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Journal articles on the topic 'Polybutadienes'

Author: Grafiati

Published: 4 June 2021

Last updated: 12 April 2025

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1

Roovers, Jacques, and Paul M. Toporowski. "Characteristic Ratio and Plateau Modulus of 1,2-Polybutadiene. A Comparison with Other Rubbers." Rubber Chemistry and Technology 63, no. 5 (1990): 734–46. http://dx.doi.org/10.5254/1.3538286.

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Abstract In the course of work on linear and ring polybutadienes with 62% 1,2 units, a number of discrepancies were noted with data on polybutadienes of various microstructure available in the literature. For example, GNο=870 kPa for our 62% 1,2-polybutadiene. This is larger than GNο=730 kPa for a 56% 1,2-polybutadiene and GNο=550 kPa for a 78% 1,2-polybutadiene sample. The cis : trans ratio of our 62% 1,2-polybutadiene, prepared with potassium counterion, is 1 : 4, On the other hand, the cis : trans ratio of 62% 1,2-polybutadiene prepared with a modified Li catalyst is estimated to be 1 : 2.

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2

Krishnamoorti, Ramanan. "Thermodynamic Interactions in Blends of Polydienes." Rubber Chemistry and Technology 72, no. 4 (1999): 580–86. http://dx.doi.org/10.5254/1.3538820.

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Abstract Thermodynamic interactions and phase behavior in binary blends of model mixed microstructure polybutadienes with model 1,4-polyisoprene were studied using small angle neutron scattering and differential scanning calorimetry (DSC). The microstructure of the polybutadiene ranged from 8% 1,2 (92% 1,4) to 90% 1,2 (10% 1,4) units, while the polyisoprene contained 93% 1,4 and 7% 3,4 units. The blends of protonated polybutadienes (HPB) with deuterated 1,4 polyisoprene (DPI) exhibited lower critical solution temperature (LCST) behavior when the polybutadiene contained 38 mol % or more of 1,2

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3

Abbasov, V. M., F. A. Nasirov, E. J. Agazade, et al. "Anti-corrosion properties of aminated epoxy liquid polybutadiene in the composition of conservation liquids." Practice of Anticorrosive Protection 28, no. 1 (2023): 12–24. https://doi.org/10.31615/j.corros.prot.2023.107.1-2.

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Epoxidized polybutadienes were synthesized by epoxidation of liquid polybutadiene (LPBD) molecular weights of 1500 and 3000 with performic acid formed in situ by the reaction of formic acid and hydrogen peroxide. The amination reaction of epoxidized polybutadienes w as used to obtain their amine derivatives. In the amination reaction of epoxidized liquid polybutadiene (ELPBD), ZnCl2 was used as a catalyst, organoaluminum compounds and solvents produced by Sigma-Aldrich and Merck, and waste turbine oil T-30. The structure of LPBD, ELPBD and its amino derivative (AELPBD) was determined on a Bruk

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4

Khayala Abbasova, Fuzuli Nasirov, Khayala Abbasova, Fuzuli Nasirov, and Sevda Rafiyeva, Vusale Bakhshiyeva Sevda Rafiyeva, Vusale Bakhshiyeva. "SYNTHESIS OF AMINATED EPOXY DERIVATIVES OF POLYBUTADIENE AND THE STUDY OF THEIR ANTI-CORROSION PROPERTIES IN THE COMPOSITION OF CONSERVATION LIQUIDS." PAHTEI-Procedings of Azerbaijan High Technical Educational Institutions 34, no. 11 (2023): 191–97. http://dx.doi.org/10.36962/pahtei34112023-191.

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The synthesis of amino derivatives of epoxidized polybutadienes was carried out by the amination reaction. The composition and structure of the amino derivatives were confirmed by NMR and IR spectroscopy. It has been established that the synthesized amine derivatives have a synergistic effect, accelerate the solubility in mineral oils and significantly improve the anticorrosion properties of conservation fluids. Samples of aminated epoxidized polybutadienes were tested for corrosion resistance in a hydro chamber, in sea water and in a sulfuric acid environment. Their high efficiency against co

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5

Díaz de León, Ramón, Florentino Soriano Corral, Francisco Javier Enríquez-Medrano, et al. "Synthesis of High cis-Polybutadiene in Styrene Solution with Neodymium-Based Catalysts: Towards the Preparation of HIPS and ABS via In Situ Bulk Polymerization." International Journal of Polymer Science 2016 (2016): 1–11. http://dx.doi.org/10.1155/2016/9841896.

