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Journal articles on the topic 'Dendritic Block Copolymers'

Author: Grafiati

Published: 6 September 2023

Last updated: 31 July 2025

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1

Brito, Mariano E., Sofia E. Mikhtaniuk, Igor M. Neelov, Oleg V. Borisov, and Christian Holm. "Implicit-Solvent Coarse-Grained Simulations of Linear–Dendritic Block Copolymer Micelles." International Journal of Molecular Sciences 24, no. 3 (2023): 2763. http://dx.doi.org/10.3390/ijms24032763.

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The design of nanoassemblies can be conveniently achieved by tuning the strength of the hydrophobic interactions of block copolymers in selective solvents. These block copolymer micelles form supramolecular aggregates, which have attracted great attention in the area of drug delivery and imaging in biomedicine due to their easy-to-tune properties and straightforward large-scale production. In the present work, we have investigated the micellization process of linear–dendritic block copolymers in order to elucidate the effect of branching on the micellar properties. We focus on block copolymers

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2

Trollsås, Mikael, Hans Claesson, Björn Atthoff, and James L. Hedrick. "Layered Dendritic Block Copolymers." Angewandte Chemie International Edition 37, no. 22 (1998): 3132–36. http://dx.doi.org/10.1002/(sici)1521-3773(19981204)37:22<3132::aid-anie3132>3.0.co;2-b.

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3

Fernandez-Megia, Eduardo, Juan Correa, and Ricardo Riguera. "“Clickable” PEG−Dendritic Block Copolymers." Biomacromolecules 7, no. 11 (2006): 3104–11. http://dx.doi.org/10.1021/bm060580d.

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4

Blasco, Eva, Milagros Piñol, and Luis Oriol. "Responsive Linear-Dendritic Block Copolymers." Macromolecular Rapid Communications 35, no. 12 (2014): 1090–115. http://dx.doi.org/10.1002/marc.201400007.

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5

Fecske, Dóra, György Kasza, Gergő Gyulai, et al. "Self-Assembling Amphiphilic ABA Triblock Copolymers of Hyperbranched Polyglycerol with Poly(tetrahydrofuran) and Their Nanomicelles as Highly Efficient Solubilization and Delivery Systems of Curcumin." International Journal of Molecular Sciences 26, no. 12 (2025): 5866. https://doi.org/10.3390/ijms26125866.

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Delivering of hydrophobic drugs by polymeric nanoparticles is an intensively investigated research and development field worldwide due to the insufficient solubility of many existing and potential new drugs in aqueous media. Among polymeric nanoparticles, micelles of biocompatible amphiphilic block copolymers are among the most promising candidates for solubilization, encapsulation, and delivery of hydrophobic drugs to improve the water solubility and thus the bioavailability of such drugs. In this study, amphiphilic ABA triblock copolymers containing biocompatible hydrophilic hyperbranched (d

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6

Babutan, Iulia, Otto Todor-Boer, Leonard Ionut Atanase, Adriana Vulpoi, and Ioan Botiz. "Crystallization of Poly(ethylene oxide)-Based Triblock Copolymers in Films Swollen-Rich in Solvent Vapors." Coatings 13, no. 5 (2023): 918. http://dx.doi.org/10.3390/coatings13050918.

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In this study, we employed a polymer processing method based on solvent vapor annealing in a confined environment to swell-rich thin films of polybutadiene-b-poly(2-vinylpyridine)-b-poly(ethylene oxide) triblock copolymers and to promote their crystallization. As revealed by optical and atomic force microscopy, thin films of triblock copolymers containing a rather short crystalline poly(ethylene oxide) block that was massively obstructed by the other two blocks were unable to crystallize following the spin-casting process, and their further swelling in solvent vapors was necessary in order to

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7

Liu, Xin, F. Max Yavitt, and Ivan Gitsov. "Supramolecular Linear-Dendritic Nanoreactors: Synthesis and Catalytic Activity in “Green” Suzuki-Miyaura Reactions." Polymers 15, no. 7 (2023): 1671. http://dx.doi.org/10.3390/polym15071671.

