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Relevant bibliographies by topics / Pausdom

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Academic literature on the topic 'Pausdom'

Author: Grafiati

Published: 4 June 2021

Last updated: 1 August 2024

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Journal articles on the topic "Pausdom"

1

Müller, Daniela. "‘s Werelds oudste institutie. Het pausdom - Frans Willem Lantink en Jeroen Koch ed., De paus en de wereld. Geschiedenis van een instituut (Boom; Amsterdam 2012) 400 p., ill., €29,90 ISBN 9789461053572." Tijdschrift voor Geschiedenis 126, no. 3 (September 1, 2013): 404–5. http://dx.doi.org/10.5117/tvgesch2013.3.b3.

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Haboud Bumachar, Marleen. "Andeetako ahots eta arbasoen jakintzetara itzul gaitezen, elkarrizketaren metodologia erabiliz: aurrerapausoak eta erronkak." BAT SOZIOLINGUISTIKA ALDIZKARIA 129, no. 10.55714 (February 7, 2024): 31–55. http://dx.doi.org/10.55714/bat-129.2.

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Artikulu honek Andeetako Ahotsak eta Arbasoen Jakintzak proiektuaren filosofia eta metodologia deskribatzen ditu, kitxuaz ez hitz egin arren, beraien burua kitxuatzat duten Ekuadorko landa eremuko zenbait komunitaterekin lotuta. Proiektu hori Pintag parrokiako (Pichincha probintzia) hiru komunitatetan egin da, Quito hiriburutik 35 km-ra. Proiektuak inguruko landare sendagarriak berriz aurkitzeko prozesua eta herritarren sendatze praktikak erakusten ditu, pausoz pauso, eta garrantzi berezia ematen dio ikerketa elkarrizketan oinarritzeari eta haren diziplinartekotasunari. Ikerlan honen ikuspegi metodologikoa ulertzeko, aurrez egindako zenbait ikerketa lan azaldu dira, lehenbizi. Ondoren, dokumentazio eta biziberritze prozesua zehaztu da, eta azpimarra egin da bidean izan diren erronka batzuetan izandako arrakastan eta beste lorpen batzuetan; izan ere, ekimen komunitarioetan epe luzerako lorpenak izan daitezkeela aurreikusten da. • Hitz gakoak: Ekuador, hizkuntza eta kultura biziberritzea, oinarrizko komunitateekin ikerketa, elkarrizketaren metodologia, diziplinartekotasuna, dokumentazio aktiboa, biziberritzea.

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Chen, Sijia, Chongguo Jiang, Nan Zheng, Zhen Yang, and Lili Shi. "Evolution of Pauson-Khand Reaction: Strategic Applications in Total Syntheses of Architecturally Complex Natural Products (2016–2020)." Catalysts 10, no. 10 (October 16, 2020): 1199. http://dx.doi.org/10.3390/catal10101199.

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Metal-mediated cyclizations are important transformations in a natural product total synthesis. The Pauson-Khand reaction, particularly powerful for establishing cyclopentenone-containing structures, is distinguished as one of the most attractive annulation processes routinely employed in synthesis campaigns. This review covers Co, Rh, and Pd catalyzed Pauson-Khand reaction and summarizes its strategic applications in total syntheses of structurally complex natural products in the last five years. Additionally, the hetero-Pauson-Khand reaction in the synthesis of heterocycles will also be discussed. Focusing on the panorama of organic synthesis, this review highlights the strategically developed Pauson-Khand reaction in fulfilling total synthetic tasks and its synthetic attractiveness is aimed to be illustrated.

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Hätzelt, André, and Sabine Laschat. "One-pot sequential PausonKhand reaction transfer hydrogenation." Canadian Journal of Chemistry 80, no. 10 (October 1, 2002): 1327–30. http://dx.doi.org/10.1139/v02-172.

