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Journal articles on the topic 'Electrolytes solide hybride polymère'

Author: Grafiati

Published: 25 May 2024

Last updated: 31 July 2025

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1

Kanai, Yamato, Koji Hiraoka, Mutsuhiro Matsuyama, and Shiro Seki. "Chemically and Physically Cross-Linked Inorganic–Polymer Hybrid Solvent-Free Electrolytes." Batteries 9, no. 10 (2023): 492. http://dx.doi.org/10.3390/batteries9100492.

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Safe, self-standing, all-solid-state batteries with improved solid electrolytes that have adequate mechanical strength, ionic conductivity, and electrochemical stability are strongly desired. Hybrid electrolytes comprising flexible polymers and highly conductive inorganic electrolytes must be compatible with soft thin films with high ionic conductivity. Herein, we propose a new type of solid electrolyte hybrid comprising a glass–ceramic inorganic electrolyte powder (Li1+x+yAlxTi2−xSiyP3−yO12; LICGC) in a poly(ethylene)oxide (PEO)-based polymer electrolyte that prevents decreases in ionic condu

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Ito, Takeru. "Polyoxometalate–Polymer Composites with Distinct Compositions and Structures as High-Performance Solid Electrolytes." Inorganics 13, no. 3 (2025): 75. https://doi.org/10.3390/inorganics13030075.

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Solid electrolytes, including polymer electrolytes, are a promising option for improving the performance of environmentally friendly batteries such as rechargeable lithium-ion batteries or fuel cells. Hydrogen–oxygen fuel cells producing only water under power generation are attracting widespread attention, and they need proton conductors as electrolytes. Fluoropolymer electrolytes such as Nafion® have been utilized for hydrogen–oxygen fuel cells below 100 °C; however, they are not applicable over the working temperature. Therefore, other types of polymer electrolytes are demanded for hydrogen

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3

Choi, Kyoung Hwan, Eunjeong Yi, Kyeong Joon Kim, et al. "(Invited) Pragmatic Approach and Challenges of All Solid State Batteries: Hybrid Solid Electrolyte for Technical Innovation." ECS Meeting Abstracts MA2023-01, no. 6 (2023): 988. http://dx.doi.org/10.1149/ma2023-016988mtgabs.

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For the growth of electric vehicle market, lithium-ion batteries (LIBS) used in the EVs still requires safety and reliability. Unfortunately, large-scale application of the LIBs is being challenged due to the fact that the use of flammable liquid electrolytes has caused safety issues such as leakage and fire explosion. In this respect, all-solid-state batteries (ASSBs) have been intensively studied to ensure the safety and mileage that are superior to the current LIBs. In terms of solid electrolytes, oxide electrolytes not only shows high ionic conductivity (10-4 ~ 10-3 S/cm) but also high mec

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4

Liao, Cheng Hung, Chia-Chin Chen, Ru-Jong Jeng, and Nae-Lih (Nick) Wu. "Application of Artificial Interphase on Ni-Rich Cathode Materials Via Hybrid Ceramic-Polymer Electrolyte in All Solid State Batteries." ECS Meeting Abstracts MA2023-01, no. 6 (2023): 1050. http://dx.doi.org/10.1149/ma2023-0161050mtgabs.

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Among many cathode materials, nickel-rich LiNi0.83Co0.12Mn0.05O2 (NCM 831205) has been spotlighted as one of the most feasible candidates for next-generation LIBs because of its high discharge capacity (~200 mAh/g). However, NCM 831205 shows significant performance degradation, which is mostly attributed to cation mixing, surface side reactions, and intrinsic structural instability originating from the large volume changes during repeated cycling. Conventional lithium ion batteries (LIB) normally use flammable nonaqueous liquid electrolytes, resulting in a serious safety issue in use. In this

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5

LI, X. D., X. J. YIN, C. F. LIN, et al. "INFLUENCE OF I2 CONCENTRATION AND CATIONS ON THE PERFORMANCE OF QUASI-SOLID-STATE DYE-SENSITIZED SOLAR CELLS WITH THERMOSETTING POLYMER GEL ELECTROLYTE." International Journal of Nanoscience 09, no. 04 (2010): 295–99. http://dx.doi.org/10.1142/s0219581x10006831.

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Thermosetting polymer gel electrolytes (TPGEs) based on poly(acrylic acid)-poly(ethylene glycol) (PAA-PEG) hybrid were prepared and applied to fabricate dye-sensitized solar cells (DSCs). N-methylpyrrolidone (NMP) and γ-butyrolactone (GBL) were used as solvents for liquid electrolytes and LiI and KI as iodide source, separately. The microstructure of PAA-PEG shows a well swelling ability in liquid electrolyte and excellent stability of the swollen hybrid. The TPGE was optimized in terms of the liquid electrolyte absorbency and ionic conductivity photovoltaic performance. Quasi-solid-state DSCs

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6

Vargas-Barbosa, Nella Marie, Sebastian Puls, and Henry Michael Woolley. "Hybrid Material Concepts for Thiophosphate-Based Solid-State Batteries." ECS Meeting Abstracts MA2023-01, no. 6 (2023): 984. http://dx.doi.org/10.1149/ma2023-016984mtgabs.