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This study describes the synthesis of novel amphiphilic linear-dendritic block copolymers and their self-assembly in water to form supramolecular nanoreactors capable of catalyzing Suzuki-Miyaura coupling reactions under “green” conditions. The block copolymers were formed through copper(I)-catalyzed alkyne-azide cycloaddition between azide functionalized poly(benzyl ether) dendrons as the perfectly branched blocks, as well as bis-alkyne modified poly(ethylene glycol), PEG, as the linear block. A first-generation poly(benzyl ether) dendron (G1) was coupled to a bis-alkyne modified PEG with mol

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8

Sousa-Herves, Ana, Christian Sánchez Espinel, Amir Fahmi, África González-Fernández, and Eduardo Fernandez-Megia. "In situ nanofabrication of hybrid PEG-dendritic–inorganic nanoparticles and preliminary evaluation of their biocompatibility." Nanoscale 7, no. 9 (2015): 3933–40. http://dx.doi.org/10.1039/c4nr06155a.

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An in situ template fabrication of inorganic nanoparticles using carboxylated PEG-dendritic block copolymers of the GATG family is described as a function of the dendritic block generation, the metal (Au, CdSe) and metal molar ratio.

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9

Chang, Youngkyu, Young Chul Kwon, Sang Cheon Lee, and Chulhee Kim. "Amphiphilic Linear PEO−Dendritic Carbosilane Block Copolymers." Macromolecules 33, no. 12 (2000): 4496–500. http://dx.doi.org/10.1021/ma9908853.

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10

Kim, Joo-Ho, Eunyoung Lee, Jun-Sik Park, Kazunori Kataoka, and Woo-Dong Jang. "Dual stimuli-responsive dendritic-linear block copolymers." Chemical Communications 48, no. 30 (2012): 3662. http://dx.doi.org/10.1039/c2cc17205d.

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11

Sousa-Herves, Ana, Ricardo Riguera, and Eduardo Fernandez-Megia. "PEG-dendritic block copolymers for biomedical applications." New J. Chem. 36, no. 2 (2012): 205–10. http://dx.doi.org/10.1039/c2nj20849k.

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12

Xie, Chao, Zhenhua Ju, Chao Zhang, Yuliang Yang, and Junpo He. "Dendritic Block and Dendritic Brush Copolymers through Anionic Macroinimer Approach." Macromolecules 46, no. 4 (2013): 1437–46. http://dx.doi.org/10.1021/ma3025317.

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13

Heidari, Alireza. "Non-Viral Gene Delivery to Human Mesenchymal Stem Cells Fluorescence Liquid Biopsy for Cancer Detection." Carcinogenesis and Chemotherapy 3, no. 2 (2024): 01–08. https://doi.org/10.31579/2835-9216/025.

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Non-Viral Gene Delivery to Human Mesenchymal Stem Cells Fluorescence Liquid Biopsy for Cancer Detection Using Cationic Dendronized Hyperbranched Polymer Combination Chemotherapy with Cisplatin and Chloroquine Encapsulation in MicellesFormed by Self-Assembling Hybrid Dendritic-Linear-Dendritic Block Copolymers Micellar Nanocarriers from Dendritic Macromolecules Containing Fluorescent Coumarin Moieties.

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14

Zhang, Weiwei, Weiwei Jiang, Delong Zhang, Guangyue Bai, Pengxiao Lou, and Zhiguo Hu. "Synthesis, characterization and association behavior of linear-dendritic amphiphilic diblock copolymers based on poly(ethylene oxide) and a dendron derived from 2,2′-bis(hydroxymethyl)propionic acid." Polymer Chemistry 6, no. 12 (2015): 2274–82. http://dx.doi.org/10.1039/c4py01385a.

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15

Leiro, Victoria, João Pedro Garcia, Pedro M. D. Moreno, et al. "Biodegradable PEG–dendritic block copolymers: synthesis and biofunctionality assessment as vectors of siRNA." Journal of Materials Chemistry B 5, no. 25 (2017): 4901–17. http://dx.doi.org/10.1039/c7tb00279c.