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The PausonKhand reaction of norbornene (1) and phenylacetylene (2) and subsequent RuCl2(PPh3)3-catalyzed transfer hydrogenation of the resulting enone (3) can be carried out in a one-pot sequence if the base is added after an induction period. The desired ketones (4a, 4b) were obtained in good yield as a mixture of diastereomers (diastereomeric ratio (dr.) 58:42). The relative rates of both the Pauson-Khand reaction and the transfer hydrogenation are decreased by a factor of 2 in the sequence, as compared with the isolated reactions.Key words: PausonKhand reaction, transfer hydrogenation.

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Escorihuela, Jorge, Daniel M. Sedgwick, Alberto Llobat, Mercedes Medio-Simón, Pablo Barrio, and Santos Fustero. "Pauson–Khand reaction of fluorinated compounds." Beilstein Journal of Organic Chemistry 16 (July 14, 2020): 1662–82. http://dx.doi.org/10.3762/bjoc.16.138.

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The Pauson–Khand reaction (PKR) is one of the key methods for the construction of cyclopentenone derivatives, which can in turn undergo diverse chemical transformations to yield more complex biologically active molecules. Despite the increasing availability of fluorinated building blocks and methodologies to incorporate fluorine in compounds with biological interest, there have been few significant advances focused on the fluoro-Pauson–Khand reaction, both in the inter- and intramolecular versions. Furthermore, the use of vinyl fluorides as olefinic counterparts had been completely overlooked. In this review, we collect the advances both on the stoichiometric and catalytic intermolecular and intramolecular fluoro-Pauson–Khand reaction, with special attention to the PKR of enynes containing a fluoride moiety.

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García-Lacuna, Jorge, Maialen Alonso, Gema Domínguez, and Javier Pérez Castells. "Study of the Pauson–Khand reaction in flow over alkynylphenyl vinyl ethers: towards the synthesis of tricyclic multisubstituted benzofurans." RSC Advances 12, no. 12 (2022): 7313–17. http://dx.doi.org/10.1039/d2ra01062c.

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García-Lacuna, Jorge, Gema Domínguez, Jaime Blanco-Urgoiti, and Javier Pérez-Castells. "Synthesis of treprostinil: key Claisen rearrangement and catalytic Pauson–Khand reactions in continuous flow." Organic & Biomolecular Chemistry 17, no. 43 (2019): 9489–501. http://dx.doi.org/10.1039/c9ob02124h.

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Manton, Jennifer C., Florian J. R. Cerpentier, Emma C. Harvey, Ian P. Clark, Gregory M. Greetham, Conor Long, and Mary T. Pryce. "Photochemical or electrochemical bond breaking – exploring the chemistry of (μ2-alkyne)Co2(CO)6 complexes using time-resolved infrared spectroscopy, spectro-electrochemical and density functional methods." Dalton Transactions 48, no. 39 (2019): 14642–52. http://dx.doi.org/10.1039/c9dt03006a.

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Zhao, Mi-Na, Ying Zhang, Ning Ge, Le Yu, Shun Wang, Zhi-Hui Ren, and Zheng-Hui Guan. "A Rh(iii)-catalyzed regioselective intermolecular oxa-Pauson–Khand reaction of alkynes, arylboronic acids and CO to form butenolides." Organic Chemistry Frontiers 7, no. 5 (2020): 763–67. http://dx.doi.org/10.1039/c9qo01486a.

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Chirkin, Egor, Chouaha Bouzidi, and François-Hugues Porée. "Tungsten-Promoted Hetero-Pauson–Khand Cycloaddition: Application to the Total Synthesis of (–)-Allosecurinine." Synthesis 51, no. 09 (February 18, 2019): 2001–6. http://dx.doi.org/10.1055/s-0037-1612063.

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Herein, we report a concise enantioselective synthesis of (–)-allosecurinine, a tetracyclic Securinega alkaloid featuring an α,β-unsaturated γ-lactone moiety. Starting from inexpensive and readily available trans-l-hydroxyproline, our strategy entails a rare late-stage [2+2+1]-hetero-Pauson–Khand cycloaddition between a ketone and an alkyne as the key complexity-generating step to rapidly install the CD-ring system. The reported W(CO)6-promoted intramolecular cyclization provides the first example of a tungsten-mediated hetero-Pauson–Khand reaction. This approach to the strained bicyclic CD motif present in allosecurinine provides some insights into the boundaries of this potentially powerful methodology that might be further extended to other butenolide-containing natural products.

