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Journal articles on the topic 'Radiolysis of uranium hexafluoride'

Author: Grafiati

Published: 5 June 2025

Last updated: 2 August 2025

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1

Kulikov, Gennady G., Anatoly N. Shmelev, Vladimir A. Apse, and Evgeny G. Kulikov. "Comprehensive analysis of proliferation protection of uranium due to the presence of 232U and its decay products." Nuclear Energy and Technology 8, no. 4 (2022): 253–60. http://dx.doi.org/10.3897/nucet.8.96564.

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For a comprehensive assessment of the protection of uranium against proliferation due to the presence of uranium-232 in it, the authors of the article propose and substantiate an integral protection criterion for this material. The criterion is based on the physical barriers against the proliferation of uranium created by uranium-232, namely: (1) the radiolysis of uranium hexafluoride, which hinders attempts to re-enrich uranium and, as a result, a significant critical mass; (2) hard γ-radiation, which leads to incapacity and death of those who try to handle this material without radiation pro

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2

Kulikov, Gennady G., Anatoly N. Shmelev, Vladimir A. Apse, and Evgeny G. Kulikov. "Comprehensive analysis of proliferation protection of uranium due to the presence of 232U and its decay products." Nuclear Energy and Technology 8, no. (4) (2022): 253–60. https://doi.org/10.3897/nucet.8.96564.

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For a comprehensive assessment of the protection of uranium against proliferation due to the presence of uranium-232 in it, the authors of the article propose and substantiate an integral protection criterion for this material. The criterion is based on the physical barriers against the proliferation of uranium created by uranium-232, namely: (1) the radiolysis of uranium hexafluoride, which hinders attempts to re-enrich uranium and, as a result, a significant critical mass; (2) hard γ-radiation, which leads to incapacity and death of those who try to handle this material without radiation pro

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3

Khromov, Konstantin Yu., Andrey V. Orlov, Ivan A. Belov, and Vladimir A. Nevinitsa. "Determination of the energy characteristics of the reactions UF6 ↔ UF5 + F and UF6 ↔ UF4 + F2." Nuclear Energy and Technology 7, no. (3) (2021): 239–44. https://doi.org/10.3897/nucet.7.74152.

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Quantum-mechanical methods are used to assess the energy barriers to dissociation and recombination reactions of UF<sub>6</sub> ↔ UF<sub>5</sub> + F and UF<sub>6</sub> ↔ UF<sub>4</sub> + F<sub>2</sub>. The energy characteristics of these reactions are found to be strongly asymmetric: the dissociation reaction barriers exceed the recombination reactions barriers by more than 4 eV. The equilibrium atomic configurations of F<sub>2</sub>, UF<sub>4</sub>, UF<sub>5</sub> and UF<sub>6</sub> have been determined using precision quantum mechanical calculations. The U-F bond lengths obtained as a result

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4

Belov, I. A., A. V. Grol’, V. A. Nevinitsa, O. Yu Poveshchenko, A. Yu Smirnov, and G. A. Sulaberidze. "Radiolysis of 232,234U-Enriched Regenerated-Uranium Hexafluoride at the Temporary Storage Stage in a Separation Plant." Atomic Energy 126, no. 5 (2019): 305–9. http://dx.doi.org/10.1007/s10512-019-00554-w.

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5

Nadezhdin, Igor S., and Nikolay S. Krinitsyn. "Harmonization Values of Downloads and Operating Modes of Interconnected Devices Production of Uranium Hexafluoride." Advanced Materials Research 1084 (January 2015): 655–60. http://dx.doi.org/10.4028/www.scientific.net/amr.1084.655.

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The article is devoted to the problem of load agreement of solid-phase components into the fluorination and capture apparatus of two technological of uranium hexafluoride production lines. The article describes the process of developing a model of the horizontal part of the combined type apparatus which was included in the dynamic mathematical model of uranium hexafluoride production. The developed algorithm of load agreement was studied on dynamic mathematical model of uranium hexafluoride production.

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6

YATO, Yumio, Osamu SUTO, and Hideyuki FUNASAKA. "Uranium Isotope Exchange between Uranium Hexafluoride and Uranium Pentafluoride." Journal of Nuclear Science and Technology 32, no. 5 (1995): 430–38. http://dx.doi.org/10.1080/18811248.1995.9731728.

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7

Vlasov, A. A., E. A. Filippov, L. L. Fadeev, and A. I. Vinnikov. "Safe shipment of uranium hexafluoride." Soviet Atomic Energy 72, no. 2 (1992): 163–64. http://dx.doi.org/10.1007/bf01121092.

