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Journal articles on the topic 'Lithium gel polymer electrolyte system'

Author: Grafiati

Published: 6 September 2023

Last updated: 31 July 2025

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1

Hoang Huy, Vo Pham, Seongjoon So, and Jaehyun Hur. "Inorganic Fillers in Composite Gel Polymer Electrolytes for High-Performance Lithium and Non-Lithium Polymer Batteries." Nanomaterials 11, no. 3 (2021): 614. http://dx.doi.org/10.3390/nano11030614.

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Among the various types of polymer electrolytes, gel polymer electrolytes have been considered as promising electrolytes for high-performance lithium and non-lithium batteries. The introduction of inorganic fillers into the polymer-salt system of gel polymer electrolytes has emerged as an effective strategy to achieve high ionic conductivity and excellent interfacial contact with the electrode. In this review, the detailed roles of inorganic fillers in composite gel polymer electrolytes are presented based on their physical and electrochemical properties in lithium and non-lithium polymer batt

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2

St-Antoine, Caroline, David Lepage, Gabrielle Foran, et al. "Flash Point of Gel-Polymer Electrolytes: Effect of the Molecular Interaction between Nitrile (HNBR) and Carbonyl (PC)." ECS Meeting Abstracts MA2023-01, no. 6 (2023): 995. http://dx.doi.org/10.1149/ma2023-016995mtgabs.

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Gel-polymer electrolytes are receiving increasing attention as they compromise between a good ionic conductivity (10-3S/cm) [1, 2] and good safety features. The solvent trapped into the polymeric matrix increases the ionic conductivity while the polymeric matrix enhances safety due to its mechanical strength repressing dendrite growth [3, 4]. Gel polymer electrolytes are almost universally presumed to be less flammable than current commercialize battery (organic liquid electrolyte) [5, 6]. However, there is no universal test to compare the flammability of a liquid and the flammability of a gel

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3

Kim, Kyeongsik, Wookil Chae, Jaehyeon Kim, Choongik Kim, and Taeshik Earmme. "Gel Polymer Electrolytes for Lithium-Ion Batteries Enabled by Photo Crosslinked Polymer Network." Gels 9, no. 12 (2023): 975. http://dx.doi.org/10.3390/gels9120975.

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We demonstrate a gel polymer electrolyte (GPE) featuring a crosslinked polymer matrix formed by poly(ethylene glycol) diacrylate (PEGDA) and dipentaerythritol hexaacrylate (DPHA) using the radical photo initiator via ultraviolet (UV) photopolymerization for lithium-ion batteries. The two monomers with acrylate functional groups undergo chemical crosslinking, resulting in a three-dimensional structure capable of absorbing liquid electrolytes to form a gel. The GPE system was strategically designed by varying the ratios between the main polymer backbone (PEGDA) and the crosslinker (DPHA) to achi

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4

Rushing, Jeramie C., Anit Gurung, and Daniel G. Kuroda. "Relation between microscopic structure and macroscopic properties in polyacrylonitrile-based lithium-ion polymer gel electrolytes." Journal of Chemical Physics 158, no. 14 (2023): 144705. http://dx.doi.org/10.1063/5.0135631.

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Polymer gel electrolytes (PGE) have seen a renewed interest in their development because they have high ionic conductivities but low electrochemical degradation and flammability. PGEs are formed by mixing a liquid lithium-ion electrolyte with a polymer at a sufficiently large concentration to form a gel. PGEs have been extensively studied, but the direct connection between their microscopic structure and macroscopic properties remains controversial. For example, it is still unknown whether the polymer in the PGE acts as an inert, stabilizing scaffold for the electrolyte or it interacts with th

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5

Razalli, S. M. M., S. I. Y. S. M. Saaid, Tengku Ishak Tengku Kudin, Muhd Zu Azhan Yahya, Oskar Hasdinor Hassan, and Ab Malik Marwan Ali. "Electrochemical Properties of Glyme Based Plasticizer on Gel Polymer Electrolytes Doped with Lithium Bis(Trifluoromethanesulfonyl)Imide." Materials Science Forum 846 (March 2016): 534–38. http://dx.doi.org/10.4028/www.scientific.net/msf.846.534.

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In this study, gel polymer electrolytes (GPEs) system is prepared by the solution cast technique. The system consists of cellulose acetate (CA) as a host polymer, lithium bis(trifluoromethanesulfonyl)imide (LiTFSI) as a dopant salt and diethylene glycol dibutylether (BDG) from glyme based family as a plasticizer. GPEs (65 wt. % CA–25 wt. % LiTFSI–10 wt. % BDG) sample is the highest conductivity of 2.88×10-3 S.cm−1 at room temperature. The lithium-electrolyte interfaced stability is established and the highest ionic conducting electrolyte is able to withstand up to 3.8V vs Li/Li+.

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Pereira, Rhyz, Taber Yim, Andrew Dopilka, Robert Kostecki, and Vibha Kalra. "Understanding Electrode-Electrolyte Interfaces in Gel Polymer Electrolytes Using in-Operando Raman Spectroscopy." ECS Meeting Abstracts MA2024-01, no. 1 (2024): 120. http://dx.doi.org/10.1149/ma2024-011120mtgabs.

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Gel polymer electrolytes hold enormous potential for advancing battery performance and technology, promising high energy densities and safe, rechargeable quasi solid-state batteries. GPEs offer higher ionic conductivities than solid electrolytes and enhanced safety in comparison to liquid electrolytes. A particular advantage of these electrolytes has been their ability to create robust electrode electrolyte interfaces that guide uniform deposition and stripping of lithium via their mechanical strength from the polymer and interface species that form during initial cycling. Herein we report tha

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7

Rajasudha, G., V. Narayanan, and A. Stephen. "Effect of Iron Oxide on Ionic Conductivity of Polyindole Based Composite Polymer Electrolytes." Advanced Materials Research 584 (October 2012): 536–40. http://dx.doi.org/10.4028/www.scientific.net/amr.584.536.