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16

Chang, Youngkyu, and Chulhee Kim. "Synthesis and photophysical characterization of amphiphilic dendritic-linear-dendritic block copolymers." Journal of Polymer Science Part A: Polymer Chemistry 39, no. 6 (2001): 918–26. http://dx.doi.org/10.1002/1099-0518(20010315)39:6<918::aid-pola1066>3.0.co;2-p.

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17

Brazkova, M. S., R. Y. Koleva, G. V. Angelova, and A. I. Krastanov. "Degradation of pyrene by laccase from Trametes versicolor." Bulgarian Chemical Communications 56, no. D2 (2024): 78–83. http://dx.doi.org/10.34049/bcc.56.d.s2p46.

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In recent years the development of eco-friendly remediation technologies with economical advantage is based on the incorporation of microorganisms or their enzyme systems in the degradation processes. In the present study purified laccase with specific activity 105.8 U/mg, obtained after submerged cultivation of the basidiomycete Trametes versicolor, was used in free and immobilized form for pyrene degradation. The alginate gel entrapment method and the encapsulation in amphiphilic dendritic-linear-dendritic block copolymers were applied as immobilization techniques. The free form of the enzym

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18

Tian, Lu, Phuong Nguyen, and Paula T. Hammond. "Vesicular self-assembly of comb–dendritic block copolymers." Chem. Commun., no. 33 (2006): 3489–91. http://dx.doi.org/10.1039/b608363c.

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19

Tang, Gang, Minqi Hu, Yongcui Ma, Dan You, and Yunmei Bi. "Synthesis and solution properties of novel thermo- and pH-responsive poly(N-vinylcaprolactam)-based linear–dendritic block copolymers." RSC Advances 6, no. 49 (2016): 42786–93. http://dx.doi.org/10.1039/c6ra04327e.

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This study describes the synthesis and solution properties of the novel linear–dendritic block copolymers (LDBCs) based on thermoresponsive poly(N-vinylcaprolactam) (PNVCL) chains and pH-responsive poly(benzyl ether) dendrons.

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20

Namazi, Hassan, and Mohsen Adeli. "Solution proprieties of dendritic triazine/poly(ethylene glycol)/dendritic triazine block copolymers." Journal of Polymer Science Part A: Polymer Chemistry 43, no. 1 (2004): 28–41. http://dx.doi.org/10.1002/pola.20471.

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21

Wei, Lin, You, Qian, Wang, and Bi. "Self-Assembly and Enzyme Responsiveness of Amphiphilic Linear-Dendritic Block Copolymers Based on Poly(N-vinylpyrrolidone) and Dendritic Phenylalanyl-lysine Dipeptides." Polymers 11, no. 10 (2019): 1625. http://dx.doi.org/10.3390/polym11101625.

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In this study, we present the synthesis, self-assembly, and enzyme responsive nature of a unique class of well-defined amphiphilic linear-dendritic block copolymers (PNVP-b-dendr(Phe-Lys)n, n = 1–3) based on linear poly(N-vinylpyrrolidone) (PNVP) and dendritic phenylalanyl-lysine (Phe-Lys) dipeptides. The copolymers were prepared via a combination ofreversible addition-fragmentation chain transfer (RAFT) /xanthates (MADIX) polymerization of N-vinylpyrrolidone and stepwise peptide chemistry. The results of fluorescence spectroscopy, 1H NMR analyses, transmission electron microscopy (TEM), and p

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22

Tavakoli Naeini, Ashkan, Manouchehr Vossoughi, and Mohsen Adeli. "Simultaneously Synthesis and Encapsulation of Metallic Nanoparticles Using Linear–Dendritic Block Copolymers of Poly(ethylene glycol)-Poly(citric acid)." Key Engineering Materials 478 (April 2011): 7–12. http://dx.doi.org/10.4028/www.scientific.net/kem.478.7.

