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Dissertations / Theses on the topic 'Nucleophilic reaction'

Author: Grafiati

Published: 4 June 2021

Last updated: 8 February 2022

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1

Duff, Jack Lawrence. "Single electron transfer in nucleophilic reactions of substituted norbornanes." Thesis, Georgia Institute of Technology, 1989. http://hdl.handle.net/1853/27444.

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2

Dehestani, Ahmad. "Exploring reactivities of oxo and nitrido ligands on high valent osmium with electrophiles, nucleophiles, alkenes, hydrogen, and methane. /." Thesis, Connect to this title online; UW restricted, 2004. http://hdl.handle.net/1773/8626.

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3

Belknap, Ethan M. "Computational Model of the Nucleophilic Acyl Substitution Pathway." Wittenberg University Honors Theses / OhioLINK, 2021. http://rave.ohiolink.edu/etdc/view?acc_num=wuhonors1623251026132848.

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4

Parker, David J. "Modelling nucleophilic substitution at main group elements by NMR spectroscopy and X-ray crystallography." Thesis, Open University, 1997. http://ethos.bl.uk/OrderDetails.do?uin=uk.bl.ethos.363493.

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5

Curry, Omadee S. "Reaction of o-Nitrobenzenesulfonyl Azide/n-Butyl Lithium with Hindered Alcohols." Youngstown State University / OhioLINK, 2013. http://rave.ohiolink.edu/etdc/view?acc_num=ysu1379945812.

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6

Omakor, Emegbero John. "The reaction mechanism and Ã-effect in nucleophilic displacement at the phosphorus center of the pesticide, fenitrothion, by oxygen nucleophiles in aqueous medium." Thesis, National Library of Canada = Bibliothèque nationale du Canada, 1998. http://www.collectionscanada.ca/obj/s4/f2/dsk2/ftp04/mq22373.pdf.

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7

Moagi, Kgotso Herbet. "Reaction Mechanism of 2-monosubstituted Quinoxalines with Organolithium Compounds : a Theoretical Study." Diss., University of Pretoria, 2020. http://hdl.handle.net/2263/75182.

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This dissertation describes the density functional theory (DFT) computational modelling of reactions between organolithium nucleophiles and various substituted quinoxalines. These reactions result in the functionalisation of the C (sp2)–H bond, thus substituting the sigma-hydrogen. The reactions are known as nucleophilic substitution of hydrogen (SNH) and are used by experimental chemists to form new C–C bonds. The SNH reactions are very important in various industries, e.g. in designing and manufacturing of pharmaceuticals. Quinoxaline is widely used in medicinal chemistry due to its various

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8

Machover, Sarah B. "Understanding the Solvent-free Nucleophilic Substitution Reaction Performed in the High Speed Ball Mill (HSBM): Reactions of Secondary Alkyl Halides and Alkali Metal-Halogen Salts." University of Cincinnati / OhioLINK, 2011. http://rave.ohiolink.edu/etdc/view?acc_num=ucin1307043848.

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9

Danielsson, Jakob. "Stereoselective Nucleophilic Additions to Aldehydes and Synthesis of α-Amino-β- Hydroxy-Esters". Licentiate thesis, KTH, Organisk kemi, 2012. http://urn.kb.se/resolve?urn=urn:nbn:se:kth:diva-95467.

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This thesis deals with the development of new reaction methodology as well as stereochemical investigations. The first part concerns the investigation of 1,2- and merged 1,2- and 1,3- asymmetric induction in Mukaiyama aldol additions to α-heteroatom and α,β- heteroatom substituted aldehydes respectively. In particular, the unexpected 1,2-syn selectivity obtained in the addition of sterically hindered nucleophiles to α-chloroaldehydes is examined, and an explanation for the observed stereochemical trends is proposed. The second part describes the development of a novel entry to α-amino-β- hydro

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10

Soper, Jake D. "Reactions at nitrogenous ligands on oxidizing group 8 metal centers /." Thesis, Connect to this title online; UW restricted, 2003. http://hdl.handle.net/1773/8589.

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11

Buquoi, John Quentin III. "Exploration Using Reaction Temperature to Tailor the Degree of Order in Micro-Block Copolymer Proton Exchange Membranes." Wright State University / OhioLINK, 2010. http://rave.ohiolink.edu/etdc/view?acc_num=wright1274493418.