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Solid-state batteries (SSBs) could replace conventional lithium-ion batteries due to the possibility of increasing the energy density of the cells by using lithium metal as the anode material.[1] Among the many electrolyte candidates for lithium SSBs, the lithium thiophosphates are particularly interesting due to their high ionic conductivities at room temperature (>1 mS/cm). However, the (electro)chemical stability of these solid electrolytes is limited and not fully compatible with state-of-the-art high-potential cathode active materials[2] or the lithium metal anode.[3] At the cell level

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Spencer Jolly, Dominic, Dominic L. R. Melvin, Isabella D. R. Stephens, et al. "Interfaces between Ceramic and Polymer Electrolytes: A Comparison of Oxide and Sulfide Solid Electrolytes for Hybrid Solid-State Batteries." Inorganics 10, no. 5 (2022): 60. http://dx.doi.org/10.3390/inorganics10050060.

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Hybrid solid-state batteries using a bilayer of ceramic and solid polymer electrolytes may offer advantages over using a single type of solid electrolyte alone. However, the impedance to Li+ transport across interfaces between different electrolytes can be high. It is important to determine the resistance to Li+ transport across these heteroionic interfaces, as well as to understand the underlying causes of these resistances; in particular, whether chemical interphase formation contributes to giving high resistances, as in the case of ceramic/liquid electrolyte interfaces. In this work, two ce

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Spencer Jolly, Dominic, Dominic L. R. Melvin, Isabella D. R. Stephens, et al. "Interfaces between Ceramic and Polymer Electrolytes: A Comparison of Oxide and Sulfide Solid Electrolytes for Hybrid Solid-State Batteries." Inorganics 10, no. 5 (2022): 60. http://dx.doi.org/10.3390/inorganics10050060.

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Hybrid solid-state batteries using a bilayer of ceramic and solid polymer electrolytes may offer advantages over using a single type of solid electrolyte alone. However, the impedance to Li+ transport across interfaces between different electrolytes can be high. It is important to determine the resistance to Li+ transport across these heteroionic interfaces, as well as to understand the underlying causes of these resistances; in particular, whether chemical interphase formation contributes to giving high resistances, as in the case of ceramic/liquid electrolyte interfaces. In this work, two ce

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9

Lee, Yan Ying, and Andre Weber. "Harmonization of Testing Procedures for All Solid State Batteries." ECS Meeting Abstracts MA2023-02, no. 2 (2023): 340. http://dx.doi.org/10.1149/ma2023-022340mtgabs.

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All Solid State Batteries (ASSBs) with lithium-ion based conducting solid state electrolytes are considered the next generation high performance batteries. They enable high power densities due to their single ion conducting solid electrolyte, eliminating salt concentration gradients and related polarization losses in the cell, and ensuring an unrivalled level of safety due to their non-combustibility. Currently, a variety of ASSBs based on different solid state electrolytes such as polymers, thiophosphates, oxides and combinations thereof are being developed. One general problem with ASSBs is

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CHENG, Xiong, Man LI, Yang Li, Seunghyun Song, Sowjanya Vallem, and Joonho Bae. "Novel DNA-Based Polymer Solid Electrolytes for Lithium-Ion Batteries." ECS Meeting Abstracts MA2024-01, no. 2 (2024): 350. http://dx.doi.org/10.1149/ma2024-012350mtgabs.

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Solid electrolytes are becoming increasingly popular due to their safety [1], and the application of organic biomolecules in electrochemical devices is also an important strategy for sustainable development [2]. Recently, we have studied the application of DNA in electrochemical energy storage devices [3]. A novel PVDF@DNA solid polymer electrolyte was designed in this work, we studied the effect of different DNA addition amounts on polymer solid electrolytes. DNA as a plasticizer-like additive, reduces the crystallinity of the polymer solid electrolyte and improves its ionic conductivity [4].

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Villaluenga, Irune, Kevin H. Wujcik, Wei Tong, et al. "Compliant glass–polymer hybrid single ion-conducting electrolytes for lithium batteries." Proceedings of the National Academy of Sciences 113, no. 1 (2015): 52–57. http://dx.doi.org/10.1073/pnas.1520394112.

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Despite high ionic conductivities, current inorganic solid electrolytes cannot be used in lithium batteries because of a lack of compliance and adhesion to active particles in battery electrodes as they are discharged and charged. We have successfully developed a compliant, nonflammable, hybrid single ion-conducting electrolyte comprising inorganic sulfide glass particles covalently bonded to a perfluoropolyether polymer. The hybrid with 23 wt% perfluoropolyether exhibits low shear modulus relative to neat glass electrolytes, ionic conductivity of 10−4 S/cm at room temperature, a cation transf

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Muñoz, Bianca K., Jorge Lozano, María Sánchez, and Alejandro Ureña. "Hybrid Solid Polymer Electrolytes Based on Epoxy Resins, Ionic Liquid, and Ceramic Nanoparticles for Structural Applications." Polymers 16, no. 14 (2024): 2048. http://dx.doi.org/10.3390/polym16142048.

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Solid polymer electrolytes (SPE) and composite polymer electrolytes (CPE) serve as crucial components in all-solid-state energy storage devices. Structural batteries and supercapacitors present a promising alternative for electric vehicles, integrating structural functionality with energy storage capability. However, despite their potential, these applications are hampered by various challenges, particularly in the realm of developing new solid polymer electrolytes that require more investigation. In this study, novel solid polymer electrolytes and composite polymer electrolytes were synthesiz

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Shah, Rajesh, Vikram Mittal, and Angelina Mae Precilla. "Challenges and Advancements in All-Solid-State Battery Technology for Electric Vehicles." J 7, no. 3 (2024): 204–17. http://dx.doi.org/10.3390/j7030012.