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Composite polymer electrolytes (CPE) have recently received a great attention due to their potential application in solid state batteries. A novel polyindole based Fe2O3 dispersed CPE containing lithium perchlorate has been prepared by sol-gel method. The crystallinity, morphology and ionic conductivity of composite polymer electrolyte were examined by XRD, scanning electron microscopy, and impedance spectroscopy, respectively. The XRD data reveals that the intensity of the Fe2O3 has decreased when the concentration of the polymer is increased in the composite. This composite polymer electroly

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8

AL-Hamdani, Nasser, Paula V. Saravia, Javier Luque Di Salvo, Sergio A. Paz, and Giorgio De Luca. "Unravelling Lithium Interactions in Non-Flammable Gel Polymer Electrolytes: A Density Functional Theory and Molecular Dynamics Study." Batteries 11, no. 1 (2025): 27. https://doi.org/10.3390/batteries11010027.

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Lithium metal batteries (LiMBs) have emerged as extremely viable options for next-generation energy storage owing to their elevated energy density and improved theoretical specific capacity relative to traditional lithium batteries. However, safety concerns, such as the flammability of organic liquid electrolytes, have limited their extensive application. In the present study, we utilize molecular dynamics and Density Functional Theory based simulations to investigate the Li interactions in gel polymer electrolytes (GPEs), composed of a 3D cross-linked polymer matrix combined with two differen

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9

Park, Habin, Anthony Engler, Nian Liu, and Paul Kohl. "Dynamic Anion Delocalization of Single-Ion Conducting Polymer Electrolyte for High-Performance of Solid-State Lithium Metal Batteries." ECS Meeting Abstracts MA2022-02, no. 3 (2022): 227. http://dx.doi.org/10.1149/ma2022-023227mtgabs.

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Lithium metal batteries (LMBs) have been considered as next-generation energy storages due to their extremely high theoretical specific capacity (3860 mAh g-1). However, current LMBs, using conventional liquid electrolytes, still could not fulfill the demand of soaring expansion of energy era, such as electrical vehicles, because of their safety issues, originated by uncontrollable electrolytic side reaction on the lithium, resulting unstable solid-electrolyte interphase (SEI) and vicious lithium dendritic growth [1]. Also, carbonate-based liquid electrolytes have an intrinsic flammability, an

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10

Rizzuto, Carmen, Dale C. Teeters, Riccardo C. Barberi, and Marco Castriota. "Plasticizers and Salt Concentrations Effects on Polymer Gel Electrolytes Based on Poly (Methyl Methacrylate) for Electrochemical Applications." Gels 8, no. 6 (2022): 363. http://dx.doi.org/10.3390/gels8060363.

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This work describes the electrochemical properties of a type of PMMA-based gel polymer electrolytes (GPEs). The gel polymer electrolyte systems at a concentration of (20:80) % w/w were prepared from poly (methyl methacrylate), lithium perchlorate LiClO4 and single plasticizer propylene carbonate (PMMA-Li-PC) and a mixture of plasticizers made by propylene carbonate and ethylene carbonate in molar ratio 1:1, (PMMA-Li-PC-EC). Different salt concentrations (0.1 M, 0.5 M, 1 M, 2 M) were studied. The effect of different plasticizers (single and mixed) on the properties of gel polymer electrolytes w

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11

Sa’adun, Nurul Nadiah, Ramesh Subramaniam, and Ramesh Kasi. "Development and Characterization of Poly(1-vinylpyrrolidone-co-vinyl acetate) Copolymer Based Polymer Electrolytes." Scientific World Journal 2014 (2014): 1–7. http://dx.doi.org/10.1155/2014/254215.

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Gel polymer electrolytes (GPEs) are developed using poly(1-vinylpyrrolidone-co-vinyl acetate) [P(VP-co-VAc)] as the host polymer, lithium bis(trifluoromethane) sulfonimide [LiTFSI] as the lithium salt and ionic liquid, and 1-ethyl-3-methylimidazolium bis(trifluoromethylsulfonyl) imide [EMImTFSI] by using solution casting technique. The effect of ionic liquid on ionic conductivity is studied and the optimum ionic conductivity at room temperature is found to be 2.14 × 10−6 S cm−1for sample containing 25 wt% of EMImTFSI. The temperature dependence of ionic conductivity from 303 K to 353 K exhibit

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12

Zhang, Lan, and Shi Chao Zhang. "Preparation and Characterization of a Novel Gel Polymer Membrane Based on a Tetra-Copolymer." Advanced Materials Research 396-398 (November 2011): 1755–59. http://dx.doi.org/10.4028/www.scientific.net/amr.396-398.1755.

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A acrylonitrile (AN)-methyl acrylate (MMA)-methoxy polyethylene glycol(350) monoacrylate (MPGA)-lithium acrylate (LiAc) tetra-copolymer was synthesized by emulsion polymerization, and phase inversion technique was adopted to prepare the as prepared polymer based microporous membrane. The gel polymer electrolytes (GPEs) were obtained by soak the as-prepared microporous membrane into 1M LiPF6/ (EC (ethylene carbonate) + DEC (diethylene carbonate)) (1:1 vol) electrolyte. FTIR, NMR and TGA/DSC measurements are used to character the components and structure of the polymer. The GPE’s ionic conductiv

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13

Li, Qi, Jian Wang, Mintao Wan, Stefano Passerini, and Dominic Bresser. "New Gel-Polymer Electrolyte for High-Performance Li‖LiFePO₄ Cells with Enhanced Safety." ECS Meeting Abstracts MA2023-02, no. 4 (2023): 788. http://dx.doi.org/10.1149/ma2023-024788mtgabs.