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Linear-dendritic triblock copolymers of linear poly(ethylene glycol) and hyperbranched poly(citric acid) (PCA-PEG-PCA) were used as the reducing and capping agents to encapsulate gold and silver nanoparticles (AuNPs and AgNPs). PCA-PEG-PCA copolymers in four different molecular weights were synthesized using 2, 5, 10 and 20 citric acid/PEG molar ratios and were called A1, A2, A3 and A4, respectively. Nanoparticles were encapsulated simultaneously during the preparation process. AuNPs were simply synthesized and encapsulated by addition a boiling aqueous solution of HAuCl4 to aqueous solutions

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23

Hamadani, Christine M., Indika Chandrasiri, Mahesh Loku Yaddehige, et al. "Improved nanoformulation and bio-functionalization of linear-dendritic block copolymers with biocompatible ionic liquids." Nanoscale 14, no. 16 (2022): 6021–36. http://dx.doi.org/10.1039/d2nr00538g.

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24

Liu, Xin, Tina Monzavi, and Ivan Gitsov. "Controlled ATRP Synthesis of Novel Linear-Dendritic Block Copolymers and Their Directed Self-Assembly in Breath Figure Arrays." Polymers 11, no. 3 (2019): 539. http://dx.doi.org/10.3390/polym11030539.

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Herein, we report the formation and characterization of novel amphiphilic linear-dendritic block copolymers (LDBCs) composed of hydrophilic dendritic poly(ether-ester), PEE, blocks and hydrophobic linear poly(styrene), PSt. The LDBCs are synthesized via controlled atom transfer radical polymerization (ATRP) initiated by a PEE macroinitiator. The copolymers formed have narrow molecular mass distributions and are designated as LGn-PSt Mn, in which LG represents the PEE fragment, n denotes the generation of the dendron (n = 1–3), and Mn refers to the average molecular mass of the LDBC (Mn = 3.5–6

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25

Sousa-Herves, Ana, Ricardo Riguera, and Eduardo Fernandez-Megia. "ChemInform Abstract: PEG-Dendritic Block Copolymers for Biomedical Applications." ChemInform 43, no. 22 (2012): no. http://dx.doi.org/10.1002/chin.201222210.

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26

Hawker, Craig J., Karen L. Wooley, and Jean M. J. Fréchet. "Novel macromolecular architectures: Globular block copolymers containing dendritic components." Macromolecular Symposia 77, no. 1 (1994): 11–20. http://dx.doi.org/10.1002/masy.19940770105.

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27

Marcos, Alejandra García, Thomas M. Pusel, Ralf Thomann, et al. "Linear-Hyperbranched Block Copolymers Consisting of Polystyrene and Dendritic Poly(carbosilane) Block." Macromolecules 39, no. 3 (2006): 971–77. http://dx.doi.org/10.1021/ma051526c.

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28

Gong, Yongji, Weihua Song, Yifan Wu, et al. "Effect of chain segment length on crystallization behaviors of poly(l-lactide-b-ethylene glycol-b-l-lactide) triblock copolymer." Polymers and Polymer Composites 28, no. 2 (2019): 77–88. http://dx.doi.org/10.1177/0967391119863951.

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The poly(l-lactide-b-ethylene glycol-b-l-lactide) (PLLA-PEG-PLLA) triblock copolymers with different chain segment length are fabricated by ring-opening polymerization. The structure, molecular weight, and crystallization behaviors of the triblock copolymers are characterized by Fourier transform infrared, nuclear magnetic resonance spectroscopy, gel permeation in chromatography, X-ray diffraction, differential scanning calorimetry, and polarizing optical microscopy (POM). The results show that the increase of block length is beneficial to improve its crystallization. In addition, the triblock

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29

Liu, Yan, Chao Lin, Jianbo Li, Yang Qu, and Jie Ren. "In vitro and in vivo gene transfection using biodegradable and low cytotoxic nanomicelles based on dendritic block copolymers." Journal of Materials Chemistry B 3, no. 4 (2015): 688–99. http://dx.doi.org/10.1039/c4tb01406e.

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30

Kalva, Nagendra, Nimisha Parekh, and Ashootosh V. Ambade. "Controlled micellar disassembly of photo- and pH-cleavable linear-dendritic block copolymers." Polymer Chemistry 6, no. 38 (2015): 6826–35. http://dx.doi.org/10.1039/c5py00792e.

