Relevant bibliographies by topics / Fischer carbenes

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  2. Dissertations / Theses
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  5. Conference papers

Academic literature on the topic 'Fischer carbenes'

Author: Grafiati
Published: 4 June 2021
Last updated: 2 February 2022

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Journal articles on the topic "Fischer carbenes"

1

Wang, Jianbo, and Kang Wang. "Transition-Metal-Catalyzed Cross-Coupling with Non-Diazo Carbene Precursors." Synlett 30, no. 05 (2018): 542–51. http://dx.doi.org/10.1055/s-0037-1611020.

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Transition-metal-catalyzed cross-coupling reactions through metal carbene migratory insertion have emerged as powerful methodology for carbon–carbon bond constructions. Typically, diazo compounds (or in situ generated diazo compounds from N-tosylhydrazones) have been employed as the metal carbene precursors for this type of cross-coupling reactions. Recently, cross-coupling reactions employing non-diazo carbene precursors, such as conjugated ene-yne-ketones, allenyl ketones, alkynes, cyclopropenes, and Cr(0) Fischer carbenes, have been developed. This account will summarize our efforts in the
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Alcaide, Benito, Luis Casarrubios, Gema Dominguez, and Miguel A. Sierra. "Reaction of chromium (Fischer) carbenes and sulfilimines." Journal of Organic Chemistry 58, no. 15 (1993): 3886–94. http://dx.doi.org/10.1021/jo00067a020.

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Padilla, Rosa, Verónica Salazar-Pereda, Daniel Mendoza-Espinosa та ін. "Activation of aldehydes by exocyclic iridium(i)-η4:π2-diene complexes derived from 1,3-oxazolidin-2-ones". Dalton Transactions 45, № 42 (2016): 16878–88. http://dx.doi.org/10.1039/c6dt02866g.

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López, Julio, Iván Velazco-Cabral, Eloy Rodríguez-deLeón, et al. "Selective synthesis of trisubstituted pyrroles through the reactions of alkynyl Fischer carbene complexes with oxazolones." Organic & Biomolecular Chemistry 18, no. 3 (2020): 538–50. http://dx.doi.org/10.1039/c9ob02411e.

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Cui, Peng, Dominic C. Babbini, and Vlad M. Iluc. "C–H activation of ethers by pyridine tethered PCsp3P-type iridium complexes." Dalton Transactions 45, no. 24 (2016): 10007–16. http://dx.doi.org/10.1039/c6dt00303f.

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An iridium complex supported by a PC<sup>Py</sup>P ligand featuring an internal pyridine tether showed selective mono-C–H activation of ethers, which represent intermediates in the synthesis of the corresponding Fischer carbenes.
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Reinheimer, Eric W., Katherine A. Kantardjieff, Xiang Ouyang, Steven R. Herron, Tiffany Lu, and Joe A. Casalnuovo. "Crystal Structures of Diphosphinated Chromium Fischer Amino Carbenes." Journal of Chemical Crystallography 37, no. 8 (2007): 507–15. http://dx.doi.org/10.1007/s10870-007-9194-9.

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Irshaidat, Tareq. "A DFT Study on Selected Physical Organic Aspects of the Fischer Carbene Intermediates [(M(CO)4(C(OMe)Me)]." E-Journal of Chemistry 7, no. 2 (2010): 437–44. http://dx.doi.org/10.1155/2010/202161.

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Fischer carbenes are important starting materials for C-C bond formation via coupling reactions between carbene and wide variety of substituted alkenes or alkynes. This DFT study shed light on unique fundamental organic/organometallic aspects for the C(OMe)Me carbene in the free form and in case of bonding with M(CO)4(M= Cr, Mo, W). The data illustrate that the structures of the title intermediates include a unique structure stabilizing intramolecular M…C-H interaction (agostic interaction). This conclusion was made based on calculated NMR data (for carbon and hydrogen), structural parameters,
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Sandoval-Chávez, César, José G. López-Cortés, Alejandro I. Gutiérrez-Hernández, María C. Ortega-Alfaro, Alfredo Toscano, and Cecilio Alvarez-Toledano. "An expedient approach to ferrocenyl thioamides via Fischer carbenes." Journal of Organometallic Chemistry 694, no. 23 (2009): 3692–700. http://dx.doi.org/10.1016/j.jorganchem.2009.07.044.