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Recent advances in all-solid-state battery (ASSB) research have significantly addressed key obstacles hindering their widespread adoption in electric vehicles (EVs). This review highlights major innovations, including ultrathin electrolyte membranes, nanomaterials for enhanced conductivity, and novel manufacturing techniques, all contributing to improved ASSB performance, safety, and scalability. These developments effectively tackle the limitations of traditional lithium-ion batteries, such as safety issues, limited energy density, and a reduced cycle life. Noteworthy achievements include fre

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Kirchberger, Anna Maria, Patrick Walke, and Tom Nilges. "Effect of Nanostructured Inorganic Ceramic Filler on Poly(ethylene oxide)-Based Solid Polymer Electrolytes." ECS Meeting Abstracts MA2023-01, no. 6 (2023): 991. http://dx.doi.org/10.1149/ma2023-016991mtgabs.

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In view of the ongoing changes in energy science and technology, the possibilities of energy storage are getting increasingly important. In particular, storing electrical energy is more complex than with fossil fuels. Lithium-Ion batteries are the most commonly used media for energy storage, but they also have some safety-related problems: toxic decomposition products can leak out and the devices can catch fire. Research is underway to find alternatives to minimize this potential hazards. Great improvements in safety matters can be achieved by replacing liquid electrolytes with ceramic/polymer

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Ji, Xiaoyu, Yiruo Zhang, Mengxue Cao, et al. "Advanced inorganic/polymer hybrid electrolytes for all-solid-state lithium batteries." Journal of Advanced Ceramics 11, no. 6 (2022): 835–61. http://dx.doi.org/10.1007/s40145-022-0580-8.

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AbstractSolid-state batteries have become a frontrunner in humankind’s pursuit of safe and stable energy storage systems with high energy and power density. Electrolyte materials, currently, seem to be the Achilles’ heel of solid-state batteries due to the slow kinetics and poor interfacial wetting. Combining the merits of solid inorganic electrolytes (SIEs) and solid polymer electrolytes (SPEs), inorganic/polymer hybrid electrolytes (IPHEs) integrate improved ionic conductivity, great interfacial compatibility, wide electrochemical stability window, and high mechanical toughness and flexibili

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16

Mohanty, Debabrata, Shu-Yu Chen, and I.-Ming Hung. "Effect of Lithium Salt Concentration on Materials Characteristics and Electrochemical Performance of Hybrid Inorganic/Polymer Solid Electrolyte for Solid-State Lithium-Ion Batteries." Batteries 8, no. 10 (2022): 173. http://dx.doi.org/10.3390/batteries8100173.

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Lithium-ion batteries are popular energy storage devices due to their high energy density. Solid electrolytes appear to be a potential replacement for flammable liquid electrolytes in lithium batteries. This inorganic/hybrid solid electrolyte is a composite of lithium bis(trifluoromethanesulfonyl)imide (LiTFSI) salt, (poly(vinylidene fluoride-hexafluoro propylene) (PVDF-HFP) polymer and sodium superionic conductor (NASICON)-type Li1+xAlxTi2−x(PO4)3 (LATP) ceramic powder. The structure, morphology, mechanical behavior, and electrochemical performance of this composite solid electrolyte, based o

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Thangadurai, Venkataraman. "(Invited) Garnet Solid Electrolytes for Advanced All-Solid-State Li Metal Batteries." ECS Meeting Abstracts MA2022-02, no. 47 (2022): 1759. http://dx.doi.org/10.1149/ma2022-02471759mtgabs.

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These days, Li metal anode-based battery has been arisen as one of the key energy storage technologies due to its high theoretical energy density compared to conventional lithium and sodium ion-based batteries. The present Li-S batteries suffer due to Li dendrite formation and capacity decay due to polysulfide dissolution effect, because of organic electrolytes used in the current research. Solid state (ceramic) electrolytes are promising to prevent Li dendrite growth and polysulfide dissolution. Among different ceramic electrolytes garnet-type structure solid inorganic electrolytes are very p

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18

Thangadurai, Venkataraman. "(Invited) Lithium – Sulfur Batteries." ECS Meeting Abstracts MA2022-02, no. 4 (2022): 545. http://dx.doi.org/10.1149/ma2022-024545mtgabs.

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These days, Li-S battery has been arisen as one of the key energy storage technologies due to its high theoretical energy density compared to conventional lithium and sodium ion-based batteries. The present Li-S batteries suffer due to Li dendrite formation and capacity decay due to polysulfide dissolution effect, due to organic electrolytes used in the current research. Solid state (ceramic) electrolytes are promising to prevent Li dendrite growth and polysulfide dissolution. Among different ceramic electrolytes garnet-type structure solid inorganic electrolytes are very promising because of

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19

Méry, Adrien, Steeve Rousselot, David Lepage, David Aymé-Perrot, and Mickael Dollé. "Limiting Factors Affecting the Ionic Conductivities of LATP/Polymer Hybrid Electrolytes." Batteries 9, no. 2 (2023): 87. http://dx.doi.org/10.3390/batteries9020087.

