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Journal articles on the topic 'CrSBr'

Author: Grafiati
Published: 2 June 2025
Last updated: 31 July 2025

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1

Hu, Chao, Huanghuang Cheng, Jiayuan Zhou, Kai Zhang, Xue Liu, and Yuxuan Jiang. "Layer Dependence of Complex Refractive Index in CrSBr." Materials 17, no. 14 (2024): 3430. http://dx.doi.org/10.3390/ma17143430.

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CrSBr is a recently discovered two-dimensional anti-ferromagnet. It has attracted much attention due to its superior properties for potential optoelectronic and spintronic applications. However, its complex refractive index with layer dependence has not been systematically studied yet. In this work, we studied the room-temperature complex refractive indices of thin CrSBr flakes of different thicknesses in the visible light range. Using micro-reflectance spectroscopy, we measured the optical contrast of thin CrSBr flakes with respect to different substrates. The complex refractive index was ext
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2

Liu, Hao, Yue-Yang Liu, Hongyu Wen, et al. "Spin-Filter Magnetic Tunnel Junctions Based on A-Type Antiferromagnetic CrSBr with Giant Tunnel Magnetoresistance." Magnetochemistry 8, no. 8 (2022): 89. http://dx.doi.org/10.3390/magnetochemistry8080089.

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CrSBr is a stable two-dimensional (2D) van der Waals (vdW) magnet with intralayer ferromagnetic and interlayer antiferromagnetic couplings. Here, we propose to use CrSBr as the barrier in spin-filter (sf) MTJ and establish the devices based on graphene/CrSBr/graphene structures. Employing density functional theory (DFT) combined with the nonequilibrium Green’s function approach, we investigated the transmission details, and the results show TMR values above 330%, 2 × 107% and 105% with two-, four- and six-layer CrSBr at zero bias, respectively. Subsequently, we systematically analyze the trans
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3

Sahu, Satyam, Oleksandr Volochanskyi, Vaibhav Varade, et al. "Tuning of MoS2 Photoluminescence in Heterostructures with CrSBr." ACS Applied Materials & Interfaces 17, no. 17 (2025): 25693–701. https://doi.org/10.1021/acsami.5c01924.

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This is the final version of the manuscript <em>"Tuning of MoS2 Photoluminescence in Heterostructures with CrSBr"</em> published in ACS Applied Materials &amp; Interfaces 2025, 17, 17, 25693-25701. Abstract: Monolayers of semiconducting transition metal dichalcogenides (TMDCs) are known for their unique excitonic photoluminescence (PL), which can be tuned by interfacing them with other materials. However, integrating TMDCs into van der Waals heterostructures often results in a significant quenching of the PL because of an increased rate of nonradiative recombination processes. We demonstrate a
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4

Craco, Luis, and Sabrina Silva Carara. "Effect of t2g-Correlations and Doping in CrSBr Ferromagnetic Semiconductor." Condensed Matter 10, no. 2 (2025): 27. https://doi.org/10.3390/condmat10020027.

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We perform a comprehensive analysis of the correlated electronic structure reconstruction of the ferromagnetic CrSBr van der Waals (vdW) bulk crystal. Using generalized gradient approximation combined with dynamical mean-field theory, we show the minor role played by multi-orbital electron–electron interactions in semiconducting CrSBr. Our study is relevant to understanding the electronic structure within the Cr3+ oxidation state with strongly spin-polarized t2g orbitals and should be applicable to other ferromagnetic vdW materials from bulk down to the low-dimensional limit. This work is rele
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5

Göser, O., W. Paul, and H. G. Kahle. "Magnetic properties of CrSBr." Journal of Magnetism and Magnetic Materials 92, no. 1 (1990): 129–36. http://dx.doi.org/10.1016/0304-8853(90)90689-n.

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6

Gao, Yinlu, Qinxi Liu, Xue Jiang, and Jijun Zhao. "Proximity coupling induced significantly enhanced Curie temperature in van der Waals CrSBr/MoTe2 heterostructure." Applied Physics Letters 121, no. 16 (2022): 162402. http://dx.doi.org/10.1063/5.0098799.

