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Dissertations / Theses on the topic 'Coordination chemistry of gold(I)'

Author: Grafiati

Published: 4 June 2021

Last updated: 15 February 2022

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1

Kifle, Hagos Tesfamariam. "New gold(I) and gold(III) coordination complexes derived from N and S heterocycles." Thesis, Stellenbosch : University of Stellenbosch, 2006. http://hdl.handle.net/10019.1/2843.

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2

Coetzee, Jacorien. "New developments in the coordination chemistry of gold(1), gold(II) and gold(III) with C-, N-, P-and S-Donor ligands /." Link to the online version, 2007. http://hdl.handle.net/10019/412.

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3

Savjani, N. "The chemistry of gold with unsaturated organics : coordination, activation and catalysis." Thesis, University of East Anglia, 2012. https://ueaeprints.uea.ac.uk/41412/.

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The aim was to understand gold‟s reactivity with unsaturated organic bonds. We focused on the role of supporting ligands, activating agents and the organic substrates employed in such reactions. Gold tetrafluorophthalimidates have been isolated, with coordination found to be surprisingly strong; no [N(CO)2C6F4]- displacement with ζ- and π-donors were observed. B(C6F5)3 and norbornene addition to [(Ph3P)Au{N(CO)2C6F4}] leads to a [Au(nbe)3]+ cation paired with a new, non-coordinating phthalimido-diborate anion. Aryl-N substituents of [(Ph3P)Au{nacnac}] influences its differing solid state struc

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4

Coetzee, Jacorien. "New developments in the coordination chemistry of Gold(I), Gold(II) and Gold(III) with C-, N- , P-and S-donor ligands." Thesis, Stellenbosch : University of Stellenbosch, 2007. http://hdl.handle.net/10019.1/1702.

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Thesis (MSc (Chemistry and Polymer Science))--University of Stellenbosch, 2007.<br>A comprehensive, comparative structural study of gold(I), gold(II) and gold(III) compounds with the general formula [Aux(C6F5)y(tht)z] (tht = tetrahydrothiophene) was performed. The series of compounds included the unprecedented dinucleur gold(II) compound, tetrakis(pentafluorophenyl)bis(tetrahydrothiophene)digold(II), which could be prepared in a rational manner. This very unique compound represents the first example of an unbridged dinucleur gold(II) compound in which the gold(II) centres are not stabilis

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5

Deligonul, Nihal. "COORDINATION AND ORGANOMETALLIC COMPLEXES OF RHODIUM, PALLADIUM, IRIDIUM, PLATINUM AND GOLD." Case Western Reserve University School of Graduate Studies / OhioLINK, 2013. http://rave.ohiolink.edu/etdc/view?acc_num=case1373109445.

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6

Wozniak, Derek Ian. "Anion effects in Homogeneous Palladium and Gold Catalysis." Diss., Temple University Libraries, 2019. http://cdm16002.contentdm.oclc.org/cdm/ref/collection/p245801coll10/id/588783.

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Chemistry<br>Ph.D.<br>The overarching theme of this work is to use weak interactions to improve transition metal catalysis by studying the ways transition metal cations interact with both traditional and novel weakly-coordinating anions. Understanding of these interactions will better allow synthetic chemists to choose appropriate counterions for catalytic transformations, as well as giving mechanistic insight for organometallic reactivity. Additionally, new anions can be synthesized with specific functionalities to improve reactions of interest. A series of ion pairs featuring the [Pd(IPr)(C(

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7

Hooper, Thomas Norman. "Elements in Low Coordination Numbers : New Frontiers in the Chemistry of Gold and Phosphorus." Thesis, University of Bristol, 2010. http://ethos.bl.uk/OrderDetails.do?uin=uk.bl.ethos.520668.

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8

Gabrielli, William Fullard. "Utilisation of various bonding modes of nitrogen-rich heterocycles in gold(I) chemistry." Thesis, Stellenbosch : University of Stellenbosch, 2006. http://hdl.handle.net/10019.1/1258.

