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Lantz, Mattias. "Investigations of Reaction Cross Sections for Protons and 3He." Doctoral thesis, Uppsala universitet, Institutionen för kärn- och partikelfysik, 2005. http://urn.kb.se/resolve?urn=urn:nbn:se:uu:diva-5813.
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The reaction cross section gives the probability that a particle will undergo a nonelastic process when passing through a nuclear medium. Therefore reaction cross section data are of importance both for theoretical studies and for applications in such diverse fields as medicine, biology, astrophysics and accelerator-driven transmutation of nuclear waste. There exist many data sets with angular distributions of elastic scattering, but very few measurements of the complementary reaction cross section have been performed. The measurement is in principle simple but has in practice proved to be very difficult to perform, and the relatively limited amount of experimental data displays some serious inconsistencies. Results from measurements of reaction cross sections are presented for: • 3He on 9Be, 12C, 16O, 28Si, 40Ca, 58,60Ni, 112,116,118,120,124Sn and 208Pb at 96, 138 and 167 MeV • protons on 12C, 40Ca, 90Zr and 208Pb at six energies in the energy range 80-180 MeV, and on 58Ni at 81 MeV. Experimental uncertainties were 3-9% for 3He and 1.5-8% for protons. The apparatus and the experimental method used for the measurements of reaction cross sections, using a modified attenuation technique, is described. The detection method enables simultaneous measurements of reaction cross sections for five different sizes of the solid angles in steps from 99.0 to 99.8% of the total solid angle. The final results are obtained by extrapolation to the full solid angle. Experimental results are compared with predictions from optical model calculations using phenomenological global optical potentials. Phenomenological parametrizations of reaction cross sections for scattering of projectiles on targets are presented. The parametrizations show that reaction cross sections are very sensitive to matter distributions at very large radii of both the projectile and the target. For protons the derived relations makes it possible to predict the reaction cross sections on targets for which no experimental data exist.
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Lantz, Mattias. "Investigations of Reaction Cross Sections for Protons and 3He." Doctoral thesis, Uppsala : Acta Universitatis Upsaliensis : Univ.-bibl. [distributör], 2005. http://urn.kb.se/resolve?urn=urn:nbn:se:uu:diva-5813.
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Hankel, Marlies. "Time-dependent wavepacket methods for the calculation of state-to-state molecular reactive cross sections." Thesis, University of Bristol, 2001. http://ethos.bl.uk/OrderDetails.do?uin=uk.bl.ethos.391180.
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Sawada, Shinya. "Differential Cross Sections for the np→dX Reaction at 1.0 and 2.0 GeV." 京都大学 (Kyoto University), 1997. http://hdl.handle.net/2433/157147.
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本文データは平成22年度国立国会図書館の学位論文(博士)のデジタル化実施により作成された画像ファイルを基にpdf変換したものであるKyoto University (京都大学)
0048
新制・課程博士
博士(理学)
甲第6934号
理博第1860号
新制||理||1012(附属図書館)
UT51-97-L155
京都大学大学院理学研究科物理学第二専攻
(主査)教授 今井 憲一, 教授 政池 明, 教授 笹尾 登
学位規則第4条第1項該当
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Carnahan, Brian. "Strangeness Photoproduction in the {gamma}p {yields} K{sup 0} {Sigma}{sup +} Reaction." Washington, D.C : Oak Ridge, Tenn. : United States. Dept. of Energy. Office of Energy Research ; distributed by the Office of Scientific and Technical Information, U.S. Dept. of Energy, 2003. http://www.osti.gov/servlets/purl/824935-CL5ICZ/native/.
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Thesis (Ph.D.); Submitted to the Catholic Univ. of America, Washington, DC (US); 1 May 2003.Published through the Information Bridge: DOE Scientific and Technical Information. "JLAB-PHY-03-40" "DOE/ER/40150-2764" Brian Carnahan. 05/01/2003. Report is also available in paper and microfiche from NTIS.
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Prokofiev, Alexander. "Nucleon-Induced Fission Cross Sections of Heavy Nuclei in the Intermediate Energy Region." Doctoral thesis, Uppsala : Acta Universitatis Upsaliensis : Univ.-bibl. [distributör], 2001. http://publications.uu.se/theses/91-554-5009-1/.
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Thiry, Jean-Claude. "Measurement of (n,xng) reaction cross sections of interest for the Generation IV reactors." Strasbourg, 2010. http://www.theses.fr/2010STRA6144.
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Le développement de réacteurs de quatrième génération demande la connaissance de sections efficaces de différentes réactions nucléaires. Les recherches du groupe GRACE concernent principalement la détermination des sections efficaces des réactions (n,xn) sur des isotopes intervenant dans les processus de transmutation et de régénération dans ces réacteurs. Le but de ces investigations est d’obtenir des sections efficaces inconnues et de réduire les incertitudes sur des données existantes. Le présent travail consiste dans l'optimisation du dispositif expérimental développé pour les mesures sur des noyaux radioactifs. Les expériences sont réalisées auprès de l’installation GELINA (IRMM, Geel, Belgique) qui produit un faisceau de neutrons blanc pulsé. Ce faisceau pulsé permet de déterminer les énergies des neutrons par la méthode du temps de vol et la spectroscopie gamme prompte est utilisée pour identifier les différents noyaux formés par les réactions (n,xnγ). L'objectif de ce travail est d'aboutir à un dispositif expérimental permettant la mesure des sections efficaces de la réaction 233U(n,xnγ), d’une très grande importance pour le processus de régénération du cycle 232ThThe presented work consists of studying 232Th(n,xnγ) and 235U(n,xnγ) reactions in the fast neutron energy domain (up to 20 MeV) with the best precision possible. The experiments are performed at GELINA which delivers a pulsed, white neutron beam at IRMM, Belgium. The time characteristics of the beam enable us to measure neutron energies with the time-of-flight (TOF) technique. The neutron induced reactions (in this case inelastic scattering, (n,2n) and (n,3n) reactions) are identified by online prompt γ spectroscopy with an experimental setup including four HPGe detectors. A double layered fission chamber is used to monitor the incident neutron flux. The obtained results are presented and a comparison between the measured cross sections and the TALYS code predictions will be discussed. In order to achieve a very high precision on the reaction cross sections, an extensive work has been realised on the detection efficiencies of the counters used in the experiment. These quantities were in fact the largest sources of uncertainty in foregoing campaigns. After important efforts including high precision measurements together with Geant4 simulations, the efficiency of the fission chambers as well as of the HPGe detectors could be determined with accuracies below 3 %, accomplishing the final goal of a cross section determination with a precision of 5 %. This work is a further step in the preparation of the measurement of 233U(n,xnγ) reactions, which are completely unknown at this stage although of very high importance in the 232Th regeneration process. For this reason, a new, segmented HPGe detector was conceived, which will complete the current experimental setup
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Ralston, James. "The 10B(n, α) and 10B(n, p) Cross-Sections in the MeV Energy Range." Ohio University Honors Tutorial College / OhioLINK, 2011. http://rave.ohiolink.edu/etdc/view?acc_num=ouhonors1315160730.
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Urdabayev, Nurtay. "Development of Photoreactive Organic Compounds with Large Two-Photon Absorption Cross Sections." Bowling Green State University / OhioLINK, 2006. http://rave.ohiolink.edu/etdc/view?acc_num=bgsu1148914562.
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Latacz, Barbara Maria. "Study of the antihydrogen atom and ion production via charge exchange reaction on positronium." Thesis, Université Paris-Saclay (ComUE), 2019. http://www.theses.fr/2019SACLS266/document.