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CrSBr monolayer is a promising ferromagnetic (FM) semiconductor with stable magnetic ground state, large bandgap, and high carrier density. However, its Curie temperature ( TC) of about 146 K is still below room temperature. Herein, electronic and magnetic properties of a CrSBr/MoTe2 heterostructure are explored to boost the TC via the proximity effect using first-principles calculations. The long-range FM ordering in the CrSBr layer is enhanced both through an extra spin superexchange channel (Cr–Te–Cr) afforded by the MoTe2 substrate and the reduced degeneracy t2 g orbitals of Cr atoms. Dire
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7

Han, Ruilin, Xiaomin Xue, and Yu Yan. "Hole-Doping-Induced Perpendicular Magnetic Anisotropy and High Curie Temperature in a CrSX (X = Cl, Br, I) Semiconductor Monolayer." Nanomaterials 13, no. 24 (2023): 3105. http://dx.doi.org/10.3390/nano13243105.

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A large perpendicular magnetic anisotropy and a high Curie temperature (TC) are crucial for the application of two-dimensional (2D) intrinsic ferromagnets to spintronic devices. Here, we investigated the electronic and magnetic properties of carrier-doped Van der Waals layered CrSX (X = Cl, Br, I) ferromagnets using first-principles calculations. It was found that hole doping can increase the magnitude of the magnetic anisotropy energy (MAE) and change the orientation of the easy magnetization axis at small doping amounts of 2.37 × 1013, 3.98 × 1012, and 3.33 × 1012/cm2 for CrSCl, CrSBr, and C
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8

Yang, Kunlin, Guorui Zhao, Yibin Zhao, et al. "A Polycarbonate-Assisted Transfer Method for van der Waals Contacts to Magnetic Two-Dimensional Materials." Micromachines 15, no. 11 (2024): 1401. http://dx.doi.org/10.3390/mi15111401.

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Magnetic two-dimensional (2D) materials have garnered significant attention for their potential to revolutionize 2D spintronics due to their unique magnetic properties. However, their air-sensitivity and highly insulating nature of the magnetic semiconductors present substantial challenges for device fabrication with effective contacts. In this study, we introduce a polycarbonate (PC)-assisted transfer method that effectively forms van der Waals (vdW) contacts with 2D materials, streamlining the fabrication process without the need for additional lithography. This method is particularly advant
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9

Lee, Kihong, Avalon H. Dismukes, Evan J. Telford, et al. "Magnetic Order and Symmetry in the 2D Semiconductor CrSBr." Nano Letters 21, no. 8 (2021): 3511–17. http://dx.doi.org/10.1021/acs.nanolett.1c00219.

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10

Xu, Murong, Chun Zhou, Zihui Wang, et al. "Solid-State Bromine for Bromide Synthesis, a Case Study of CrSBr." Acta Chimica Sinica 82, no. 12 (2024): 1234. https://doi.org/10.6023/a24090276.

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11

Beck, Johannes. "�ber Chalkogenidhalogenide des Chroms Synthese, Kristallstruktur und Magnetismus von Chromsulfidbromid, CrSBr." Zeitschrift f�r anorganische und allgemeine Chemie 585, no. 1 (1990): 157–67. http://dx.doi.org/10.1002/zaac.19905850118.

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12

Bo, Xiangyan, Feng Li, Xinyu Xu, Xiangang Wan, and Yong Pu. "Calculated magnetic exchange interactions in the van der Waals layered magnet CrSBr." New Journal of Physics, January 17, 2023. http://dx.doi.org/10.1088/1367-2630/acb3ee.

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Abstract Intrinsic van der Waals materials layered magnets have attracted much attention, especially the air-stable semiconductor CrSBr. Herein, we carry out a comprehensive investigation of both bulk and monolayer CrSBr using the first-principles linear-response method. Through the calculation of the magnetic exchange interactions, it is confirmed that the ground state of bulk CrSBr is A-type antiferromagnetic, while there are five sizable large intralayer exchange interactions with small magnetic frustration, which results in a relatively high magnetic transition temperature of both bulk and
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13

Pei, Fangfang, Jingjing Yu, Jiayuan Zhou, et al. "Surface‐Sensitive Detection of Magnetic Phase Transition in Van Der Waals Magnet CrSBr." Advanced Functional Materials, December 10, 2023. http://dx.doi.org/10.1002/adfm.202309335.

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Abstract2D magnets have recently drawn enormous interest. As an air‐stable A‐type van der Waals antiferromagnet (AFM), CrSBr has attracted great attention but has also led to controversies about its large‐span ordering temperatures. Herein, a systematic study of the magnetic phase transition in single‐crystalline CrSBr with ultrahigh‐quality through surface‐sensitive X‐ray magnetic linear dichroism and X‐ray magnetic circular dichroism measurements combined with vibrating sample magnetometry for characterization of bulk magnetization is reported. The interlayer AFM order of both surface and bu
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14

Mosina, Kseniia, Bing Wu, Nikolas Antonatos, et al. "Electrochemical Intercalation and Exfoliation of CrSBr into Ferromagnetic Fibers and Nanoribbons." Small Methods, December 29, 2023. http://dx.doi.org/10.1002/smtd.202300609.