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8

Orlov, Аleksey A., and Roman V. Malyugin. "Way to Obtain Uranium Hexafluoride." Advanced Materials Research 1084 (January 2015): 338–41. http://dx.doi.org/10.4028/www.scientific.net/amr.1084.338.

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The article contains an analytical overview of technologies used for obtaining UF6. The structures of devices for obtaining UF6 have been considered. Their advantages and drawbacks have been outlined. It has been shown that plasma reactors using uranium tetrafluoride as a raw material are the most efficient in obtaining UF6.

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9

Orlov, Aleksey A., and Roman V. Malyugin. "Methods of Uranium Hexafluoride Purification." Advanced Materials Research 1084 (January 2015): 46–49. http://dx.doi.org/10.4028/www.scientific.net/amr.1084.46.

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The article contains an analytical overview of techniques used for UF6 purification. Structures of respective devices have been considered. Their advantages and drawbacks have been outlined. It has been shown that heat discharge desublimators and multi-chamber devices with two heated walls are the most efficient in UF6 purification.

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10

Armstrong, D. P., D. A. Harkins, R. N. Compton, and D. Ding. "Multiphoton ionization of uranium hexafluoride." Journal of Chemical Physics 100, no. 1 (1994): 28–43. http://dx.doi.org/10.1063/1.467270.

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11

Belyntsev, A. M., G. S. Sergeev, O. B. Gromov, et al. "Intensification of evaporation of uranium hexafluoride." Theoretical Foundations of Chemical Engineering 47, no. 4 (2013): 499–504. http://dx.doi.org/10.1134/s0040579513040040.

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12

Klouda, Karel, Václav Rak, and Josef Vachuška. "Intercalation of uranium hexafluoride into graphite." Collection of Czechoslovak Chemical Communications 50, no. 4 (1985): 947–55. http://dx.doi.org/10.1135/cccc19850947.

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Intercalation of UF6 into graphite, both from the gaseous phase and from the Ledon 113 solution, was studied. The amount of intercalated UF6 from the gaseous phase was found to be inversely proportional to the size of graphite particles. Intercalation increases with the increasing temperature and surface area of graphite. The contact of gaseous UF6 with graphite led to the formation of β-UF5 that is not intercalated. In the Ledon solution, β-UF5 is not formed. "Passivation" of graphite by elementary fluorine also prevents the formation of β-UF5 but the amount of intercalated UF6 decreases. The

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13

Morel, Bertrand, Ania Selmi, Laurent Moch, et al. "Surface reactivity of uranium hexafluoride (UF6)." Comptes Rendus Chimie 21, no. 8 (2018): 782–90. http://dx.doi.org/10.1016/j.crci.2018.05.006.

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14

Bacher, W., W. Bier, and A. Guber. "Reaction of uranium hexafluoride with fluoroelastomers." Journal of Fluorine Chemistry 35, no. 1 (1987): 207. http://dx.doi.org/10.1016/0022-1139(87)95164-5.

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15

Lyman, John L., Glenn Laguna, and N. R. Greiner. "Reactions of uranium hexafluoride photolysis products." Journal of Chemical Physics 82, no. 1 (1985): 175–82. http://dx.doi.org/10.1063/1.448791.

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16

Gordon, E. B., V. A. Dubovitskii, V. I. Matyushenko, V. D. Sizov, and Yu A. Kolesnikov. "Uranium hexafluoride reduction with hydrogen atoms." Kinetics and Catalysis 47, no. 1 (2006): 148–56. http://dx.doi.org/10.1134/s0023158406010204.

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17

Babenko, S., and A. Bad'in. "On the Dose Coefficient of Uranium Hexafluoride." Medical Radiology and radiation safety 66, no. 5 (2021): 11–17. http://dx.doi.org/10.12737/1024-6177-2021-66-5-11-17.

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Introduction: Uranium hexafluoride (UF6, UHF) is a gaseous product containing uranium and fluorine. Once in the air, it interacts with water vapor and produces hydrolysis products that can penetrate the human body and lead to the chemical effects of uranium and fluorine, as well as the radiation effects of uranium on the body. This action can be very strong and therefore serious attention has been paid to its study for a long time. Purpose: Quantitative calculation of the radiation effects of uranium on humans and their analysis in the conditions of daily work at nuclear power plants, as

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18

Hunt, Rodney D., Lester Andrews, and L. Mac Toth. "Matrix infrared spectra of hydrogen chloride complexes with uranium hexafluoride, tungsten hexafluoride and molybdenum hexafluoride." Inorganic Chemistry 30, no. 20 (1991): 3829–32. http://dx.doi.org/10.1021/ic00020a011.