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Le but principal de la collaboration GBAR est de mesurer le comportement d'atomes d'antihydrogène sous l'effet de la gravité terrestre. Ceci est fait en mesurant la chute libre classique d'atomes d'antihydrogène, qui est un test direct du principe d'équivalence faible pour l'antimatière. La première étape de l'expérience est de produire des ions d'antihydrogène et de les amener dans un piège de Paul, où ils peuvent être refroidis à une température de l'ordre du μK en utilisant la technique du refroidissement sympathique avec des ions Be⁺ eux-mêmes mis dans leur état fondamental par la technique Raman à bande latérale. Une température de l'ordre du μK correspond à une vitesse de la particule de l'ordre de 1 m/s. Une fois cette vitesse atteinte, l'ion antihydrogène peut être neutralisé et commence sa chute. Ceci permet une précision de 1 % sur la mesure de l’accélération gravitationnelle g pour l’antimatière avec environ 1500 événements. Cependant, pour mesurer la chute libre, il faut d'abord produire l'ion antihydrogène. Celui-ci est formé dans les réactions d'échange de charge entre des antiprotons et des antihydrogènes avec du positronium. Positronium et atomes d'antihydrogène peut se trouver soit à l’état fondamental, soit dans un état excité. Une étude expérimentale de la mesure de la section efficace de ces deux réactions est décrite dans cette thèse. La production de l'atome d'antihydrogène ainsi que de l'ion se passe à l’intérieur d'une cavité. La formation d'un antihydrogène ion lors d'une interaction entre faisceaux requiert environ 5x10⁶ antiprotons/paquet et quelques 10¹¹ Ps/cm⁻³ de densité de positronium à l’intérieur d'une cavité. Celle-ci est produite par un faisceau contenant 5x10¹⁰ positrons par paquet. La production de faisceaux aussi intenses avec les propriétés requises est en soi un challenge. Le développement de la source de positrons de GBAR est décrite. Celle-ci est basée sur un accélérateur linéaire à électrons de 9 MeV. Le faisceau d’électrons est incident sur une cible de tungstène où les positrons sont créés par rayonnement de freinage (gammas) et création de paires. Une partie des positrons ainsi créés diffusent à nouveau dans un modérateur de tungstène en réduisant leur énergie à environ 3 eV. Ces particules sont re-accélérées à une énergie d'environ 53 eV. Aujourd'hui, le flux mesuré de positrons est au niveau de 6x10⁷ e⁺/s, soit quelques fois. Puis la thèse comporte une courte description des préparatifs pour les faisceaux d'antiprotons ou de protons, terminée par un chapitre sur le taux de production attendu d'atomes et d'ions d'antihydrogène. En aval de la réaction, les faisceaux d'antiprotons, d'atomes et d'ions d'antihydrogène sont guidés vers leur système de détection. Ceux-ci ont été conçus de façon à permettre la détection d'un à plusieurs milliers d'atomes d'antihydrogène, un seul ion antihydrogène et tous les 5x10⁶ antiprotons. Ceci est particulièrement difficile parce que l'annihilation des antiprotons crée beaucoup de particules secondaires qui peuvent perturber la mesure d'un atome ou ion. La majeure partie de la thèse consiste en la description des bruits de fond attendus pour la détection des atomes et ions d'antihydrogène. De plus, le système de détection permet de mesurer les sections efficaces pour les réactions symétriques de production d'atomes et d'ions hydrogèene par échange de charge entre protons et positronium. La partie production d’antihydrogène ions de l’expérience a été complètement installée au CERN en 2018. Les premiers tests avec des antiprotons provenant du décélérateur ELENA ont été effectués. Actuellement, l’expérience est testée avec des positrons et des protons, de façon à former des atomes et ions hydrogène. Une optimisation de la production de ces ions de matière aidera à se préparer pour la prochaine période de faisceau d'antiprotons en 2021The main goal of the GBAR collaboration is to measure the Gravitational Behaviour of Antihydrogen at Rest. It is done by measuring the classical free fall of neutral antihydrogen, which is a direct test of the weak equivalence principle for antimatter. The first step of the experiment is to produce the antihydrogen ion and catch it in a Paul trap, where it can be cooled to μK temperature using ground state Raman sideband sympathetic cooling. The μK temperature corresponds to particle velocity in the order of 1 m/s. Once such velocity is reached, the antihydrogen ion can be neutralised and starts to fall. This allows reaching 1 % precision on the measurement of the gravitational acceleration g for antimatter with about 1500 events. Later, it would be possible to reach 10⁻⁵ - 10⁻⁶ precision by measuring the gravitational quantum states of cold antihydrogen. However, in order to measure the free fall, firstly the antihydrogen ion has to be produced. It is formed in the charge exchange reactions between antiproton/antihydrogen and positronium. Positronium and antihydrogen atoms can be either in a ground state or in an excited state. An experimental study of the cross section measurement for these two reactions is described in the presented thesis. The antihydrogen atom and ion production takes place in a cavity. The formation of one antihydrogen ion in one beam crossing requires about 5x10⁶ antiprotons/bunch and a few 10¹¹ Ps/cm⁻³ positronium density inside the cavity, which is produced with a beam containing 5x10¹⁰ positrons per bunch. The production of such intense beams with required properties is a challenging task. First, the development of the positron source is described. The GBAR positron source is based on a 9 MeV linear electron accelerator. The relatively low energy was chosen to avoid activation of the environment. The electron beam is incident on a tungsten target where positrons are created from Bremsstrahlung radiation (gammas) through the pair creation process. Some of the created positrons undergo a further diffusion in the tungsten moderator reducing their energy to about 3 eV. The particles are re-accelerated to about 53 eV energy and are adiabatically transported to the next stage of the experiment. Presently, the measured positron flux is at the level of 6x10⁷ e⁺/s, which is a few times higher than intensities reached with radioactive sources. Then, the thesis features a short description of the antiproton/proton beam preparations, finalised with a chapter about the expected antihydrogen atom and ion production yield. After the reaction, antiproton, antihydrogen atom, and ion beams are guided to the detection system. It is made to allow for detection from 1 to a few thousand antihydrogen atoms, a single antihydrogen ion and all 5x10⁶ antiprotons. It is especially challenging because antiproton annihilation creates a lot of secondary particles which may disturb measurements of single antihydrogen atoms and ions. The main part of the Thesis is the description of the expected background for the antihydrogen atom and ion detection. Additionally, the detection system allows measuring the cross sections for the symmetric reactions of a hydrogen atom and ion production through charge exchange between protons and positronium. The antihydrogen ion production part of the experiment was fully installed at CERN in 2018. The first tests with antiprotons from the ELENA decelerator were done. Currently, the experiment is being commissioned with positrons and protons, in order to perform the hydrogen atom and ion formation. The optimisation of the ion production with matter will help to be fully prepared for the next antiproton beam time in 2021
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Wright, Victoria E. "Ion mobility-mass spectrometry studies of organic and organometallic complexes and reaction monitoring." Thesis, Loughborough University, 2013. https://dspace.lboro.ac.uk/2134/14275.
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Ion mobility (IM) spectrometry is a gas-phase electrophoretic technique in which ions are separated on the basis of their relative mobility in the presence of a weak electric field gradient and a buffer gas. Ion mobility-mass spectrometry (IM-MS) has the capability of separating ions based on m/z, size and shape, providing additional structural information compared to using mass spectrometry on its own. In this thesis, IM-MS has been used to investigate organic and organometallic complexes and identify reactants, intermediates and products in reaction mixtures. Collision cross sections (CCS) have been measured for three salen ligands, and their complexes with copper and zinc using travelling-wave ion mobility-mass spectrometry (TWIMS) and drift tube ion mobility-mass spectrometry (DTIMS), allowing a comparative size evaluation of the ligands and complexes. CCS measurements using TWIMS were determined using peptide and TAAH calibration standards with good intra-day and inter-day reproducibility. TWIMS measurements gave significantly larger CCS than DTIMS derived data in helium, indicating that the choice of calibration standards is important in ensuring the accuracy of TWIMS derived CCS measurements. The CCS data obtained from IM-MS measurements have been compared to CCS values obtained from X-ray coordinates and modelled structures. The analysis of small organic and organometallic molecules has been extended to investigations of the potential of IM-MS for reaction monitoring and structural studies of the components of catalytic cycles. Reaction mixtures of an organocatalysed Diels-Alder cycloaddition reaction have been monitored using IM-MS and high-field asymmetric waveform ion mobility-mass spectrometry (FAIMS-MS). Reactant, product, catalyst and reaction intermediates, including an intermediate not previously detected, were identified and the catalyst and intermediates monitored over time. An organometallic catalytic cycle using a palladium catalyst has been analysed using IM-MS and the CCS of reactants, intermediates and products have been measured and compared to theoretical CCS calculations. Good agreement was observed between measured and calculated data. Species not amenable to electrospray ionisation were covalently bound to an ionisable tag containing a quaternary ammonium ion allowing the tagged molecules to be detected by IM-MS.
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Chai, Zhengwei. "Study of the N to Delta Transition via p({rvec e}, e'{rvec p}){pi}{sup 0} Reaction." Washington, D.C : Oak Ridge, Tenn. : United States. Dept. of Energy. Office of Energy Research ; distributed by the Office of Scientific and Technical Information, U.S. Dept. of Energy, 2003. http://www.osti.gov/servlets/purl/816501-VTYjov/native/.
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Thesis (Ph.D.); Submitted to the Massachusetts Inst. of Tech., Cambridge, MA (US); 1 Oct 2003.Published through the Information Bridge: DOE Scientific and Technical Information. "JLAB-PHY-03-174" "DOE/ER/40150-2571" Zhengwei Chai. 10/01/2003. Report is also available in paper and microfiche from NTIS.
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Horst, Felix Ernst [Verfasser]. "Measurement of Nuclear Reaction Cross Sections for Applications in Radiotherapy with Protons, Helium and Carbon Ions / Felix Ernst Horst." Gießen : Universitätsbibliothek, 2020. http://d-nb.info/1209159503/34.
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Horst, Felix [Verfasser]. "Measurement of Nuclear Reaction Cross Sections for Applications in Radiotherapy with Protons, Helium and Carbon Ions / Felix Ernst Horst." Gießen : Universitätsbibliothek, 2020. http://d-nb.info/1209159503/34.
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Deboer, Richard J. "Measurement of cross sections for 65Cu([alpha],p) 68Zn nuclear reaction at low energy with comparison to Hauser-Feshbach statistical model." Virtual Press, 2005. http://liblink.bsu.edu/uhtbin/catkey/1319221.
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Where did the elements come from? Why are they found in the abundance that they are? These are two of the fundamental questions that the field of astrophysics has sought to answer. The first major studies of elemental synthesis were done in the 1950's and 1960's. Most notable among them was the Burbidge, Burbidge, Fowler, and Hoyle paper [Clayton 73]. This paper set forth the general theory of elemental synthesis in stars and supernovae by means of nuclear reactions. It remains the leading theory for elemental abundance today.As with most theories, the picture of elemental synthesis remains incomplete. While it is thought that the overall theory is correct, there are still many mysteries in the details. There are several kinds of nuclear reactions that occur in stars and supernova that create the elements heavier than iron. They include the r-process, s-process, and p-process, along with several others. However, there are some elements whose creation is not fully understood. There are a variety of reasons for this, which will be discussed.In our experiment we studied the nuclear reaction properties of an isotope of Copper (65Cu). It is theorized that it is produced by the p-process during a supernova explosion. The p-process can be described simply as the collision of an alpha particle with a large atomic nucleus with a proton byproduct. Little actual experimental data has been taken involving the p-process, which is why we chose this reaction. The experiment was done using the Tandem Van de Graaff Accelerator at Ohio University.Department of Physics and Astronomy
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Corn, Philip B. "Measurement of the ⁸Li(d,n)⁹Be and ⁸Li(a,n)¹¹B reaction cross sections at astrophysical energies by radioactive beam techniques /." The Ohio State University, 1989. http://rave.ohiolink.edu/etdc/view?acc_num=osu1487671108308862.
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Powrie, Calum John Young. "A study of the '1'2C(#gamma#,pp) reaction." Thesis, University of Glasgow, 1999. http://ethos.bl.uk/OrderDetails.do?uin=uk.bl.ethos.301509.
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Liatard, Éric. "Mesures de sections efficaces totales de réaction avec des faisceaux d'ions lourds stables et radioactifs par la méthode du rayonnement associé." Grenoble 1, 1989. http://www.theses.fr/1989GRE10143.