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The use of lithium-metal anodes promises batteries with substantially higher energy densities due to their high theoretical capacity of 3860 mAh g-1 and low redox plateau of -3.04 V vs. the standard hydrogen electrode [1, 2]. Of particular interest in this regard is the combination with (quasi-)solid electrolytes, potentially enabling a stabilized interface with the lithium electrode compared to solely liquid electrolyte systems [3]. Herein, a new gel-polymer electrolyte based on a non-toxic, nitrogen-containing polymer is reported that provides flame-retarding properties and decreases the vol

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14

Zailani, N. A. M., F. A. Latif, Z. S. M. Al Shukaili, Pramod K. Singh, S. F. M. Zamri, and M. A. A. Rani. "Ionic Liquid Encapsulated Poly (Methyl Methacrylate) Electrolyte Film in Electrical Double Layer Capacitor." International Journal of Emerging Technology and Advanced Engineering 12, no. 11 (2022): 89–97. http://dx.doi.org/10.46338/ijetae1122_10.

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One of the main components of electrical double layer capacitor (EDLC) is the electrolyte. Gel-type electrolyte has shown good performance in EDLC. However, not much information is available on film-type electrolytes, which are known to provide better mechanical stability than the gel-type electrolyte. In present study, we have reported the performance of film-type poly(methyl methacrylate (PMMA) as electrolyte in electrical double layer capacitor (EDLC) systems and compared with the gel-type PMMA electrolytes. This film-type PMMA electrolyte is modified by encapsulating 1-methyl-3-pentamethyl

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15

Chernyak, Alexander V., Nikita A. Slesarenko, Anna A. Slesarenko, et al. "Effect of the Solvate Environment of Lithium Cations on the Resistance of the Polymer Electrolyte/Electrode Interface in a Solid-State Lithium Battery." Membranes 12, no. 11 (2022): 1111. http://dx.doi.org/10.3390/membranes12111111.

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The effect of the composition of liquid electrolytes in the bulk and at the interface with the LiFePO4 cathode on the operation of a solid-state lithium battery with a nanocomposite polymer gel electrolyte based on polyethylene glycol diacrylate and SiO2 was studied. The self-diffusion coefficients on the 7Li, 1H, and 19F nuclei in electrolytes based on LiBF4 and LiTFSI salts in solvents (gamma-butyrolactone, dioxolane, dimethoxyethane) were measured by nuclear magnetic resonance (NMR) with a magnetic field gradient. Four compositions of the complex electrolyte system were studied by high-reso

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16

Martinez, Victor, Nis Fisker-Bødker, Smobin Vincent, and Jin Hyun Chang. "Design of High-Entropy Electrolytes Enabled By the High-Throughput and Autonomous Procedure." ECS Meeting Abstracts MA2023-02, no. 2 (2023): 375. http://dx.doi.org/10.1149/ma2023-022375mtgabs.

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Electrolytes in Li-ion batteries play a significant role as they influence different aspects directly related to the battery performance, such as safety, voltage window, electrochemical stability, and the formation of solid-electrolyte interphase (SEI). Conventionally, these electrolytes are composed of a lithium salt dissolved in an organic solvent such as ethylene carbonate and propylene carbonate. Regarding safety, these organic electrolytes can be replaced by room-temperature ionic liquids (RTILs), which present lower vapor pressure and non-flammability.1 Moreover, adding polymer to these

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17

Ari, Muhammad Syahir Sak, Siti Zafirah Zainal Abidin, Mohamad Fariz Mohamad Taib, and Muhd Zu Azhan Yahya. "Electrical and Electrochemical Studies of Polymer Gel Electrolytes Based on Agarose-LiBOB and P(VP-co-VAc)-LiBOB." Solid State Phenomena 317 (May 2021): 385–92. http://dx.doi.org/10.4028/www.scientific.net/ssp.317.385.

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This study focuses on preparation and characterization of polymer gel electrolytes (PGEs) based on agarose–LiBOB–DMSO and poly(1-vinylpyrrolidone-co-vinyl acetate)–LiBOB–DMSO. Two systems of PGEs were prepared by dissolving a different amount (1-8 wt.%) of agarose and (1-8 wt.%) P(VP-co-VAc) as host polymer in 0.8 M of LiBOB–DMSO solution. The addition of host polymer into 0.8 M of LiBOB–DMSO solution will result an optimum conductivity which is 6.91 x 10-3 S.cm-1 for agarose–LiBOB–DMSO system and 7.83 x 10-3 S.cm-1 for P(VP-co-VAc)–LiBOB–DMSO system. In the temperature range of conductivity s

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18

Domalanta, Marcel Roy, and Julie Anne del Rosario. "(Digital Presentation) An Electrochemical-Thermal Coupled Thermal Runaway Multiphysics Model for Lithium Polymer Battery." ECS Meeting Abstracts MA2022-01, no. 2 (2022): 439. http://dx.doi.org/10.1149/ma2022-012439mtgabs.

