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Relevant bibliographies by topics / Deuterium Isotope Effect

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Academic literature on the topic 'Deuterium Isotope Effect'

Author: Grafiati

Published: 4 June 2021

Last updated: 1 February 2022

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Journal articles on the topic "Deuterium Isotope Effect"

1

Armesto, X. L., M. Canle L., V. García, and J. A. Santaballa. "Solvent isotope effects in the oxidation of dipeptides by aqueous chlorine." Canadian Journal of Chemistry 77, no. 5-6 (1999): 997–1004. http://dx.doi.org/10.1139/v99-105.

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A kinetic study of the mechanism of oxidation of Ala-Gly and Pro-Gly by aqueous chlorine has been carried out. Among other experimental facts, the deuterium solvent isotope effects were used to clarify the mechanisms involved. In a first stage, N-chlorination takes place, and then the (N-Cl)-dipeptide decomposes through two possible mechanisms, depending on the acidity of the medium. The initial chlorination step shows a small isotope effect. In alkaline medium, two consecutive processes take place: first, the general base-catalyzed formation of an azomethine (β ca. 0.27), which has an inverse

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2

Trequattrini, Francesco, Oriele Palumbo, Silvano Tosti, Alessia Santucci, and Annalisa Paolone. "Promising Isotope Effect in Pd77Ag23 for Hydrogen Separation." ChemEngineering 5, no. 3 (2021): 51. http://dx.doi.org/10.3390/chemengineering5030051.

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Pd–Ag alloys are largely used as hydrogen separation membranes and, as a consequence, the Pd–Ag–H system has been intensively studied. On the contrary, fewer information is available for the Pd–Ag–D system; thus, the aim of this work is to improve the knowledge of the isotope effect on the commercial Pd77Ag23 alloy, especially for temperature above 200 °C. In particular, deuterium absorption measurements are carried out in the Pd77Ag23 alloy in the temperature range between 79 and 400 °C and in the pressure range between 10−2 and 16 bar. In this exploited pressure (p) and composition (c) range

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3

Koerner, Terry, Kenneth Charles Westaway, Raymond A. Poirier та Y. Wang. "An unusually large secondary α-deuterium kinetic isotope effect in hydride ion SN2 reactions". Canadian Journal of Chemistry 78, № 8 (2000): 1067–72. http://dx.doi.org/10.1139/v00-100.

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Theoretical calculations at the HF/6-31+G* level suggest the secondary α-deuterium kinetic isotope effects for hydride ion SN2 reactions are much larger than expected for the structure of the transition state. The secondary α-deuterium kinetic isotope effects for the SN2 reactions between sodium borohydride (hydride ion) and para-methyl- and para-chlorobenzyl chlorides are much larger than expected as the theoretical calculations suggest. It appears the secondary α-deuterium isotope effects are larger than expected for the structure of the SN2 transition state because the hydride ion is too sm

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4

Away, Kenneth Charles West, and Zhu-Gen Lai. "Solvent effects on SN2 transition state structure. II: The effect of ion pairing on the solvent effect on transition state structure." Canadian Journal of Chemistry 67, no. 2 (1989): 345–49. http://dx.doi.org/10.1139/v89-056.

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Identical secondary α-deuterium kinetic isotope effects (transition state structures) in the SN2 reaction between n-butyl chloride and a free thiophenoxide ion in aprotic and protic solvents confirm the validity of the Solvation Rule for SN2 Reactions. These isotope effects also suggest that hydrogen bonding from the solvent to the developing chloride ion in the SN2 transition state does not have a marked effect on the magnitude of the chlorine (leaving group) kinetic isotope effects. Unlike the free ion reactions, the secondary α-deuterium kinetic isotope effect (transition state structure) f

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5

Pozio and Tosti. "Pd-Ag Electrical Resistivity in Hydrogen and Deuterium: Temperature Effect." Materials 12, no. 21 (2019): 3551. http://dx.doi.org/10.3390/ma12213551.

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The electrical resistivity of Pd-Ag (silver 21 wt.%) in hydrogen and deuterium atmosphere at 100 kPa has been investigated via electrochemical impedance spectroscopy. The electrical resistivity of Pd-Ag vs. the temperature presents the characteristic S-shaped curve with a minimum and a maximum of the resistivity in different positions for the tests in hydrogen and deuterium. The results have been related to: (1) the different isotope ratios, H/M and D/M, and (2) their position in the Pd-Ag lattice. The behavior of the electrical resistivity is discussed in details by considering the hydrogen a

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6

Chan, Jefferson, Ariel Tang та Andrew J. Bennet. "Transition-state structure for the hydronium-ion-promoted hydrolysis of α-d-glucopyranosyl fluoride". Canadian Journal of Chemistry 93, № 4 (2015): 463–67. http://dx.doi.org/10.1139/cjc-2014-0451.