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Thesis (PhD (Chemistry and Polymer Science))—University of Stellenbosch, 2006.<br>This study describes the exploitation of numerous donor ligand possibilities presented by selected nitrogen-rich heterocyclic ligands towards gold(I). The preparation and structural characterisation of novel gold(I) complexes, apart from conventional gold(I) bonding possibilities, also encompassed a study of bi- and polytopic bonding modes within a range of multifunctional ligands.

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9

Deetlefs, Maggel. "Carbene and coordination complexes of gold, palladium, platinum and manganese derived from N-containing heterocycles." Thesis, Stellenbosch : Stellenbosch University, 2001. http://hdl.handle.net/10019.1/52155.

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10

De, Jongh Leigh-Anne. "Imine-donor complexes with group 6 and group 11 transition metals : coordination and dynamics." Thesis, Stellenbosch : Stellenbosch University, 2008. http://hdl.handle.net/10019.1/2001.

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Thesis (MSc (Chemistry and Polymer Science))--Stellenbosch University, 2008.<br>In this study the coordination of ligands with several coordination sites, 2-aminoazoles (2- amino-4-methylthiazole), 2-aminobenzothiazole, 2-aminobenzoimidazole and 2- aminothiazoline and a biguanidine (N-(2-methylphenyl)imidodicarbonimidic diamide) to soft metal centres [gold(I) (group 11), chromium(0) (group 6) and tungsten (0) (group 6)] was investigated. The aminoazoles have three coordination sites, an exocyclic amine nitrogen, an endocyclic imine nitrogen and an endocyclic thioether sulphur. The biguan

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11

Rampazzi, Vincent. "Chimie de coordination du phosphore aux métaux du groupe 11 : progrès en catalyse de couplage C-N au Cu(I) et nouveaux complexes polyphosphines de l'Au(I)." Thesis, Dijon, 2014. http://www.theses.fr/2014DIJOS025/document.

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De nos jours et depuis quelques années maintenant, le principe de développement durable encourage les chimistes de tous horizons à développer de nouvelles méthodes de synthèse économiques et écologiques, les ressources naturelles de notre planète ne sont pas illimitées. Parmi les ressources les plus exploitées, nous trouvons le pétrole et le gaz. Outre ces derniers et le gaz, les métaux précieux sont également devenus indispensables.Cette thèse se concentre sur la valorisation de complexes de cuivre et d’or, obtenus à partir de ligands phosphorés synthétisés au sein du laboratoire. Dans un pre

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12

Rousselle, Benjamin. "Synthèse d’arylphosphines ortho-fonctionnalisées et leurs applications." Thesis, Bourgogne Franche-Comté, 2020. http://www.theses.fr/2020UBFCK024.

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Ce travail de thèse porte sur la synthèse d’arylphosphines ortho- fonctionnalisées par des groupements phosphonium et 1,2,3-triazole.La synthèse de phosphines-phosphoniums, utilisant comme étape clé un réarrangement de Phospha-Fries et une réaction d’Appel, est décrite. Huit nouvelles phosphines- phosphoniums, possédant des groupements alkyle, aryle et ferrocényle sur la partie phosphonium ont été préparées avec des rendements globaux atteignants 48%. Les phosphines-phosphoniums ont été utilisées pour la préparation de complexes d’or (I) qui ont été caractérisés par des méthodes spectroscopiqu

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13

Aitchison, Hannah. "Self-assembly of monolayers of aromatic carboxylic acid molecules on silver and copper modified gold surfaces at the liquid-solid interface." Thesis, University of St Andrews, 2015. http://hdl.handle.net/10023/6950.

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Exploiting coordination bonding of aromatic carboxylic acids at metal surfaces, this thesis explores new directions in the design and application of self-assembled monolayers (SAMs). The SAMs are investigated using a multi-technique approach comprising of a complementary combination of scanning tunneling microscopy (STM), X-ray photoelectron spectroscopy (XPS) and near-edge X-ray absorption fine structure (NEXAFS) spectroscopy. In addition, the X-ray standing wave technique (XSW) was used to characterise the substrates. The process of layer formation and the final structures of the SAMs are fo

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14

Noack, Cassandra, and n/a. "Studies in Coordination Chemistry." Griffith University. School of Science, 2003. http://www4.gu.edu.au:8080/adt-root/public/adt-QGU20031030.145610.