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Nous avons mis au point une nouvelle methode de mesure directe de sections efficaces totales de reaction fondee sur l'utilisation d'un detecteur 4 pi modulaire. Dans un premier temps, des mesures ont ete effectuees avec des faisceaux d'ions lourds delivres par les accelerateurs sara et ganil dans la gamme d'energie 30-80 mev/u. Nous avons ensuite adapte notre dispositif aux mesures avec des faisceaux secondaires radioactifs (ligne lise du ganil). Les resultats obtenus couvrent une large gamme de projectiles legers comprenant des isotopes exotiques situes a la limite de la stabilite vis-a-vis de l'emission de neutrons. A partir des sections efficaces totales de reaction, les rayons carres moyens de ces projectiles sont calcules a l'aide d'un formalisme microscopique simple dont la validite est demontree par les resultats obtenus avec des faisceaux stables. Malgre la presence d'effets de structure marques (n pair- n impair), l'ensemble des isotopes etudies presente un rayon carre moyen normal excepte le #1#1be, le #1#4be et le #1#7b. Enfin, en utilisant les resultats de recents calculs haartree-fock, il est possible de determiner, a partir de nos donnees experimentales, les rayons carres moyens des distributions de neutrons des projectiles de n pairs. Ces rayons se comparent favorablement aux valeurs theoriques issues du meme calcul hartree-fock, excepte pour les cas ou l'extension spatiale des neutrons est tres importante (#1#4be et #1#7b)
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Kessedjian, Grégoire. "Mesures de sections efficaces d'actinides mineurs d'intérêt pour la transmutation." Thesis, Bordeaux 1, 2008. http://www.theses.fr/2008BOR13672/document.
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Les réacteurs actuels produisent deux types de déchets dont la gestion et le devenir soulèvent des problèmes. Il s’agit d’abord de certains produits de fission et de noyaux lourds (isotopes de l’Américium et du Curium) au-delà de l’uranium appelés actinides mineurs. Deux options sont envisagées : le stockage en site géologique profond et/ou l’incinération de ces déchets dans un flux de neutrons rapides, c’est-à-dire, la transmutation par fission. Ces études font appel à de nombreuses données neutroniques. Malheureusement, les bases de données présentent encore de nombreuses insuffisances pour parvenir à des résultats fiables. L’objectif de ce travail est ici d’actualiser des données nucléaires et de les compléter. Nous avons ainsi mesuré la section efficace de fission de l’243Am (7370 ans) en référence à la diffusion élastique (n,p) afin de fournir des données indépendantes des mesures existantes dans la gamme des neutrons rapides (1 - 8 MeV). La réaction 243Am(n,f) a été analysée en utilisant un modèle statistique décrivant les voies de désexcitation du noyau composé d’244Am. Ainsi les sections efficaces de capture radiative (n,?) et de diffusion inélastique (n,n’) ont pu être évaluées. La mesure directe des sections efficaces neutroniques d’actinides mineurs constitue très souvent un véritable défi compte tenu de la forte activité des actinides mineurs. Pour cela, une méthode indirecte a été développée utilisant les réactions de transfert dans le but d’étudier certains isotopes du curium. Les réactions 243Am(3He,d)244Cm, 243Am(3He,t)243Cm et 243Am(3He,alpha)242Am nous ont permis de mesurer les probabilités de fission des noyaux de 243,244Cm et de l’242Am. Les sections efficaces de fission des curiums 242,243Cm(162,9 j, 28,5 ans) et de l’américium 241Am sont obtenues en multipliant ces probabilités par les sections efficaces calculées de formation des noyaux composés. Pour chaque mesure, une évaluation précise des erreurs a été réalisée à travers une étude des variances-covariances des résultats présentés. Pour les mesures de la réaction 243Am(n,f), une analyse des corrélations d’erreurs a permis d’interpréter la portée de ces mesures au sein des mesures existantesThe existing reactors produce two kinds of nuclear waste : the fission products and heavy nuclei beyond uranium called minor actinides (Americium and Curium isotopes). Two options are considered: storage in deep geological site and/or transmutation by fast neutron induced fission. These studies involve many neutron data. Unfortunately, these data bases have still many shortcomings to achieve reliable results. The aim of these measurements is to update nuclear data and complement them. We have measured the fission cross section of 243Am (7370y) in reference to the (n,p) elastic scattering to provide new data in a range of fast neutrons (1 - 8 MeV). A statistical model has been developed to describe the reaction 243Am(n,f). Moreover, the cross sections from the following reactions have been be extracted from these calculations: inelastic scattering 243Am(n,n’) and radiative capture 243Am(n,?) cross sections. The direct measurements of neutron cross sections are often a challenge considering the short half-lives of minor actinides. To overcome this problem, a surrogate method using transfer reactions has been used to study few isotopes of curium. The reactions 243Am(3He, d)244cm, 243Am(3He, t)243cm and 243Am(3He, alpha)242Am allowed to measure the fission probabilities of 243,244Cm and 242Am. The fission cross sections of 242,243Cm(162,9d, 28,5y) and 241Am(431y) have been obtained by multiplying these fission probabilities by the calculated compound nuclear neutron cross section relative to each channel. For each measurement, an accurate assessment of the errors was realized through variance-covariance studies. For measurements of the reaction 243Am(n,f), the analysis of error correlations allowed to interpret the scope of these measures within the existing measurements
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Lamirand, Vincent. "Détermination de sections efficaces pour la production de champs neutroniques monoénergétiques de basse énergie." Phd thesis, Université de Grenoble, 2011. http://tel.archives-ouvertes.fr/tel-00683170.
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La réponse d'un détecteur de neutrons varie avec l'énergie du neutron incident. La détermination expérimentale de cette variation se réalise au moyen de champs neutroniques monoénergétiques. Ceux-ci sont produits par l'interaction entre un faisceau d'ions accélérés et une cible fine constituée d'un dépôt réactif sur un support métallique. En utilisant différentes réactions telles que 7Li(p,n), 3H(p,n), 2H(d,n) et 3H(d,n), il est possible de produire des neutrons entre 120 keV et 20 MeV dans la direction du faisceau incident (0°).Pour atteindre des énergies inférieures, il est possible d'augmenter l'angle du point de mesure par rapport à la direction du faisceau d'ions. Cependant, cette méthode présente des problèmes d'homogénéité en énergie et en fluence des neutrons à la surface du détecteur, ainsi qu'une augmentation de la proportion de neutrons diffusés. Une alternative est l'utilisation d'autres réactions nucléaires, notamment la réaction 45Sc(p,n) qui permet de descendre jusqu'à des énergies de 8 keV à 0°.Une étude complète de cette réaction et de sa section efficace a été menée au sein d'une coopération scientifique entre le laboratoire de métrologie et de dosimétrie des neutrons (LMDN) de l'IRSN, deux instituts de métrologie européens, le NPL (National Physical Laboratory, RU) et le PTB (Physikalisch-Technische Bundesanstalt, All), et l'IRMM (Institute for Reference Materials and Measurements, CEE). Parallèlement, d'autres réactions envisageables ont été étudiées : 65Cu(p,n), 51V(p,n), 57Fe(p,n), 49Ti(p,n), 53Cr(p,n) et 37Cl(p,n). Elles ont été comparées en termes d'émission neutronique et d'énergie minimale des neutrons produits.
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Boutoux, Guillaume. "Sections efficaces neutroniques via la méthode de substitution." Phd thesis, Bordeaux 1, 2011. http://tel.archives-ouvertes.fr/tel-00654677.
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Les sections efficaces neutroniques des noyaux de courte durée de vie sont des données cruciales pour la physique fondamentale et appliquée dans des domaines tels que la physique des réacteurs ou l'astrophysique nucléaire. En général, l'extrême radioactivité de ces noyaux ne nous permet pas de procéder à des mesures induites par neutrons. Cependant, il existe une méthode de substitution (" surrogate " dans la littérature) qui permet de déterminer ces sections efficaces neutroniques par l'intermédiaire de réactions de transfert ou de réactions de diffusion inélastique. Son intérêt principal est de pouvoir utiliser des cibles moins radioactives et ainsi d'accéder à des sections efficaces neutroniques qui ne pourraient pas être mesurées directement. La méthode est basée sur l'hypothèse de formation d'un noyau composé et sur le fait que la désexcitation ne dépend essentiellement que de l'énergie d'excitation et du spin et parité de l'état composé peuplé. Toutefois, les distributions de moments angulaires et parités peuplés dans des réactions de transfert et celles induites par neutrons sont susceptibles d'être différentes. Ce travail fait l'état de l'art sur la méthode substitution et sa validité. En général, la méthode de substitution fonctionne très bien pour extraire des sections efficaces de fission. Par contre, la méthode de substitution dédiée à la capture radiative est mise à mal par la comparaison aux réactions induites par neutrons. Nous avons réalisé une expérience afin de déterminer les probabilités de désexcitation gamma du 176Lu et du 173Yb à partir des réactions de substitution 174Yb(3He,p)176Lu* et 174Yb(3He,alpha)173Yb*, respectivement, et nous les avons comparées avec les probabilités de capture radiative correspondantes aux réactions 175Lu(n,gamma) et 172Yb(n,gamma) qui sont bien connues. Cette expérience a permis de comprendre pourquoi, dans le cas de la désexcitation gamma, la méthode de substitution donne des écarts importants par rapport à la réaction neutronique correspondante. Ce travail dans la région de terres rares a permis d'évaluer dans quelle mesure la méthode de substitution peut s'appliquer pour extraire des probabilités de capture dans la région des actinides. Des expériences précédentes sur la fission ont aussi pu être réinterprétées. Ce travail apporte donc un éclairage nouveau sur la méthode de substitution.
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Hermes, Jan Philipp [Verfasser]. "Geant4 simulation of a time-of-flight spectrometer for measurements of nuclear cross sections relevant to particle therapy and development of a reconstruction algorithm for the identification of reaction products / Jan Philipp Hermes." Aachen : Hochschulbibliothek der Rheinisch-Westfälischen Technischen Hochschule Aachen, 2013. http://d-nb.info/1047324997/34.
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Rvachev, Marat. "Study of the Quasielastic {sup 3}He(e,e{prime}p) Reaction at Q{sup 2}=1.5 (GeV/c){sup 2} up to Missing Momenta of 1 GeV/c." Washington, D.C : Oak Ridge, Tenn. : United States. Dept. of Energy. Office of Energy Research ; distributed by the Office of Scientific and Technical Information, U.S. Dept. of Energy, 2003. http://www.osti.gov/servlets/purl/824894-w3sMWi/native/.
