons May Leak through Pure Lipid Bilayers via a Concerted Mechanism." Biophysical Journal 88, no. 5 (May 2005): 3095–108. http://dx.doi.org/10.1529/biophysj.104.056184.

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36

Xu, Yiying, and Paul E. Dietze. "Evidence for a concerted mechanism in the solvolysis of phenyldimethylsilyl ethers." Journal of the American Chemical Society 115, no. 23 (November 1993): 10722–27. http://dx.doi.org/10.1021/ja00076a033.

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37

Angelis, Yiannis, Xiaojun Zhang, and Michael Orfanopoulos. "Secondary isotope effects in dioxirane epoxidations. Concerted or step-wise mechanism?" Tetrahedron Letters 37, no. 33 (August 1996): 5991–94. http://dx.doi.org/10.1016/0040-4039(96)01256-7.

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38

Guthrie, J. Peter. "Concerted mechanism for alcoholysis of esters: an examination of the requirements." Journal of the American Chemical Society 113, no. 10 (May 1991): 3941–49. http://dx.doi.org/10.1021/ja00010a040.

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39

Millman, Jonathan S., and David W. Andrews. "Switching the Model: A Concerted Mechanism for GTPases in Protein Targeting." Cell 89, no. 5 (May 1997): 673–76. http://dx.doi.org/10.1016/s0092-8674(00)80248-2.

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40

Yoshizawa, Kazunari, Takehiro Ohta, Masataka Eda, and Tokio Yamabe. "Two-Step Concerted Mechanism for the Hydrocarbon Hydroxylation by Cytochrome P450." Bulletin of the Chemical Society of Japan 73, no. 2 (February 2000): 401–7. http://dx.doi.org/10.1246/bcsj.73.401.

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41

Lu, Jin-Yong, John A. Keith, Wei-Zheng Shen, Markus Schürmann, Hans Preut, Timo Jacob, and Hans-Dieter Arndt. "Regioselective De Novo Synthesis of Cyanohydroxypyridines with a Concerted Cycloaddition Mechanism." Journal of the American Chemical Society 130, no. 40 (October 8, 2008): 13219–21. http://dx.doi.org/10.1021/ja804078v.

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42

Hutter, Michael C., and Volkhard Helms. "Phosphoryl transfer by a concerted reaction mechanism in UMP/CMP-kinase." Protein Science 9, no. 11 (2000): 2225–31. http://dx.doi.org/10.1110/ps.9.11.2225.

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43

GRIDNEV, I. D., A. V. SHASTIN, and E. S. BALENKOVA. "ChemInform Abstract: Concerted Mechanism of Acylamidation. syn-Stereospecificity of the Reaction." ChemInform 22, no. 42 (August 22, 2010): no. http://dx.doi.org/10.1002/chin.199142226.

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44

Snyder, Christopher H., Emma Berta Gutierrez-Cirlos, and Bernard L. Trumpower. "Evidence for a Concerted Mechanism of Ubiquinol Oxidation by the Cytochromebc1Complex." Journal of Biological Chemistry 275, no. 18 (April 28, 2000): 13535–41. http://dx.doi.org/10.1074/jbc.275.18.13535.

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45

Starnes,, William H., Joshua A. Wallach, and Hongyang Yao. "Six-Center Concerted Mechanism for Poly(vinyl chloride) Dehydrochlorination.Requiescat in Pace?" Macromolecules 29, no. 23 (January 1996): 7631–33. http://dx.doi.org/10.1021/ma9609036.

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46

Baranovskiy, Andrey G., Nigar D. Babayeva, Yinbo Zhang, Jianyou Gu, Yoshiaki Suwa, Youri I. Pavlov, and Tahir H. Tahirov. "Mechanism of Concerted RNA-DNA Primer Synthesis by the Human Primosome." Journal of Biological Chemistry 291, no. 19 (March 14, 2016): 10006–20. http://dx.doi.org/10.1074/jbc.m116.717405.

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47

Li, Yan, Chi-Wing Tsang, Eve Man Hin Chan, Eugene Yin Cheung Wong, Danny Chi Kuen Ho, Xiao-Ying Lu, and Changhai Liang. "Sustainable Option for Hydrogen Production: Mechanistic Study of the Interaction between Cobalt Pincer Complexes and Ammonia Borane." Catalysts 10, no. 7 (June 28, 2020): 723. http://dx.doi.org/10.3390/catal10070723.

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The mechanism of the solvolysis/hydrolysis of ammonia borane by iridium (Ir), cobalt (Co), iron (Fe) and ruthenium (Ru) complexes with various PNP ligands has been revisited using density functional theory (DFT). The approach of ammonia borane (NH3BH3) to the metal center has been tested on three different possible mechanisms, namely, the stepwise, concerted and proton transfer mechanism. It was found that the theoretical analyses correlate with the experimental results very well, with the activities of the iridium complexes with different PNP ligands following the order: (tBu)2P > (iPr)2P > (Ph)2P through the concerted mechanism. The reaction barriers of the rate-determining steps for the dehydrogenation of ammonia borane catalyzed by the active species [(tBu)2PNP-IrH] (Complex I-8), are found to be 19.3 kcal/mol (stepwise), 15.2 kcal/mol (concerted) and 26.8 kcal/mol (proton transfer), respectively. Thus, the concerted mechanism is the more kinetically favorable pathway. It is interesting to find that stable (tBu)2PNP Co-H2O and (tBu)2PNP Co-NH3 chelation products exist, which could stabilize the active I-8 species during the hydrolysis reaction cycle. The use of more sterically hindered and electron-donating PNP ligands such as (adamantyl)2P- provides similar activity as the t-butyl analogue. This research provides insights into the design of efficient cobalt catalysts instead of using precious and noble metal, which could benefit the development of a more sustainable hydrogen economy.
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48

Stamminger, Andreas R., Benedikt Ziebarth, Matous Mrovec, Thomas Hammerschmidt, and Ralf Drautz. "Fast diffusion mechanism in Li4P2S6via a concerted process of interstitial Li ions." RSC Advances 10, no. 18 (2020): 10715–22. http://dx.doi.org/10.1039/d0ra00932f.

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A new diffusion path comprising the concerted migration of lithium ions is proposed for Li4P2S6. Detailed analysis of the underlying migration process reveals a significantly reduced energy barrier compared to purely interstitial migration.
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49

Jalem, Randy, Yoshihiro Yamamoto, Hiromasa Shiiba, Masanobu Nakayama, Hirokazu Munakata, Toshihiro Kasuga, and Kiyoshi Kanamura. "Concerted Migration Mechanism in the Li Ion Dynamics of Garnet-Type Li7La3Zr2O12." Chemistry of Materials 25, no. 3 (January 18, 2013): 425–30. http://dx.doi.org/10.1021/cm303542x.

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50

Mazilova, T. I., E. V. Sadanov, V. N. Voyevodin, V. A. Ksenofontov, and I. M. Mikhailovskij. "Impact-induced concerted mass transport on W surfaces by a voidion mechanism." Surface Science 669 (March 2018): 10–15. http://dx.doi.org/10.1016/j.susc.2017.11.002.

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