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The research reported in this thesis was carried out in Brisbane, Australia and Calgary, Canada. The aim of the research conducted in Brisbane was to prepare a series of copper(I) and ruthenium(II) based complexes incorporating a hemilabile phosphine ligand and to determine whether or not these compounds possessed catalytic activity. The history, uses, properties and recent work incorporating hemilabile phosphine ligands is discussed in detail as well as the application of hemilabile ligands to atom transfer radical polymerization (ATRP) and the usefulness of the 'windscreen wiper' action of

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15

Keene, Frank Richard. "Aspects of coordination chemistry /." Title page, contents and abstract only, 1998. http://web4.library.adelaide.edu.au/theses/09SD/09sdk26.pdf.

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16

Coetzee, Karolien. "Gold complexes obtained from gold ylide preparations." Thesis, Stellenbosch : Stellenbosch University, 2005. http://hdl.handle.net/10019.1/21206.

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Thesis (MSc)--University of Stellenbosch, 2005.<br>ENGLISH ABSTRACT: This investigation comprised the synthesis and characterisation of new Au(I) phosphonium ylide complexes and other compounds formed during coordination reactions. These complexes could exploit the synergism between two pharmacologically active substances (gold complex unit and phosphorus ylide) to furnish an even more active substance. Four phosphonium salts were prepared, [C6H5CH2PPh3]Br (1), [Ph3P(CH2)3PPh3]Br2 (2a), p-[{Ph3PCH2}2C6H4]Br2 (3a) and m- [{Ph3PCH2}2C6H4]Br2 (4a), by reacting PPh3 with the corresponding a

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17

Moore, Charles H. M. "Coordination chemistry of guanidine derivatives." Thesis, University of Nottingham, 1987. http://eprints.nottingham.ac.uk/14354/.

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This thesis describes an investigation of the coordination chemistry of l-cyanoguanidine (cnge), l-carbamoylguanidine (clge) and l-amidino-O-ethylurea (aOeu). Various copper(II) complexes of these analogous molecules were synthesised and characterised using mainly X-ray crystallographic and spectroscopic (infrared and UV-visible) techniques. Only bis (cnge) complexes were observed for copper(II) ions. The monodentate cnge ligands coordinated the copper(II) via their nitrile nitrogen atoms which were located in trans equatorial positions of the copper(II) ions's tetragonally distorted octahedra

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18

Grundy, Joanna. "Bifunctional amidines in coordination chemistry." Thesis, University of Sussex, 2003. http://ethos.bl.uk/OrderDetails.do?uin=uk.bl.ethos.398786.

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19

Mansfield, Natalie Emma. "Phosphaguanidines : coordination chemistry and catalysis." Thesis, University of Sussex, 2006. http://ethos.bl.uk/OrderDetails.do?uin=uk.bl.ethos.435610.

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20

Aucott, Stephen Mark. "Coordination chemistry of aminophosphine ligands." Thesis, Loughborough University, 1999. https://dspace.lboro.ac.uk/2134/34492.

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The reaction of [MCl2(cod)] (M = Pt, Pd) with two equivalents of 2-(diphenylphosphinoamino)pyridine, Ph2PNHpy, in warm acetonitrile led to cationic complexes of the type cis-[MCl(Ph2PNHpy-P,N){Ph2PNHpy-P}][Cl] (M = Pt, Pd) which exhibit broad single 31P{1H} NMR resonances due to their dynamic pyridyl exchange behaviour in solution. A single crystal X-ray diffraction study of the platinum species confirmed the proposed structure and revealed that adjacent complex molecules were held together by hydrogen bonding to the same chloride counter-ion. The bromo- and iodo-cis[MX(Ph2PNHpy-P,N){Ph2PNHpy-

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21

Wu, Haiying. "Coordination chemistry of tetraneopentoxyphthalocyaninatocobalt(II)." Thesis, University of British Columbia, 1991. http://hdl.handle.net/2429/29822.