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ALCAIDE, B., L. CASARRUBIOS, G. DOMINGUEZ, and M. A. SIERRA. "ChemInform Abstract: Reaction of Chromium (Fischer) Carbenes and Sulfilimines." ChemInform 24, no. 45 (2010): no. http://dx.doi.org/10.1002/chin.199345166.

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López-Alberca, María P., María J. Mancheño, Israel Fernández, Mar Gómez-Gallego, Miguel A. Sierra, and Rosario Torres. "Divergent Pathways in the Reaction of Fischer Carbenes and Palladium." Organic Letters 9, no. 9 (2007): 1757–59. http://dx.doi.org/10.1021/ol070431n.

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Dissertations / Theses on the topic "Fischer carbenes"

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Bezuidenhout, Daniela Ina. "Multimetal complexes of Fischer carbenes." Thesis, University of Pretoria, 2010. http://hdl.handle.net/2263/28973.

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Fischer carbene complexes of the Group VI transition metals (Cr, Mo and W) containing at least two or three different transition metal substituents, all in electronic contact with the carbene carbon atom, were synthesized and studied both in solution and in the solid state. For the complexes of the type [M(CO)5{C(OR)R’}], the substituents chosen included (hetero)aromatic (benzene or thiophene) rings π-bonded to a chromium tricarbonyl fragment or ferrocene as the R’-substituent, while the OR-substituent was systematically varied between an ethoxy or a titanoxy group, to yield the complexes 1 (M
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2

Germaneau, Romain. "Amphiphilic sugar metal carbenes : from fischer type to N-Heterocyclic carbenes (NHCs) : investigations on potential gelation and catalytic activities." Paris 6, 2007. http://www.theses.fr/2007PA066209.

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Le travail présenté ici décrit, en quatre parties, la synthèse d’une nouvelle famille de complexes N-hétérocycliques carbèniques amphiphiles. Le remplacement du carbène de Fischer, présent dans la structure sur laquelle le travail est basé, par un groupe NHC est apparu difficile. Ce problème a pu être résolu par l’utilisation de différents espaceurs. Utilisant une méthode à base d’oxyde d’argent, une nouvelle famille de systèmes amphiphiles comportant un carbène de type NHC du chrome fut accessible. Une étude sur la combinaison possible de la chimie des carbènes de Fischer avec celle des carbè
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Le, Poul Pascal. "Sels de pyrylium et carbenes de fischer action des carbanions des carbenes de fischer sur des sels de pyrylium. Synthese de benzophenones hautement substituees et de carbenes de fischer insatures de type donneur - accepteur, directement ou non directement stabilises par un heteroatome." Rennes 1, 1999. http://www.theses.fr/1999REN10111.

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Les sels de pyrylium sont des heterocycles aromatiques oxygenes presentant un caractere de carbocation. Cette propriete est a l'origine de leur utilisation comme synthon pour la synthese de produits naturels et ils ont joue un role clef dans le developpement de la chimie heterocyclique. Par contre, la chimie organometallique des metaux de transition de ces sels a ete tres peu etudiee. Pour contribuer au developpement de cette chimie, nous avons teste la reactivite du noyau pyrylium avec des carbanions des carbenes de fischer. Dans ce memoire, nous presentons la reactivite des carbanions des ca
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4

Du, Toit Aletta. "Anioniese Fischer-tipe karbeenkomplekse as ligande." Thesis, Stellenbosch : Stellenbosch University, 2003. http://hdl.handle.net/10019.1/53280.

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Stander, Elzet. "Nuwe reaksies van gedeprotoneerde Fischer-tipe karbeenkomplekse." Thesis, Link to the online version, 2005. http://hdl.handle.net/10019/1222.

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Baba, Eduard. "N-Heterocyclic Carbenes of the Late Transition Metals: A Computational and Structural Database Study." Thesis, University of North Texas, 2005. https://digital.library.unt.edu/ark:/67531/metadc4792/.