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The transition state for the hydronium-ion-promoted hydrolysis of α-d-glucopyranosyl fluoride in water has been characterized by combining multiple kinetic isotope effect measurements with theoretical modelling. The measured kinetic isotope effects for the C1-deuterium, C2-deuterium, C5-deuterium, anomeric carbon-13, and ring oxygen-18 are 1.219 ± 0.021, 1.099 ± 0.024, 0.976 ± 0.014, 1.014 ± 0.005, and 0.991 ± 0.013, respectively. The transition state for the hydronium ion reaction is late with respect to both C–F bond cleavage and proton transfer.

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7

Pal, Haridas, Yutaka Nagasawa, Keisuke Tominaga, Shigeichi Kumazaki, and Keitaro Yoshihara. "Deuterium isotope effect on the solvation dynamics." Journal of Chemical Physics 102, no. 19 (1995): 7758–60. http://dx.doi.org/10.1063/1.469028.

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8

Westaway, Kenneth Charles, and Zhu-Gen Lai. "Isotope effects in nucleophilic substitution reactions. VI. The effect of ion pairing on the transition state structure of SN2 reactions." Canadian Journal of Chemistry 66, no. 5 (1988): 1263–71. http://dx.doi.org/10.1139/v88-205.

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Spectroscopic and conductivity studies of sodium thiophenoxide solutions in four different solvents and the secondary α-deuterium kinetic isotope effects found in the presence of 15-crown-5 ether demonstrate that the secondary α-deuterium kinetic isotope effect and transition state structure for the SN2 reaction between sodium thiophenoxide and n-butyl chloride are significantly different, depending on whether the ionic reactant is a solvent-separated ion-pair complex or a free ion. In all three solvents in which the form of the ionic reactant changes, a smaller isotope effect and tighter tran

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9

Pham, T. V., and K. C. Westaway. "Solvent effects on nucleophilic substitution reactions. III. The effect of adding an inert salt on the structure of the SN2 transition state." Canadian Journal of Chemistry 74, no. 12 (1996): 2528–30. http://dx.doi.org/10.1139/v96-283.

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The nitrogen and secondary α-hydrogen–deuterium kinetic isotope effects found for the SN2 reaction between thiophenoxide ion and benzyldimethylphenylammonium ion at different ionic strengths in DMF at 0 °C indicate that the structure of the transition state changes markedly with the ionic strength of the reaction mixture. In fact, a more reactant-like, more ionic, transition state is found at the higher ionic strength. This presumably occurs because a more ionic transition state is more stable in the more ionic solvent. Key words: transition state, ionic strength, secondary α deuterium kinetic

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10

Keeffe, J. R., and A. J. Kresge. "Medium isotope effect for isobutyrophenone in aqueous solution. Solvent isotope effects on carbonyl group hydration." Canadian Journal of Chemistry 67, no. 5 (1989): 792–93. http://dx.doi.org/10.1139/v89-119.

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A medium solvent isotope effect of Φ = 0.827 ± 0.013 was determined for transfer of isobutyrophenone from H2O to D2O. This result, in conjunction with the average solvent isotope effect on hydration of a number of carbonyl compounds, leads to [Formula: see text] as the fractionation factor for the hydroxyl group hydrogens of the hydration reactions' gem-diol products, which is consistent with the expectation that fractionation factors for uncharged hydroxyl groups should be unity. Keywords: isobutyrophenone, fractionation factors, solvent isotope effects, deuterium oxide.

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Dissertations / Theses on the topic "Deuterium Isotope Effect"

1

Kuperman, Joshua Minoru. "Applications of NMR techniques : the anomeric effect and secondary deuterium isotope effects /." Diss., Connect to a 24 p. preview or request complete full text in PDF format. Access restricted to UC campuses, 2003. http://wwwlib.umi.com/cr/ucsd/fullcit?p3112850.

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2

Ingle, Shakti Singh. "RNA structure investigation: a deuterium kinetic isotope effect/hydroxyl radical cleavage experiment." Thesis, Boston University, 2013. https://hdl.handle.net/2144/12787.