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AbstractRecent studies dedicated to layered van der Waals crystals have attracted significant attention to magnetic atomically thin crystals offering unprecedented opportunities for applications in innovative magnetoelectric, magneto‐optic, and spintronic devices. The active search for original platforms for the low‐dimensional magnetism study has emphasized the entirely new magnetic properties of two dimensional (2D) semiconductor CrSBr. Herein, for the first time, the electrochemical exfoliation of bulk CrSBr in a non‐aqueous environment is demonstrated. Notably, crystal cleavage governed by
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15

Mosina, Kseniia, Bing Wu, Nikolas Antonatos, et al. "Electrochemical Intercalation and Exfoliation of CrSBr into Ferromagnetic Fibers and Nanoribbons." December 29, 2023. https://doi.org/10.1002/smtd.202300609.

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Recent studies dedicated to layered van der Waals crystals have attracted significant attention to magnetic atomically thin crystals offering unprecedented opportunities for applications in innovative magnetoelectric, magneto-optic, and spintronic devices. The active search for original platforms for the low-dimensional magnetism study has emphasized the entirely new magnetic properties of&nbsp;two dimensional (2D) semiconductor CrSBr. Herein, for the first time, the electrochemical exfoliation of bulk CrSBr in a non-aqueous environment is demonstrated. Notably, crystal cleavage governed by th
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16

Rudenko, Alexander N., Malte Rösner, and Mikhail I. Katsnelson. "Dielectric tunability of magnetic properties in orthorhombic ferromagnetic monolayer CrSBr." npj Computational Materials 9, no. 1 (2023). http://dx.doi.org/10.1038/s41524-023-01050-3.

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AbstractMonolayer CrSBr is a recently discovered semiconducting spin-3/2 ferromagnet with a Curie temperature of around 146 K. In contrast to many other known 2D magnets, the orthorhombic lattice of CrSBr gives rise to spatial anisotropy of magnetic excitations within the 2D plane. Triaxial magnetic anisotropy and considerable magnetic dipolar interactions in CrSBr challenge its theoretical description in terms of spin Hamiltonians. Here, we employ a Green’s function formalism combined with first-principles calculations to study the magnetic properties of monolayer CrSBr in different regimes o
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17

Wei, Xin, Mengdi Li, Xiangxiang He, et al. "Spin–phonon coupling and phonon dynamics in van der Waals antiferromagnetic CrSBr." Applied Physics Letters 126, no. 25 (2025). https://doi.org/10.1063/5.0277983.

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As a vander Waals antiferromagnetic semiconductor, CrSBr exhibits unique anisotropy and hosts various physical phenomena (e.g., magnons, phonons, excitons, and polarons), showing great application potential. However, extensive investigations of its spin–phonon coupling and phonon dynamics are still limited. In this study, we employed a combination of group theory analysis and first-principles calculations and carried out comprehensive angle-resolved polarization-dependent and temperature-dependent Raman spectroscopy measurements on CrSBr single crystals. The abnormal shifts in phonon frequency
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18

Cheng, Huanghuang, Jiayuan Zhou, Chao Hu, et al. "Magnetic sensitive mechanical response in CrSBr and its composite resonators." Applied Physics Letters 125, no. 18 (2024). http://dx.doi.org/10.1063/5.0233033.

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We study the mechanical response of bulk CrSBr in temperature using a CrSBr string resonator. We observe two abrupt changes in eigenfrequency and quality factor of the resonator with decreasing temperature, a strong one around 140 K due to an antiferromagnetic phase transition, and a weaker one around 200 K possibly related to a change of spin correlations. We find that the antiferromagnetic transition persists through a temperature window of 30 K rather than showing a narrow sharp change, indicating a gradual spin transition process. In addition, the quality factor exhibits an unexpected incr
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19

Rizzo, Daniel J., Eric Seewald, Fangzhou Zhao, et al. "Engineering anisotropic electrodynamics at the graphene/CrSBr interface." Nature Communications 16, no. 1 (2025). https://doi.org/10.1038/s41467-025-56804-y.