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A computational chemistry analysis combined with a crystallographic database study of the bonding in late transition metal N-heterocyclic carbene (NHC) complexes is reported. The results illustrate a metal-carbon bond for these complexes, approximately 4% shorter than that of a M-C single bond found in metal alkyl complexes. As a consequence of this result, two hypotheses are investigated. The first hypothesis explores the possibility of multiple-bond character in the metal-carbon linkage of the NHC complex, and the second, considers the change in the hybridization of the carbenoid carbon to
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Meyer, Annalene. "The synthesis of α-alkoxy and α-aminostannanes as precursors to Novel Chromium Fischer Carbenes". Thesis, Rhodes University, 2012. http://hdl.handle.net/10962/d1005036.

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The present study involves the use of main group organometallics: organostannanes and organolithiums as precursors to chromium Fischer carbene complexes. Fischer carbenes are well stabilized by the π‐donor substituents such as alkoxy and amino groups and low oxidation state metals such as Group 6 (Chromium, Molybdenum or Tungsten). Carbenes are an important intermediate in the synthesis of a range of compounds through cyclopropanations, insertions, coupling and photochemical reactions. Synthesis and successful characterisation of three α‐alkoxystannanes was achieved via nucleophilic addition o
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Makanjee, Che Azad. "An experimental and theoretical investigation of unstable Fischer chromium carbene complexes." Thesis, Rhodes University, 2013. http://hdl.handle.net/10962/d1002953.

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This organometallic study involves the use organostannanes and organolithiums as precursors to chromium Fischer carbene complexes. Fischer carbenes are typically electrophilic and are stabilized by a single π-donor substituent, and contain low oxidation state metals (often but not always from Group 6). They are highly reactive and can give access to a range of biologically active compounds through cyclopropanations, insertions, coupling and photochemical reactions. Synthesis and characterization of three MOM-protected α-alkoxy organostannanes was successfully carried out via a nucleophilic add
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Jiménez, Halla José Óscar Carlos. "Theoretical study of catalytic reactions of carbenes: haptotropic rearrangements and the Dötz reaction." Doctoral thesis, Universitat de Girona, 2009. http://hdl.handle.net/10803/7942.

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En aquesta tesi s'han estudiat mecanismes de reaccions de cicloanulació en carbens de Fischer a través de mètodes teòrics, concretament fent servir el nivell de teoria B3LYP/(Wachters' basis / 6-31G**). Els alcoxi- i amino carbens de pentacarbonil crom, ja siguin vinílics o aromàtics, reaccionen amb acetilè per produir fenols, naftols o derivats ciclopentadiè o indè substituïts amb el Cr(CO)3 coordinat, d'una manera regioselectiva. L'objectiu d'aquest treball és discutir ambudes reaccions competitives particularment a la reacció de Dötz, la qual durant els darrers anys ha estat explorada exper
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Stander-Grobler, Elzet. "Carbene ligand and complex design directed towards application in synthesis and homogeneous catalysis." Thesis, Stellenbosch : Stellenbosch University, 2008. http://hdl.handle.net/10019.1/1139.

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Thesis (PhD (Chemistry and Polymer Science))--Stellenbosch University, 2008.<br>Alkylated acetonitrile that forms during the synthesis of the sulfonium salt, [(Me3)2(MeS)S][BF4], is involved in the formation of new , -unsaturated Fischer-type carbene complexes from (CO)5M=C(OMe)CH2Li (M = Cr, W). Metal migration observed when the substitution product obtained from the reaction of the anionic carbene complexes (CO)5M=C(NMe2)CºC¯ (M = Cr, W) with Ph3PAu+ was left in solution, was also kinetically and theoretically investigated. 1H NMR and quantum mechanical (at the B3LYP level of theory) d
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Books on the topic "Fischer carbenes"

1

Powers, Timothy S. Asymmetric Diels-Alder and aldol reactions using Fischer carbene complexes. 1993.

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Gilbertson, Scott R. New reactions of Fischer type carbene complexes and their use in the total synthesis of natural products. 1988.

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3

Bauta, William E. Synthetic strategies employing Fischer carbene complexes. 1990.

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4

Murray, Christopher K. Synthesis with Fischer carbene complexes: Carbene ligand transfer and rearrangements. 1990.

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5

Peterson, Glen Albin. Reactions of unsaturated organotriflates and Fischer-type carbene complexes. 1988.

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Bao, Jianming. Synthetic application of Fischer carbene complexes and catalytic asymmetric reactions. 1993.

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7

Kim, Oak Kyung. Reactions of Fischer carbene complexes with 1,6-enynes: Stereoselectivity and mechanism. 1990.