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19

Hunt, Rodney D., Lester Andrews, and L. M. Toth. "Infrared spectra of uranium hexafluoride, tungsten hexafluoride, molybdenum hexafluoride, and sulfur hexafluoride complexes with hydrogen fluoride in solid argon." Journal of Physical Chemistry 95, no. 3 (1991): 1183–88. http://dx.doi.org/10.1021/j100156a028.

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20

Muratov, O. E. "Handling problems of depleted uranium hexafluoride (review)." Theoretical and Applied Ecology, no. 4 (2020): 13–21. http://dx.doi.org/10.25750/1995-4301-2020-4-013-021.

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21

Klouda, Karel, V/'alav Rak, Antonín Poŝta, and Václav Dêdek. "The intercalation of uranium hexafluoride into graphite." Journal of Fluorine Chemistry 29, no. 1-2 (1985): 63. http://dx.doi.org/10.1016/s0022-1139(00)83298-4.

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22

Achour, Mickaël, Laure Martinelli, Sylvie Chatain, et al. "Corrosion of iron in liquid uranium hexafluoride." Corrosion Engineering, Science and Technology 52, no. 8 (2017): 611–17. http://dx.doi.org/10.1080/1478422x.2017.1344039.

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23

van der Merwe, P. du T. "On the infrared‐active overtonesnν3of uranium hexafluoride". Journal of Chemical Physics 99, № 7 (1993): 5030–35. http://dx.doi.org/10.1063/1.466004.

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24

Lind, Maria C., Stephen L. Garrison, and James M. Becnel. "Trimolecular Reactions of Uranium Hexafluoride with Water." Journal of Physical Chemistry A 114, no. 13 (2010): 4641–46. http://dx.doi.org/10.1021/jp909368g.

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25

Menghini, M., A. Montone, P. Morales, L. Nencini, and P. Dore. "Effects of collisions on uranium hexafluoride fluorescence." Chemical Physics Letters 150, no. 3-4 (1988): 204–10. http://dx.doi.org/10.1016/0009-2614(88)80028-9.

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26

Lubnin, S. S., E. V. Maslyukov, and V. A. Palkin. "Optimization of double cascades by the bee colony algorithm for purification of regenerated uranium hexafluoride from isotopes232, 234, 236U." Izvestiya vysshikh uchebnykh zavedenii. Fizika, no. 5 (2022): 56–62. http://dx.doi.org/10.17223/00213411/65/5/56.

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We propose a double cascade scheme for reducing the concentration of232, 234, 236U isotopes in regenerated uranium hexafluoride. In the product of the first ordinary cascade the greatest decrease in the236U /235U mass ratio with enrichment in235U to a concentration of less than 20% is provided. To ensure the required concentrations, a special mode of operation of the stages. In the second ordinary cascade, which is fed by the product of the first, enrichment in isotopes232,234U is performed. The waste flow, purified from232, 234U, is diluted to a concentration of235U less than 5%. A method for

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27

Gubanov, S. M., and K. M. Moiseeva. "Modeling of heat transfer during the desublimation of substances into refrigerated containers." Journal of Physics: Conference Series 2211, no. 1 (2022): 012018. http://dx.doi.org/10.1088/1742-6596/2211/1/012018.

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Abstract This paper presents the results of the theoretical and computational analysis of the thermal processes during the desublimation of uranium hexafluoride and hydrogen fluoride in refrigerated containers. The technological scheme of the hydrogen fluoride desublimation in the containers refrigerated by the cold air is presented. We have substantiated the desublimation method of the uranium hexafluoride residues and hydrogen fluoride from the process stream into one container. The paper also provides the estimation of the maximum container loading, when the pressure of the saturated vapors

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28

Semenov, Evgeny V., and Vladimir V. Kharitonov. "Calculation of the cost of enriched uranium products in multi-stream cascades of enrichment process." Nuclear Energy and Technology 9, no. 1 (2023): 19–25. http://dx.doi.org/10.3897/nucet.9.100752.