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In a first step, 1,3-butadiene was selectively polymerized at 60°C in styrene as solvent using NdV3/DIBAH/EASC as the catalyst system. The catalyst system activation process, the addition order of monomers and catalyst components, and the molar ratios [Al]/[Nd] and [Cl]/[Nd] were studied. The catalyst system allowed the selective 1,3-butadiene polymerization, reaching conversions between 57.5 and 88.1% with low polystyrene contents in the order of 6.3 to 15.4%. Molecular weights ranging from 39,000 to 150,000 g/mol were obtained, while cis-1,4 content was found in the interval of 94.4 to 96.4%

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6

Pleska, Alexander, Iva Klichová, and Jindřich Pytela. "Grafting of Hydroxy-Terminated Polybutadiene with 2-Mercaptoethanol." Collection of Czechoslovak Chemical Communications 67, no. 12 (2002): 1899–910. http://dx.doi.org/10.1135/cccc20021899.

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A method for functionalization of hydroxy-terminated polybutadiene with 2-sulfanylethan-1-ol (2-mercaptoethanol) leading to a controlled increase in the OH functionality of the polymer was developed. The polybutadiene used contained about 65% of unsaturation in the form of 1,2-vinyl groups. The reaction was carried out without using volatile solvents. The radical addition of 2-sulfanylethan-1-ol on the polymer proceeded quantitatively and the products were free of the mercaptan odour. A series of functionalized polybutadienes were synthesized and characterized by their physical and chemical pr

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7

Ceauşescu, E., R. Bordeianu, E. Buzdugan, I. Cerchez, P. Ghioca, and R. Stancu. "Polybutadiene Modification: Reactions of Halogen-Containing Polybutadienes with Organolithium Compounds." Journal of Macromolecular Science: Part A - Chemistry 22, no. 5-7 (1985): 803–18. http://dx.doi.org/10.1080/00222338508056637.

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8

Dechent, Sarah-Elisabeth, Arjan W. Kleij, and Gerrit A. Luinstra. "Fully bio-derived CO2 polymers for non-isocyanate based polyurethane synthesis." Green Chemistry 22, no. 3 (2020): 969–78. http://dx.doi.org/10.1039/c9gc03488a.

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9

Zhou, L.-L., N. Hadjichristidis, P. M. Toporowski, and J. Roovers. "Synthesis and Properties of Regular Star Polybutadienes with 32 Arms." Rubber Chemistry and Technology 65, no. 2 (1992): 303–14. http://dx.doi.org/10.5254/1.3538613.

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Abstract A dendrimer carbosilane containing 32 Si—Cl bonds in the perimeter has been prepared and has been used as a coupling agent to prepare 32-arm star polybutadienes. The dilute-solution properties 〈RG2〉, A2, [η], and D0 have been measured in one good solvent and in one ¸ -solvent. The dimensions of the 32-arm star polymers are compared with those of linear polymers at constant molecular weight. It is shown that the 32-arm star polybutadiene has the characteristic properties of a hard-sphere molecule in dilute solution. The equivalent hard-sphere radii calculated from A2, D0 and [η] are id

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10

Ying, Weilun, Weijing Pan, Qiao Gan, Xiaoyu Jia, Alfonso Grassi, and Dirong Gong. "Correction: Preparation and property investigation of chain end functionalized cis-1,4 polybutadienes via de-polymerization and cross metathesis of cis-1,4 polybutadienes." Polymer Chemistry 10, no. 32 (2019): 4495. http://dx.doi.org/10.1039/c9py90121c.

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Correction for ‘Preparation and property investigation of chain end functionalized cis-1,4 polybutadienes via de-polymerization and cross metathesis of cis-1,4 polybutadienes’ by Weilun Ying et al., Polym. Chem., 2019, 10, 3525–3534.

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11

Hempenius, Mark A., Walter Michelberger, and Martin Möller. "Arborescent Graft Polybutadienes." Macromolecules 30, no. 19 (1997): 5602–5. http://dx.doi.org/10.1021/ma970280b.

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12

Doi, Yoshiharu, Akihiro Yano, Kazuo Soga, and David R. Burfield. "Hydrogenation of polybutadienes. Microstructure and thermal properties of hydrogenated polybutadienes." Macromolecules 19, no. 9 (1986): 2409–12. http://dx.doi.org/10.1021/ma00163a013.

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13

Wang, Beibei, Heng Liu, Tao Tang та Xuequan Zhang. "cis-1,4 Selective Coordination Polymerization of 1,3-Butadiene and Copolymerization with Polar 2-(4-Methoxyphenyl)-1,3-butadiene by Acenaphthene-Based α-Diimine Cobalt Complexes Featuring Intra-Ligand π-π Stacking Interactions". Polymers 13, № 19 (2021): 3329. http://dx.doi.org/10.3390/polym13193329.