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Dissertations / Theses on the topic "Pausdom"

1

Ishaq, Salma. "New substrates for Pauson-Khand reaction." Thesis, University College London (University of London), 2006. http://ethos.bl.uk/OrderDetails.do?uin=uk.bl.ethos.428148.

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Kaufmann, Karina Anne Celia. "A study of the Pauson-Khand reaction." Thesis, Imperial College London, 2007. http://ethos.bl.uk/OrderDetails.do?uin=uk.bl.ethos.486323.

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The introduction to this thesis commences with a description of the mechanism of the Pauson-Khand reaction (PKR) as postulated by Magnus. Three examples of biologically active compounds synthesised using the stoichiometric PKR are presented, and the cobalt catalysed PKR is surveyed together with the asymmetric cobalt catalysed PKR. The first half of Chapter 2 describes research into the reaction pathway of a cobalt catalysed asymmetric PKR. Three enynes 68, 81 and 82 were synthesised together with the novel alkyne 80. Compounds 68, 80, 81 and 82 were used to synthesise the novel (BINAP)(enyne)C02(CO)4 complexes 89-92. X-Ray crystal structures were obtained for novel complexes 89 and 90. Variable temperature 31p NMR experiments were first carried out on complexes 89, 91 and 92 under nitrogen and all four complexes (89-92) were examined in the same way under an atmosphere of carbon monoxide. The variable temperature 31p NMR experiments under carbon monoxide with novel complexes 89, 91 and 92 resulted in the observation of a new resonance at 0 54 ppm. Observation of the resonance at 0 54 was found to be dependant on the presence ofan alkene moiety within the complexes. A (J bonded cobalt-alkyne complex (93) was identified by X-ray crystallography, which stimulated the synthesis of two enynes 94 and 95, containing internal alkyne moieties. Novel (BINAP)(enyne)C02(CO)4 complexes 98 and 99 were synthesised from enynes 94 and 95 and subjected to variable temperature 31p NMR experiments under carbon monoxide whereupon the new resonance at 054 was observed. The novel (BINAP)Co(CO)(CI) complex 100 was isolated and examined by X-ray crystallography, and the resonance at 0 54 was characterised by NMR spectroscopy and X-ray crystallography as the novel HCo(COh(BINAP) complex 101. The enynes (89, 91 and 92), water and the Pauson-Khand adduct 69 were investigated as a hydrogen source for the formation of complex 101 but the search was inconclusive. 31p NMR spectroscopy of the catalytic PKR revealed the presence of 101 in the PKR together with (BINAP)C02(CO)6 75. The second half of Chapter 2 describes the application of the catalytic PKR in the synthesis of drug candidates. Three reversible covalent inhibitors of cathepsin Sand K enzymes were designed. The development of a new intermolecular PKR utilising alkene reactants tert-butyl-2,5-dihydropyrrole carboxylate 124 and tert-butyl-2,3-dihydropyrrole carboxylate 125 was a~empte~.. An intramole~u~ar PKR was used to synthesise five potential inhibitor sequences, U8a-e, which exhibited poor selectlvity and low inhibition of the cathepsin Sand K enzymes.

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Lindsay, David Montgomery. "Development of the asymmetric Pauson Khand reaction." Thesis, University of Strathclyde, 2000. http://ethos.bl.uk/OrderDetails.do?uin=uk.bl.ethos.248568.

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Sezer, Serdar. "Remote Control Of The Diastereoselectivity In The Pauson." Phd thesis, METU, 2011. http://etd.lib.metu.edu.tr/upload/12613908/index.pdf.