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Abstract Graphene is a privileged 2D platform for hosting confined light-matter excitations known as surface plasmon polaritons (SPPs), as it possesses low intrinsic losses and a high degree of optical confinement. However, the isotropic nature of graphene limits its ability to guide and focus SPPs, making it less suitable than anisotropic elliptical and hyperbolic materials for polaritonic lensing and canalization. Here, we present graphene/CrSBr as an engineered 2D interface that hosts highly anisotropic SPP propagation across mid-infrared and terahertz energies. Using scanning tunneling mic
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20

Cham, Thow Min Jerald, Reiley J. Dorrian, Xiyue S. Zhang, et al. "Exchange Bias between Van Der Waals Materials: Tilted Magnetic States and Field‐Free Spin‐Orbit‐Torque Switching." Advanced Materials, October 6, 2023. http://dx.doi.org/10.1002/adma.202305739.

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AbstractMagnetic van der Waals heterostructures provide a unique platform to study magnetism and spintronics device concepts in the two‐dimensional limit. Here, we report studies of exchange bias from the van der Waals antiferromagnet CrSBr acting on the van der Waals ferromagnet FeGeTe (FGT). The orientation of the exchange bias is along the in‐plane easy axis of CrSBr, perpendicular to the out‐of‐plane anisotropy of the FGT, inducing a strongly tilted magnetic configuration in the FGT. Furthermore, the in‐plane exchange bias provides sufficient symmetry breaking to allow deterministic spin‐o
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21

Huang, Xinyue, Zhigang Song, Yuchen Gao, et al. "Intrinsic Localized Excitons in MoSe2/CrSBr Heterostructure." Advanced Materials, December 18, 2024. https://doi.org/10.1002/adma.202413438.

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AbstractDespite extensive studies on magnetic proximity effects, the fundamental excitonic properties of the 2D semiconductor‐magnet heterostructures remain elusive. Here, the presence of localized excitons in MoSe2/CrSBr heterostructures is unveiled, represented by a new photoluminescence emission feature, X*. Our findings reveal that X* originates from excitons confined by intrinsic defects in the CrSBr layer. Additionally, the degrees of valley polarization of the X* and trion peaks exhibit opposite polarities under a magnetic field and closely correlate with the magnetic order of CrSBr. Th
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22

Khan, Muhammad Asghar, Muhammad Farooq Khan, Muhammad Nasim, et al. "Photonic Synapse of CrSBr/PtS2 Transistor for Neuromorphic Computing and Light Decoding." Advanced Functional Materials, October 15, 2024. http://dx.doi.org/10.1002/adfm.202410974.

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Abstract Field effect transistors based on 2D layered material have gained significant potential in emerging technologies, such as neuromorphic computing and ultrafast memory response for artificial intelligence applications. This study proposes a facile approach to fabricate an optoelectronic artificial synapse for neuromorphic computing and light‐decoding information system by utilizing the 2D heterostructure of CrSBr/PtS2 to overcome circuit complexity. The CrSBr layer serves as a trapping layer, while PtS2, mounted on top of CrSBr, acts as a channel layer. PtS2 exhibits n‐type semiconducto
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23

Rybakov, Andrey, Carla Boix‐Constant, Diego Alba Venero, Herre S. J. van der Zant, Samuel Mañas‐Valero, and Eugenio Coronado. "Probing Short‐Range Correlations in the van der Waals Magnet CrSBr by Small‐Angle Neutron Scattering." Small Science, June 13, 2024. http://dx.doi.org/10.1002/smsc.202400244.

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The layered metamagnet CrSBr offers a rich interplay between magnetic, optical, and electrical properties that can be extended down to the two‐dimensional (2D) limit. Despite the extensive research regarding the long‐range magnetic order in magnetic van der Waals materials, short‐range correlations have been loosely investigated. By using small‐angle neutron scattering (SANS) the formation of short‐range magnetic regions in CrSBr with correlation lengths that increase upon cooling up to ≈3 nm at the antiferromagnetic ordering temperature (T N ≈ 140 K) is shown. Interestingly, these ferromagnet
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24

Klein, Julian, and Frances M. Ross. "Materials beyond monolayers: The magnetic quasi-1D semiconductor CrSBr." Journal of Materials Research, November 6, 2024. http://dx.doi.org/10.1557/s43578-024-01459-6.

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AbstractThe all-surface nature of atomically thin van der Waals materials can present challenges for practical applications. Fortunately, new layered materials are on the horizon that preserve their useful properties even when thicker than a monolayer. Here, we summarize our interest in one of these emergent materials, the magnetic semiconductor CrSBr. We describe monolayer properties exhibited by this material in its bulk form, discussing how the quasi-1D electronic structure of CrSBr allows mono- or bilayer physics to be displayed even in thick crystals. Long-range magnetic order offers addi
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25

Tschudin, Märta A., David A. Broadway, Patrick Siegwolf, et al. "Imaging nanomagnetism and magnetic phase transitions in atomically thin CrSBr." Nature Communications 15, no. 1 (2024). http://dx.doi.org/10.1038/s41467-024-49717-9.