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Thesis (Ph.D.); Submitted to Massachusetts Inst. of Tech., Cambridge, MA (US); 1 Sep 2003.Published through the Information Bridge: DOE Scientific and Technical Information. "JLAB-PHY-03-167" "DOE/ER/40150-2745" Marat Rvachev. 09/01/2003. Report is also available in paper and microfiche from NTIS.
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Uemura, Sho. "Differential cross section measurement for the d(n,np) reaction." Thesis, Massachusetts Institute of Technology, 2010. http://hdl.handle.net/1721.1/61004.
Full textAbstract:
Thesis (S.B.)--Massachusetts Institute of Technology, Dept. of Physics, 2010.This electronic version was submitted by the student author. The certified thesis is available in the Institute Archives and Special Collections.
Cataloged from student-submitted PDF version of thesis.
Includes bibliographical references (p. 83-84).
The differential cross section for the quasielastic d(n,np) neutron-induced deuteron breakup reaction was measured as a function of incident and scattered particle energies and angles, using a liquid deuterium target at the Weapons Neutron Research (WNR) spallation neutron beam at the Los Alamos Neutron Science Center at the Los Alamos National Laboratory. Cross sections were computed for the incident neutron energy ranges of 10010, 20010, and 30010 MeV. We used proton detectors covering a range of = 17 - 25 in the lab frame, and neutron detectors covering a range of = 55 - 76 in the lab frame. Experiment setup and data analysis are discussed, and preliminary results are presented for the cross section.
by Sho Uemura.
S.B.
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Chadwick, Helen J. "Angular momentum polarisation effects in inelastic scattering." Thesis, University of Oxford, 2012. http://ora.ox.ac.uk/objects/uuid:474b04fa-4f50-4618-88ab-c85878723f2a.
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In this thesis, a joint experimental and theoretical investigation of the vector properties that describe the inelastic scattering of a diatomic radical with an atomic collision partner is presented. A particular emphasis is placed on those correlations that include the final rotational angular momentum, j', of the radical. The depolarisation of both NO(A) and OH(A) brought about through collisions with krypton has been studied, providing a measure of the j-j' correlation, where j is the initial rotational angular momentum associated with the diatom. The total depolarisation cross- sections for both collisional disorientation and disalignment have been measured using quantum beat spectroscopy, and modelled theoretically using quasi-classical trajectory (QCT) calculations. The agreement between experiment and theory for NO(A)-Kr is excellent, but is not observed for OH(A)-Kr under thermal conditions. This has been attributed to the importance of electronic quenching in OH(A)-Kr. The depolarisation cross-sections have also been determined at a higher collision energy for OH(A)-Kr where electronic quenching is less significant, and the experimental results are in better agreement with those obtained theoretically. The NO(A)-Kr depolarisation cross-sections fall with increasing rotational quantum number, N, whereas for OH(A)-Kr, they exhibit less of an N dependence. This trend is mirrored in the elastic depolarisation cross-sections, which have also been determined experimentally for OH(A)-Kr. The significantly attractive and anisotropic nature of the OH(A)-Kr potential energy surface (PES) accounts for these observations. The j-j' correlation is extended to include the initial (relative) velocity (k) in a new theoretical treatment of the k-j-j' correlation. The formalism developed is used with the results from the QCT calculations for NO(A)-Kr and OH(A)-Kr to provide further insight into the mechanism of depolarisation in the two systems. Collisions of NO(A) with krypton do not cause significant depolarisation due to their impulsive nature, and the projection of j onto the kinematic apse is conserved. In contrast, collisions of OH(A) with krypton effectively randomise the direction of j, again showing the influence of the anisotropic and attractive nature of the PES. However, the projection of j onto the kinematic apse is still conserved. The inelastic scattering of NO(X) with argon and krypton has also been investigated, using a crossed molecular beam apparatus. The initial Λ-doublet state of the NO(X) was selected using hexapole focussing, and the products of the collision detected using velocity mapped ion imaging. The state to state differential cross-sections (equivalent to the k-k' correlation, where k' is the final relative velocity) have been measured for collisions which conserve the initial spin-orbit level of the NO(X) with krypton. The same parity dependent effects were seen as have been observed previously for NO(X)-Ar. The collision induced alignment (equivalent to the k-k'-j' correlation) of NO(X) as a result of scattering with argon has also been determined experimentally. The results can be explained classically by considering the conservation of the projection of j onto the kinematic apse.
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Ducasse, Quentin. "Etude de la méthode de substitution à partir de la mesure simultanée des probabilités de fission et d'émission gamma des actinides 236U, 238U, 237Np et 238Np." Thesis, Bordeaux, 2015. http://www.theses.fr/2015BORD0109/document.
Full textAbstract:
Les sections efficaces induites par neutrons des noyaux de courte durée de vie jouent un rôle important dans des domaines variés parmi la physique fondamentale, l'astrophysique ou l'énergie nucléaire. Malheureusement de nombreuses contraintes liées à la radiotoxicité des cibles rendent la mesure de ces sections efficaces souvent très difficiles. La méthode de substitution est une technique de mesure indirecte de sections efficaces neutroniques de noyaux radioactifs qui à l'avantage de s'affranchir de ces contraintes. Pour la première fois dans ce type d'expérience,les probabilités de fission et d'émission gamma sont mesurées simultanément, pour les actinides236U, 238U, 237Np et 238Np dans le but d'étudier la validité de la méthode. Une des difficultés provient de la soustraction des gammas des fragments de fission et cette mesure constitue en cela un véritable défi. Cette expérience de mesure simultanée a été effectuée au cyclotron d'Oslo.A une énergie d'excitation fixée du noyau formé, les résultats montrent que les probabilités de fission de substitution sont en bon accord avec celles induites par neutron alors que les probabilités d'émission gamma mesurées sont plusieurs fois plus élevées. Ces écarts sont liés à la différence distribution spin peuplée par le noyau entre les deux méthodes. Des calculs de modèles statistiques avec des paramètres standards n'ont pas permis de reproduire cette insensibilité de la probabilité de fission vis à vis du spin du noyau. La reproduction des observations expérimentales devient possible en considérant un moment d'inertie du noyau fissionnant qui augmente plus rapidement avec la déformation du noyau que ne le préconisent les paramètres standards. De nouveaux efforts théoriques sont à fournir pour améliorer la compréhension de nos résultatsNeutron-induced cross sections of short-lived nuclei are important in various fields such as fundamental physics, astrophysics or nuclear energy. However, these cross sections are often extremely difficult to measure due to high radioactivity of the targets involved. The surrogate-reaction method is an indirect way to determine neutron-induced cross sections of short-lived nuclei. In order to study the validity of the method, we have measured for the very first time in a surrogate-reaction experiment simultaneously fission and gamma-decay probabilities for the actinides 236U, 238U, 237Np and 238Np. This is challenging because one has to remove the gamma rays emitted by the fission fragments. The measurement was performed at the Oslocyclotron.Our results show that for a given excitation energy, our gamma-decay probabilities are several times higher than neutron-induced probabilities, which can be attributed to differences in spin distribution between the two types of reactions. On the other hand, our fission probabilities are in good agreement with neutron-induced data. Statistical-model calculations applied with standardparameters cannot reproduce the weak spin sensibility to variations of the angular momentum observed for the fission probabilities. However, it is possible to reproduce the experimental observations by considering a stronger increase of the moment of inertia of the fissionning nucleus with deformation. Further theoretical efforts are needed to improve the understanding of our results
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Barthel, Robert. "Growth of unsaturated, cyclic, and polycyclic aromatic hydrocarbons: Reactions under the conditions of the interstellar medium." Doctoral thesis, Saechsische Landesbibliothek- Staats- und Universitaetsbibliothek Dresden, 2009. http://nbn-resolving.de/urn:nbn:de:bsz:14-ds-1238024025498-21465.
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Hydrocarbons, in particular polycyclic aromatic hydrocarbons (PAHs), have been long discussed to be carriers of interstellar infrared (IR) emission and ultraviolet (UV) absorption features. Yet, their origin in dense phases of the interstellar medium (ISM), such as molecular clouds, remains unclear. In this work, growth mechanisms based on ion-molecule reactions between cationic PAHs/hydrocarbons and methyne (CH) were investigated. The reaction type and the precursor were derived and selected from known chemical and physical properties of the ISM. These chemical reactions were characterised by calculating branching ratios (based on cross sections) and capture rate coefficients, minimum reaction paths, reaction enthalpies, thermal equilibrium constants, and microcanonic isomerisation and radiative deactivation rate coefficients. In order to cope with the variety of reaction parameters, a hierarchic workflow scheme was set up. First, the reaction potential energy surface was sampled by molecular dynamics simulations. Then, minimum energy paths of the most probable reaction channels were investigated. Finally, molecular and kinetic properties of stationary points were calculated. The quantum chemical level of theory was increased at each step from DFTB (tight-binding density-functional), to DFT, and finally to post-Hartree-Fock methods. Results on CH based hydrocarbon growth showed the transition from non-cyclic hydrocarbons to cyclic and aromatic structures and from cyclic to polycyclic aromatic hydrocarbons. Additionally, the reactive collisions between hydrocarbons and CH were found to produce sufficient energy for isomerisation and fragmentation processes even at ultra low temperatures. In all, the results indicate that methyne might be a proper precursor for the formation of large interstellar PAHsKohlenwasserstoffe, insbesondere polyzyklische Kohlenwasserstoffe (engl. PAHs), werden seit einigen Jahren als Mitverursacher interstellar IR-Emissions- und UV-Absorptionsbanden angesehen und diskutiert. Dabei ist die Herkunft dieser Moleküle in den dichten Phasen des interstellaren Mediums (ISM) aber noch nicht aufgeklärt. In dieser Arbeit wurden daher die Bildungsmechanismen, welche auf Ion-Molekül-Reaktionen zwischen kationischen PAHs und Kohlenwasserstoffen und dem Molekül CH beruhen, untersucht. Sowohl der Reaktionstyp als auch der Präkursor wurden anhand von bekannten physikalischen und chemischen Eigenschaften des ISM abgeleitet und ausgewählt. Die Analyse der chemischen Reaktionen basierte auf Berechnungen zur Produktzusammensetzung und Einfangsratenkoeffizienten (welche wiederum aus berechneten Reaktionsquerschnitten hervorgingen) Minimumenergiepfade (MEP), Reaktionsenthalpien, thermische Gleichgewichtskonstanten und mikrokanonische Isomerisierungs- und Strahlungsdeaktivierungs-Ratenkoeffizienten. Um der Vielzahl an Reaktionsparameter gerecht zu werden, wurden die Berechnungsmethoden entsprechend eines hierarischen Fließschemas kombiniert. Hierzu wurden zuerst durch Molekulardynamik-Simulationen die Reaktionspotentialenergieflächen abgerastert. Auf der nächsten Stufe wurden statistisch bedeutsame Reaktionskanäle bezüglich ihrer Minimumenergiepfade untersucht. Den Abschluss bildete die Berechnung molekularer und kinetischer Charakteristika stationärer Punkte auf einem MEP. Entsprechend dieses Schemas wurde die quantenchemische Genauigkeit auf jeder Stufe von approximativer DFT über DFT zu post-Hartree-Fock verändert. Die Ergebnisse des CH-basierten Kohlenwasserstoffwachstums zeigten einen Übergang von nichtzyklischen zu zyklischen and aromatischen Strukturen, sowie von zyklischen zu polyzyklischen Kohlenwasserstoffen. Außerdem zeigte sich, dass reaktive Kollisionen zwischen Kohlenwasserstoffen und CH auch bei Tiefsttemperaturen immer ausreichend Energie für Isomerisierungs- und Fragmentationsprozesse liefert. Die Ergebnisse dieser Arbeit lassen den Schluss zu, dass CH ein geeigneter Präkursor für die Bildung großer interstellarer PAH ist
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VIEIRA, de MORAES MARCO A. P. "Reacoes fotonucleares induzidas por radiacao gama de captura de neutrons, nos nucleos de U-233 e Pu-239, junto ao limiar." reponame:Repositório Institucional do IPEN, 1990. http://repositorio.ipen.br:8080/xmlui/handle/123456789/10226.