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With the rising energy demand, safe and efficient energy storage technologies have been increasing in importance. Lithium-ion batteries (LIBs) have been dynamically prevalent as energy storage and power sources for various electrical systems, from communication purposes to transportation applications. Lithium Polymer (LiPo) batteries are a subcategory of LIBs that use a solid or semisolid (gel) polymer to act as both a separator and electrolyte for the system. Compared to a conventional liquid electrolyte, gel polymer electrolyte is more thermally and electrochemically stable and relatively sa

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Chen, Wenting, Yikun Yi, Feng Hai, et al. "A Flexible and Self-Healing Ionic Gel Electrolyte Based on a Zwitterion (ZI) Copolymer for High-Performance Lithium Metal Batteries." Batteries 9, no. 9 (2023): 452. http://dx.doi.org/10.3390/batteries9090452.

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Ionic gel electrolyte retains the characteristics of non-volatilization, non-flammability and outstanding electrochemical stability of ionic liquid, and shows good electrochemical performance combined with the excellent characteristics of different matrix materials, which is considered to be the best choice to achieve high energy density and safety at the same time. In this paper, a flexible and self-healing ionic gel electrolyte was prepared using a solvent-assisted method based on a zteric ion (ZI) copolymer. Abundant hydrogen bonds and synergistic interaction of ions in the electrolyte syst

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Feng, Ningning, Chaoqiang Wang, Jing Wang, Yang Lin, and Gang Yang. "A High-Performance Li-O2/Air Battery System with Dual Redox Mediators in the Hydrophobic Ionic Liquid-Based Gel Polymer Electrolyte." Batteries 9, no. 5 (2023): 243. http://dx.doi.org/10.3390/batteries9050243.

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Lithium–oxygen (Li-O2) batteries have captured worldwide attention owing to their highest theoretical specific energy density. However, this promising system still suffers from huge discharge/charge overpotentials and poor cycling stability, which are related to the leakage/volatilization of organic liquid electrolytes and the inefficiency of solid catalysts. A mixing ionic liquid-based gel polymer electrolyte (IL-GPE)-based Li-O2 battery, consisting of a 20 mM 2,5-di-tert-butyl-1,4-benzoquinone (DBBQ) 40 mM N-methylphenothiazine (MPT)-containing IL-GPE and a single-walled carbon nanotube cath

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Wang, Jingwei, Zejia Zhao, Shenhua Song, Qing Ma, and Renchen Liu. "High Performance Poly(vinyl alcohol)-Based Li-Ion Conducting Gel Polymer Electrolyte Films for Electric Double-Layer Capacitors." Polymers 10, no. 11 (2018): 1179. http://dx.doi.org/10.3390/polym10111179.

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With 1-methyl-2-pyrrolidinone (NMP) as the solvent, the biodegradable gel polymer electrolyte films are prepared based on poly(vinyl alcohol) (PVA), lithium bis(trifluoromethane)sulfonimide (LiTFSI), and 1-ethyl-3 methylimidazoliumbis(trifluoromethylsulfonyl)imide (EMITFSI) by means of solution casting. The films are characterized to evaluate their structural and electrochemical performance. The 60PVA-40LiTFSI + 10 wt.% EMITFSI system exhibits excellent mechanical properties and a high ionic transference number (0.995), indicating primary ionic conduction in the film. In addition, because of t

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Liu, Feng-Quan, Wen-Peng Wang, Ya-Xia Yin, et al. "Upgrading traditional liquid electrolyte via in situ gelation for future lithium metal batteries." Science Advances 4, no. 10 (2018): eaat5383. http://dx.doi.org/10.1126/sciadv.aat5383.

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High-energy lithium metal batteries (LMBs) are expected to play important roles in the next-generation energy storage systems. However, the uncontrolled Li dendrite growth in liquid electrolytes still impedes LMBs from authentic commercialization. Upgrading the traditional electrolyte system from liquid to solid and quasi-solid has therefore become a key issue for prospective LMBs. From this premise, it is particularly urgent to exploit facile strategies to accomplish this goal. We report that commercialized liquid electrolyte can be easily converted into a novel quasi-solid gel polymer electr

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Slesarenko, Nikita A., Alexander V. Chernyak, Kyunsylu G. Khatmullina, et al. "Nanocomposite Polymer Gel Electrolyte Based on TiO2 Nanoparticles for Lithium Batteries." Membranes 13, no. 9 (2023): 776. http://dx.doi.org/10.3390/membranes13090776.

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In this article, the specific features of competitive ionic and molecular transport in nanocomposite systems based on network membranes synthesized by radical polymerization of polyethylene glycol diacrylate in the presence of LiBF4, 1-ethyl-3-methylimidazolium tetrafluoroborate, ethylene carbonate (EC), and TiO2 nanopowder (d~21 nm) were studied for 1H, 7Li, 11B, 13C, and 19F nuclei using NMR. The membranes obtained were studied through electrochemical impedance, IR-Fourier spectroscopy, DSC, and TGA. The ionic conductivity of the membranes was up to 4.8 m Scm−1 at room temperature. The opera

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Wright, Peter V. "Developments in Polymer Electrolytes for Lithium Batteries." MRS Bulletin 27, no. 8 (2002): 597–602. http://dx.doi.org/10.1557/mrs2002.194.

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AbstractRecent developments in polymer electrolyte materials for lithium batteries are reviewed in this article. Four general classifications are recognized: (1) solvent-containing systems in which a liquid electrolyte solution either is fully miscible with a single-phase swollen polymer matrix (gel) or is a two-phase system in which “free” liquid occupies micropores within a swollen polymer network (hybrid), and conductivity (≥∼1 mS cm-1 at ambient temperature) is essentially independent of the polymer segmental motion (the thermal motion of segments of atoms along the backbone of a flexible

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Nikodimos, Yosef, Wei-Nien Su, and Bing-Joe Hwang. "Lithium Dendrite Growth Suppression in Anode-Free Lithium Battery Using Bifunctional Electrospun Gel Polymer Electrolyte Membrane." ECS Meeting Abstracts MA2023-01, no. 6 (2023): 998. http://dx.doi.org/10.1149/ma2023-016998mtgabs.