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Thesis (Ph.D.)--Boston University PLEASE NOTE: Boston University Libraries did not receive an Authorization To Manage form for this thesis or dissertation. It is therefore not openly accessible, though it may be available by request. If you are the author or principal advisor of this work and would like to request open access for it, please contact us at open-help@bu.edu. Thank you.<br>The hydroxyl radical is widely used as a high-resolution footprinting agent for DNA and RNA. The hydroxyl radical abstracts a hydrogen atom from the sugar- phosphate backbone of a nucleic acid molecule, creatin

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3

Yu, Jian. "Synthesis and mechanistic studies on the monoamine oxidase (MAO) catalyzed oxidation of 1,4-disubstituted-1,2,3,6-tetrahydropyridines." Diss., Virginia Tech, 1998. http://hdl.handle.net/10919/30688.

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The parkinsonian inducing drug 1-methyl-4-phenyl-1,2,3,6-tetrahydropyridine (MPTP) is bioactivated in a reaction catalyzed by the flavoenzyme monoamine oxidase B (MAO-B) to form the corresponding dihydropyridinium (MPDP+) subsequently pyridinium (MPP+) metabolites. As part of our ongoing studies to characterize the structural features responsible for this unexpected biotransformation, we have synthesized and examined the MAO-B substrate properties of a variety of MPTP analogs bearing various heteroaryl groups at the 4-position of the tetrahydropyridinyl ring. The results of these SAR studies

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4

Owens, Simon. "Kinetics and mechanisms of hydrogen isotope exchange over solid storage media." Thesis, University of Bath, 2015. https://ethos.bl.uk/OrderDetails.do?uin=uk.bl.ethos.687343.

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Hydrogen isotope separation systems using palladium (Pd) are currently being designed for both reactor designs with the aim of separating and purifying the reactor exhaust products which contain valuable unspent hydrogen isotopes. Hydrogen isotope exchange in Pd offers an efficient, ambient condition process that can produce pure isotopic species in a process far simpler and less costly than the current state of the art cryogenic distillation processes. The method is applicable whether separating hydrogen (protium), deuterium or tritium and any combination of these. If practical fusion devices

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5

Debleds, François. "Complexation d'électrophiles aromatiques par des bases hétérocycliques ambidentes : structure et réactivité d'adduits carbones et azotes pyrroliques indoliques et imidazoliques." Paris 6, 1987. http://www.theses.fr/1987PA066330.

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Structure et formation des complexes de Meisenheimer du trinitro-1,3,5 benzène avec divers indoles, pyrroles, imidazoles ; étude cinétique de la décomposition de ces complexes. Etude cinétique de la protonation du kryptopyrrole en solution aqueuse.

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Lavigne, André. "Oxydations cupro-catalysees des amines aliphatiques : etudes mecanistiques et applications synthetiques." Paris 6, 1987. http://www.theses.fr/1987PA066470.

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Preparation de nitriles a partir d'amines primaires et d'alpha -aminoacides. Les acides amines monosubstutitues rch(nh::(2))co::(2)h donnent le nitrile rcn, alors que les acides amines disubstitues rr'c(nh::(2))co::(2)h conduisent a l'azine rr'c=n-n=cr'r. Les mecanismes proposes font intervenir le cuivre (iii), forme in situ a partir du cuivre (i) et de l'oxygene

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Majournat, Béatrice. "Interférences et prédissociation par interaction spin-orbite dans HgH." Grenoble 1, 1988. http://www.theses.fr/1988GRE10107.

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Pour les mesures d'intensites dans hgh, l'etalonnage du systeme optique de detection est effectue. Etude des interferences entre transitions de symetrie differente, et de la predissociation avec effet tunnel sur la gauche

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8

Sobrado, Pablo. "Studies of the chemical mechanisms of flavoenzymes." Texas A&M University, 2003. http://hdl.handle.net/1969/565.

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9

Rossi, François-Noël. "Etude théorique des collisions non réactives entre atomes alcalins et molécules d'hydrogène ou de deuterium : Calcul et analyse des surfaces de potentiel, application aux transitions de structure fine du rubidium." Paris 13, 1986. http://www.theses.fr/1986PA132015.

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Calcul des courbes de potentiel adiabatiques pour les géométries colinéaires et perpendiculaires, à l'aide d'un pseudopotentiel dépendant du moment orbital électronique et d'une approche à deux centres; bon accord avec les calculs ab initio existants. Examen des différentes symétries de ces systèmes dans le formalisme de la théorie des groupes, afin d'étudier les valeurs propres et facteurs propres de l'hamiltonien électronique. Calcul quantique des sections efficaces relatives des transitions de structure fine de Rb induites par collision avec H(2) ou D(2). En tenant compte des niveaux rotati

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10

Vakonakis, Ioannis. "Structure and function of circadian clock proteins and deuterium isotope effects in nucleic acid hydrogen bonds." Diss., Texas A&M University, 2003. http://hdl.handle.net/1969.1/2195.