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Modern uranium enrichment facilities can simultaneously use several raw materials as feed, including natural uranium, regenerated uranium obtained as a result of SNF reprocessing, or depleted uranium (all in the form of uranium hexafluoride). As the output of the separating cascade, several types of enriched uranium product with different levels of enrichment can be fabricated simultaneously. The paper proposes a methodology, absent in literature, for calculating the cost of each enriched uranium product in multi-stream separating cascades. The proposed methodology uses standard definitions of

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29

Semenov, Evgeny V., and Vladimir V. Kharitonov. "Calculation of the cost of enriched uranium products in multi-stream cascades of enrichment process." Nuclear Energy and Technology 9, no. (1) (2023): 19–25. https://doi.org/10.3897/nucet.9.100752.

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Modern uranium enrichment facilities can simultaneously use several raw materials as feed, including natural uranium, regenerated uranium obtained as a result of SNF reprocessing, or depleted uranium (all in the form of uranium hexafluoride). As the output of the separating cascade, several types of enriched uranium product with different levels of enrichment can be fabricated simultaneously. The paper proposes a methodology, absent in literature, for calculating the cost of each enriched uranium product in multi-stream separating cascades. The proposed methodology uses standard definitions of

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30

Tayurskii, Dmitriy, Evgeniy Podoplelov, and Anatoliy Dement'ev. "THE CAPTURE OF URANIUM HEXAFLUORIDE FROM COLLECTED GASES." Bulletin of the Angarsk State Technical University 1, no. 15 (2022): 93–97. http://dx.doi.org/10.36629/2686-777x-2021-1-15-93-97.

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The article presents an analytical review of methods for capturing uranium hexafluoride, its regeneration from waste gases. The types and designs of the corresponding devices are con-sidered. Their advantages and disadvantages are shown. The most effective methods that can be used to solve the problem of complex modernization of sublimate and separation plants have been identified

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31

Menghini, M., P. Morales, P. Dore, and M. I. Schisano. "On the photodissociation of uranium hexafluoride in theBband." Journal of Chemical Physics 84, no. 11 (1986): 6521–22. http://dx.doi.org/10.1063/1.450699.

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32

Vorster, S. W., and F. P. A. Robinson. "Corrosion of copper alloys by gaseous uranium hexafluoride." British Corrosion Journal 27, no. 2 (1992): 151–56. http://dx.doi.org/10.1179/bcj.1992.27.2.151.

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33

Croft, Stephen, Martyn T. Swinhoe, and Karen A. Miller. "Alpha particle induced gamma yields in uranium hexafluoride." Nuclear Instruments and Methods in Physics Research Section A: Accelerators, Spectrometers, Detectors and Associated Equipment 698 (January 2013): 192–95. http://dx.doi.org/10.1016/j.nima.2012.10.003.

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34

Sherrow, Susan A., and Rodney D. Hunt. "FTIR spectra of the hydrolysis of uranium hexafluoride." Journal of Physical Chemistry 96, no. 3 (1992): 1095–99. http://dx.doi.org/10.1021/j100182a015.

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35

Benzi, V., та D. Mostacci. "Neutrons from (α, n) reactions in uranium hexafluoride". Applied Radiation and Isotopes 48, № 2 (1997): 213–14. http://dx.doi.org/10.1016/s0969-8043(96)00180-7.

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36

Gromov, O. B., A. A. Mikhalichenko, P. I. Mikheev, V. I. Nikonov, and V. G. Soloviov. "Reduction of uranium hexafluoride adsorbed on sodium fluoride." Atomic Energy 109, no. 2 (2010): 96–101. http://dx.doi.org/10.1007/s10512-010-9329-5.

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37

Asprey, Larned B., Scott A. Kinkead, and P. Gary Eller. "Low-Temperature Conversion of Uranium Oxides to Uranium Hexafluoride Using Dioxygen Difluoride." Nuclear Technology 73, no. 1 (1986): 69–71. http://dx.doi.org/10.13182/nt86-a16202.

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38

Hubbard, Joshua A., Meng-Dawn Cheng, Lawrence Cheung, Jared R. Kirsch, Jason M. Richards, and Glenn A. Fugate. "UO2F2 particulate formation in an impinging jet gas reactor." Reaction Chemistry & Engineering 6, no. 8 (2021): 1428–47. http://dx.doi.org/10.1039/d1re00105a.

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39

Babenko, S. P., and A. V. Bad'in. "Recommendations for Choosing a Model Describing the Human Exposure to Uranium Hexafluoride." Radio Engineering, no. 1 (March 5, 2020): 31–42. http://dx.doi.org/10.36027/rdeng.0120.0000161.