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Anode free Li metal battery (AFLMB) are being intensively investigating in recent years as a means to achieve higher capacity when compared with standard Li metal batteries. However, the severe electrolyte decomposition during plating/stripping cycles, that causes fast Li dendrite growth and quick capacity fading, is challenging for its commercialization. Herein, poly (vinylidene fluoride-hexafluoropropylene) polymer containing Li1.6Al0.4Mg0.1Ge1.5(PO4)3 ceramic filler (90:10 w% ratio, PVDF-HFP-10) gel polymer electrolyte (GPE) is employed for the first time in AFLMB to suppress the Li dendrit

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Butnicu, Dan, Daniela Ionescu, and Maria Kovaci. "Structure Optimization of Some Single-Ion Conducting Polymer Electrolytes with Increased Conductivity Used in “Beyond Lithium-Ion” Batteries." Polymers 16, no. 3 (2024): 368. http://dx.doi.org/10.3390/polym16030368.

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Simulation techniques implemented with the HFSS program were used for structure optimization from the point of view of increasing the conductivity of the batteries’ electrolytes. Our analysis was focused on reliable “beyond lithium-ion” batteries, using single-ion conducting polymer electrolytes, in a gel variant. Their conductivity can be increased by tuning and correlating the internal parameters of the structure. Materials in the battery system were modeled at the nanoscale with HFSS: electrodes–electrolyte–moving ions. Some new materials reported in the literature were studied, like poly(e

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Khatmullina, Kyunsylu G., Nikita A. Slesarenko, Alexander V. Chernyak, et al. "New Network Polymer Electrolytes Based on Ionic Liquid and SiO2 Nanoparticles for Energy Storage Systems." Membranes 13, no. 6 (2023): 548. http://dx.doi.org/10.3390/membranes13060548.

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Elementary processes of electro mass transfer in the nanocomposite polymer electrolyte system by pulse field gradient, spin echo NMR spectroscopy and the high-resolution NMR method together with electrochemical impedance spectroscopy are examined. The new nanocomposite polymer gel electrolytes consisted of polyethylene glycol diacrylate (PEGDA), salt LiBF4 and 1—ethyl—3—methylimidazolium tetrafluoroborate (EMIBF4) and SiO2 nanoparticles. Kinetics of the PEGDA matrix formation was studied by isothermal calorimetry. The flexible polymer–ionic liquid films were studied by IRFT spectroscopy, diffe

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Shimbori, Yuma, and Kiyoshi Kanamura. "Preparation of 3DOM PI–Ion Gel Composite Electrolyte Membranes for Li Metal Batteries." ECS Meeting Abstracts MA2024-02, no. 7 (2024): 961. https://doi.org/10.1149/ma2024-027961mtgabs.

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The electrolyte used in Li metal batteries (LMBs) contributes to high cycle performance, coulombic efficiency and safety. In particular, highly flammable electrolytes limit an operating temperature of LMBs around room temperature to keep safety, so that an introduction of cooling system is necessary, resulting in a reduction of the energy density of LMBs. Therefore, a use of safer electrolytes is required. Ion gel (IG) electrolytes have attracted attention as a candidate for electrolytes with high safety. Ionic liquid (IL) electrolytes have been incorporated in a polymer matrix. A large amount

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Chelfouh, Nora, Steeve Rousselot, Gaël Coquil, et al. "Using Pectin for Energy Storage Devices." ECS Meeting Abstracts MA2023-01, no. 5 (2023): 891. http://dx.doi.org/10.1149/ma2023-015891mtgabs.

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Wearable and flexible printed electronics are more than ever in demand. The value of the flexible electronics market reached USD 26.5 million in 2021 and its revenue forecast will reach USD 63.1 million in 2030.[1] Increasing investments in research & development in these fields have already led to several achievements in the past years. Nevertheless, serious remains concerns about the ecological footprint of such technologies must be addressed early in their conception and throughout the whole electronics life cycle.[2] In printed electronics, electrical energy is supplied by energy stora

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Kong, Sungho, Myung-keun Oh, Hui-tae Sim, et al. "Monomer Engineering in Gel Polymer Electrolytes for Practical-Level Lithium Metal Battery Performance." ECS Meeting Abstracts MA2025-01, no. 9 (2025): 3164. https://doi.org/10.1149/ma2025-0193164mtgabs.

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Gel polymer electrolytes (GPEs) are highly attractive for developing high-performance rechargeable lithium metal batteries due to their excellent electrochemical performances and enhanced safety. However, when it comes to reach high energy density lithium metal battery with practical conditions such as high areal capacity (> 4 mAh/cm2), high C-rate, wide operating temperature range and etc, the GPEs are still facing hurdles, especially large interfacial resistances and low ionic conducitivity. To breakthrough this, the key component of the GPE, which is monomer, plays critical roles in dete

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He, Xiang Ming, Wei Hua Pu, Jian Jun Li, Chang Yin Jiang, Chun Rong Wan, and Shi Chao Zhang. "Nano Sulfur Composite for Li/S Polymer Secondary Batteries." Key Engineering Materials 336-338 (April 2007): 541–44. http://dx.doi.org/10.4028/www.scientific.net/kem.336-338.541.