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All-Solid-State Lithium Batteries (ASSLB) are promising candidates for next generation lithium battery systems due to their increased safety, stability, and energy density. Ceramic and solid composite electrolytes (SCE), which consist of dispersed ceramic particles within a polymeric host, are among the preferred technologies for use as electrolytes in ASSLB systems. Synergetic effects between ceramic and polymer electrolyte components are usually reported in SCE. Herein, we report a case study on the lithium conductivity of ceramic and SCE comprised of Li1.4Al0.4Ti1.6(PO4)3 (LATP), a NASICON-

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Zhang, L. X., Y. Z. Li, L. W. Shi, et al. "Electrospun Polyethylene Oxide (PEO)-Based Composite polymeric nanofiber electrolyte for Li-Metal Battery." Journal of Physics: Conference Series 2353, no. 1 (2022): 012004. http://dx.doi.org/10.1088/1742-6596/2353/1/012004.

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Abstract Composite polymer electrolytes (CPEs) based on polyethylene oxide (PEO) offer manufacturing feasibility and outstanding mechanical flexibility. However, the low ionic conductivity of the CPEs at room temperature, as well as the poor mechanical properties, have hindered their commercialization. In this work, Solid-state electrolytes based on polyethylene oxide (PEO) with and without fumed SiO2 (FS) nanoparticles are prepared by electrostatic spinning process. The as-spun PEO hybrid nanofiber electrolyte with 6.85 wt% FS has a relatively high lithium ion conductivity and electrochemical

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Nakajima, Hironori, Linda Bolay, Henrik Ekström, Asuka Shima, Göran Lindbergh, and Yoshitsugu Sone. "Numerical Modeling of Water Transport in a Microporous Layer-Coated Porous Transport Layer for a Polymer Electrolyte Membrane Water Electrolyzer with an Interdigitated Flow Field for Internal Gas-Liquid Separation." ECS Meeting Abstracts MA2024-02, no. 46 (2024): 3279. https://doi.org/10.1149/ma2024-02463279mtgabs.

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We have developed a novel interdigitated flow field for polymer electrolyte membrane electrolyzers (proton exchange membrane water electrolysis cells) for ground and space applications1),2), which are supposed to work in a hybrid system with a low temperature Sabatier reactor for effective use of heat3),4). This design separates the oxygen and liquid water inside the anode of the cell. It dispenses with water circulators and external separators that use natural or centrifugal buoyancy. To date, we have developed a numerical model for optimizing cell structures. Finite element modeling (COMSOL

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Zhai, Yanfang, Wangshu Hou, Zongyuan Chen, et al. "A hybrid solid electrolyte for high-energy solid-state sodium metal batteries." Applied Physics Letters 120, no. 25 (2022): 253902. http://dx.doi.org/10.1063/5.0095923.

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Exploring solid electrolytes with promising electrical properties and desirable compatibility toward electrodes for safe and high-energy sodium metal batteries remains a challenge. In this work, these issues are addressed via an in situ hybrid strategy, viz., highly conductive and thermally stable 1-ethyl-3-methylimidazolium bis(fluorosulfonyl)imide is immobilized in nanoscale silica skeletons to form ionogel via a non-hydrolytic sol-gel route, followed by hybridizing with polymeric poly(ethylene oxide) and inorganic conductor Na3Zr2Si2PO12. Such hybrid design yields the required solid electro

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Giffin, Guinevere A., Mara Goettlinger, Hendrik Bohn, et al. "Development of a Polymer-Based Silicon-NMC Solid-State Cell." ECS Meeting Abstracts MA2023-02, no. 2 (2023): 373. http://dx.doi.org/10.1149/ma2023-022373mtgabs.

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Solid-state batteries are seen as the next generation of battery technology with the promise of high energy density and improved safety as compared to conventional lithium-ion batteries. To achieve these goals, high-capacity negative electrodes, e.g., silicon or lithium, need to be combined with high capacity and high voltage positive electrodes, e.g., Ni-rich NMC. This combination of active materials provides a number of significant challenges for the solid-state electrolyte. If silicon is used as the anode active material, significant volume changes during lithiation/delithiation occur. Thes

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Ryu, Kun, Kyungbin Lee, Hyun Ju, Jinho Park, Ilan Stern, and Seung Woo Lee. "Ceramic/Polymer Hybrid Electrolyte with Enhanced Interfacial Contact for All-Solid-State Lithium Batteries." ECS Meeting Abstracts MA2022-02, no. 7 (2022): 2621. http://dx.doi.org/10.1149/ma2022-0272621mtgabs.

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All solid-state lithium batteries (ASSLBs) with a high energy density are challenging, yet desired by the rising energy demands. Its intrinsic safety of solid-state electrolytes (SSEs) compared to flammable liquid electrolytes makes ASSLBs a modern-day necessity. NASICON-type Li1.5Al0.5Ge1.5P3O12 (LAGP) has high ionic conductivity, high stability against air and water, and a wide electrochemical window. However, the application of LAGP is significantly hindered by its slow interfacial kinetics and brittle nature. In addition, the ionic conductivity of LAGP is relatively low at room temperature

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De Cachinho Cordeiro, Ivan Miguel, Ao Li, Bo Lin, et al. "Solid Polymer Electrolytes for Zinc-Ion Batteries." Batteries 9, no. 7 (2023): 343. http://dx.doi.org/10.3390/batteries9070343.