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AbstractSince their first observation in 2017, atomically thin van der Waals (vdW) magnets have attracted significant fundamental, and application-driven attention. However, their low ordering temperatures, Tc, sensitivity to atmospheric conditions and difficulties in preparing clean large-area samples still present major limitations to further progress, especially amongst van der Waals magnetic semiconductors. The remarkably stable, high-Tc vdW magnet CrSBr has the potential to overcome these key shortcomings, but its nanoscale properties and rich magnetic phase diagram remain poorly understo
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26

Jo, Junhyeon, Manuel Suárez‐Rodríguez, Samuel Mañas‐Valero, et al. "Anomalous Nonlinear Magnetoconductivity in van der Waals Magnet CrSBr." Advanced Materials, March 10, 2025. https://doi.org/10.1002/adma.202419283.

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AbstractNonlinear magnetoconductivity (NLMC) is a nonreciprocal transport response arising in non‐centrosymmetric materials. However, this ordinary NLMC signal vanishes at zero magnetic field, limiting its potential for applications. Here, the observation of an anomalous NLMC controlled by internal order parameters such as the magnetization or Néel vectors is reported. This response is achieved by breaking both inversion and time‐reversal symmetry in artificial van der Waals heterostructures based on the magnetic CrSBr and insulating hBN. The nonreciprocal signal can be tuned between two diffe
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27

Mondal, Priyanka, Daria I. Markina, Lennard Hopf, et al. "Raman polarization switching in CrSBr." npj 2D Materials and Applications 9, no. 1 (2025). https://doi.org/10.1038/s41699-025-00542-8.

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Abstract Semiconducting CrSBr is a layered A-type antiferromagnet, with individual layers antiferromagnetically coupled along the stacking direction. Due to its unique orthorhombic crystal structure, CrSBr exhibits highly anisotropic mechanical and optoelectronic properties acting itself as a quasi-1D material. CrSBr demonstrates complex coupling phenomena involving phonons, excitons, magnons, and polaritons. Here we show through polarization-resolved resonant Raman scattering the intricate interaction between the vibrational and electronic properties of CrSBr. For samples spanning from few-la
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28

Dey, Sourav, Dorye L. Esteras, and José J. Baldoví. "Tailoring the properties of the 2D ferromagnet CrSBr by lanthanide doping." Journal of Physics: Materials, March 21, 2025. https://doi.org/10.1088/2515-7639/adc3cd.

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Abstract The increasing fascination with 2D van der Waals (vdW) magnetic materials arises from their distinctive properties and promising applications in spintronics, magnonics, and quantum information technologies. Among them, CrSBr is a semiconductor that stands out owing to its high Curie temperature (TC ~ 146 K), air stability and tunable electronic and magnetic properties. Here, we present a systematic investigation of the effects of Dy doping (12.5%, 25%, and 50%) on the structural, electronic and magnetic properties of CrSBr monolayer. Our results reveal that Dy incorporation enhances m
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29

Long, Fangchao, Yi Li, Yu Cheng, et al. "Rise and Fall of the Ferromagnetism in CrSBr Flakes by Non‐Magnetic Ion Irradiation." Advanced Physics Research, June 13, 2024. http://dx.doi.org/10.1002/apxr.202400053.

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AbstractThe magnetic phase transition is explored in CrSBr flakes through non‐magnetic ion irradiation, revealing a novel method for magnetic control in two‐dimensional (2D) materials. The rise and fall of the ferromagnetic phase is observed in antiferromagnetic CrSBr with increasing the irradiation fluence. The irradiated CrSBr shows ferromagnetic critical temperature ranging from 110 to 84 K, well above liquid N2 temperature. Raman spectroscopy reveals phonon softening, suggesting the formation of defects. These findings not only highlight CrSBr's potential in spintronics, but also present i
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Pang, Chi, Rang Li, Fangchao Long, et al. "Optical Whispering‐Gallery Mode as a Fingerprint of Magnetic Ordering in Van der Waals Layered CrSBr." Advanced Functional Materials, April 24, 2025. https://doi.org/10.1002/adfm.202505275.