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Tese (Doutoramento)
IPEN/T
Instituto de Pesquisas Energeticas e Nucleares - IPEN/CNEN-SP
29
Barthel, Robert. "Growth of unsaturated, cyclic, and polycyclic aromatic hydrocarbons: Reactions under the conditions of the interstellar medium." Doctoral thesis, Technische Universität Dresden, 2008. https://tud.qucosa.de/id/qucosa%3A23589.
Full textAbstract:
Hydrocarbons, in particular polycyclic aromatic hydrocarbons (PAHs), have been long discussed to be carriers of interstellar infrared (IR) emission and ultraviolet (UV) absorption features. Yet, their origin in dense phases of the interstellar medium (ISM), such as molecular clouds, remains unclear. In this work, growth mechanisms based on ion-molecule reactions between cationic PAHs/hydrocarbons and methyne (CH) were investigated. The reaction type and the precursor were derived and selected from known chemical and physical properties of the ISM. These chemical reactions were characterised by calculating branching ratios (based on cross sections) and capture rate coefficients, minimum reaction paths, reaction enthalpies, thermal equilibrium constants, and microcanonic isomerisation and radiative deactivation rate coefficients. In order to cope with the variety of reaction parameters, a hierarchic workflow scheme was set up. First, the reaction potential energy surface was sampled by molecular dynamics simulations. Then, minimum energy paths of the most probable reaction channels were investigated. Finally, molecular and kinetic properties of stationary points were calculated. The quantum chemical level of theory was increased at each step from DFTB (tight-binding density-functional), to DFT, and finally to post-Hartree-Fock methods. Results on CH based hydrocarbon growth showed the transition from non-cyclic hydrocarbons to cyclic and aromatic structures and from cyclic to polycyclic aromatic hydrocarbons. Additionally, the reactive collisions between hydrocarbons and CH were found to produce sufficient energy for isomerisation and fragmentation processes even at ultra low temperatures. In all, the results indicate that methyne might be a proper precursor for the formation of large interstellar PAHs.Kohlenwasserstoffe, insbesondere polyzyklische Kohlenwasserstoffe (engl. PAHs), werden seit einigen Jahren als Mitverursacher interstellar IR-Emissions- und UV-Absorptionsbanden angesehen und diskutiert. Dabei ist die Herkunft dieser Moleküle in den dichten Phasen des interstellaren Mediums (ISM) aber noch nicht aufgeklärt. In dieser Arbeit wurden daher die Bildungsmechanismen, welche auf Ion-Molekül-Reaktionen zwischen kationischen PAHs und Kohlenwasserstoffen und dem Molekül CH beruhen, untersucht. Sowohl der Reaktionstyp als auch der Präkursor wurden anhand von bekannten physikalischen und chemischen Eigenschaften des ISM abgeleitet und ausgewählt. Die Analyse der chemischen Reaktionen basierte auf Berechnungen zur Produktzusammensetzung und Einfangsratenkoeffizienten (welche wiederum aus berechneten Reaktionsquerschnitten hervorgingen) Minimumenergiepfade (MEP), Reaktionsenthalpien, thermische Gleichgewichtskonstanten und mikrokanonische Isomerisierungs- und Strahlungsdeaktivierungs-Ratenkoeffizienten. Um der Vielzahl an Reaktionsparameter gerecht zu werden, wurden die Berechnungsmethoden entsprechend eines hierarischen Fließschemas kombiniert. Hierzu wurden zuerst durch Molekulardynamik-Simulationen die Reaktionspotentialenergieflächen abgerastert. Auf der nächsten Stufe wurden statistisch bedeutsame Reaktionskanäle bezüglich ihrer Minimumenergiepfade untersucht. Den Abschluss bildete die Berechnung molekularer und kinetischer Charakteristika stationärer Punkte auf einem MEP. Entsprechend dieses Schemas wurde die quantenchemische Genauigkeit auf jeder Stufe von approximativer DFT über DFT zu post-Hartree-Fock verändert. Die Ergebnisse des CH-basierten Kohlenwasserstoffwachstums zeigten einen Übergang von nichtzyklischen zu zyklischen and aromatischen Strukturen, sowie von zyklischen zu polyzyklischen Kohlenwasserstoffen. Außerdem zeigte sich, dass reaktive Kollisionen zwischen Kohlenwasserstoffen und CH auch bei Tiefsttemperaturen immer ausreichend Energie für Isomerisierungs- und Fragmentationsprozesse liefert. Die Ergebnisse dieser Arbeit lassen den Schluss zu, dass CH ein geeigneter Präkursor für die Bildung großer interstellarer PAH ist.
30
Keller, Steven Ede. "Flux-limited Diffusion Coefficient Applied to Reactor Analysis." Diss., Georgia Institute of Technology, 2007. http://hdl.handle.net/1853/16126.
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A new definition of the diffusion coefficient for use in reactor physics calculations is evaluated in this thesis. It is based on naturally flux-limited diffusion theory (FDT), sometimes referred to as Levermore-Pomraning diffusion theory. Another diffusion coefficient more loosely based on FDT is also evaluated in this thesis. Flux-limited diffusion theory adheres to the physical principle of flux-limiting, which is that the magnitude of neutron current is not allowed to exceed the scalar flux. Because the diffusion coefficients currently used in the nuclear industry are not flux-limited they may violate this principle in regions of large spatial gradients, and because they encompass other assumptions, they are only accurate when used in the types of calculations for which they were intended.
The evaluations were performed using fine-mesh diffusion theory. They are in one spatial dimension and in 47, 4, and 2 energy groups, and were compared against a transport theory benchmark using equivalent energy structures and spatial discretization.
The results show that the flux-limited diffusion coefficient (FD) outperforms the standard diffusion coefficient in calculations of single assemblies with vacuum boundaries, according to flux- and eigenvalue-errors. In single assemblies with reflective boundary conditions, the FD yielded smaller improvements, and tended to improve only the fast-group results. The results also computationally confirm that the FD adheres to flux-limiting, while the standard diffusion coefficient does not.
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Scott, David Andrew. "Underground study of the 17 O(p,γ )18F reaction at Gamow energies for classical novae." Thesis, University of Edinburgh, 2014. http://hdl.handle.net/1842/9697.
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Classical novae are explained as thermonuclear explosions on the surface of white dwarf stars accreting hydrogen-rich material from less evolved companions in binary star systems. These events occur frequently within our galaxy and have been proposed as significant contributors to the galactic abundance of 13C, 15N, 17/18O and 18/19F. The short-lived isotope 18F (t1/2 = 110 min) is of particular importance since it may provide a signature of novae events through the detection of 511 keVγ-ray emission following the β+ decay of a 18F nucleus. During classical novae the 17O(p,γ)18F reaction governs the production of 18F and affects the synthesis of the rare isotopes mentioned above. Prior to the present study, the 17O(p,γ)18F reaction rate was poorly determined owing to a lack of low-energy experimental data. The present work reports on the first accurate measurements of the resonant and non-resonant contributions to the 17O(p,γ)18F reaction cross section in the energy region relevant for classical novae. Measurements were performed at the Laboratory for Underground Nuclear Astrophysics (LUNA) accelerator facility of the Laboratori Nazionali del Gran Sasso (LNGS) in Italy. Here the γ-ray background is suppressed by up to 3 orders of magnitude, thus providing a unique environment for low-energy measurements of reaction cross sections. Prompt γ rays associated with the formation and decay of states in 18F were analysed to determine the resonant and non-resonant contributions to the reaction cross section. The total non-resonant S-factor was determined at energies between Ecm ≈ 200 - 370 keV and the strength of a key resonance at Ecm = 183 keV was obtained with the best precision to date. The uncertainty in the reaction rate is now sufficiently low to place firmer constraints on nucleosynthesis predictions from accurate models of novae.
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De, Dominicis Lucia. "Proton-induced cross sections on V-nat target: focus on Sc-47 production." Master's thesis, Alma Mater Studiorum - Università di Bologna, 2019. http://amslaurea.unibo.it/18777/.