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The thesis work reports developments in the coordination chemistry of tetra-neopentoxyphthalocyaninatocobalt(II) (CoTNPc) complexes. The preparation, characterization, and ligand binding measurements in solution of seven new compounds are described in this thesis. Some additional complexes are studied in situ. Measurement of the equilibrium constants by UV-visible spectroscopy for the 1:1 binding reactions of the axial ligands (L = imidazole, N-methylimidazole, pyridine, 4-picoline, 4-tert-butylpyridine, piperidine, tetrahydrofuran) to CoTNPc in toluene solution allow for an estimation of th

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22

Setyawati, Ika Agustin. "Coordination chemistry : basics to bioactive molecules." Thesis, National Library of Canada = Bibliothèque nationale du Canada, 1999. http://www.collectionscanada.ca/obj/s4/f2/dsk1/tape7/PQDD_0020/NQ46420.pdf.

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23

Amantia, David. "Coordination chemistry of chelate-tethered nucleobases." Thesis, University of Newcastle Upon Tyne, 2004. http://ethos.bl.uk/OrderDetails.do?uin=uk.bl.ethos.417527.

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24

Thompsett, Andrew Robert. "The coordination chemistry of unusual alkynes." Thesis, University of Warwick, 1998. http://ethos.bl.uk/OrderDetails.do?uin=uk.bl.ethos.302650.

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25

Wilson, Thomas Charles. "Coordination chemistry of the pentacyanocyclopentadienide anion." Thesis, University of Cambridge, 2014. https://ethos.bl.uk/OrderDetails.do?uin=uk.bl.ethos.708033.

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26

Balaraman, Lakshmi. "COORDINATION CHEMISTRY OF N,N’- AZODOXIDES." Cleveland State University / OhioLINK, 2019. http://rave.ohiolink.edu/etdc/view?acc_num=csu1556986156564604.

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27

Davies, Scott. "Catalysis by gold." Thesis, Cardiff University, 2017. http://orca.cf.ac.uk/100727/.

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The oxidation of benzyl alcohol over supported Au, Pd and AuPd catalysts on a range of metal oxide supports was investigated using a Radley’s Starfish Reactor. Reaction conditions such as temperature, solvent, support and metal loading were varied in order to obtain insight into benzyl alcohol oxidation. All catalysts were prepared using the sol immobilisation technique. It was discovered that AuPd bimetallic catalysts were most active for benzyl alcohol oxidation, in a ratio of 1:1 Au:Pd. Further, substituted benzyl alcohol compounds were oxidised using AuPd catalysts in order to investigate

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28

Yau, John. "The chemistry of gold(I) compounds." Thesis, Imperial College London, 1996. http://ethos.bl.uk/OrderDetails.do?uin=uk.bl.ethos.338901.

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29

Forward, Jennifer Mary. "Aspects of metallocarborane and gold chemistry." Thesis, University of Oxford, 1993. http://ethos.bl.uk/OrderDetails.do?uin=uk.bl.ethos.316885.

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30

Jelliss, Paul A. "Chemistry of gold(I) carbaborane complexes." Thesis, University of Bristol, 1993. http://ethos.bl.uk/OrderDetails.do?uin=uk.bl.ethos.358045.

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31

MuÌˆller, Thomas Ernst. "Studies of polyaromatic phosphines and their coordination to noble metals." Thesis, Imperial College London, 1995. http://ethos.bl.uk/OrderDetails.do?uin=uk.bl.ethos.309833.

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32

Chapman, Erich G. 1984. "Platinum coordination to RNA." Thesis, University of Oregon, 2010. http://hdl.handle.net/1794/11072.