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Highly cis-1,4 selective (up to 98%) coordination–insertion polymerization of 1,3-butadiene (BD) has been achieved herein using acenaphthene-based α-diimine cobalt complexes. Due to the presence of intra-ligand π-π stacking interactions, the complexes revealed high thermostability, affording polybutadiene products in high yields. Moreover, all of the obtained polymers possessed a relatively narrow molecular weight distribution as well as high molecular weight (up to 92.2 × 104 Dalton). The molecular weights of the resultant polybutadienes could be finely tuned by varying polymerization paramet

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14

Nir, Moira Marx, and Robert E. Cohen. "Mechanical Properties of Blends of Crystallizable Polybutadienes Containing Amorphous Polybutadiene Diblock Copolymers." Rubber Chemistry and Technology 67, no. 2 (1994): 342–47. http://dx.doi.org/10.5254/1.3538679.

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Abstract Tensile failure properties of syndiotactic 1,2 polybutadiene/trans 1,4 polybutadiene crystalline blends are improved by addition of 5–10% amorphous 1,2 polybutadiene/1,4 polybutadiene diblock copolymer. The effect of block molecular weight and microphase behavior of the diblock copolymer was investigated. Heterogeneous diblocks enhance blend properties to a greater extent than homogeneous diblocks. In blends with enhanced properties, percent coverage of interfacial surface area by diblock is on the order of 10%.

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15

Poshyachinda, S., H. G. M. Edwards, and A. F. Johnson. "Dynamic mechanical thermal analysis of homopolymeric and diblock polybutadienes and polybutadiene blends." Polymer 37, no. 23 (1996): 5171–77. http://dx.doi.org/10.1016/0032-3861(96)00342-4.

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16

TADAKI, Toshihiro. "Recent Advances in Polybutadienes." NIPPON GOMU KYOKAISHI 76, no. 12 (2003): 441–45. http://dx.doi.org/10.2324/gomu.76.441.

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17

Tadaki, T. "Recent Advances in Polybutadienes." International Polymer Science and Technology 31, no. 8 (2004): 5–10. http://dx.doi.org/10.1177/0307174x0403100802.

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18

Urbano, Juan, Brigitte Korthals, M. Mar Díaz-Requejo, Pedro J. Pérez, and Stefan Mecking. "Catalytic cyclopropanation of polybutadienes." Journal of Polymer Science Part A: Polymer Chemistry 48, no. 20 (2010): 4439–44. http://dx.doi.org/10.1002/pola.24231.

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19

Robles-Vásquez, O., A. González-Álvarez, J. E. Puig, and O. Manero. "A Composition Rule to Predict the Linear Viscoelastic Properties of Polybutadienes with Varying Microstructure." Rubber Chemistry and Technology 79, no. 5 (2006): 859–69. http://dx.doi.org/10.5254/1.3547970.

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Abstract A composition rule is proposed here to predict the glass transition temperature (Tg), the zero shear-rate dynamic viscosity (η0′), the plateau modulus (G0) and the terminal relaxation time (λ) of narrow molecular weight distribution (MWD) polybutadienes with various vinyl contents in solution and in the melt from the knowledge of the vinyl fraction, polymer fraction in solution and average molecular weight. The predictions of the composition rule are compared with data of a variety of narrow MWD polybutadienes with varying microstructure.

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20

Roovers, Jacques. "Tube renewal in the relaxation of 4-arm-star polybutadienes in linear polybutadienes." Macromolecules 20, no. 1 (1987): 148–52. http://dx.doi.org/10.1021/ma00167a025.

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21

Livanova, Nadezhda, and Svetlana Karpova. "The Structure of Polybutadienes and Butadiene-Acrylonitrile Copolymers." Chemistry & Chemical Technology 5, no. 4 (2011): 423–28. http://dx.doi.org/10.23939/chcht05.04.423.

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22

Amato, R., and G. Marot. "Functional Characterization of Hydroxy-Polybutadienes." Journal of Liquid Chromatography 14, no. 1 (1991): 79–95. http://dx.doi.org/10.1080/01483919108049599.

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23

Alessi, Paolo, Angelo Cortesi, Pablo Sacomani, and E. Valles. "Solvent-polymer interactions in polybutadienes." Macromolecules 26, no. 23 (1993): 6175–79. http://dx.doi.org/10.1021/ma00075a006.