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AbstractAn ultra‐sensitive nanoscale magnetism sensing of van der Waals layered CrSBr is demonstrated by employing optical whispering‐gallery‐mode (WGM) resonances in a self‐rolled‐up microcavity. CrSBr nanoflakes with and without intercalation are probed by monitoring the WGM resonant modes shift as a function of magnetic field intensity and temperature, revealing the presence of ferromagnetic (FM) and antiferromagnetic (AFM) order. The minimum detectable amount of CrSBr nanoflakes reaches the femtogram scale, and the detection limit is as low as 1.25 × 10−16 emu. This study demonstrates a pr
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Shi, Wenqiang, Junming Guo, Xing Chen, et al. "Controllable Antiferromagnetic to Ferromagnetic Transition of CrSBr by Organic Cation Intercalation." Advanced Electronic Materials, May 27, 2025. https://doi.org/10.1002/aelm.202500125.

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AbstractThe exploration of magnetism in 2D systems has emerged as a compelling topic, offering insights into novel physical theories and potential applications while expanding the scope of 2D material research. Electrochemical intercalation has been proven to be an effective method to achieve antiferromagnetic‐ferromagnetic phase transition of van der Waals magnetic materials but the mechanism is still unclear. In this study, we present a strategy for modulating 2D magnetism through the electrochemical intercalation of organic cations. Specifically, we demonstrate the controllable transformati
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Guo, Junming, Wenqiang Shi, Kaipeng Ni, et al. "Non-synchronous Strain Effects on a Hetero-Bonded van der Waals Material CrSBr." Chinese Physics B, May 15, 2025. https://doi.org/10.1088/1674-1056/add90d.

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Abstract The van der Waals (vdW) material CrSBr exhibits a distinctive hetero-bonded structure, characterized by fence-like and rectangular configurations viewed from different crystallographic orientations. Mechanical deformation of this unique structure can induce significant anisotropic electronic and optical properties. In this study, we systematically investigate the non-synchronous strain response of CrSBr through theoretical and experimental approaches. Our results reveal that the electronic band structure of CrSBr is predominantly governed by the intralayer Cr-S bonds along the b-axis,
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Ghiasi, Talieh S., Michael Borst, Samer Kurdi, et al. "Nitrogen-vacancy magnetometry of CrSBr by diamond membrane transfer." npj 2D Materials and Applications 7, no. 1 (2023). http://dx.doi.org/10.1038/s41699-023-00423-y.

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AbstractMagnetic imaging using nitrogen-vacancy (NV) spins in diamonds is a powerful technique for acquiring quantitative information about sub-micron scale magnetic order. A major challenge for its application in the research on two-dimensional (2D) magnets is the positioning of the NV centers at a well-defined, nanoscale distance to the target material required for detecting the small magnetic fields generated by magnetic monolayers. Here, we develop a diamond “dry-transfer” technique akin to the state-of-the-art 2D-materials assembly methods and use it to place a diamond micro-membrane in d
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Jo, Junhyeon, Yuan Peisen, Haozhe Yang, et al. "Local control of superconductivity in a NbSe2/CrSBr van der Waals heterostructure." Nature Communications 14, no. 1 (2023). http://dx.doi.org/10.1038/s41467-023-43111-7.

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AbstractTwo-dimensional magnets and superconductors are emerging as tunable building-blocks for quantum computing and superconducting spintronic devices, and have been used to fabricate all two-dimensional versions of traditional devices, such as Josephson junctions. However, novel devices enabled by unique features of two-dimensional materials have not yet been demonstrated. Here, we present NbSe2/CrSBr van der Waals superconducting spin valves that exhibit infinite magnetoresistance and nonreciprocal charge transport. These responses arise from a unique metamagnetic transition in CrSBr, whic
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Tabataba-Vakili, Farsane, Huy P. G. Nguyen, Anna Rupp, et al. "Doping-control of excitons and magnetism in few-layer CrSBr." Nature Communications 15, no. 1 (2024). http://dx.doi.org/10.1038/s41467-024-49048-9.

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AbstractMagnetism in two-dimensional materials reveals phenomena distinct from bulk magnetic crystals, with sensitivity to charge doping and electric fields in monolayer and bilayer van der Waals magnet CrI3. Within the class of layered magnets, semiconducting CrSBr stands out by featuring stability under ambient conditions, correlating excitons with magnetic order and thus providing strong magnon-exciton coupling, and exhibiting peculiar magneto-optics of exciton-polaritons. Here, we demonstrate that both exciton and magnetic transitions in bilayer and trilayer CrSBr are sensitive to voltage-
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36

Hou, Yusheng, Feng Xue, Liang Qiu, Zhe Wang, and Ruqian Wu. "Multifunctional two-dimensional van der Waals Janus magnet Cr-based dichalcogenide halides." npj Computational Materials 8, no. 1 (2022). http://dx.doi.org/10.1038/s41524-022-00802-x.