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To date, zinc-ion batteries (ZIBs) have been attracting extensive attention due to their outstanding properties and the potential to be the solution for next-generation energy storage systems. However, the uncontrollable growth of zinc dendrites and water-splitting issues seriously restrict their further scalable application. Over the past few years, solid polymer electrolytes (SPEs) have been regarded as a promising alternative to address these challenges and facilitate the practical advancement of zinc batteries. In this review, we revisit the research progress of SPEs applied in zinc batter

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Babkova, Tatiana, Rudolf Kiefer, and Quoc Bao Le. "Hybrid Electrolyte Based on PEO and Ionic Liquid with In Situ Produced and Dispersed Silica for Sustainable Solid-State Battery." Sustainability 16, no. 4 (2024): 1683. http://dx.doi.org/10.3390/su16041683.

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This work introduces the synthesis of hybrid polymer electrolytes based on polyethylene oxide (PEO) and electrolyte solution bis(trifluoromethane)sulfonimide lithium salt/ionic liquid 1-ethyl-3-methyl-imidazolium bis(trifluoromethylsulfonyl)imide (LiTFSI/EMIMTFSI) with in situ produced and dispersed silica particles by the sol–gel method. Conventional preparation of solid polymer electrolytes was followed by desolvation of lithium salt in a polymer matrix of PEO, which, in some cases, additionally contains plasticizers. This one-pot synthesis is an alternative route for fabricating a solid pol

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Gerbig, Felix, Anshuman Chauhan, and Hermann Nirschl. "Multi-Scale Modeling and Simulation of All-Solid-State Sodium-Ion Batteries with Polymer-Ceramic Hybrid Electrolytes." ECS Meeting Abstracts MA2024-01, no. 45 (2024): 2499. http://dx.doi.org/10.1149/ma2024-01452499mtgabs.

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Lithium-ion batteries (LIBs) have been widely considered as the most promising power source for mobile devices. However, LIBs cannot meet the increasing global demand for electrochemical energy storage in the foreseeable future. Sodium ion-batteries (SIBs) are based on more ecofriendly and earth-abandoned materials. Commonly researched SIBs are based on liquid electrolytes. They pose leakage and thermal runaway risks. Solid polymer electrolytes solve these problems but need to operate at temperatures between 60-80°C to compensate insufficient ionic conductivity of polymer electrolytes at ambie

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Pham, Quoc-Thai, Badril Azhar, and Chorng-Shyan Chern. "Novel Acrylonitrile-Based Polymers for Solid–State Polymer Electrolyte and Solid-State Lithium Ion Battery." ECS Meeting Abstracts MA2022-01, no. 2 (2022): 160. http://dx.doi.org/10.1149/ma2022-012160mtgabs.

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Rechargeable lithium-ion batteries (LIBs) involving lithium metal oxides, liquid electrolyte and graphite have been widely used in portable electronic devices due to their relatively high energy density and long cycle life. These desirable features make LIBs very attractive as the power source for electronic devices, hybrid electric vehicles (HEVs) and electric vehicles (EVs) applications [1, 2]. For future EV applications, higher energy density of LIBs up to 360 Wh kg-1 is required. Currently, the energy density of the state-of-the-art LIBs using conventional graphite anode, LiFePO4 (denoted

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Falco, Marisa, Gabriele Lingua, Silvia Porporato, et al. "An Overview on Polymer-Based Electrolytes with High Ionic Mobility for Safe Operation of Solid-State Batteries." ECS Meeting Abstracts MA2023-02, no. 4 (2023): 604. http://dx.doi.org/10.1149/ma2023-024604mtgabs.

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Liquid electrolytes used in commercial Li-ion batteries are generally based on toxic volatile and flammable organic carbonate solvents, thus raising safety concerns in case of thermal runaway. The most striking solution at present is to switch on all solid-state designs exploiting polymer materials, films, ceramics, low-volatile, green additives, etc. The replacement of liquids component with low-flammable solids is expected to improve the safety level of the device intrinsically. Moreover, a solid-state configuration is expected to guarantee improved energy density systems. However, low ionic

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Röttgen, Niklas, Michael Holzapfel, Franziska Klein, and Jens Tübke. "Development and Characterization of Hybrid Inorganic-Organic Solid Electrolytes for Their Application in Solid State Sodium Batteries." ECS Meeting Abstracts MA2024-02, no. 9 (2024): 1390. https://doi.org/10.1149/ma2024-0291390mtgabs.

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In recent years sodium-ion batteries (SIB) have received significant attention from academia and industry. Switching the charge carrier inside the battery from lithium to sodium enables the use of non-critical, widely available, affordable resources and in turn offers the potential for low-cost batteries. One drawback of SIB is their lower energy-density compared to state-of-the-art lithium-ion batteries. [1] To increase the energy density of sodium-based batteries, researchers are exploring strategies to implement sodium metal anodes because of their high specific capacity (1165 mAh g-1) and

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Park, MoonJeong. "All-Solid-State Lithium–Sulfur Batteries Enabled By Single-Ion Conducting Particle Electrolytes." ECS Meeting Abstracts MA2024-02, no. 8 (2024): 1108. https://doi.org/10.1149/ma2024-0281108mtgabs.