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12

Chan, Mary S. W. "Factors influencing the regiochemistry of nucleophilic addition to the radical cation of alkenes and dienes studied in the context of the photochemical nucleophile-olefin combination, aromatic substitution (photo-NOCAS) reaction." Thesis, National Library of Canada = Bibliothèque nationale du Canada, 1998. http://www.collectionscanada.ca/obj/s4/f2/dsk2/ftp02/NQ36574.pdf.

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13

Métivier, Pascal. "Synthese organique assistee par ordinateur : l'approche synthetique." Université Louis Pasteur (Strasbourg) (1971-2008), 1987. http://www.theses.fr/1987STR13190.

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Deux programmes fonctionnant dans le sens synthetique, c'est a dire permettant de simuler les reactions, ont ete realises l'un a l'universite louis pasteur a strasbourg (france), et l'autre, a l'universite john purdue (usa). Ce memoire decrit les choix developpes lors de la realisation de ces programmes ainsi que leur fonctionnement. Differents aspects, tels la reconnaissance des caracteristiques d'interet synthetique d'une molecule, un modele de la chimie nucleophile ainsi qu'un modele des reactions de reductions, correspondant au travail d'interet chimique effectue sont particulierement deta

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14

Kahef, Lana el. "Oxydation des mesotetraphenyl porphyrines : beta-substitution par voie electrochimique directe." Université Louis Pasteur (Strasbourg) (1971-2008), 1987. http://www.theses.fr/1987STR13221.

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15

Dlubala, Alain. "Etude de la reactivite de dianions formes par double deprotonation de dithioesters beta-thiosubstitues." Caen, 1987. http://www.theses.fr/1987CAEN2010.

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16

Sullivan, Shannon M. "Synthesis of 2,4-disubstituted pyrimidine derivatives as potential 5-HT7 receptor antagonist." unrestricted, 2008. http://etd.gsu.edu/theses/available/etd-05052008-153400/.

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Thesis (M.S.)--Georgia State University, 2008.<br>Title from file title page. Lucjan Strekowski, committee chair; A.L. Baumstark, Gabor Patonay, Doyle Barrow , committee members. Electronic text (68 p. : ill.) : digital, PDF file. Description based on contents viewed June 23, 2008. Includes bibliographical references (p. 42-430.

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17

MacMillar, Susanna. "Isotopes as Mechanism Spies : Nucleophilic Bimolecular Substitution and Monoamine Oxidase B Catalysed Amine Oxidation Probed with Heavy Atom Kinetic Isotope Effects." Doctoral thesis, Uppsala : Acta Universitatis Upsaliensis (AUU), 2006. http://urn.kb.se/resolve?urn=urn:nbn:se:uu:diva-7441.

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18

Annandale, Michael Thomas. "NMR spectroscopic studies of nucleophilic attack on dinitroaniline herbicides, reactions of selected nucleophiles with trifluralin and benefin." Thesis, National Library of Canada = Bibliothèque nationale du Canada, 1997. http://www.collectionscanada.ca/obj/s4/f2/dsk2/ftp04/mq22268.pdf.

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19

Beji, Mohamed. "Heterocumulenes alpha -sulfonyles et leurs applications a la synthese de nouvelles structures heterocycliques : alkylation des esters sulfamiques en catalyse par transfert de phase." Paris 7, 1987. http://www.theses.fr/1987PA077183.

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20

Millan, Michael John. "The attachment of dyes to amino acids /." Title page, contents and abstract only, 1996. http://web4.library.adelaide.edu.au/theses/09PH/09phm6448.pdf.

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21

Xie, Sheng. "Perfluroaryl azides : Reactivities, Unique Reactions and their Applications in the Synthesis of Theranostic Agents." Doctoral thesis, KTH, Organisk kemi, 2015. http://urn.kb.se/resolve?urn=urn:nbn:se:kth:diva-172950.

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The work centersaround perfluoroaryl azides (PFAAs), and theirability to undergo certain fast and robusttransformations. The chemistry was furtherappliedfor biomedical applications. The first section focuses on the azide-aldehyde-amine cycloaddition using PFAAs. Experimental and computational investigations uncovered a fast azide-enamine cycloaddition to form triazolines, which spontaneously rearrange into stable amidine products. In addition, this transformation was explored in the formulation of pure nanodrugs. Because this reaction can introduce a phenyl and a perfluoroaryl moiety enabling

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22

Martin, Peter Arnold. "Nucleophilic substitution reactions of some polyhalogenated compounds." Thesis, Durham University, 1987. http://etheses.dur.ac.uk/6876/.