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24

Grebowicz, Janusz, Wonji Aycock, and Bernhard Wunderlich. "Heat capacities of 1,4-polybutadienes." Polymer 27, no. 4 (1986): 575–82. http://dx.doi.org/10.1016/0032-3861(86)90243-0.

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25

Cassano, Guillermo A., Enrique M. Vallés, and Lidia M. Quinzani. "Structure of partially hydrogenated polybutadienes." Polymer 39, no. 22 (1998): 5573–77. http://dx.doi.org/10.1016/s0032-3861(97)10080-5.

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26

Sabnis, Sanket, Vijesh A. Tanna, Chao Li, et al. "Exfoliation of two-dimensional zeolites in liquid polybutadienes." Chemical Communications 53, no. 52 (2017): 7011–14. http://dx.doi.org/10.1039/c7cc03256k.

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27

Kössler, I., J. Vodehnal, M. Štolka, J. Kálal, and E. Hartlová. "Cyclo- and cyclized diene polymers. VIII. Cyclization of polybutadienes and ir spectra of cyclized polybutadiene." Journal of Polymer Science Part C: Polymer Symposia 16, no. 3 (2007): 1311–25. http://dx.doi.org/10.1002/polc.5070160309.

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28

Antipov, Evgueni M., Evguenia A. Mushina, Manfred Stamm, and Erhard W. Fischer. "Structure of Polybutadienes Synthesized with a New Catalyst System, 2. Blends oftrans-andcis-1,4-Polybutadiene." Macromolecular Chemistry and Physics 202, no. 1 (2001): 73–81. http://dx.doi.org/10.1002/1521-3935(20010101)202:1<73::aid-macp73>3.0.co;2-3.

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29

Rozentsvet, Victor A., Daria M. Ulyanova, Nelly A. Sablina, Sergei V. Kostjuk, Peter M. Tolstoy, and Ivan A. Novakov. "Cationic polymerization of butadiene using alkyl aluminum compounds as co-initiators: an efficient approach toward solid polybutadienes." Polymer Chemistry 13, no. 11 (2022): 1596–607. http://dx.doi.org/10.1039/d1py01684a.

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30

Roovers, Jacques. "Synthesis and Properties of Ring Polybutadienes." Rubber Chemistry and Technology 62, no. 1 (1989): 33–41. http://dx.doi.org/10.5254/1.3536233.

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Abstract Much of polymer science is concerned with the linear joining of monomers and the properties of the new materials that emerge from this process. Of almost equal importance is the formation of tridimensional networks as the result of branching and crosslinking reactions. Ring formation has always been considered an unavoidable consequence of extensive crosslinking and, from the theoretical point, it is often neglected. Nevertheless, rings may contribute to the network properties by means of permanent entanglements. Indeed, rings alone can form special permanent networks without any chem

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31

Pekar, M. "Inverse gas chromatography of liquid polybutadienes." Polymer 43, no. 3 (2002): 1013–15. http://dx.doi.org/10.1016/s0032-3861(01)00651-6.

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32

Sokolova, L. V., O. A. Chesnokova, and V. A. Shershnev. "High-temperature structural transition of polybutadienes." Polymer Science U.S.S.R. 29, no. 1 (1987): 27–34. http://dx.doi.org/10.1016/0032-3950(87)90076-1.

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33

LIU, W., Y. YANG, and T. HE. "Monomeric friction coefficient of 1,2-polybutadienes." Polymer 29, no. 10 (1988): 1789–92. http://dx.doi.org/10.1016/0032-3861(88)90392-8.

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34

Li, Si Wan, Heon E. Park, John M. Dealy, et al. "Detecting Structural Polydispersity in Branched Polybutadienes." Macromolecules 44, no. 2 (2011): 208–14. http://dx.doi.org/10.1021/ma101803h.

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35

Varghese, Abraham, K. J. Scariah, S. C. Bera, M. Rama Rao, and K. S. Sastri. "Processability characteristics of hydroxy terminated polybutadienes." European Polymer Journal 32, no. 1 (1996): 79–83. http://dx.doi.org/10.1016/0014-3057(95)00116-6.

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36

Peka?, Miloslav. "On the miscibility of liquid polybutadienes." Journal of Applied Polymer Science 78, no. 9 (2000): 1628–35. http://dx.doi.org/10.1002/1097-4628(20001128)78:9<1628::aid-app80>3.0.co;2-i.

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37

Takeda, Masatami, Ryūichi Endõ, and Yoshikatsu Matsuura. "Solution properties of chlorinated stereoregular polybutadienes." Journal of Polymer Science Part C: Polymer Symposia 23, no. 2 (2007): 487–98. http://dx.doi.org/10.1002/polc.5070230206.