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The demand for safer alternatives to liquid electrolytes in lithium-ion batteries has stimulated the development of all-solid-state lithium batteries. These advanced batteries aim to mitigate potential hazards associated with flammability and dendrite formation during operation. Additionally, the integration of solid-state electrolytes creates opportunities to improve the energy and power densities of lithium batteries by enabling the direct utilization of lithium metal as the anode. In this study, we designed solid-state hybrid electrolytes with single-ion conducting properties by co-assembli

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Kuppusamy, Hari Gopi, Prabhakaran Dhanasekaran, Niluroutu Nagaraju, et al. "Anion Exchange Membranes for Alkaline Polymer Electrolyte Fuel Cells—A Concise Review." Materials 15, no. 16 (2022): 5601. http://dx.doi.org/10.3390/ma15165601.

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Solid anion exchange membrane (AEM) electrolytes are an essential commodity considering their importance as separators in alkaline polymer electrolyte fuel cells (APEFC). Mechanical and thermal stability are distinguished by polymer matrix characteristics, whereas anion exchange capacity, transport number, and conductivities are governed by the anionic group. The physico-chemical stability is regulated mostly by the polymer matrix and, to a lesser extent, the cationic head framework. The quaternary ammonium (QA), phosphonium, guanidinium, benzimidazolium, pyrrolidinium, and spirocyclic cation-

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Rawat, Suneyana, Monika Michalska, Pramod K. Singh, et al. "Ion Conduction Dynamics, Characterization, and Application of Ionic Liquid Tributyl Methyl Phosphonium Iodide (TMPI)-Doped Polyethylene Oxide Polymer Electrolyte." Polymers 17, no. 14 (2025): 1986. https://doi.org/10.3390/polym17141986.

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The increasing demand for high-performance energy storage devices has stimulated interest in advanced electrolyte materials. Among them, ionic liquids (ILs) stand out for their thermal stability, wide electrochemical windows, and good ionic conductivity. When doped into polymeric matrices, these ionic liquids form hybrid polymeric electrolytes that synergize the benefits of both liquid and solid electrolytes. This study explores a polymeric electrolyte based on polyethylene oxide (PEO) doped with tributylmethylphosphonium iodide (TMPI) and ammonium iodide (NH4I), focusing on its synthesis, str

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Sankara Raman, Ashwin, Samik Jhulki, Billy Johnson, Aashray Narla, and Gleb Yushin. "Facile in-Situ Polymerized Polymer Electrolytes in All Solid-State Lithium-Ion Batteries." ECS Meeting Abstracts MA2022-02, no. 3 (2022): 316. http://dx.doi.org/10.1149/ma2022-023316mtgabs.

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With the push towards renewable energy sources and “green” technologies, lithium-ion batteries (LIBs) have proven to be necessary across multiple technological realms, the biggest of which is currently the electric vehicle (EV) and grid storage markets. But the popular choice of liquid organic electrolytes in LIBs suffers from safety concerns, which motivated significant innovations in safer solid-state electrolytes. Among them, solid polymer electrolytes (SPEs) have shown great potential due to their processability, flexibility and tunability of physical properties. The past decade has seen r

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35

Shah, Vaidik, and Yong Lak Joo. "Rationally Designed in-Situ Gelled Polymer-Ceramic Hybrid Electrolyte Enables Superior Performance and Stability in Quasi-Solid-State Lithium-Sulfur Batteries." ECS Meeting Abstracts MA2023-02, no. 4 (2023): 535. http://dx.doi.org/10.1149/ma2023-024535mtgabs.

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Despite boasting giant leaps in performance improvement over the years, the current commercial standard, Li-ion batteries, are fast approaching their theoretical limits. Meanwhile, Lithium-Sulfur (Li-S) batteries offering ultra-high theoretical energy density (～2600 Whkg-1), cost-effectiveness, and nontoxicity are being seen as promising alternatives. Despite their plentiful advantages, the practicality of Li-S batteries has been largely stymied by several challenges: a) deleterious polysulfide dissolution and ‘shuttle effect’, b) significant volume change of S cathodes during cycling, c) safe

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Okos, Alexandru, Cristina Florentina Ciobota, Adrian Mihail Motoc, and Radu-Robert Piticescu. "Review on Synthesis and Properties of Lithium Lanthanum Titanate." Materials 16, no. 22 (2023): 7088. http://dx.doi.org/10.3390/ma16227088.

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The rapid development of portable electronic devices and the efforts to find alternatives to fossil fuels have triggered the rapid development of battery technology. The conventional lithium-ion batteries have reached a high degree of sophistication. However, improvements related to specific capacity, charge rate, safety and sustainability are still required. Solid state batteries try to answer these demands by replacing the organic electrolyte of the standard battery with a solid (crystalline, but also polymer and hybrid) electrolyte. One of the most promising solid electrolytes is Li3xLa2/3−

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Aruchamy, Kanakaraj, Subramaniyan Ramasundaram, Sivasubramani Divya, Murugesan Chandran, Kyusik Yun, and Tae Hwan Oh. "Gel Polymer Electrolytes: Advancing Solid-State Batteries for High-Performance Applications." Gels 9, no. 7 (2023): 585. http://dx.doi.org/10.3390/gels9070585.

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Gel polymer electrolytes (GPEs) hold tremendous potential for advancing high-energy-density and safe rechargeable solid-state batteries, making them a transformative technology for advancing electric vehicles. GPEs offer high ionic conductivity and mechanical stability, enabling their use in quasi-solid-state batteries that combine solid-state interfaces with liquid-like behavior. Various GPEs based on different materials, including flame-retardant GPEs, dendrite-free polymer gel electrolytes, hybrid solid-state batteries, and 3D printable GPEs, have been developed. Significant efforts have al

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Lin, Ruifan, Yingmin Jin, Yumeng Li, Xuebai Zhang, and Yueping Xiong. "Recent Advances in Ionic Liquids—MOF Hybrid Electrolytes for Solid-State Electrolyte of Lithium Battery." Batteries 9, no. 6 (2023): 314. http://dx.doi.org/10.3390/batteries9060314.