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31

Wang, Fang, Zhiqing Zhang, Tao Wang, Yunze Li, and Mei Cui. "Synthesis, Characterization, and Demulsification Behavior of Amphiphilic Dendritic Block Copolymers." Journal of Dispersion Science and Technology 36, no. 8 (2014): 1097–105. http://dx.doi.org/10.1080/01932691.2014.950741.

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32

Trollsås, Mikael, Björn Atthoff, Hans Claesson, and James L. Hedrick. "Dendritic homopolymers and block copolymers: Tuning the morphology and properties." Journal of Polymer Science Part A: Polymer Chemistry 42, no. 5 (2004): 1174–88. http://dx.doi.org/10.1002/pola.11088.

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33

Lang, Andreas S., Franz René Kogler, Michael Sommer, Ulrich Wiesner, and Mukundan Thelakkat. "Semiconductor Dendritic-Linear Block Copolymers by Nitroxide Mediated Radical Polymerization." Macromolecular Rapid Communications 30, no. 14 (2009): 1243–48. http://dx.doi.org/10.1002/marc.200900203.

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34

Bi, Yunmei, Caixian Yan, Lidong Shao, Yufei Wang, Yongcui Ma, and Gang Tang. "Well-defined thermoresponsive dendritic polyamide/poly(N -vinylcaprolactam) block copolymers." Journal of Polymer Science Part A: Polymer Chemistry 51, no. 15 (2013): 3240–50. http://dx.doi.org/10.1002/pola.26716.

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35

Lu, Yuliang, Dongtao Liu, Xinjie Wei та ін. "Synthesis and Thermoreversible Gelation of Coil–Rod Copolymers with a Dendritic Polyethylene Core and Multiple Helical Poly(γ-benzyl-L-glutamate) Arms". Polymers 15, № 22 (2023): 4351. http://dx.doi.org/10.3390/polym15224351.

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Coil–rod copolymers with a dendritic polyethylene (DPE) core and multiple helical poly(γ-benzyl-L-glutamate) (PBLG) arms (DPE-(PBLG)n) were prepared by palladium-catalyzed copolymerization in tandem with ring-opening polymerization (ROP). Macroinitiator (DPE–(NH2)11) was firstly prepared by the group transformation of DPE–(OH)11 generated from palladium-catalyzed copolymerization of ethylene and acrylate comonomer. Coil–helical DPE-(PBLG)11 copolymers were prepared by ROP of γ-benzyl-L-glutamate-N-carboxyanhydride (BLG-NCA). These DPE-(PBLG)11 copolymers could form thermoreversible gels in tol

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36

Lebedeva, Inna O., Ekaterina B. Zhulina, and Oleg V. Borisov. "Self-Assembly of Linear-Dendritic and Double Dendritic Block Copolymers: From Dendromicelles to Dendrimersomes." Macromolecules 52, no. 10 (2019): 3655–67. http://dx.doi.org/10.1021/acs.macromol.9b00140.

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37

Qian, Yangyang, Dan You, Feng Lin, Junwu Wei, Yujia Wang, and Yunmei Bi. "Enzyme triggered disassembly of amphiphilic linear-dendritic block copolymer micelles based on poly[N-(2-hydroxyethyl-l-glutamine)]." Polymer Chemistry 10, no. 1 (2019): 94–105. http://dx.doi.org/10.1039/c8py01231h.

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New amphiphilic linear-dendritic diblock copolymers based on poly[N-(2-hydroxyethyl-l-glutamine)] have been synthesized, and their micellar assemblies can disassemble and release encapsulated molecular cargo upon enzymatic activation.

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38

Jeong, Moon Gon, Jan C. M. van Hest, and Kyoung Taek Kim. "Self-assembly of dendritic-linear block copolymers with fixed molecular weight and block ratio." Chemical Communications 48, no. 30 (2012): 3590. http://dx.doi.org/10.1039/c2cc17231c.

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39

Abad, Miriam, Alejandro Martínez-Bueno, Gracia Mendoza, et al. "Supramolecular Functionalizable Linear–Dendritic Block Copolymers for the Preparation of Nanocarriers by Microfluidics." Polymers 13, no. 5 (2021): 684. http://dx.doi.org/10.3390/polym13050684.