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The Li/S polymer secondary batteries presents higher capacity, lower materials cost and much better performance in higher operation temperature. A nano-scale sulfur polymer composite cathode material has been developed for these batteries, and its cycle capacity is over 700mAh/g when the lithium metal is used as the anode; A nano-scale Cu/Sn alloy powder has been synthesized by a novel micro-emulsion process, its cycle capacity is over 300 mAh/g; The performance of PVdF gel electrolyte has been improved through the addition of the nanometer SiO2 synthesized in-situ. The advanced Li/S polymer s

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Sawada, Komei, Daisuke Okuda, and Masashi Ishikawa. "Electrochemical Properties of Solid Electrolytes with High Content of Non-Sintered Ceramics." ECS Meeting Abstracts MA2024-02, no. 8 (2024): 1196. https://doi.org/10.1149/ma2024-0281196mtgabs.

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1.Introduction All-solid-state lithium-ion batteries are rechargeable batteries that use either polymeric or inorganic solid ionic conductor as the electrolyte1). All-solid-state lithium-ion batteries with solid polymer electrolytes have long been investigated because of their ease of handling. There are two types of solid polymer electrolytes currently under consideration: gel-based and dry types2). Gel type has high ionic conductivity because this is swollen by organic solvents, but safety is compromised due to leakage of organic solvents. On the other hand, dry type does not use organic sol

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Mohd Noor, Siti Aminah, Chow Peng Wong, Mariah Zuliana Dzulkipli, Mohd Sukor Su'ait, Lee Tian Khoon та Nur Hasyareeda Hassan. "Properties of Gel Polymer Electrolyte Based Poly(Vinylidine Fluoride-сo-Hexafluoropropylene) (PVdF-HFP), Lithium Perchlorate (LiClO₄) and 1-Butyl-3-Methylimmidazoliumhexafluorophosphate [PF₆]". Solid State Phenomena 317 (травень 2021): 434–39. http://dx.doi.org/10.4028/www.scientific.net/ssp.317.434.

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This study reported the preparation and characterization of gel polymer electrolyte (GPE) using poly (vinylidine fluoride-co-hexafluoropropylene) (PVdF-HFP), lithium perchlorate (LiClO4) and 1-butyl-3-metilimmidazoliumhexafluorophosphate [PF6]. The GPE were prepared by solution casting technique. [Bmim] [PF6] ionic liquid is used as an additive for the purpose of increasing the ionic conductivity of GPE. Morphological analysis showed that the electrolyte gel polymer sample had a smooth and flat surface with the addition of [Bmim] [PF6] and no phase separation effect was observed. This shows th

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Wang, Zeru, and Ke Wang. "Balancing the Mechanical and Electrochemical Properties of Multifunctional Composite Electrolyte for Structural Batteries." ECS Meeting Abstracts MA2024-01, no. 5 (2024): 754. http://dx.doi.org/10.1149/ma2024-015754mtgabs.

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The pursuit of energy-efficient for electric vehicles and aircraft has driven the exploration of structural batteries. In the material-level design of structural batteries, electrode and electrolyte materials act as both load-bearing structures and energy storage elements. During these developments, carbon fibers with excellent mechanical and electrical conductive properties were used as electroactive materials and current collectors. However, most of these systems are combined with electrolytes without mechanical integrity (such as liquid or gel-type electrolytes), thus limiting the load-carr

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Yoo, Seojeong, Sung Ryul Choi, and Jun-Young Park. "Advancements in Thin Solid-State Electrolytes for High-Energy Lithium Metal Batteries." ECS Meeting Abstracts MA2024-02, no. 8 (2024): 1164. https://doi.org/10.1149/ma2024-0281164mtgabs.

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ABSTRACT In the next generation of lithium-ion batteries (LIBs) utilizing lithium metal as the anode material, a theoretical capacity of 3860 mAh·g-1 can be expected [1]. However, several challenges such as safety issues due to lithium dendrite diffusion during charge-discharge cycling still remain unresolved [2]. The penetration of lithium dendrites remains a concern in traditional solution-based LIBs [3]. As an alternative approach to address the challenges of LIBs, solid-state electrolytes (SSEs) with high ionic conductivity and lithium metal stability have garnered attention [4]. The SSE c

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Sugiyama, Takaya, Keisuke Muramatsu, Wataru Sugimoto, and Bruce S. Dunn. "Pseudo-Solid Aqueous Electrolyte with Widened Potential Window By Encapsulating Water-in-Salt in Silica Matrix." ECS Meeting Abstracts MA2024-02, no. 67 (2024): 4529. https://doi.org/10.1149/ma2024-02674529mtgabs.

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Pseudo-solidification of liquid electrolytes is an effective means to prevent electrolyte leakage, and various polymeric materials have been proposed. Recently, silica gel prepared by sol-gel methods has been proposed as an inorganic polymer than can confine liquid electrolytes and has shown to be a promising pseudo-solidification method providing rigidity and stability owing to the inorganic matrix while maintaining the ionic conductivity of liquid electrolytes. For example, silica gel containing an ionic liquid, known as an ionogel, enables solidification while maintaining the properties of

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Nazir, Khuzaimah, Mohamad Fariz Mohamad Taib, Rosnah Zakaria, et al. "Conductivity Studies of Epoxidized PMMA Grafted Natural Rubber Doped Lithium Triflate Gel Polymer Electrolytes." International Journal of Engineering & Technology 7, no. 4.14 (2019): 502. http://dx.doi.org/10.14419/ijet.v7i4.14.27778.