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Circadian oscillators or clocks are a widespread, endogenous class of oscillatory mechanisms that control the ~24h temporal pattern of diverse organism functions. In cyanobacteria this mechanism is formed by three proteins, KaiA, KaiB and KaiC. KaiA is shown here to be a two domain protein that directly interacts with KaiC and enhances the KaiC autokinase activity. The amino-terminal domain of KaiA can be structurally categorized as a pseudo-receiver, a class of proteins used in signaling cascades and activated by direct protein??protein interactions. The carboxy-terminal domain interacts dire

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Books on the topic "Deuterium Isotope Effect"

1

Osborne, Craig. Measuring the rate constant and secondary a-deuterium kinetic isotope effect for the SN2 reaction between para-nitrobenzyl choride and cyanide ion in 15% aqueous DMSO. Laurentian University, 1996.

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2

Bruce, Cook. The Feasibility of measuring the rate constant and secondary [alpha]-deuterium kinetic isotope effect for the Sn2 reaction between sodium phenoxide and benzyl chloride at low concentrations of phenoxide ion. Laurentian University, 1995.

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3

Thompson, D. A. ITER task T26/28 (1994): Preliminary results on the solubility, diffusion and permeability of hydrogen isotopes in potentional fusion reactor ceramics. CFFTP, 1995.

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4

Quigley, Kim. The use of deuterium kinetic solvent isotope effects and the proton inventory method in the elucidation of the catalyticmechanism of the cysteine protease papain. University of Birmingham, 1987.

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Book chapters on the topic "Deuterium Isotope Effect"

1

Lochbrunner, S., K. Stock, C. Schriever, and E. Riedle. "Ultrafast double proton transfer: symmetry breaking wavepacket motion and absence of deuterium isotope effect." In Springer Series in Chemical Physics. Springer Berlin Heidelberg, 2005. http://dx.doi.org/10.1007/3-540-27213-5_150.

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2

Shackelford, Scott A. "Mechanistic Investigations of Condensed Phase Energetic Material Decomposition Processes Using the Kinetic Deuterium Isotope Effect." In Chemistry and Physics of Energetic Materials. Springer Netherlands, 1990. http://dx.doi.org/10.1007/978-94-009-2035-4_18.

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3

Shackelford, Scott A. "Mechanistic Relationships of the Decomposition Process to Combustion and Explosion Events from Kinetic Deuterium Isotope Effect Investigations." In Chemistry and Physics of Energetic Materials. Springer Netherlands, 1990. http://dx.doi.org/10.1007/978-94-009-2035-4_19.

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4

Limbach, Hans-Heinrich. "Dynamic NMR Spectroscopy in the Presence of Kinetic Hydrogen/Deuterium Isotope Effects." In Deuterium and Shift Calculation. Springer Berlin Heidelberg, 1990. http://dx.doi.org/10.1007/978-3-642-75932-1_2.

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5

Berger, S. "Chemical Models for Deuterium Isotope Effects in 13C- and 19F-NMR." In Isotope Effects in NMR Spectroscopy. Springer Berlin Heidelberg, 1990. http://dx.doi.org/10.1007/978-3-642-74835-6_1.

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6

Schleucher, J., P. Vanderveer, J. L. Markley, and T. D. Sharkey. "Disequilibrium of Chloroplastic Phosphoglucose Isomerase Inferred from Deuterium Isotope Discrimination." In Photosynthesis: Mechanisms and Effects. Springer Netherlands, 1998. http://dx.doi.org/10.1007/978-94-011-3953-3_821.

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Sunko, Dionis E., and Warren J. Hehre. "Secondary Deuterium Isotope Effects on Reactions Proceeding Through Carbocations." In Progress in Physical Organic Chemistry. John Wiley & Sons, Inc., 2007. http://dx.doi.org/10.1002/9780470171936.ch5.

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8

Tu, Shiao-Chun, Lee-Ho Wang, and Yimin Yu. "Applications of deuterium and tritium isotope effects to the elucidation of kinetic mechanisms of flavoprotein hydroxylases." In Flavins and Flavoproteins 1987, edited by D. E. Edmondson and D. B. McCormick. De Gruyter, 1987. http://dx.doi.org/10.1515/9783110884715-091.

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9

Balaban, Alexandru T. "Steric Versus Electronic Components of Secondary Deuterium Isotope Effects Depend on the Size of Electrophilic Probes." In Water and Ions in Biological Systems. Springer US, 1985. http://dx.doi.org/10.1007/978-1-4899-0424-9_63.