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Rate measurements for the reactions of a series of polyfluoro - and polychloro - pyridines with aniline and ammonia in 60/40 dioxan/water at 25ºC has shown that chlorine, when ortho and para to the position of attack, is activating with respect to fluorine, but at the position meta to the point of attack, chlorine and fluorine are virtually equivalent in their effect on reaction rate. The trifluoromethyl and nitrile groups were found to be activating relative to fluorine when ortho and para to the position of substitution and the nitrile group was thus found to be ortho/para directing. The ort

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23

Haleem, Asad Bilal. "Crosslinking nucleophilic dyes on cotton." Thesis, University of Leeds, 2002. http://ethos.bl.uk/OrderDetails.do?uin=uk.bl.ethos.250890.

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24

Cino, Silvia <1985&gt. "Coupling Reactions Between Aromatic Carbon - and Nitrogen - Nucleophiles and Electrophiles: Reaction Intermediates, Products and their Properties." Doctoral thesis, Alma Mater Studiorum - Università di Bologna, 2016. http://amsdottorato.unibo.it/7566/.

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During my PhD I was involved in many studies concerning the nucleophilic (SNAr) and electrophilic (SEAr) aromatic substitution reactions. My research activity was focused on the study of different electrophile/nucleophile combinations between strongly activated species, with the purpose to investigate on their reactivity, to detect new intermediates of the aromatic substitution reaction and to obtain new higly conjugated structures bearing contemporaneously electron donor and acceptor moieties on the same unit for application in different fields. Different reactions between both neutral or c

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25

HADDAD-FAHED, OMAIMA. "Catalyse micellaire de reactions de substitution nucleophile aromatique comportant des reactifs electriquement charges." Paris 6, 1987. http://www.theses.fr/1987PA066419.

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26

Beaumont, Andrew J. "A study of some selective nucleophilic fluorination reactions." Thesis, University of York, 1992. http://ethos.bl.uk/OrderDetails.do?uin=uk.bl.ethos.306248.

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27

Iagrossi, Anna. "Stereochemical studies of reactions of phosphate and thiophosphate esters." Thesis, University of Leicester, 1988. http://hdl.handle.net/2381/33748.

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Nucleophilic substitution reactions involving phosphate monoesters have been investigated. Two general syntheses of O-alkyl or O-aryl [16O,18O] thiophosphate monoesters are reported. An independent and general method for the determination of the enantiomeric excess of isotopically chiral thiophosphate monoesters has been developed and the absolute configurations of the diastereoisomers of (2R)-O-(O-ethyl thiophosphoryl)-3, 4S-dimethyl-5S-phenyl-l,3,2-oxazaphos- pholidin-2-one have been assigned. The solvolysis of p-nitrophenyl [R-16O,18O] thiophosphate in ethanol gives rise to ethyl [16O, 18O]

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28

Jones, Craig Warren. "Nucleophilic aromatic substitution using supported copper(I) reagents." Thesis, University of York, 1989. http://ethos.bl.uk/OrderDetails.do?uin=uk.bl.ethos.236184.

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29

Diep, Nhut Kiet. "Studies of nucleophile ring opening of oxabicyclic systems in highly polar media application to a total synthesis of antitumor agent, (-)-epothilone B /." Diss., Montana State University, 2006. http://etd.lib.montana.edu/etd/2006/diep/DiepN0806.pdf.

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Polyketides constitute an important family of natural products, having a broad spectrum of biological activity such as antitumor, antibiotic, antifungal, or immunomodulatory action.Â¹ Many of these compounds possess polypropionates (units with alternating hydroxyl and methyl groups), reflecting their common biosynthesis that is found within nature. Their structural complexity and importance of these compounds as therapeutical agents have made them attractive targets for synthetic organic chemists.Â¹ Excellent chiral propionate reagents have been developed over the years,

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30

Popp, Ann E. "Investigation of the lifetimes of electrochemically generated anthracene cation radicals in the presence of selected nucleophiles." Thesis, Georgia Institute of Technology, 1988. http://hdl.handle.net/1853/27173.