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A gel polymer electrolytes (GPEs) comprising of 62.3 mol% of epoxidized-30% poly(methyl methacrylate) grafted natural rubber (EMG30) as a polymer host, LiCF3SO3 as a dopant salt and ethylene carbonate (EC) as a plasticizer was prepared by solution-casting technique. The effect of plasticizer on the EMG30- LiCF3SO3 on the ionic conductivity is explained in terms of the plasticizer loading of the film. The temperature dependence of the conductivity of the polymer films obeys the Vogel-Tamman-Fulcher (VTF) relationship. The ionic transference number is calculated using Wagner’s polarization techn

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Farhan, Muhammad, Rimsha Naeem, Hafiz Muhammad Shoaib, et al. "Comprehensive Review of Emerging Lithium and Sodium-Ion Electrochemical Systems for Advanced Energy Storage Applications." Scholars Journal of Physics, Mathematics and Statistics 12, no. 05 (2025): 188–98. https://doi.org/10.36347/sjpms.2025.v12i05.005.

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The need for effective, scalable, and sustainable energy storage solutions has increased due to the quick spread of electric cars, portable gadgets, and renewable energy sources. Because of their extended cycle life, high energy density, and established manufacturing infrastructure, lithium-ion (Li-ion) batteries have long dominated the energy storage market. However, the hunt for substitute technologies, especially sodium-ion (Na-ion) batteries, which take advantage of the cheap and plentiful sodium, has accelerated due to the limited supply and growing expense of lithium resources. This pape

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Anderson, Ethan, Antranik Jonderian, and Eric McCalla. "High Throughput Studies of Li-La-Zr-O Garnet Solid Electrolytes." ECS Meeting Abstracts MA2022-02, no. 3 (2022): 226. http://dx.doi.org/10.1149/ma2022-023226mtgabs.

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Development of next-generation Li-ion batteries has increasingly focused on all-solid batteries employing either ceramic, polymer, or glass electrolytes in order to address shortcomings in currently commercialized liquid electrolyte Li-ion batteries including safety, limited lifetime, and lower energy densities resulting from instability with respect to Li metal anodes.[1] Lithium lanthanum zirconium oxide (LLZO) is a leading candidate for solid Li-batteries due to its high Li-ion conductivity, stability in air and against Li metal, and compatibility with high-voltage cathodes.[2],[3] Despite

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Shah, Vaidik, and Yong Lak Joo. "Incorporating Heteroatom-Doped Graphene in Electrolyte for High-Performance Lithium-Sulfur Batteries." ECS Meeting Abstracts MA2022-02, no. 8 (2022): 656. http://dx.doi.org/10.1149/ma2022-028656mtgabs.

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Despite dominating the current commercial energy storage landscape, Li-ion batteries are fast approaching their theoretical limit. Meanwhile, Lithium Sulphur (Li-S) batteries, owing to their ultrahigh theoretical energy density of about 2600 Whkg-1, low-cost, Earth-abundant, and environmentally friendly sulfur (S) cathode, are seen as promising replacements to realize energy densities beyond 500 Whkg-1. Despite these advantages, the large-scale implementation of Li-S technology has been stymied due to several issues, one of the most deleterious of them is the dissolution and shuttling of polys

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Lee, Sangyeop, Im Kyung Han, Youn Soo Kim, and Soojin Park. "Promoting Homogeneous Zinc-Ion Transfer through Preferential Ion Coordination Effect in Gel Electrolyte for Stable Zinc Metal Batteries." ECS Meeting Abstracts MA2024-02, no. 9 (2024): 1355. https://doi.org/10.1149/ma2024-0291355mtgabs.

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In an era increasingly defined by climate change, the shift towards sustainable energy solutions has become a critical global imperative. This shift underscores the importance of developing eco-friendly electricity sources as viable alternatives to fossil fuels, addressing both environmental concerns and the issues of intermittency and instability that plague renewable energy sources. Electrochemical energy storage, exemplified by rechargeable batteries, has emerged as a key technology in this context, offering a means to store renewable energy efficiently. Notably, lithium-ion batteries (LIBs

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NARA, Hiroki, Toshiyuki MOMMA, and Tetsuya OSAKA. "Feasibility of an Interpenetrated Polymer Network System Made of Di-block Copolymer Composed of Polyethylene Oxide and Polystyrene as the Gel Electrolyte for Lithium Secondary Batteries." Electrochemistry 76, no. 4 (2008): 276–81. http://dx.doi.org/10.5796/electrochemistry.76.276.

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Hassan, Md Mehadi, Brett Conners, Mojtaba Ebrahimian Mashhadi, Jinguang Hu, Xia Li, and Qingye Lu. "Electrospinning and Solution-Casting Assisted Aligned Nanocomposite Solid Electrolyte Based on Cellulose Acetate and Chitosan Biopolymers for Sodium-Ion Batteries." ECS Meeting Abstracts MA2025-01, no. 62 (2025): 2947. https://doi.org/10.1149/ma2025-01622947mtgabs.

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The growing popularity and global demand for flexible and wearable microelectronics underscore the need for a cost-effective, eco-friendly, safe, and readily available resource-based clean energy storage system to replace the market-dominating lithium-ion batteries (LIBs)[1],[2]. In particular, concerns about the limited availability and rising costs of lithium resources have heightened the urgency to develop sustainable alternatives. Conventional LIBs, which rely on liquid or gel electrolytes, face significant challenges: corrosion, poor thermal stability, flammability, leakage, and quick den

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Navarra, Maria Assunta, Matteo Palluzzi, Akiko Tsurumaki, and Sergio Brutti. "Electrochemical storage systems: Safer and more sustainable batteries." EPJ Web of Conferences 310 (2024): 00005. http://dx.doi.org/10.1051/epjconf/202431000005.