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8

Challener, Cynthia A. New reactions of Fischer carbene complexes with acetylenes: A synthetic and mechanistic investigation. 1990.

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9

Faron, Katherine L. Reactions of Fischer carbene complexes with unsaturated organic substrates: Studies of the Ene, [2+2] and alkyne annulation processes. 1989.

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Book chapters on the topic "Fischer carbenes"

1

Barluenga, José, Félix Rodríguez, Francisco J. Fañanás, and Josefa Flórez. "Cycloaddition Reactions of Group 6 Fischer Carbene Complexes." In Metal Carbenes in Organic Synthesis. Springer Berlin Heidelberg, 2004. http://dx.doi.org/10.1007/b98763.

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Wu, Yao-Ting, and Armin de Meijere. "The Multifaceted Chemistry of Variously Substituted α,β-Unsaturated Fischer Metalcarbenes." In Metal Carbenes in Organic Synthesis. Springer Berlin Heidelberg, 2004. http://dx.doi.org/10.1007/b98762.

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Reißig, H. U. "Donor-Acceptor-Substituted Cyclopropanes via Fischer Carbene Complexes." In Organometallics in Organic Synthesis 2. Springer Berlin Heidelberg, 1989. http://dx.doi.org/10.1007/978-3-642-74269-9_17.

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Solà, Miquel, Miquel Duran, and Maricel Torrent. "The Dötz Reaction: A Chromium Fischer Carbene-Mediated Benzannulation Reaction." In Catalysis by Metal Complexes. Springer US, 2002. http://dx.doi.org/10.1007/0-306-47718-1_11.

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Weiss, Karin, and Kurt Hoffmann. "Studies on Stoichiometric and Catalytic Metathesis and Other Reactions of Imines With Fischer Type Carbene Tungsten Complexes. Part XVI (1)." In Advances in Metal Carbene Chemistry. Springer Netherlands, 1989. http://dx.doi.org/10.1007/978-94-009-2317-1_38.

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Fernández, Israel, and Miguel A. Sierra. "β-Lactams from Fischer Carbene Complexes: Scope, Limitations, and Reaction Mechanism." In Topics in Heterocyclic Chemistry. Springer Berlin Heidelberg, 2012. http://dx.doi.org/10.1007/7081_2012_87.

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Aumann, R. "Formation of C=C Double Bonds by Novel Insertion Reactions of Allenes, Heterocumulenes and Acid Amides into M=C Bonds of Fischer Carbene Complexes." In Advances in Metal Carbene Chemistry. Springer Netherlands, 1989. http://dx.doi.org/10.1007/978-94-009-2317-1_26.

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Weiss, Karin, Wilfried Guthmann, Michael Denzner, and Sergio Maisuls. "Syntheses of Heterogeneous, Bimetallic Metathesis Catalysts by Reactions of Fischer Type Carbene and Carbyne Complexes with Reduced Phillips Catalyst. Part XVIII (1)." In Olefin Metathesis and Polymerization Catalysts. Springer Netherlands, 1990. http://dx.doi.org/10.1007/978-94-011-3328-9_20.

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Coates, C., J. Kabir, and E. Turos. "Additions of Fischer Carbenes to Imines." In Three Carbon-Heteroatom Bonds: Esters and Lactones; Peroxy Acids and R(CO)OX Compounds; R(CO)X, X=S, Se, Te. Georg Thieme Verlag KG, 2005. http://dx.doi.org/10.1055/sos-sd-021-00596.

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Surman, M. D., and R. H. Hutchings. "Annulation of Fischer Carbenes with Azadienes." In Six-Membered Hetarenes with Two Unlike or More than Two Heteroatoms and Fully Unsaturated Larger-Ring Heterocycles. Georg Thieme Verlag KG, 2004. http://dx.doi.org/10.1055/sos-sd-017-01160.

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Conference papers on the topic "Fischer carbenes"

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Aguilar, Enrique, Alexandra Pérez-Anes, Patricia García-García, and Manuel Fernández-Rodríguez. "Microwave-Accelerated Multi-Component Cascade Reactions Involving Fischer Alkoxy Alkynyl Carbene Complexes." In The 12th International Electronic Conference on Synthetic Organic Chemistry. MDPI, 2008. http://dx.doi.org/10.3390/ecsoc-12-01264.

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