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In this thesis, an intramolecular Pauson-Khand reaction of chiral enynes derived from homoallyl, allyl and homopropargyl alcohols is described. For this purpose, 2-heteroaryl substituted homoallyl, allyl and homopropargyl alcohols are easily and efficiently resolved through enzymatic resolution in a high ee (91-99%) with a known stereochemistry. Each enantiomerically enriched enyne derived from homoallyl and homopropargyl alcohols affords the conformationally most stable diastereomeric cyclopenta[c]pyran ring system as a sole product, whereas enantiomerically enriched enynes derived from allyl alcohols give the diastereomeric cis:trans mixture of cyclopenta[c]furan ring system. In addition these, an intramolecular Pauson&ndash
Khand reaction of camphor tethered enynes derived from homoallyl, homomethallyl, and homopropargyl alcohols is also described. Accordingly, homoallyl, homomethallyl, and homopropargyl moieties are easily constructed on the camphor carbonyl group with excellent diastereoselectivity due to endo-face selectivity, and with known stereochemistry. Each enantiomerically pure enyne affords the conformationally most stable diastereomeric spirocyclic cyclopenta[c]pyran ring system.

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Robert, Frédéric. "Utilisation de diphosphinoamines dans la réaction Pauson-Khand." Université Joseph Fourier (Grenoble), 1999. http://www.theses.fr/1999GRE10241.

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La reaction de pauson-khand est une des methodes les plus efficaces pour la formation de cyclopentenones. La reaction etant catalysee par des complexes de dicobalt, nous avons entrepris une etude sur la substitution de deux monoxydes de carbone du complexe par des diphosphinoamines pontant les deux atomes de cobalt. Tout d'abord, l'utilisation de substituants electroattracteurs sur les phosphores a augmente le pouvoir accepteur des phosphines. Cela a favorise le depart de monoxyde de carbone, stabilise les complexes et augmente les rendements de la reaction de pauson-khand. D'autre part, l'introduction de chiralite sur le ligand, sur l'amine puis sur les substituants du phosphore, a ouvert la voie pour une nouvelle approche asymetrique de la reaction. Sous pression de monoxyde de carbone, les diphosphinoamines ont permis l'utilisation d'une quantite catalytique de complexe en reaction intermoleculaire. Des problemes concernant le mecanisme et la regioselectivite observee et les moyens mis en uvre pour tenter d'y repondre ont aussi ete abordes.

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Verdaguer, i. Espaulella Xavier. "Reaccions de Pauson-Khand amb alcoxialquins derivats d'alcohols quirals." Doctoral thesis, Universitat de Barcelona, 1994. http://hdl.handle.net/10803/667766.

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Se han estudiado las reacciones intramoleculares de Pauson-Khand de los eteres 3-alcoxialil propargílicos y 3-alcoxipropargil alílicos derivados del 2-neopentiloxi-3-bornanol y del 3-neopentiloxi-iso-borneol. Las diastereoselectividades observadas en las reacciones de estos sistemas llegó hasta 14/1 (aproximación del inductor unido al alquino). Se ha abordado, también, el estudio de la inducción asimétrica en las reacciones intermoleculares de Pauson-Khand y en este contexto se diseñó y preparó un nuevo tipo de auxiliar quiral quelante. Las reacciones del complejo de dicobaltohexacarbonilo del 10-metiltio-iso-borniloxietino con olefinas tensionadas transcurre con elevada selectividad. En el caso del norbornadieno se llegó al 91% D.E.. En ambas aproximaciones, la intra y la intermolecular, se recuperaron los auxiliares quirales con excelentes rendimientos, y se determinaron las configuraciones absolutas de los respectivos aductos de Pauson-Khand.

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Blunt, Gillian. "Developing novel synthetic methods for the Pauson Khand reaction." Thesis, University of Glasgow, 2002. http://ethos.bl.uk/OrderDetails.do?uin=uk.bl.ethos.248289.

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Fjermestad, Torstein. "Computacional studies on the mechanism of the pauson-khand reaction." Doctoral thesis, Universitat Rovira i Virgili, 2010. http://hdl.handle.net/10803/9112.