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The article notes the fact that uranium hexafluoride (UHF) is the only uranium compound in a gaseous state under conditions close to normal to be used in the enrichment of natural uranium with an isotope. It is noted that during the hydrolysis of UHF in the air of a working room, this room is polluted with gases and aerosols that are carriers of uranium and fluorine atoms, which have a negative chemical and radiation effect on the human body. This, of course, poses problems when using uranium hexafluoride at the enterprises of the nuclear industry both in everyday work and, especially, in poss

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40

Babenko, S. P., and Andrey V. Badin. "ABOUT CALCULATION OF THE DETERMINISTIC EFFECT OF PROTEINURIA IN EMPLOYEES OF ENRICHMENT PLANTS OF NUCLEAR INDUSTRY." Hygiene and sanitation 97, no. 4 (2018): 315–21. http://dx.doi.org/10.18821/0016-9900-2018-97-4-315-321.

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In this paper, we consider the impacts of gaseous uranium hexafluoride used at concentrating plants of the nuclear industry on the human body. The appearance of uranium hexafluoride in the air of the working premises is accompanied by hydrolysis and the formation of substances that can enter the human body and bring atoms of uranium and fluorine. The article describes the method of the determination of the working conditions preventing the development of occupational diseases in employees. The method is based both on the calculation of the number of toxic substances entering the human body in

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41

Chan, George C. Y., Xianglei Mao, Leigh R. Martin, Lee D. Trowbridge, and Richard E. Russo. "Direct uranium enrichment assay in gaseous uranium hexafluoride with laser induced breakdown spectroscopy." Journal of Radioanalytical and Nuclear Chemistry 331, no. 3 (2022): 1409–21. http://dx.doi.org/10.1007/s10967-022-08215-2.

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42

But, L. A., V. D. Vdovichenko, O. B. Gromov, et al. "Synthesis of powder uranium tetrafluoride from depleted uranium hexafluoride in hydrogen fluoride flame." Theoretical Foundations of Chemical Engineering 50, no. 5 (2016): 884–89. http://dx.doi.org/10.1134/s0040579516050043.

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43

But, L. A., V. D. Vdovichenko, O. B. Gromov, et al. "Synthesis of powder uranium tetrafluoride from depleted uranium hexafluoride in hydrogen fluorine flame." Theoretical Foundations of Chemical Engineering 51, no. 4 (2017): 594–98. http://dx.doi.org/10.1134/s0040579517040030.

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44

Seneda, J. A., F. F. Figueiredo, A. Abrão, F. M. S. Carvalho, and E. U. C. Frajndlich. "Recovery of uranium from the filtrate of ‘ammonium diuranate’ prepared from uranium hexafluoride." Journal of Alloys and Compounds 323-324 (July 2001): 838–41. http://dx.doi.org/10.1016/s0925-8388(01)01156-2.

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45

Avtandilashvili, Maia, Matthew Puncher, Stacey L. McComish, and Sergei Y. Tolmachev. "US Transuranium and Uranium Registries case study on accidental exposure to uranium hexafluoride." Journal of Radiological Protection 35, no. 1 (2015): 129–51. http://dx.doi.org/10.1088/0952-4746/35/1/129.

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46

Kalinin, B. A., V. E. Atanov, and O. E. Aleksandrov. "Metastable ions in the mass spectrum of uranium hexafluoride." Technical Physics 47, no. 5 (2002): 648–50. http://dx.doi.org/10.1134/1.1479997.

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47

Richards, Jason M., Leigh R. Martin, Glenn A. Fugate, and Meng-Dawn Cheng. "Kinetic investigation of the hydrolysis of uranium hexafluoride gas." RSC Advances 10, no. 57 (2020): 34729–31. http://dx.doi.org/10.1039/d0ra05520d.

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48

El-Sheikh, S. M. "The structure of different phases for solid uranium hexafluoride." Acta Crystallographica Section A Foundations of Crystallography 63, a1 (2007): s162. http://dx.doi.org/10.1107/s0108767307096341.

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49

Miyazawa, T., Y. Tezuka, A. Shimoda, H. Takahashi, and M. Aritomi. "Development of ‘MST-30’ Packaging for Enriched Uranium Hexafluoride." International Journal of Radioactive Materials Transport 12, no. 4 (2001): 225–32. http://dx.doi.org/10.1179/rmt.2001.12.4.225.

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50

Kunakov, S. K., and E. E. Son. "Probe diagnostics of nuclear-excited plasma of uranium hexafluoride." High Temperature 48, no. 6 (2010): 789–805. http://dx.doi.org/10.1134/s0018151x10060052.

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