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38

Roovers, J., and P. M. Toporowski. "Synthesis and characterization of ring polybutadienes." Journal of Polymer Science Part B: Polymer Physics 26, no. 6 (1988): 1251–59. http://dx.doi.org/10.1002/polb.1988.090260609.

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39

Makhiyanov, N. "13C NMR spectra of 1,4-polybutadienes." Journal of Applied Spectroscopy 61, no. 1-2 (1994): 509–13. http://dx.doi.org/10.1007/bf02606394.

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40

Jung, Haeji, and Yeong-Gweon Lim. "Fe(ii)-Catalyzed azidation of polybutadienes using the Zhdankin reagent." Polymer Chemistry 10, no. 39 (2019): 5348–52. http://dx.doi.org/10.1039/c9py01009b.

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41

Januszewski, Rafał, Michał Dutkiewicz, Ireneusz Kownacki, and Bogdan Marciniec. "The effect of organosilicon modifier structure on the efficiency of the polybutadiene hydrosilylation process." Catalysis Science & Technology 10, no. 21 (2020): 7240–48. http://dx.doi.org/10.1039/d0cy01376e.

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Real-time FT-IR spectroscopy permitted us to determine the influence of steoelectronic properties of functional groups on hydrosilylation. This allowed the synthesis of polybutadienes equipped with attractive silicon-based functional groups.

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42

Berkovich, Inbal, Sudheendran Mavila, Olga Iliashevsky, Sebastian Kozuch, and N. Gabriel Lemcoff. "Single-chain polybutadiene organometallic nanoparticles: an experimental and theoretical study." Chemical Science 7, no. 3 (2016): 1773–78. http://dx.doi.org/10.1039/c5sc04535e.

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High molecular weight polybutadienes and rhodium complexes were used to produce single chain organometallic nanoparticles. A relationship was found between the cis double bond content of the polymer and metal binding kinetics.

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43

Huang, Shuai, Li Han, Hongwei Ma, et al. "Determination of refractive index increment of synthetic polybutadienes and microstructural control of grafting density and liquid crystalline properties." Polymer Chemistry 11, no. 14 (2020): 2559–67. http://dx.doi.org/10.1039/d0py00050g.

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Polybutadienes (PBs) with microstructural control of 8% to 94% moles of 1,2-olefins synthesized via living anionic polymerization (LAP) were used as precursors for the synthesis of PB-based liquid crystalline polymers (LCPs) with well-controlled grafting densities.

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44

Pan, Weijing, Huafeng Chen, Jingshan Mu, et al. "Synthesis of high crystalline syndiotactic 1,2-polybutadienes and study on their reinforcing effect on cis-1,4 polybutadiene." Polymer 111 (February 2017): 20–26. http://dx.doi.org/10.1016/j.polymer.2017.01.022.

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45

Antipov, Evgueni M., Boris F. Schklyaruk, Manfred Stamm, and Erhard W. Fischer. "Structure of Polybutadienes Synthesised with a New Catalyst System, 3. Random Copolymers oftrans-1,4- and 1,2-Polybutadiene." Macromolecular Chemistry and Physics 202, no. 1 (2001): 82–89. http://dx.doi.org/10.1002/1521-3935(20010101)202:1<82::aid-macp82>3.0.co;2-7.

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46

Narayanan, Pondicherry, Barry Kaye, and David J. Cole-Hamilton. "Polycarboxylic acids via catalytic hydrocarboxylation of polybutadienes." Journal of Materials Chemistry 3, no. 1 (1993): 19. http://dx.doi.org/10.1039/jm9930300019.

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47

Roovers, Jacques, Paul Toporowski, and James Martin. "Synthesis and characterization of multiarm star polybutadienes." Macromolecules 22, no. 4 (1989): 1897–903. http://dx.doi.org/10.1021/ma00194a064.

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48

Cais, Rudolf E., and Shahabuddin Siddiqui. "Chemical modification of 1,4-polybutadienes by fluorochlorocarbene." Macromolecules 20, no. 5 (1987): 1004–12. http://dx.doi.org/10.1021/ma00171a021.

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49

Makhiyanov, N., and E. V. Temnikova. "Glass-transition temperature and microstructure of polybutadienes." Polymer Science Series A 52, no. 12 (2010): 1292–300. http://dx.doi.org/10.1134/s0965545x10120072.

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50

Ismail, Ahmed E., Flint Pierce, and Gary S. Grest. "Diffusion of small penetrant molecules in polybutadienes." Molecular Physics 109, no. 16 (2011): 2025–33. http://dx.doi.org/10.1080/00268976.2011.608085.

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