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Il gruppo NUCL-EX si interessa a misure di sezioni d’urto di produzione di isotopi instabili selezionati, presso i Laboratori Nazionali di Legnaro appartenenti all'Istituto Nazionale di Fisica Nucleare (INFN-LNL). Poiché il progetto SPES, il futuro dei LNL, è attualmente in fase di costruzione, si è creata una collaborazione con il gruppo LARAMED, operante nel campo della produzione di radionuclidi con applicazione medicale. In particolare, questa tesi è incentrata sull'analisi dei dati sperimentali nell'ambito delle misure di sezioni d’urto, indotte da protoni, di interesse si in fisica nucleare che interdisciplinare. Il lavoro realizzato e presentato in questa tesi rientra nel contesto del progetto, il cui scopo è lo studio della produzione dello Sc-47 e dei suoi contaminanti, tutti prodotti mediante reazioni nucleari indotte da un fascio di protoni, di energia variabile, su un bersaglio di V-nat. L’interesse nello Sc-47 è motivato dalla sua promettente applicazione in campo medico, in particolare nella teragnostica, un nuovo approccio alla medicina che sfrutta le radiazioni emesse (γ e β-) sia per la terapia che per la diagnosi, indirizzata alla cura dei tumori. Dato che per tali applicazioni è richiesto un livello di purezza elevato per lo Sc-47 prodotto, in questo lavoro sono state calcolate (e sono presentate) anche le sezioni d’urto di produzione di tutti i radionuclidi contaminanti. Tra essi il più problematico è lo Sc-46 dato che, essendo un altro isotopo dello scandio, non può essere separato chimicamente e, poiché la sua vita media è più lunga di quella dello Sc-47, non è possibile aspettare che decada. Lo scopo di questa tesi è di trovare un intervallo di energia, se possibile, in cui lo Sc-47 ha una un valore di sezione d’urto più alto di quello che si ha per lo Sc-46. Tale intervallo potrebbe essere sfruttato per produrre Sc-47 sufficientemente puro da poter essere utilizzato in futuri studi preclinici che ne testino l'efficacia terapeutica.
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Orme, Wesley John. "Cross sections used to elucidate differences in wavelet transforms of ground force reactions." [Boise, Idaho] : Boise State University, 2009. http://scholarworks.boisestate.edu/td/70/.
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Saayman, Jean. "Combined hydrodynamic and reaction analysis of a bubbling to turbulent Fluidized Bed Reactor." Thesis, University of Pretoria, 2013. http://hdl.handle.net/2263/40221.
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There are many large-scale contacting methods for gas reactions requiring a solid catalyst. The catalytic gas-solid Fluidized Bed Reactor (FBR) is one of the popular methods in industry. In FBRs the bulk of the gas throughput is present as lean bubbles, mostly deprived of solids, bubbling through a solids-rich emulsion phase. The movement of gas into and out of the emulsion often dictates the performance of an FBR. During the past five decades major contributions have been made towards the understanding of FBRs, although numerous gaps still exist, especially at higher bubbling regime velocities.
This work follows an integrated approach for the simultaneous measurement of hydrodynamics and reactor performance. Hydrodynamics are measured using fast X-Ray Tomography (XRT), pressure analysis techniques and an optical fibre probe. Reactor performance is measured by utilizing the ozone decomposition reaction. Performance is quantified using a basic two-phase reactor model with an apparent overall interphase mass transfer (K0) parameter. Two 14 cm (ID) fluidized bed columns are used, one setup supporting the ozone decomposition reaction and the other installed within a fast XRT facility. Special emphasis is placed on superficial velocities (U0) spanning the entire bubbling regime up to the onset of the turbulent regime (Uc). The particle types employed are Geldart B sand particles and highly dense ferro-silicon (FeSi) particles. Fines are added to both particle types, resulting in a total of four particle systems (sand baseline; sand with fines; FeSi baseline; FeSi with fines). Time constraints on the XRT equipment limited the tomography measurements to the sand baseline particle system. The hydrodynamics of the
other particle systems were limited to the pressure signal and optical probe measurements of the ozone decomposition setup.
The results of the sand baseline system suggest that a distinction should be made between the low-interaction bubbling regime and the high-interaction bubbling regime. A change in mass transfer behaviour occurs around a U0/Uc value of 0.25. Reactor performance increases up to U0/Uc = 0.7, after which a decreasing trend is observed. An empirical correlation is proposed for the specific interphase mass transfer (kbe) of the higher velocity bubbling regime. This correlation is based on the integration of the hydrodynamics determined by means of XRT and reactor performance:
4-12
The hydrodynamic parameter β gives the best fit for the entire velocity range with an average error of 8%, although it is not recommended for U0/Uc<0.17. It is observed that the classical approach of penetration theory for interphase mass transfer, performs exceptionally well at low velocities (U0/Uc<0.34).
The addition of fines to the FeSi particle type decreases the overall reactor performance, despite decreased bubble sizes. The solids fraction, however, unexpectedly increases with the addition of fines and a collapse of the emulsion phase is measured. It is therefore postulated that though flow in the emulsion phase is much higher for the FeSi baseline system and decreases with the addition of fines. For the sand particle type, the behaviour expected from literature is observed: reactor performance increases, bubble sizes decrease and the solids fraction decreases.
Very distinct hydrodynamic behaviour is observed for all the fluidization regimes with XRT. Probability density distributions show there are still two phases present in the turbulent regime and that the emulsion-phase solids fraction remains independent of velocity until fast fluidization sets in. The turbulent regime has unique hydrodynamic behaviour, although voids appear to be a transient structure between the structures of the bubbling and fast fluidization regimes.Thesis (PhD)--University of Pretoria, 2013.
gm2014
Chemical Engineering
unrestricted
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SEMMLER, RENATO. "Medidas das secções de choque de fotonêutrons do sup(9)Be, sup(13)Ce sup(17)O com radiação gama de captura de neutrons térmicos." reponame:Repositório Institucional do IPEN, 2006. http://repositorio.ipen.br:8080/xmlui/handle/123456789/11421.
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Tese (Doutoramento)
IPEN/T
Instituto de Pesquisas Energeticas e Nucleares - IPEN/CNEN-SP
36
Auce, Agris. "Reaction Cross Section Measurements for p,d,3He and 4He at Intermediate Energies." Doctoral thesis, Uppsala universitet, Institutionen för kärn- och partikelfysik, 2004. http://urn.kb.se/resolve?urn=urn:nbn:se:uu:diva-4633.
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Reaction cross sections were measured for protons at 65.5 MeV, for deuterons at 37.8, 65.5, 97.4 MeV, for 3He at 96.4, 137.8, 167.3 MeV, and for 4He at 69.6, 117.2, 163.9 and 192.4 MeV. Targets were 9Be, 12C, 16O, 28Si, 40,48Ca, 58,60Ni, 112,116,118,120,124Sn and 208Pb. 48Ca and 118Sn targets were used only for some of the measurements. Rest of the targets have been measured for all energies and projectiles but 4He at 69.6 MeV where reaction cross sections were measured for 9Be, 12C, 16O, 28Si, 40Ca targets. A modification of a standard attenuation technique was used. Details of the experimental design are presented. Experimental uncertainties were 2-3% for p, 3% for d and 3-10% for 3,4He. A strong forward peaking of the reaction products was observed for 3,4He. Therefore the standard reaction cross section measurement technique was not applicable for these projectiles. The forward peaking is also responsible for the increase of experimental uncertainties for these projectiles. The forward peaking of the reaction products is not known for other projectiles and has also not been observed with 3,4He at different - both higher and lower - energies. Possible explanations for this phenomenon are discussed. Optical model calculations of the reaction cross sections are in good agreement with the measured values. The measurements were performed with beams from the Gustav Werner cyclotron at the The Svedberg Laboratory, Uppsala.
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Candalino, Robert Wilcox. "Engineering analysis of low enriched uranium fuel using improved zirconium hydride cross sections." Texas A&M University, 2006. http://hdl.handle.net/1969.1/4347.
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A neutronic and thermal hydraulic analysis of the 1-MW TRIGA research reactor
at the Texas A&M University Nuclear Science Center using a new low enriched uranium
fuel (named 30/20 fuel) was completed. This analysis provides safety assessment for the
change out of the existing high enriched uranium fuel to this high-burnup, low enriched
uranium fuel design. The codes MCNP and Monteburns were utilized for the neutronic
analysis while the code PARET was used to determine fuel and cladding temperatures.
All of these simulations used improved zirconium hydride cross sections that were
provided by Dr. Ayman Hawari at North Carolina State University. The neutronic and
thermal analysis showed that the reactor will operate with approximately the same fuel
lifetime as the current high enriched uranium fuel and stay within the thermal and safety
limits for the facility. It was also determined that the control rod worths and the
temperature coefficient of reactivity would provide sufficient negative reactivity to
control the reactor during the fuelâÂÂs complete lifetime.
An assessment of the fuelâÂÂs viability for use with the Advanced Fuel Cycle
InitiativeâÂÂs Reactor Accelerator Coupling Experiments program was also performed.
The objective of this study was to confirm the continued viability of these experiments with the reactor operating using this new fuel. For these experiments, the accelerator
driven system must produce fission heating in excess of 1 kW when driven by a 20 kW
accelerator system. This criterion was met using the new fuel. Therefore the change out
of the fuel will not affect the viability of these experiments.
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Street, A. M. "Methods for the calculation of cross-sections of interest to nuclear reactor design." Thesis, University of Oxford, 1987. http://ethos.bl.uk/OrderDetails.do?uin=uk.bl.ethos.379981.
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Salter, Philip James Charles. "Time-reversed measurement of the 18Ne(α,p)21Na cross-section for Type I X-ray bursts." Thesis, University of Edinburgh, 2012. http://hdl.handle.net/1842/6239.