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xix, 111 p. : ill. (some col.)<br>Since discovery of its biological effects in the late 1960's, cisplatin (cis-diamminedichloroplatinum( II)) has become one of the most broadly-prescribed cancer drugs in use today. A majority of efforts to understand the metallobiochemistry of this drug have focused on describing the interactions of cisplatin-derived Pt(II) complexes with DNA. Drug binding to this "high value" cellular target is believed to trigger the apoptotic pathways that underlie cisplatin's cytotoxic effects. Although RNA is chemically similar to DNA and responsible for accurately transf

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33

Farkas, Ildiko. "Coordination Chemistry of Actinide and Lanthanide Ions." Doctoral thesis, KTH, Chemistry, 2001. http://urn.kb.se/resolve?urn=urn:nbn:se:kth:diva-3236.

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34

Farkas, Ildikó. "Coordination chemistry of actinide and lanthanide ions /." Stockholm, 2001. http://urn.kb.se/resolve?urn=urn:nbn:se:kth:diva-3236.

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35

Al-Rasbi, Nawal K. "The coordination chemistry of new multidentate ligands." Thesis, University of Sheffield, 2008. http://ethos.bl.uk/OrderDetails.do?uin=uk.bl.ethos.489370.

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The content of this thesis is concerned with two distinctly independent areas of research: (i) the synthesis and coordination chemistry of new multidentate ligands and investigate their emission properties; (ii) the synthesis and study of new poly(pyrazol-1-yl)borate and Pt(II) based ligands and their lanthanide complexes.

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36

Tatchell, Thomas. "Coordination chemistry of pendant aniline aza-macrocycles." Thesis, Cardiff University, 2005. http://orca.cf.ac.uk/56099/.

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The selective functionalisation of triazamacrocycles is investigated herein, with the focus on 1, 4, 7-triazacyclononane (tacn) The ligands tris (5-fluoro, 2- aminophenyl) 1, 4, 7-triazacyclononane (L1), tris (4-fluoro, 2-aminophenyl) 1,4, 7- triazacyclononane (L") and tris (3-fluoro, 2-ammophenyl) 1, 4, 7-triazacyclononane (L ) were studied. X-Ray crystal data was obtained for (L,)M (C104)2.x:MeCN where M=Mn,,/FeII/Ni"/CuII/Znn/CdII/Hgn, (L2)M (C104)2 xMeCN where M=Mn1I/Fe,I/NiII/CuII/ZnII/Cdn and (L3)M (C104)2 xMeCN where M=Mn,1/NiI,/Cun/Zn,I/Cd,,/Pb11 complexes. The (L,)Cu (C104)2 complex e

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37

Schleep, Mario [Verfasser], and Ingo [Akademischer Betreuer] Krossing. "Molecular and coordination chemistry of Tin(II)." Freiburg : Universität, 2017. http://d-nb.info/1143602927/34.

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38

Metcalfe, John Edwin. "Studies in nickel and manganese coordination chemistry." Thesis, Queen's University Belfast, 1998. http://ethos.bl.uk/OrderDetails.do?uin=uk.bl.ethos.263502.

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39

Bishop, P. T. "The coordination chemistry of sterically hindered theolates." Thesis, University of Essex, 1987. http://ethos.bl.uk/OrderDetails.do?uin=uk.bl.ethos.381248.

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40

Champness, Neil Robert. "Studies in ruthenium and osmium coordination chemistry." Thesis, University of Southampton, 1993. http://ethos.bl.uk/OrderDetails.do?uin=uk.bl.ethos.239648.

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41

Orchard, Simon David. "Synthesis and coordination chemistry of telluroether ligands." Thesis, University of Southampton, 2000. http://ethos.bl.uk/OrderDetails.do?uin=uk.bl.ethos.326303.

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42

Mistry, Rakesh. "Synthesis and coordination chemistry of carboranyl phosphines." Thesis, University of Bristol, 2007. http://ethos.bl.uk/OrderDetails.do?uin=uk.bl.ethos.442207.

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43

Khalaf, Majid Shannon. "Coordination chemistry of bicyclic guanidines and guanidinates." Thesis, University of Sussex, 2011. http://sro.sussex.ac.uk/id/eprint/7347/.