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AbstractTwo-dimensional van der Waals Janus materials and their heterostructures offer fertile platforms for designing fascinating functionalities. Here, by means of systematic first-principles studies on van der Waals Janus monolayer Cr-based dichalcogenide halides CrYX (Y = S, Se, Te; X = Cl, Br, I), we find that CrSX (X = Cl, Br, I) are the very desirable high TC ferromagnetic semiconductors with an out-of-plane magnetization. Excitingly, by the benefit of the large magnetic moments on ligand S2− anions, the sought-after large-gap quantum anomalous Hall effect and sizable valley splitting c
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Yang, Shiqi, Zhigang Song, Yuchen Gao, et al. "Multi-parameter control of photodetection in van der Waals magnet CrSBr." Light: Science & Applications 14, no. 1 (2025). https://doi.org/10.1038/s41377-024-01737-2.

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Abstract Photodetectors equipped with multi-parameter control hold the potential to deliver exceptional performance in a wide range of scenarios, paving the way for developing novel spin-opto-electronic devices. Nevertheless, the integration of such capabilities within a single device is challenging due to the necessity of harmonizing multiple materials with varying degrees of freedom. In this study, we introduce the van der Waals magnet CrSBr, featuring inherent anisotropy and distinctive spin-electronic coupling, to this realm. The linear dichroic ratio of the photocurrent in CrSBr tunneling
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Lan, Guibin, Hongjun Xu, Yu Zhang, et al. "Giant tunnelling magnetoresistance in spin-filter magnetic tunnel junctions based on van der Waals A-type antiferromagnet CrSBr." Chinese Physics Letters, April 3, 2023. http://dx.doi.org/10.1088/0256-307x/40/5/058501.

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Abstract Two-dimensional (2D) van der Waals (vdW) magnetic materials have demonstrated great potential for new-generation high-performance and versatile spintronic devices. Among them, magnetic tunnel junctions (MTJs) based on A-type antiferromagnets, such as CrI3, possess record-high tunnelling magnetoresistance (TMR) because of the spin filter effect of each insulating unit ferromagnetic layer. However, the relatively low working temperature and the instability of the chromium halides hinder the applications of this system. Using a different technical scheme, we fabricated the MTJs based on
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39

Weile, Mads, Sergii Grytsiuk, Aubrey Penn, et al. "Defect Complexes in CrSBr Revealed Through Electron Microscopy and Deep Learning." Physical Review X 15, no. 2 (2025). https://doi.org/10.1103/physrevx.15.021080.

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Atomic defects underpin the properties of van der Waals materials, and their understanding is essential for advancing quantum and energy technologies. Scanning transmission electron microscopy is a powerful tool for defect identification in atomically thin materials, and extending it to multilayer and beam-sensitive materials would accelerate their exploration. Here, we establish a comprehensive defect library in a bilayer of the magnetic quasi-1D semiconductor CrSBr by combining atomic-resolution imaging, deep learning, and calculations. We apply a custom-developed machine learning work flow
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Bae, Youn Jue, Taketo Handa, Yanan Dai, et al. "Transient magnetoelastic coupling in CrSBr." Physical Review B 109, no. 10 (2024). http://dx.doi.org/10.1103/physrevb.109.104401.

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41

Tschudin, Märta, David Broadway, Patrick Reiser, et al. "Nanoscale magnetism and magnetic phase transitions in atomically thin CrSBr." Nature Communications, May 29, 2024. https://doi.org/10.5281/zenodo.11375831.

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42

Uykur, E., A. A. Tsirlin, F. Long, et al. "Phonon and magnon dynamics across the antiferromagnetic transition in the two-dimensional layered van der Waals material CrSBr." Physical Review B 111, no. 17 (2025). https://doi.org/10.1103/physrevb.111.174434.

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We report temperature-dependent reflectivity spectra of the layered van der Waals magnet CrSBr in the far-infrared region. Polarization-dependent measurements resolve the vibrational modes along the E∥a and b axes and reveal clear structural anisotropy. While the a-axis phonons notably harden on cooling, the b-axis phonon frequencies are almost temperature independent. A phonon splitting due to the antiferromagnetic phase transition is observed for the 180 cm−1 a-axis vibrational mode, accompanied by a phonon softening below TN. Furthermore, an additional mode with strong magnetic characterist
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43

Komar, Rafał, Aleksandra Łopion, Kseniia Mosina, et al. "The polarization switching in nanoscale with an anisotropic 2D magnetic semiconductor." December 16, 2024. https://doi.org/10.1016/j.ssc.2024.115798.