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La aplicación de los métodos de la química computacional ha llevado a una mejor comprensión del mecanismo de la reacción de Pauson-Khand para la síntesis de ciclopentenonas, en especial en su variante enantioselectiva.
Se han analizado tres métodos distintos para introducir enantioselectividad en esta reacción, que en su modelo original no es selectiva. Se han estudiado tres casos: a) la activación del catalizador convencional dicobalto octacarbonilo mediante un N-óxido quiral, b) la modificación de este mismo catalizador mediante la sustitución de dos ligandos carbonilo por una difosfina quiral, y c) la sustitución del catalizador dinuclear de cobalto por un catalizador mononuclear de rodio con ligandos quirales.
El estudio teórico ha llevado a la caracterización de aspectos mecanísticos que son inaccesibles al estudio puramente experimental, y contribuye así al desarrollo de métodos catalíticos más eficientes para esta importante reacción.
The application of computational methods has lead to a better understanding of the mechanism of the Pauson-Khand reaction (PKR) for the synthesis of cyclopentenone compounds. In particular the enantioselective PKR has been considered.

Different methods for inducing enantioselectivity in this originally unselective reaction have been analyzed. Three cases have been considered: a) Activation of the conventional dicobalt octacarbonyl catalyst by a chiral N-oxide, b) A modification of the dicobalt catalyst by means of a substitution of two carbonyl ligands by a chiral diphosphine ligand. and c) the substitution of the dinuclear cobalt catalyst by a mononuclear rhodium catalyst with chiral ligands.

The theoretical study has lead to the characterization of mechanistic aspects that would be inaccessible from a purely experimental study. The study therefore contributes to the development of more efficient catalytic methods for this important reaction.

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Miller, Ian. "The application of temporary tethers to the Pauson-Khand reaction." Thesis, University of Exeter, 2005. http://ethos.bl.uk/OrderDetails.do?uin=uk.bl.ethos.421557.

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Lewis, Sara Estelle. "Probing the role of phosphines in the Pauson-Khand reaction." Thesis, King's College London (University of London), 2003. http://ethos.bl.uk/OrderDetails.do?uin=uk.bl.ethos.407447.

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Books on the topic "Pausdom"

1

Bäumer, Remigius. Martin Luther und der Papst. 4th ed. Münster: Aschendorff, 1985.

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Walter, Ullmann. A short history of the Papacy in the Middle Ages. London: Routledge, 2002.

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Duffy, Eamon. Saints & sinners: A history of the Popes. [New Haven, Conn.]: Yale University Press, in association with S4C, 1997.

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Duffy, Eamon. Saints & sinners: A history of the Popes. 2nd ed. New Haven: Yale University Press, 2002.

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Holmes, George. Florence, Rome, and the origins of the Renaissance. Oxford: Clarendon Press, 1986.

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Housley, Norman. The Avignon papacy and the Crusades, 1305-1378. Oxford [Oxfordshire]: Clarendon Press, 1986.

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Graham, Robert A. Vatican diplomacy: A study of church and state on the international plane. Princeton, N.J: Princeton University Press, 1985.

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Saizarbitoria, Ramón. Hamaika pauso. Donostia [Spain]: Erein, 1995.

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1943-, Ryan Christopher, and Pontifical Institute of Mediaeval Studies., eds. The Religious role of the papacy: Ideals and realities, 1150-1300. Toronto, Ont: Pontifical Institute of Mediaeval Studies, 1989.

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Charles, Villa-Vicencio, ed. Between Christ and Caesar: Classic and contemporary texts on church and state. Grand Rapids, Mich: W.B. Eerdmans Pub. Co., 1986.

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Book chapters on the topic "Pausdom"

1

Laue, Thomas, and Andreas Plagens. "Pauson-Khand-Reaktion." In Teubner Studienbücher Chemie, 248–50. Wiesbaden: Vieweg+Teubner Verlag, 1994. http://dx.doi.org/10.1007/978-3-322-94015-5_80.

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Laue, Thomas, and Andreas Plagens. "Pauson-Khand-Reaktion." In Teubner Studienbücher Chemie, 249–52. Wiesbaden: Vieweg+Teubner Verlag, 1998. http://dx.doi.org/10.1007/978-3-322-94077-3_81.

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Laue, Thomas, and Andreas Plagens. "Pauson-Khand-Reaktion." In Teubner Studienbücher Chemie, 248–50. Wiesbaden: Vieweg+Teubner Verlag, 1994. http://dx.doi.org/10.1007/978-3-322-94726-0_80.