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Li-ion batteries are currently considered promising energy storage devices for the future. However, the use of liquid electrolytes poses certain challenges, including lithium dendrite penetration and flammable liquid leakage. Encouragingly, solid electrolytes endowed with high stability and safety appear to be a potential solution to these problems. Among them, ionic liquids (ILs) packed in metal organic frameworks (MOFs), known as ILs@MOFs, have emerged as a hybrid solid-state material that possesses high conductivity, low flammability, and strong mechanical stability. ILs@MOFs plays a crucia

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Devaux, Didier, Natalia Stankiewicz, Thomas Boulmier, et al. "PEO Electrolyte As Interlayer for Li Metal Battery Comprising an Halide Based Hybrid Electrolyte." ECS Meeting Abstracts MA2024-02, no. 7 (2024): 777. https://doi.org/10.1149/ma2024-027777mtgabs.

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In the context of the energetic transition, lithium (Li) metal is considered as the most promising material for battery anode electrodes regarding its physico-chemical and electrochemical properties with its high capacity leading to high energy density of the device. However, safety issues, such as the well-known dendrites causing short-circuits, limits its use. Solid-state-electrolytes1 such as hybrid electrolyte based on halides2 that are designed to generate synergy between an organic and inorganic phase is foreseen as promising contenders to overcome the current Li-ion limitations. Despite

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CHENG, Xiong, Man Li, and Joonho Bae. "Novel DNA-Based Nanomaterials for High- Performance Lithium-Ion Batteries." ECS Meeting Abstracts MA2025-01, no. 37 (2025): 1771. https://doi.org/10.1149/ma2025-01371771mtgabs.

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In recent years, research on lithium-ion batteries and the application of organic biomolecules in electrochemical devices has attracted considerable attention from researchers.[1][2] Recently, we have studied the application of DNA in electrochemical energy storage devices.[3][4][5] In our latest work, we designed a novel PVDF@DNA solid polymer electrolyte and developed DNA-guided fabrication of LFP micro-roses. In the first study, DNA was used as an additive in polymer solid electrolytes, reducing crystallinity, enhancing ionic conductivity [6], and increasing free lithium ions through its Le

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Park, Jinkyu, and Jungdon Suk. "Rational Design of Hybrid Electrolyte for All-Solid-State Lithium Battery Based on Investigation of Lithium-Ion Transport Mechanism." ECS Meeting Abstracts MA2024-01, no. 5 (2024): 745. http://dx.doi.org/10.1149/ma2024-015745mtgabs.

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Lithium-ion batteries (LIBs) are widely used in various applications, including personal electronic devices, electric vehicles, and energy storage systems. Given the increasing demand for LIBs, there is need to develop rechargeable batteries with high energy densities, long cycle life, and enhanced safety. Lithium all-solid-state batteries (ASSBs) could improve operational safety by eliminating flammable liquid electrolytes and using non-flammable solid electrolytes. Among the various types of solid electrolytes explored, solid polymer electrolytes (SPEs) have garnered significant attention ow

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Toghyani, Somayeh, Florian Baakes, Ningxin Zhang, Helmut Kühnelt, Walter Cistjakov, and Ulrike Krewer. "(Digital Presentation) Model-Assisted Design of Oxide-Based All-Solid-State Li-Batteries with Hybrid Electrolytes for Aviation." ECS Meeting Abstracts MA2022-02, no. 4 (2022): 484. http://dx.doi.org/10.1149/ma2022-024484mtgabs.

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There is a growing interest in the sustainability of the aviation industry sector over the past years due to the environmental issues associated with traditional aviation engines. Electric and hybrid aircrafts are considered promising technologies for reducing fuel consumption and enhancing system efficiency [1]. However, electrical energy storage systems require a higher capacity-to-weight ratio than today’s Li-ion batteries to fulfil the high demands in this area. Safety restrictions imposed by liquid electrolytes motivate the development of next-generation chemistries, such as oxide-based a

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Chometon, Ronan, Marc Dechamps, Jean-Marie Tarascon, and Christel Laberty-Robert. "Meaningful Metrics for an Efficient Solvent-Free Formulation of Polymer – Argyrodite Hybrid Solid Electrolyte." ECS Meeting Abstracts MA2023-02, no. 6 (2023): 929. http://dx.doi.org/10.1149/ma2023-026929mtgabs.

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Solid-state batteries generate huge excitement with the promise of higher energy density than current Li-ion technology, thanks to the use of lithium metal at the anode1. Recent advancements in ceramic electrolytes demonstrate comparable conductivity with liquid ones2. However, the brittleness of ceramics results in mechanical limitations, during both assembly and cycling3, constraining the scale-up of pure-ceramic batteries. Hybrid solid electrolytes (HSE) can overcome this hurdle by combining the superior ionic conductivity of inorganic fillers with the scalable process of polymer electrolyt

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Tronstad, Zachary, and Bryan D. McCloskey. "Exploring the Interaction between EC and Ta-Doped LLZO." ECS Meeting Abstracts MA2024-02, no. 8 (2024): 1227. https://doi.org/10.1149/ma2024-0281227mtgabs.