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31

BOUAYAD, ZOHEIR. "Ouverture nucleophile d'aziridines fonctionnalisees par des composes a methylene actif : synthese de pyrrolidones-2 fonctionnalisees." Clermont-Ferrand 2, 1987. http://www.theses.fr/1987CLF2S884.

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32

Baxter, Nicholas James. "The mechanisms of reactions of #beta#-sultams." Thesis, University of Huddersfield, 1998. http://ethos.bl.uk/OrderDetails.do?uin=uk.bl.ethos.285584.

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33

Drew, S. M. "Photochemical nucleophilic substitution reactions of quinones and related systems." Thesis, University of Leeds, 1986. http://ethos.bl.uk/OrderDetails.do?uin=uk.bl.ethos.374182.

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34

Van, der Westhuizen Carl Johan. "Nucleophilic substitution reactions of α-haloketones : a computational study". Diss., University of Pretoria, 2017. http://hdl.handle.net/2263/63346.

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This dissertation describes the computational modelling of reactions between α-haloketones and various nucleophiles. Nucleophilic substitution reactions of α-haloketones (also known as α- halocarbonyls in literature) are utilised in synthetic laboratories to obtain 1,2-disconnections; which are typically difficult to obtain otherwise. To gain insight into these reactions, DFT modelling was carried out in this project, with further understanding into these reactions being obtained using Quantum Fragment Along Reaction Pathway (QFARP) which is an extension of Interacting Quantum Atoms (IQA

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35

Liu, Jiangqiong. "Kinetic Studies of 6-Halopurine Nucleoside in SNAr Reactions; 6-(Azolyl, Alkylthio and Fluoro)-purine Nucleosides as Substrates for Suzuki Reactions." Diss., CLICK HERE for online access, 2007. http://contentdm.lib.byu.edu/ETD/image/etd1821.pdf.

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36

Rafiq, Adnan. "Synthesis and reactions of therapeutic nucleophiles." Thesis, University of Newcastle Upon Tyne, 1998. http://ethos.bl.uk/OrderDetails.do?uin=uk.bl.ethos.262891.

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37

Sakamoto, Ryu. "Development of Amine-catalyzed Asymmetric Reactions Using Hetero-functionalized Acetaldehydes as Nucleophiles." 京都大学 (Kyoto University), 2014. http://hdl.handle.net/2433/188503.

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38

HURTAUD, DOMINIQUE. "Reactions chimioselectives des epoxydes gem-dinitriles avec des reactifs nucleophiles : preparation et interet synthetique d'epoxyimidates." Rennes 1, 1993. http://www.theses.fr/1993REN10064.

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L'objectif de ce travail est d'une part l'etude de la chimioselectivite de la reaction des epoxydes gem-dinitriles avec des reactifs nucleophiles en milieu basique et d'autre part l'evaluation de l'interet synthetique des epoxyiminoethers. Nous montrons que les bases s'additionnent rapidement de facon reversible sur l'un des nitriles de l'epoxyde. L'evolution de cet adduit primaire depend de l'encombrement de l'epoxyde, de la nature du nucleophile et de la stabilite du produit de reaction. Nous isolons: soit des produits d'addition sur le nitrile: epoxyiminoethers, epoxyamidines et epoxyimidaz

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39

Zioga, Georgia. "Studies on the reaction of pyrrolobenzodiazepines with nucleophiles." Thesis, University of Portsmouth, 1999. http://ethos.bl.uk/OrderDetails.do?uin=uk.bl.ethos.298374.

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40

Balan, Gayatri. "Studies on the nucleophilic substitution reactions of a dimeric cyclopentadienone." Diss., Columbia, Mo. : University of Missouri-Columbia, 2007. http://hdl.handle.net/10355/6265.

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Thesis (M.S.)--University of Missouri-Columbia, 2007.<br>The entire dissertation/thesis text is included in the research.pdf file; the official abstract appears in the short.pdf file (which also appears in the research.pdf); a non-technical general description, or public abstract, appears in the public.pdf file. Title from title screen of research.pdf file (viewed on January 11, 2008) Includes bibliographical references.

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41

James, Rachel Anne. "Nucleophilic substitution reactions of (alkoxymethylene) dimethylammonium chloride and cyclopropane methodology." Thesis, Imperial College London, 1999. http://ethos.bl.uk/OrderDetails.do?uin=uk.bl.ethos.342180.