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Lithium-ion batteries (LIBs) are the predominant power source for portable electronic devices, and in recent years their use has extended to higherenergy and larger devices. However, to satisfy the stringent requirements of safety and energy density, further material advancements are required. Due to the inherent flammability of organic solvent-based liquid electrolytes and their instability against materials utilized in high-energy systems, a transition to alternative ionconductive media becomes urgent. In this paper, some possible solutions, shifting from molecular liquids to a class of mate

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Brehm, Wolfgang, and Julia Kowal. "Conversion Electrodes for Rechargeable Li-Sulfur, Na-Ion and Zn-Air Batteries." ECS Meeting Abstracts MA2024-01, no. 36 (2024): 2053. http://dx.doi.org/10.1149/ma2024-01362053mtgabs.

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Rechargeable batteries are reliable and highly efficient energy storage devices providing high energy density at high voltages with the lead of the Li-ion technology since the early 1990s. Despite these promising advantages, the strongly limited abundance of Li and also that of other elements contained in a Li-ion battery (LIB) leads to the search for low-cost and more abundant alternatives. Especially for stationary storage devices alternative battery technologies are required. Alternative chemistries, such as those based on lithium conversion or alloying, can actually lead to higher energy d

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Li, Kairui, Biao jin, Tong zhang, Qiang Fei, Shubing Zhen, and Jingyu Xu. "Investigation on the properties of PVDF matrix composite porous gel polymer electrolyte doped with lithium silicon gel." E3S Web of Conferences 520 (2024): 03014. http://dx.doi.org/10.1051/e3sconf/202452003014.

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Gel polymer electrolytes are safer because they do not contain liquid phase components. On this basis, the introduction of inorganic fillers effectively overcame the problem of low ionic conductivity of polymer electrolyte at room temperature, and the constructed composite polymer electrolyte (CPEs) combined the advantages of inorganic fillers and polymer segments. In this paper, lithium silicon gel SiO2(Li+) was prepared by in-situ polymerization and sol-gel method, and doped in PVDF composite porous gel polymer electrolyte film prepared by immersion precipitation method. The electrochemical

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Luo, Wenhan, Kuirong Deng, Shuanjin Wang, et al. "A Novel Gel Polymer Electrolyte by Thiol-Ene Click Reaction Derived from CO2-Based Polycarbonate for Lithium-Ion Batteries." Advances in Polymer Technology 2020 (July 17, 2020): 1–12. http://dx.doi.org/10.1155/2020/5047487.

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Here, we describe the synthesis of a CO2-based polycarbonate with pendent alkene groups and its functionalization by grafting methoxypolyethylene glycol in view of its application possibility in gel polymer electrolyte lithium-ion batteries. The gel polymer electrolyte is prepared by an in-situ thiol-ene click reaction between polycarbonate with pendent alkene groups and thiolated methoxypolyethylene glycol in liquid lithium hexafluorophosphate electrolyte and exhibits conductivity as remarkably high as 2.0×10−2 S cm−1 at ambient temperature. To the best of our knowledge, this gel polymer elec

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Owensby, Kyra, Wan-Yu Tsai, Ritu Sahore, and Xi Chen. "Lithium Morphology Evolution through Crosslinked Poly(ethylene oxide) Solid Polymer Electrolyte." ECS Meeting Abstracts MA2023-01, no. 7 (2023): 2820. http://dx.doi.org/10.1149/ma2023-0172820mtgabs.

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Solid-state, lithium metal batteries are promising candidates for developing the safe, energy-dense devices needed to transition to an electrified economy. However, lithium is highly reactive, making it thermodynamically unstable when in contact with many electrolyte materials. Achieving uniform Li plating and stripping during cycling is the key for enabling high energy Li metal batteries. The lithium stripping and plating mechanism is complicated as it can be affected by the cathode, electrolyte and lithium anode, and the resulting solid electrolyte interphase (SEI). In particular, the mechan

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Boz, Buket, Hunter O. Ford, Alberto Salvadori, and Jennifer L. Schaefer. "Porous Polymer Gel Electrolytes Influence Lithium Transference Number and Cycling in Lithium-Ion Batteries." Electronic Materials 2, no. 2 (2021): 154–73. http://dx.doi.org/10.3390/electronicmat2020013.

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To improve the energy density of lithium-ion batteries, the development of advanced electrolytes with enhanced transport properties is highly important. Here, we show that by confining the conventional electrolyte (1 M LiPF6 in EC-DEC) in a microporous polymer network, the cation transference number increases to 0.79 while maintaining an ionic conductivity on the order of 10−3 S cm−1. By comparison, a non-porous, condensed polymer electrolyte of the same chemistry has a lower transference number and conductivity, of 0.65 and 7.6 × 10−4 S cm−1, respectively. Within Li-metal/LiFePO4 cells, the i

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Lipkin, M. S., Y. V. Verdi, O. Y. Reznikova, et al. "Study of tin-based composite anode in gel-polymer electrolyte." PERSPEKTIVNYE MATERIALY 8 (2024): 23–30. http://dx.doi.org/10.30791/1028-978x-2024-8-23-30.

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The aim of the work was to study the cycling of composite electrode tin-ultradisperse tin powder in gel-polymer electrolyte based on polyvinylidene difluoride. It was shown by the conducted studies that the cathodic introduction of lithium into the composite electrode tin-ultradisperse tin powder from gel-polymer electrolyte on the basis of PVDF is accompanied by disordered of the initial structure, which reduces the difficulties of the subsequent intercalation and leads to an increase in the lithium diffusion coefficient from 10–14 up to 10–10 cm2/s with increasing stoichiometry of the interc

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