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Solid-state electrolytes are a primary strategy for unlocking the use of lithium metal anodes and enabling batteries with higher energy density.1 Garnet-type Li7La3Zr2O12 (LLZO) is a leading candidate among ceramic-type materials due to its high ionic conductivity and kinetic stability against lithium metal.2 However, LLZO is air sensitive, spontaneously reacting with CO2 in ambient air to form lithium carbonate layers.3–6 Additionally, we have recently collected evidence, as described below, that suggests that LLZO may even be reactive towards ethylene carbonate (EC), a key liquid electrolyte

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Song, Shufeng, Masashi Kotobuki, Feng Zheng, et al. "Al conductive hybrid solid polymer electrolyte." Solid State Ionics 300 (February 2017): 165–68. http://dx.doi.org/10.1016/j.ssi.2016.12.023.

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46

Zhang, Yinghui, and Jean-François Gohy. "Design of Novel Types of Phosphorus-Containing Flame-Retardant Hybrid Solid Electrolytes with Enhanced Ionic Conductivities." ECS Meeting Abstracts MA2023-02, no. 3 (2023): 483. http://dx.doi.org/10.1149/ma2023-023483mtgabs.

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Hybrid polymer/inorganic solid electrolytes have been considered one of the promising routes toward improved safety and higher energy density compared to today’s liquid electrolytes. Herein, flame-retardant phosphorus-containing random copolymers, namely poly(oligo(ethylene glycol) methyl ether methacrylate)-co-(dimethyl(methacryloyloxy)methyl phosphonate) (P(xPEGMA-co-yMAPC1)), were synthesized with different ratio of monomer compositions and further used as the polymer matrix. By mixing P(xPEGMA-co-yMAPC1) with lithium perchlorate (LiClO4) and acetonitrile (ACN), the solid polymer electrolyt

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47

Bubulinca, Constantin, Natalia E. Kazantseva, Viera Pechancova, et al. "Development of All-Solid-State Li-Ion Batteries: From Key Technical Areas to Commercial Use." Batteries 9, no. 3 (2023): 157. http://dx.doi.org/10.3390/batteries9030157.

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Innovation in the design of Li-ion rechargeable batteries is necessary to overcome safety concerns and meet energy demands. In this regard, a new generation of Li-ion batteries (LIBs) in the form of all-solid-state batteries (ASSBs) has been developed, attracting a great deal of attention for their high-energy density and excellent mechanical-electrochemical stability. This review describes the current state of research and development on ASSB technology. To this end, study of the literature and patents as well as market analysis over the last two decades were carried out, highlighting how sci

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Novakov, Christo, Radostina Kalinova, Svetlana Veleva, Filip Ublekov, Ivaylo Dimitrov, and Antonia Stoyanova. "Flexible Polymer-Ionic Liquid Films for Supercapacitor Applications." Gels 9, no. 4 (2023): 338. http://dx.doi.org/10.3390/gels9040338.

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Mechanically and thermally stable novel gel polymer electrolytes (GPEs) have been prepared and applied in supercapacitor cells. Quasi-solid and flexible films were prepared by solution casting technique and formulated by immobilization of ionic liquids (ILs) differing in their aggregate state. A crosslinking agent and a radical initiator were added to further stabilize them. The physicochemical characteristics of the obtained crosslinked films show that the realized cross-linked structure contributes to their improved mechanical and thermal stability, as well as an order of magnitude higher co

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Foran, Gabrielle, Nina Verdier, David Lepage, Cédric Malveau, Nicolas Dupré, and Mickaël Dollé. "Use of Solid-State NMR Spectroscopy for the Characterization of Molecular Structure and Dynamics in Solid Polymer and Hybrid Electrolytes." Polymers 13, no. 8 (2021): 1207. http://dx.doi.org/10.3390/polym13081207.

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Solid-state NMR spectroscopy is an established experimental technique which is used for the characterization of structural and dynamic properties of materials in their native state. Many types of solid-state NMR experiments have been used to characterize both lithium-based and sodium-based solid polymer and polymer–ceramic hybrid electrolyte materials. This review describes several solid-state NMR experiments that are commonly employed in the analysis of these systems: pulse field gradient NMR, electrophoretic NMR, variable temperature T1 relaxation, T2 relaxation and linewidth analysis, excha

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Lim, Seung, Juyoung Moon, Uoon Baek, Jae Lee, Youngjin Chae, and Jung Park. "Shape-Controlled TiO2 Nanomaterials-Based Hybrid Solid-State Electrolytes for Solar Energy Conversion with a Mesoporous Carbon Electrocatalyst." Nanomaterials 11, no. 4 (2021): 913. http://dx.doi.org/10.3390/nano11040913.

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One-dimensional (1D) titanium dioxide (TiO2) is prepared by hydrothermal method and incorporated as nanofiller into a hybrid polymer matrix of polyethylene glycol (PEG) and employed as a solid-electrolyte in dye-sensitized solar cells (DSSCs). Mesoporous carbon electrocatalyst with a high surface area is obtained by the carbonization of the PVDC-g-POEM double comb copolymer. The 1D TiO2 nanofiller is found to increase the photoelectrochemical performance. As a result, for the mesoporous carbon-based DSSCs, 1D TiO2 hybrid solid-state electrolyte yielded the highest efficiencies, with 6.1% under

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