Full textAbstract:
Type I X-ray bursts (XRB) are highly energetic and explosive astrophysical events, observed as very sudden and intense emissions of X-rays. X-ray bursts are believed to be powered by a thermonuclear runaway on the surface of a neutron star in a binary system. XRB models are dependent on the accurate information of the nuclear reactions involved. The 18Ne(α,p)21Na reaction is considered to be of great importance as a possible breakout route from the Hot-CNO cycle preceding the thermonuclear runaway. In this thesis work, the 18Ne(α,p)21Na reaction cross-section was indirectly measured at Ecm(α,p) = 2568, 1970, 1758, 1683, 1379 and 1194 keV, using the time-reverse 21Na(p,α)18Ne reaction. Since the time-reverse approach only connects the ground states of 21Na and 18Ne, the cross sections measured here represent lower limits of the 18Ne(α,p)21Na cross-section. An experiment was performed using the the ISAC-II facility at TRIUMF, Vancouver, Canada. A beam of 21Na ions was delivered to a polyethylene (CH2)n target placed within the TUDA scattering chamber. The reaction 18Ne and 4He ions were detected using silicon strip detectors, with time-of-flight and ΔE/E particle identification techniques used to distinguish the ions from background. The measurement at Ecm = 1194 keV is the lowest energy measurement to date of the 18Ne(α,p)21Na cross section. The measured cross sections presented in this thesis were compared to the NON-SMOKER Hauser-Feshbach statistical calculations of the cross section and to the unpublished results of another time-reverse investigation performed by a collaboration at the Argonne National Laboratory. A 18Ne(α,p)21Na reaction rate calculation based on the measured cross sections was performed. In comparison with previous reaction rate estimates, our results indicate a rate that is about a factor 2-3 lower than Hauser-Feshbach calculations, suggesting that a statistical approach may not be appropriate for cross section calculations for nuclei in this mass region. The astrophysical consequences of our new results appear to remain nevertheless negligible. These are also presented in this thesis.
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Szames, Esteban Alejandro. "Few group cross section modeling by machine learning for nuclear reactor." Thesis, université Paris-Saclay, 2020. http://www.theses.fr/2020UPASS134.
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Pour estimer la répartition de la puissance au sein d’un réacteur nucléaire, il est nécessaire de coupler des modélisations neutroniques et thermohydrauliques. De telles simulations doivent disposer des valeurs sections efficaces homogénéisées à peu de groupes d’énergies qui décrivent les interactions entre les neutrons et la matière. Cette thèse est consacrée à la modélisation des sections efficaces par des techniques académiques innovantes basées sur l’apprentissage machine. Les premières méthodes utilisent les modèles à noyaux du type RKHS (Reproducing Kernel Hilbert Space) et les secondes par réseaux de neurones. La performance d’un modèle est principalement définie par le nombre de coefficients qui le caractérisent (c’est-à-dire l’espace mémoire nécessaire pour le stocker), la vitesse d’évaluation, la précision, la robustesse au bruit numérique, la complexité, etc. Dans cette thèse, un assemblage standard de combustible UOX REP est analysé avec trois variables d’état : le burnup, la température du combustible et la concentration en bore. La taille de stockage des bibliothèques est optimisée en cherchant à maximiser la vitesse et la précision de l’évaluation, tout en cherchant à réduire l’erreur de reconstruction des sections efficaces microscopiques, macroscopiques et du facteur de multiplication infini. Trois techniques d’approximation sont étudiées. Les méthodes de noyaux, qui utilisent le cadre général d’apprentissage machine, sont capables de proposer, dans un espace vectoriel normalisé, une grande variété de modèles de régression ou de classification. Les méthodes à noyaux peuvent reproduire différents espaces de fonctions en utilisant un support non structuré, qui est optimisé avec des techniques d’apprentissage actif. Les approximations sont trouvées grâce à un processus d’optimisation convexe facilité par "l’astuce du noyau”. Le caractère modulaire intrinsèque de la méthode facilite la séparation des phases de modélisation : sélection de l’espace de fonctions, application de routines numériques, et optimisation du support par apprentissage actif. Les réseaux de neurones sont des méthodes d’approximation universelles capables d’approcher de façon arbitraire des fonctions continues sans formuler de relations explicites entre les variables. Une fois formés avec des paramètres d’apprentissage adéquats, les réseaux à sorties multiples (intrinsèquement parallélisables) réduisent au minimum les besoins de stockage tout en offrant une vitesse d’évaluation élevée. Les stratégies que nous proposons sont comparées entre elles et à l’interpolation multilinéaire sur une grille cartésienne qui est la méthode utilisée usuellement dans l’industrie. L’ensemble des données, des outils, et des scripts développés sont disponibles librement sous licence MITModern nuclear reactors utilize core calculations that implement a thermo-hydraulic feedback requiring accurate homogenized few-group cross sections.They describe the interactions of neutrons with matter, and are endowed with the properties of smoothness and regularity, steaming from their underling physical phenomena. This thesis is devoted to the modeling of these functions by industry state-of-theart and innovative machine learning techniques. Mathematically, the subject can be defined as the analysis of convenient mapping techniques from one multi-dimensional space to another, conceptualize as the aggregated sum of these functions, whose quantity and domain depends on the simulations objectives. Convenient is intended in terms of computational performance, such as the model’s size, evaluation speed, accuracy, robustness to numerical noise, complexity,etc; always with respect to the engineering modeling objectives that specify the multidimensional spaces of interest. In this thesis, a standard UO₂ PWR fuel assembly is analyzed for three state-variables, burnup,fuel temperature, and boron concentration.Library storage requirements are optimized meeting the evaluation speed and accuracy targets in view of microscopic, macroscopic cross sections and the infinite multiplication factor. Three approximation techniques are studied: The state-of-the-art spline interpolation using computationally convenient B-spline basis, that generate high order local approximations. A full grid is used as usually donein the industry. Kernel methods, that are a very general machine learning framework able to pose in a normed vector space, a large variety of regression or classification problems. Kernel functions can reproduce different function spaces using an unstructured support,which is optimized with pool active learning techniques. The approximations are found through a convex optimization process simplified by the kernel trick. The intrinsic modular character of the method facilitates segregating the modeling phases: function space selection, application of numerical routines and support optimization through active learning. Artificial neural networks which are“model free” universal approximators able Artificial neural networks which are“model free” universal approximators able to approach continuous functions to an arbitrary degree without formulating explicit relations among the variables. With adequate training settings, intrinsically parallelizable multi-output networks minimize storage requirements offering the highest evaluation speed. These strategies are compared to each other and to multi-linear interpolation in a Cartesian grid, the industry standard in core calculations. The data set, the developed tools, and scripts are freely available under aMIT license
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GONCALEZ, ODAIR L. "Fotoproducao de neutrons no sup232Th e sup238U com radiacao gama de captura de neutrons termicos no intervalo de energia entre 5,61 a 10,83 MeV." reponame:Repositório Institucional do IPEN, 1998. http://repositorio.ipen.br:8080/xmlui/handle/123456789/10695.
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Made available in DSpace on 2014-10-09T12:43:06Z (GMT). No. of bitstreams: 0Made available in DSpace on 2014-10-09T14:05:36Z (GMT). No. of bitstreams: 1 06125.pdf: 6631284 bytes, checksum: 0d7cb7ea79949cb8c3121b13b630793a (MD5)
Tese (Doutoramento)
IPEN/T
Instituto de Pesquisas Energeticas e Nucleares - IPEN/CNEN-SP
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Sahin, Latife. "Measurement of the cross section and reaction rate of ⁸Li(²H,⁴HE)⁶He reaction at the energies of astrophysical interest /." The Ohio State University, 2001. http://rave.ohiolink.edu/etdc/view?acc_num=osu148640189520717.
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Giri, Rekam. "Cross Section Measurements of the 12C(α, γ)16O Reaction at E_c.m. = 3.7, 4.0, and 4.2 MeV." Ohio University / OhioLINK, 2019. http://rave.ohiolink.edu/etdc/view?acc_num=ohiou1553421450433669.
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Jansson, Kaj. "Measurements of Neutron-induced Nuclear Reactions for More Precise Standard Cross Sections and Correlated Fission Properties." Doctoral thesis, Uppsala universitet, Tillämpad kärnfysik, 2017. http://urn.kb.se/resolve?urn=urn:nbn:se:uu:diva-329953.
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It is difficult to underestimate the importance of neutron cross section standards in the nuclear data field. Accurate and precise standards are prerequisites for measuring neutron cross sections. Two different projects are presented here with the aim of improving on neutron standards. A simulation study was performed for an experiment intended to measure the cross sections of H(n,n), 235U(n,f), and 238U(n,f) relative to each other. It gave the first estimates of the performance of the experimental setup. Its results have aided the development of the experimental setup by setting limits on the target and detector design. A second neutron-standard project resulted in three measurements of 6Li(n,α)t relative to 235U(n,f). Each subsequent measurement improved upon the previous one and changed the experimental setup accordingly. Although, preliminary cross sections were agreeing well with evaluated data files in some energy intervals, the main goal to measure the cross section up to 3 MeV was not reached. Mass yields and energy spectra are important outcomes of many fission experiments, but in low yield regions the uncertainties are still high even for recurrently studied nuclei. In order to understand the fission dynamics, one also needs correlated fission data. One particular important property is the distribution of excitation energy between the two nascent fission fragments. It is closely connected to the prompt emission of neutrons and γ’s and reveals information about how nucleons and energy are transferred within the fissioning nucleus. By measuring both the pre and post neutron-emission fragment masses, the cumbrance of detecting neutrons directly is overcome. This is done using the fission spectrometer VERDI and the 2E-2v method. In this work I describe how both the spectrometer, the analysis method, and the calibration procedures have been further developed. Preliminary experimental data show the great potential of VERDI, but also areas that call for more attention. A previously overlooked consequence of a central assumption was found and a correction method is proposed that can correct previously obtained data as well. The last part of this thesis concerns the efficiencies of the fission product extraction at the IGISOL facility. The methodology of the fission yield measurements at IGISOL are reliant on assumptions that have not been systematically investigated. The presented work is a first step of such an investigation that can also be used as a tool for optimising the setup for measurements of exotic nuclei. A simulation framework connecting three different simulation codes was developed to investigate the produced yield of fission products in a buffer gas. Several different variants of the setup were simulated and the findings were generally accordant with previous estimates. A reasonable agreement between experimental data and the simulation results is demonstrated.
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Gilardy, Gwenaelle. "Measuring the 7Li(a ; g)11B reaction rate at temperatures relevant for the n-process." Thesis, Bordeaux, 2018. http://www.theses.fr/2018BORD0398/document.