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A [5:5] ligand based on the bicyclic guanidine 1,4,6-triazabicyclo[3.3.0]oct-4-ene [Htbo] has been synthesised. Two of these tbo units have been linked via a carbon bridgehead to form a novel bidentate ligand. Based on the knowledge that the electronic properties and specific steric interactions at a metal can lead to new insights into the relationship between crystal structure and ligand activity, the synthesised compounds have been investigated as polydentate ligands on the assumption that that they could be used to precisely control coordination environment. The corresponding [6:6] system w

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44

Cullen, William M. "Host-guest chemistry of polyhedral coordination cages." Thesis, University of Sheffield, 2015. http://etheses.whiterose.ac.uk/11545/.

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Chapter 1 – Introduction Chapter 2 – Synthesis, characterisation and manipulation of a three component self-assembled system Chapter 3 – Development and utilisation of a fluorescence displacement assay for guest screening Chapter 4 – Prediction of guest binding using molecular docking Chapter 5 – The use of pH changes to control guest binding in water Chapter 6 – Highly efficient catalysis of the Kemp Elimination in the cage cavity.

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45

Benson, Callum Giles Maxwell. "Synthesis and coordination chemistry of functionalised phosphazanes." Thesis, University of Cambridge, 2016. https://www.repository.cam.ac.uk/handle/1810/264415.

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This thesis focuses on the chemistry of novel phosphazane species derived from the chloro-phosphazanes [ClP(μ-NR)]$_2$ and their use as ligands and building blocks for macrocyclic compounds. The introduction (Chapter 1) surveys previous literature in the area, which is pertinent to the new studies. One of the most important issues is the various ways in which dimeric phosph(III)azanes can be employed as precursors for new ligands and in the design of new types of inorganic macrocycles. In Chapter 2 the synthesis of new chloro-dimers of the type [ClP(μ-NR)]$_2$ is described, which are the prima

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46

Hannon, Michael John. "Metal ion control in oligopyridine coordination chemistry." Thesis, University of Cambridge, 1993. https://www.repository.cam.ac.uk/handle/1810/272558.

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47

Clifton, Jamie. "Phosphinothiophene ligands : coordination chemistry, catalysis, and polymerisation." Thesis, University of Bristol, 2016. http://ethos.bl.uk/OrderDetails.do?uin=uk.bl.ethos.687601.

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48

Van, Veelen Arjen. "Uranium coordination chemistry in Mg-rich systems." Thesis, University of Manchester, 2014. https://www.research.manchester.ac.uk/portal/en/theses/uranium-coordination-chemistry-in-mgrich-systems(707b1576-699c-4f0a-b945-7482cfb7f51f).html.

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In the UK, large quantities of intermediate level waste pose complex radiological remediation challenges. Chemical understanding of uranium in these Mg-rich sludges is vital. Previous studies have examined uranium uptake by calcium carbonate minerals (calcite and aragonite) under conditions pertinent to both natural and anthropogenically perturbed systems. However, research on uranyl uptake by magnesium-rich minerals such as magnesite [MgCO3], brucite [Mg(OH)2], nesquehonite [MgCO3·3H2O] and hydromagnesite-[Mg5(CO3)4(OH)2·4H2O] has not, to the best of our knowledge, been previously conducted.

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49

Youfu, Katsuyuki. "Coordination chemistry and reactivities of expanded porphyrins." 京都大学 (Kyoto University), 2006. http://hdl.handle.net/2433/144223.

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50

Mjos, Katja Dralle. "Coordination chemistry of antimicrobial and anticancer agents." Thesis, University of British Columbia, 2015. http://hdl.handle.net/2429/54682.

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The World Health Organization has named the resistance of microbes to known antimicrobial drugs as an increasingly serious threat to global public health. Isolates of the ESKAPE pathogens (E. faecium, S. aureus, K. pneumonia, A. baumanii, P. aeruginosa, and Enterobacter species) are responsible for many nosocomial infections each year that require complicated, and therefore expensive, medical treatment, often leading to death in immune-compromised patients. Over the past 50 years, (fluoro-)quinolone antimicrobial agents have been widely used in the clinic as broad-spectrum antibiotics, but lat

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