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Here we present a proof-of-concept device demonstrating the feasibility to control the light polarization using the properties of the magnetic 2D materials. The studied structure consists of a diluted magnetic semiconductor quantum well and a thin layer of CrSBr. We show that by application of the external field we can switch the sign of the polarization of the emitted light. The theoretical modeling confirms that such a switching is a direct consequence of a colossal shift of the exciton lines observed in the high energy range of the CrSBr spectra. Owing to this mechanism, the full rotation o
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Cham, Thow Min Jerald, Daniel G. Chica, Xiaoxi Huang, et al. "Spin-filter tunneling detection of antiferromagnetic resonance with electrically tunable damping." Science, July 10, 2025. https://doi.org/10.1126/science.adq8590.

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Antiferromagnetic spintronics offers the potential for higher-frequency operations and improved insensitivity to magnetic fields compared to ferromagnetic spintronics. However, previous electrical techniques to detect antiferromagnetic dynamics have utilized large, millimeter-scale bulk crystals. Here we demonstrate direct electrical detection of antiferromagnetic resonance in structures on the few-micrometer scale using spin-filter tunneling in PtTe 2 /bilayer CrSBr/graphite junctions in which the tunnel barrier is the van der Waals antiferromagnet CrSBr. This sample geometry allows not only
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Chen, Yuliang, Kartik Samanta, Naafis A. Shahed, et al. "Twist-assisted all-antiferromagnetic tunnel junction in the atomic limit." Nature, August 14, 2024. http://dx.doi.org/10.1038/s41586-024-07818-x.

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AbstractAntiferromagnetic spintronics1,2 shows great potential for high-density and ultrafast information devices. Magnetic tunnel junctions (MTJs), a key spintronic memory component that are typically formed from ferromagnetic materials, have seen rapid developments very recently using antiferromagnetic materials3,4. Here we demonstrate a twisting strategy for constructing all-antiferromagnetic tunnel junctions down to the atomic limit. By twisting two bilayers of CrSBr, a 2D antiferromagnet (AFM), a more than 700% nonvolatile tunnelling magnetoresistance (TMR) ratio is shown at zero field (Z
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Long, Fangchao, Kseniia Mosina, René Hübner, et al. "Intrinsic magnetic properties of the layered antiferromagnet CrSBr." Applied Physics Letters 123, no. 22 (2023). http://dx.doi.org/10.1063/5.0175185.

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van der Waals magnetic materials are an ideal platform to study low-dimensional magnetism. Opposed to other members of this family, the magnetic semiconductor CrSBr is highly resistant to degradation in air, which, in addition to its exceptional optical, electronic, and magnetic properties, is the reason the compound is receiving considerable attention at the moment. For many years, its magnetic phase diagram seemed to be well-understood. Recently, however, several groups observed a magnetic transition in magnetometry measurements at temperatures of around 40 K that is not expected from theore
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Rizzo, Daniel J., Alexander S. McLeod, Caitlin Carnahan, et al. "Visualizing Atomically‐Layered Magnetism in CrSBr." Advanced Materials, May 3, 2022, 2201000. http://dx.doi.org/10.1002/adma.202201000.

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48

Jo, Junhyeon, Samuel Mañas-Valero, Eugenio Coronado, Fèlix Casanova, Marco Gobbi, and Luis E. Hueso. "Nonvolatile Electric Control of Antiferromagnet CrSBr." Nano Letters, April 8, 2024. http://dx.doi.org/10.1021/acs.nanolett.4c00348.

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Semina, M. A., F. Tabataba-Vakili, A. Rupp, A. S. Baimuratov, A. Högele, and M. M. Glazov. "Excitons and trions in CrSBr bilayers." Physical Review B 111, no. 20 (2025). https://doi.org/10.1103/physrevb.111.205301.

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Moaied, Mohammed Salah Mohammed, and Mahmoud A. Salem. "Strain-tunable electronic and magnetic properties of two-dimensional CrSBr material." Physica Scripta, October 29, 2024. http://dx.doi.org/10.1088/1402-4896/ad8cac.

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Abstract Two-dimensional (2D) materials, particularly those with intrinsic magnetism, hold promise for next-generation spintronic devices due to their unique electronic and magnetic properties. This study investigates the impact of in-plane uniaxial and biaxial strain on the properties of monolayer CrSBr using density functional theory (DFT) and Monte Carlo (MC) simulations. We demonstrate that strain engineering can effectively modulate the electronic band structure and Curie temperature (Tc) of the CrSBr monolayer. Under uniaxial strains, transitions from indirect to direct bandgaps are obse
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