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Hybrid linear–dendritic block copolymers (LDBCs) having dendrons with a precise number of peripheral groups that are able to supramolecular bind functional moieties are challenging materials as versatile polymeric platforms for the preparation of functional polymeric nanocarriers. PEG2k-b-dxDAP LDBCs that are based on polyethylene glycol (PEG) as hydrophilic blocks and dendrons derived from bis-MPA having 2,6-diacylaminopyridine (DAP) units have been efficiently synthesized by the click coupling of preformed blocks, as was demonstrated by spectroscopic techniques and mass spectrometry. Self-as

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40

Dong, Chang-Ming, and Gang Liu. "Linear–dendritic biodegradable block copolymers: from synthesis to application in bionanotechnology." Polym. Chem. 4, no. 1 (2013): 46–52. http://dx.doi.org/10.1039/c2py20441j.

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41

Gitsov, Ivan, and Jean M. J. Frechet. "Solution and solid-state properties of hybrid linear-dendritic block copolymers." Macromolecules 26, no. 24 (1993): 6536–46. http://dx.doi.org/10.1021/ma00076a035.

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42

Lee, Hyung-il, Jung Ah Lee, Zhiyong Poon, and Paula T. Hammond. "Temperature-triggered reversible micellar self-assembly of linear–dendritic block copolymers." Chemical Communications, no. 32 (2008): 3726. http://dx.doi.org/10.1039/b807561a.

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43

Trolls�s, Mikael, Craig J. Hawker, Jules F. Remenar, et al. "Highly branched radial block copolymers via dendritic initiation of aliphatic polyesters." Journal of Polymer Science Part A: Polymer Chemistry 36, no. 15 (1998): 2793–98. http://dx.doi.org/10.1002/(sici)1099-0518(19981115)36:15<2793::aid-pola16>3.0.co;2-m.

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44

Gitsov, Ivan, Karen L. Wooley, Craig J. Hawker, Pavlina T. Ivanova, and Jean M. J. Frechet. "Synthesis and properties of novel linear-dendritic block copolymers. Reactivity of dendritic macromolecules toward linear polymers." Macromolecules 26, no. 21 (1993): 5621–27. http://dx.doi.org/10.1021/ma00073a014.

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45

Al-Muallem, Hasan A., and Daniel M. Knauss. "Synthesis of hybrid dendritic-linear block copolymers with dendritic initiators prepared by convergent living anionic polymerization." Journal of Polymer Science Part A: Polymer Chemistry 39, no. 1 (2000): 152–61. http://dx.doi.org/10.1002/1099-0518(20010101)39:1<152::aid-pola170>3.0.co;2-s.

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46

Namazi, Hassan, and Mohsen Adeli. "Synthesis of barbell-like triblock copolymers, dendritic triazine-block-poly(ethylene glycol)-block-dendritic triazine and investigation of their solution behaviors." Polymer 46, no. 24 (2005): 10788–99. http://dx.doi.org/10.1016/j.polymer.2005.09.020.

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47

Yu, Dong, Nikolay Vladimirov, and Jean M. J. Fréchet. "MALDI-TOF in the Characterizations of Dendritic−Linear Block Copolymers and Stars." Macromolecules 32, no. 16 (1999): 5186–92. http://dx.doi.org/10.1021/ma981734n.

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48

Zhang, Zhiqing, and Fang Wang. "Aggregation Behavior of Polyether Block Copolymers with Dendritic Structure in Aqueous Solutions." Journal of Dispersion Science and Technology 29, no. 8 (2008): 1092–97. http://dx.doi.org/10.1080/01932690701817669.

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49

Wurm, Frederik, and Holger Frey. "Linear–dendritic block copolymers: The state of the art and exciting perspectives." Progress in Polymer Science 36, no. 1 (2011): 1–52. http://dx.doi.org/10.1016/j.progpolymsci.2010.07.009.

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50

García-Juan, Hugo, Aurora Nogales, Eva Blasco, et al. "Self-assembly of thermo and light responsive amphiphilic linear dendritic block copolymers." European Polymer Journal 81 (August 2016): 621–33. http://dx.doi.org/10.1016/j.eurpolymj.2015.12.021.

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