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Li, Jie Jack. "Pauson–Khand reaction." In Name Reactions, 462–63. Cham: Springer International Publishing, 2014. http://dx.doi.org/10.1007/978-3-319-03979-4_206.

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Li, Jie Jack. "Pauson–Khand reaction." In Name Reactions, 419–20. Berlin, Heidelberg: Springer Berlin Heidelberg, 2009. http://dx.doi.org/10.1007/978-3-642-01053-8_193.

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Li, Jie Jack. "Pauson-Khand Reaction." In Name Reactions, 430–32. Cham: Springer International Publishing, 2021. http://dx.doi.org/10.1007/978-3-030-50865-4_117.

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Kerr, William J. "The Pauson-Khand Reaction - an Introduction." In The Pauson-Khand Reaction, 1–21. Chichester, UK: John Wiley & Sons, Ltd, 2012. http://dx.doi.org/10.1002/9781119941934.ch1.

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Rios Torres, Ramon, and Jan Vesely. "Other Transition Metal-Mediated Cyclizations Leading to Cyclopentenones." In The Pauson-Khand Reaction, 275–305. Chichester, UK: John Wiley & Sons, Ltd, 2012. http://dx.doi.org/10.1002/9781119941934.ch10.

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Cambeiro, Xacobe C., and Miquel A. Pericàs. "The Mechanism of the Pauson-Khand Reaction: Hypothesis, Experimental Facts, and Theoretical Investigations." In The Pauson-Khand Reaction, 23–48. Chichester, UK: John Wiley & Sons, Ltd, 2012. http://dx.doi.org/10.1002/9781119941934.ch2.

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Shibata, Takanori. "Non Chiral Pauson-Khand Reaction." In The Pauson-Khand Reaction, 49–68. Chichester, UK: John Wiley & Sons, Ltd, 2012. http://dx.doi.org/10.1002/9781119941934.ch3.

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Conference papers on the topic "Pausdom"

1

Ruiz Suaña, José Antonio, and Antonio García Blay. "Acceso en el castillo de Portell. *** Entrance in the Castle of Portell." In 8º Congreso Internacional de Arquitectura Blanca - CIAB 8. Valencia: Universitat Politècnica València, 2018. http://dx.doi.org/10.4995/ciab8.2018.7432.

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La plaza de l’Esglèsia forma parte del antiguo castillo de Portell. En esta plaza, una antigua escalera, en mal estado y con excesiva pendiente, conectaba el desnivel entre la población y la parte superior del recinto amurallado. Se sustituye la escalera existente construyendo un nuevo acceso más cómodo, ocupando un pequeño solar municipal recayente a la plaza. El nuevo acceso asciende entendiéndose como depositado sobre el terreno natural, facilita un recorrido más pausado y cómodo que invita a parar y sentarse, al encuentro y la conversación. Los nuevos muros construyen un pequeño recinto y, por otra parte, se relacionan con lo existente. Un muro de hormigón configura los límites de la plaza. sin mostrar directamente el nuevo acceso, sino más bien, se sugiere detrás de él e invitan a entrar y recorrerlo.***The church square is part of the old castle of Portell. In this square, an old staircase, in poor condition and with excessive slope, connected the gap between the town and the upper part of the walled enclosure. The existing staircase is replaced by building a new more convenient access, occupying a small municipal plot located next to the square. The new access comes up as if it were deposited on the natural ground, thus facilitates a more leisurely and comfortable promenade that invites to stop and sit down, join and converse. A small enclosure is built with the new walls and, on the other hand, they co-exist with what already existed. A concrete wall configures the boundaries of the square not directly showing the new entrance.

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Reports on the topic "Pausdom"

1

Enchev, Dobromir D., and Irina R. Yotova. 1,2-Alkadienephosphonates in Pauson–Khand Reaction. "Prof. Marin Drinov" Publishing House of Bulgarian Academy of Sciences, April 2020. http://dx.doi.org/10.7546/crabs.2020.04.06.

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