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42

Kim, Jong Chul. "Nucleophilic Addition Reactions to Carbonyl Compounds under High Pressure Environment." Kyoto University, 2003. http://hdl.handle.net/2433/148945.

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Kyoto University (京都大学)<br>0048<br>新制・課程博士<br>博士(人間・環境学)<br>甲第10308号<br>人博第195号<br>14||159(吉田南総合図書館)<br>新制||人||48(附属図書館)<br>UT51-2003-H729<br>京都大学大学院人間・環境学研究科人間・環境学専攻<br>(主査)教授松本澄, 教授山内淳, 教授山口良平<br>学位規則第4条第1項該当

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43

Giles, Robert G. "Some reactions of acyl cation equivalents with nucleophilic aromatic systems." Thesis, Loughborough University, 1986. https://dspace.lboro.ac.uk/2134/11087.

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Trimethyloxonium fluoroborate rapidly reacts with nitriles at elevated temperatures, to afford N-methylnitrilium salts. Subsequent reaction with π-excessive heterocyclic aromatic systems has been shown to give rise to iminium salts in moderate to excellent yields. The related imines may be obtained by deprotonation, and these compounds can be converted further by reduction or hydrolysis to secondary amines or ketones respectively. The reactions studied provide access to acylated indoles and pyrroles which are obtainable by other methods in inferior yields. The related reactions with carbocycli

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44

Nomura, Kenichi. "Studies on a Nucleophilic Cyclopropanation Reactions with Bis(iodozincio)methane." 京都大学 (Kyoto University), 2010. http://hdl.handle.net/2433/120873.

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45

Bhavaraju, Sitaram. "Study of nucleaphilicity of an enol tosylate fragment of [alpha]- formylglycine ([alpha]-FGly-Ots) /." View online ; access limited to URI, 2007. http://0-digitalcommons.uri.edu.helin.uri.edu/dissertations/AAI3292101.

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46

Khodaei, M. M. "The reactions of diazo compounds with nucleophiles." Thesis, University of Liverpool, 1988. http://ethos.bl.uk/OrderDetails.do?uin=uk.bl.ethos.384393.

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47

Williams, Kenneth Bruce. "The effect of methyl groups on nucleophilic substitution reactions of chlorocyclotriphosphazenes." Diss., Virginia Polytechnic Institute and State University, 1985. http://hdl.handle.net/10919/49962.

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The reactions of methyl-substituted chlorocyclotriphosphazenes with aryl Grignard reagents and with bifunctional amines, aminoalcohols, and alkoxides were investigated. The characterization data for the compounds formed in the reactions of monomethylpentachlorocyclotriphosphazene and the Grignard reagents were found to be informative with respect to the extent and nature of the interaction between the phosphazene ring and its exocyclic substituents. This interaction was found to be responsible for significant effects on the reactions of the phosphazene ring with nucleophiles. The reactions o

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48

Morgan, J. J. G. "The reactions of endoperoxides with nucleophiles and bases." Thesis, Cardiff University, 1993. http://ethos.bl.uk/OrderDetails.do?uin=uk.bl.ethos.388230.

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49

Sarkar, Md Ruhul Amin. "Palladium catalysed reactions of allene with heterocyclic nucleophiles." Thesis, University of Leeds, 2006. http://ethos.bl.uk/OrderDetails.do?uin=uk.bl.ethos.427786.

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50

Firdous, Samia. "Synthesis and Reactions of α-Azido Alcohols". Doctoral thesis, Universitätsbibliothek Chemnitz, 2012. http://nbn-resolving.de/urn:nbn:de:bsz:ch1-qucosa-86012.

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Die vorliegende Arbeit beschäftigt sich mit der Untersuchung von a-Azidoalkoholen, welche über die Reaktion von aliphatischen sowie aromatischen Aldehyden mit HN3 leicht zugänglich sind und die im Gleichgewicht mit den jeweiligen Ausgangsstoffen vorliegen. Bei Raumtemperatur stellt sich dieses Gleichgewicht sehr schnell ein und man erhält spezifische Konzentrationen an Eduktaldehyd, Stickstoffwasserstoffsäure und a-Azidoalkohol. Die Reaktion von Aldehyden mit HN3 generiert dabei ein neues Chriralitätszentrum, wodurch die Umsetzung chiraler Aldehyde, wie z. B. von Zuckerderivaten, zwei anomere

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