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Lydakis-Simantiris, N., C. W. Hoganson, D. F. Ghanotakis, and G. T. Babcock. "Deuterium Isotope Effects on the Kinetics of Y Z · Reduction in Oxygen Evolving Photosystem II Membranes." In Photosynthesis: from Light to Biosphere. Springer Netherlands, 1995. http://dx.doi.org/10.1007/978-94-009-0173-5_295.

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Conference papers on the topic "Deuterium Isotope Effect"

1

Shek, Gordon K., and Harry Seahra. "Effect of Hydrogen Isotope and Concentration on Delayed Hydride Crack Growth Rates in Zr-2.5Nb Pressure Tubes." In 18th International Conference on Nuclear Engineering. ASMEDC, 2010. http://dx.doi.org/10.1115/icone18-29786.

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CANDU Zr-2.5 Nb pressure tubes are susceptible to a cracking mechanism known as Delayed Hydride Cracking (DHC), which is a repetitive process that involves hydrogen diffusion, hydride precipitation and fracture at a crack tip. As defense-in-depth, when DHC is postulated to have initiated from a flaw, it is required to demonstrate that the crack can be detected by the leak monitoring system and the reactor safely shut down before the crack reaches the critical length for pressure tube rupture. DHC growth rates (DHCR) in the axial direction of the tube are required for such leak-before-break ass

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Boens, Noel, Luc D. Janssens, Luc Van Dommelen, Frans C. De Schryver, and Jacques Gallay. "Photophysics of tryptophan: global analysis of the fluorescence decay surface as a function of pH, temperature, quencher concentration, excitation and emission wavelengths, timing calibration and deuterium isotope effect." In OE/LASE '92, edited by Joseph R. Lakowicz. SPIE, 1992. http://dx.doi.org/10.1117/12.58201.

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3

Lee, Jin-Ha, Mamoru Nishimoto, Masayuki Okuyama, et al. "ALPHA-SECONDARY DEUTERIUM KINETIC ISOTOPE EFFECTS FOR HYDROLYSIS OF TREHALOSE BY TREHALASE." In XXIst International Carbohydrate Symposium 2002. TheScientificWorld Ltd, 2002. http://dx.doi.org/10.1100/tsw.2002.731.

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4

Lin, C. H., M. H. Lee, B. C. Hsu, and C. W. Liu. "Novel Methods to Incorporate Deuterium in the MOS Structures and Isotope Effects on Soft Breakdown and Interface States." In 2001 International Conference on Solid State Devices and Materials. The Japan Society of Applied Physics, 2001. http://dx.doi.org/10.7567/ssdm.2001.p-1-12.

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5

Rossegger, Bernhard, Michael Engelmayer, and Andreas Wimmer. "Challenges in Measuring Lube Oil Consumption of Internal Combustion Engines Using Deuterium As a Tracer." In ASME 2019 Internal Combustion Engine Division Fall Technical Conference. American Society of Mechanical Engineers, 2019. http://dx.doi.org/10.1115/icef2019-7111.

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Abstract Lube oil emission is thought to have a negative influence on hydrocarbon and particle emissions, autoignition and the life-cycle cost of internal combustion engines. Thus, one of the major goals of combustion engine research and development is to optimize lube oil consumption, for example by optimizing the tribological behavior of the piston group (interaction between piston rings and cylinder liner). This requires the application of a fast and accurate lube oil consumption measurement method. Methods such as gravimetric and volumetric measurement are outdated for R&D applications

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Lashkul, S. I., A. B. Altukhov, E. Z. Gusakov, et al. "Isotopic effect study in the LHCD and LHH experiments in hydrogen/deuterium plasmas of the FT-2 tokamak." In RADIOFREQUENCY POWER IN PLASMAS: Proceedings of the 20th Topical Conference. American Institute of Physics, 2014. http://dx.doi.org/10.1063/1.4864573.

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Ludeman, Susan M., Michael A. D'Alessandro, R. Stephanie Huang, Ivan Spasojevic, and M. Eileen Dolan. "Abstract 4766: The use of deuterium isotope effects to shift the partitioning of cyclophosphamide and ifosfamide among competing, P450-dependent, oxidative pathways." In Proceedings: AACR 103rd Annual Meeting 2012‐‐ Mar 31‐Apr 4, 2012; Chicago, IL. American Association for Cancer Research, 2012. http://dx.doi.org/10.1158/1538-7445.am2012-4766.

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