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L’étude des réaction (a,g) d’intérêt astrophysique est vaste. Ces réactions ont un rôle important dans la phase de fusion d’hélium des étoiles, dans la nucléosynthèse au moment du big bang ainsi que dans une grande partie des scénarios d'explosions stellaires. L’étude des réactions (a,g) impliquant des faisceaux stables peut être réalisée de diverse façon. Je me suis concentrée sur deux d'entre elles. La première est l’étude en cinématique directe en détectant les rayons gamma produits. C'est ce que j'ai fait durant ma thèse pour mesurer la section efficace de 7Li(a,g)11B. Cette réaction a été étudiée au cours des années pour différentes raisons en astrophysique nucléaire. Par exemple, il a été postule que cette réaction pourrait résoudre, au moment de la nucléosynthèse du big bang, le problème du Lithium. Il est clair, aujourd'hui, que ce n'est pas la solution, cependant, elle a un rôle dans la production de boron lors des supernovae de type Ic. Une autre façon d’étudier les réactions (a,g) est d'utiliser la cinématique inverse. L’idée est d'envoyer un faisceau d'ions lourd sur une cible d’hélium. Ce type de cinématique permet de détecter, avec une bonne efficacité, le noyau lourd de recul produit si le faisceau qui n'a pas interagit avec la cible, en est correctement séparé. Les séparateurs de masses, comme St. George, sont construit dans ce but. St. George sera impliquer dans la mesure de sections efficaces de réaction d’importance pour le processus s comme 16O(a,g)20NeThe study of (a,g) reactions of astrophysical interest is quite vast. These reactions play an important role in the quiescent Helium burning phase of stars, in big bang nucleosynthesis and in most explosive stellar scenarios. The studies of (a,g) reactions involving stable beams are performed in various ways. I have been concentrating on two of them. The first one is studying these reactions in direct kinematics by detecting the produced gamma rays. This is what I did during my thesis to measure the cross section of 7Li(a,g)11B. It has been studied throughout the years for several purposes in nuclear astrophysics. For example, it was postulated it could solve the big bang nucleosynthesis Lithium problem. Nowadays, it is clear it does not.However, this reaction plays a role in the production of Boron during type Ic Supernovae. Another way to study (a,g) reactions is to use inverse kinematics. The idea is to send a heavy element beam on a Helium target. This kind of kinematics allows for the detection, with good efficiency, of the heavy recoil product if the beam that did not interact in the target is properly separated. Recoil mass separators, like St. George, are built for this purpose. St. George will be involved in measuring cross sections of reaction important for the s-process like 16O(a,g)20Ne
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Röder, Marko. "Measurement of the Coulomb dissociation cross sections of the neutron rich nitrogen isotopes 20,21N." Doctoral thesis, Saechsische Landesbibliothek- Staats- und Universitaetsbibliothek Dresden, 2014. http://nbn-resolving.de/urn:nbn:de:bsz:14-qucosa-157725.
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Many neutron rich nuclei are involved in the astrophysical r-process (rapid neutron capture process). The r-process forms an important path for heavy element nucleosynthesis and runs along the neutron drip line. Astrophysicists suggested core-collapse supernovae within a neutrino-driven wind scenario where the neutrino wind dissociates all previously formed elements into protons, neutrons and α particles, to be a possible astrophysical scenario for the r-process. Furthermore, reaction network calculations reported a high impact of light neutron rich nuclei to the r-process abundance. Reactions on these exotic nuclei can only be studied with radioactive ion beams as their half lifes, in the order of a few hundred milliseconds (T1/2,19N=330ms), are too low to fabricate target material out of them. Two examples of reactions along the path of the r-process are the 19N(n,γ)20N and the 20N(n, γ)21N reactions. Using 20N (resp. 21N) as a beam, these reactions were studied at the GSI Fragment Separator (FRS) in time-reversed conditions via Coulomb dissociation in the S393 experiment exploiting the virtual gamma field of a lead target. The experiment was performed at the LAND/R3B setup (Large Area Neutron Detector, Reactions with Relativistic Radioactive Beams) in a kinematically complete measurement, i.e., detecting all particles leaving the nuclear reaction. The neutrons flying at relativistic velocity were observed by the LAND detector, the calibration of which plays a crucial role for the present reaction. The Smiley effect, meaning that the measured energy of impinging particles in long scintillators is not independent of the hit position of the particle, has been investigated. It will be shown that reflections of the light traveling through the scintillator and the resulting longer path length of the light when not emitted directly towards the ends of the bar were identified to cause the Smiley effect. Gamma spectra in coincidence with outgoing 19N (resp. 20N) were generated. These fit well to recent publications and were utilized to separate transitions of the projectile nucleus into the ground state or first excited state of the ejectile nucleus. The Coulomb dissociation cross section was calculated for the total reaction, transitions into the ground state and the first excited state of the ejectile nucleus. Furthermore, excitation energy spectra were derived for both reactions separately for ground state transitions and for the dominating transitions into the first excited state. In order to facilitate future experiments on exotic nuclei, two detector solutions for the NeuLAND detector (the successor of LAND) were investigated. Utilizing minimum ionizing electrons of 30MeV at the ELBE facility, time resolutions and detection efficiencies were studied for an MRPC (Multi-gap Resistive Plate Chamber) based neutron detector with passive iron converters, on the one hand, and a pure scintillator based neutron ToF detector on the other hand. The ELBE data show good time resolutions (σt,electron < 120 ps) and detection efficiencies (ǫelectron > 90%) for both systems. Small MRPC prototypes were irradiated with 175MeV quasi-monochromatic neutrons at The Svedberg Laboratory (TSL) in Uppsala measuring efficiencies of ǫMRPC,neutron = 1.0%. It will be shown that MRPCs with passive steel converters may be included as neutron detectors in experiments where a lower multi-neutron capability than the one needed for NeuLAND is sufficientViele neutronenreiche Kerne sind im schnellen Neutroneneinfangprozess (r-Prozess, engl. für rapid) involviert. Der r-Prozess bildet einen wichtigen Pfad für die Nukleosynthese schwerer Elemente und verläuft entlang der Neutronen-Dripline. Astrophysiker schlugen Kernkollaps-Supernovae innerhalb eines neutrinogetriebenen Windes als mögliches astrophysikalisches Szenario für den r-Prozess vor. Dabei werden alle zuvor gebildeten Elemente in Protonen, Neutronen und Alphapartikel dissoziiert. Außerdem ist von Berechnungen mit Reaktionsnetzwerken bekannt, dass leichte neutronenreiche Kerne einen hohen Einfluss auf die Elementverteilung des r-Prozesses haben. Reaktionen dieser exotischen Kerne können nur mit radioaktiven Ionenstrahlen studiert werden, da ihre Halbwertszeiten im Bereich von wenigen hundert Millisekunden (T1/2,19N=330ms) zu gering sind, um Probenmaterial daraus herzustellen. Zwei Beispiele solcher Reaktionen, die auf dem Pfad des r-Prozesses liegen, sind die 19N(n,γ)20N und die 20N(n,γ)21N Reaktionen. Unter Verwendung von 20N (bzw. 21N) als Strahl wurden diese Reaktionen am Fragment Separator (FRS) der GSI unter zeitumgekehrten Bedingungen mittels Coulomb-Aufbruch gemessen, indem das virtuelle Photonenfeld einer Bleiprobe ausgenutzt wurde. Das Experiment wurde am LAND/R3B Aufbau (Large Area Neutron Detector, Reactions with Relativistic Radioactive Beams) in einer kinematisch vollständigen Messung durchgeführt, d.h. alle ausgehenden Reaktionsprodukte wurden detektiert. Die relativistischen Neutronen wurden mit dem LAND-Detektor untersucht. Dessen Kalibration spielt eine wichtige Rolle für die hier analysierten Reaktionen. Dabei wurde der Smiley-Effekt studiert, welcher beinhaltet, dass die gemessene Energie von einfallenden Teilchen mittels langen Szintillatorstreifen nicht unabhängig von der Position ist, an der die Teilchen auf den Detektor treffen. Es wird gezeigt, dass Reflexionen des Lichtes beim Durchgang durch den Szintillator und die größere Weglänge, die das Licht zurücklegen muss, wenn es nicht direkt in Richtung der Enden des Szintillators emittiert wird, den Smiley-Effekt verursachen. Gamma-Spektren in Koinzidenz mit ausgehenden 19N (bzw. 20N) wurden gewonnen und stimmen gut mit früheren Veröffentlichungen überein. Diese Spektren wurden dazu verwendet, die Übergänge des Projektilkerns in den Grundzustand und den ersten angeregten Zustand des Ejektilkerns zu identifizieren. Die Wirkungsquerschnitte des Coulombaufbruchs der Projektilkerne und die Anregungsenergiespektren beider Reaktionen wurden berechnet und separiert in Übergänge in den Grundzustand und die dominierenden Übergänge in den ersten angeregten Zustand. Um künftige Experimente an exotischen Kernen zu ermöglichen, wurden zusätzlich zwei Detektorkonzepte für NeuLAND (Nachfolger von LAND) untersucht. Mit minimal ionisierenden Elektronen mit Energien von 30MeV aus dem Elektronenbeschleuniger ELBE wurden die Zeitauflösungen und Detektionseffizienzen zum einen für einen MRPC (Multi-gap Resistive Plate Chamber) basierenden Neutronendetektor mit passiven Stahlkonverter und zum anderen für einen reinen szintillatorbasierenden Neutronendetektor studiert. Die ELBE-Daten zeigen gute Zeitauflösungen (σt,electron < 120ps) und Detektionseffizienzen (ǫelectron > 90%) für beide Systeme. Kleine MRPC-Prototypen wurden mit quasi-monochromatischen Neutronen mit einer Energie von 175MeV am TSL (The Svedberg Laboratory) in Uppsala bestrahlt. Dabei wurden Effizienzen von ǫMRPC,neutron = 1.0% gemessen. Es wird gezeigt, dass MRPCs mit passiven Stahlkonvertern als Neutronendetektoren bei Experimenten, bei denen eine geringere Multineutronenfähigkeit als für NeuLAND ausreichend ist, eingesetzt werden können
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Grøtner, Katrine, and Huy Hoang Pham. "Kinetik ved løb med dagligdagsprotese og løbespecifikprotese hos transtibial amputerede: Et cross-sectional studie." Thesis, Hälsohögskolan, Jönköping University, HHJ, Avd. för rehabilitering, 2020. http://urn.kb.se/resolve?urn=urn:nbn:se:hj:diva-49495.
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Formål: Formålet med studiet er at undersøge hvordan løb med en dagligdagsprotese og en løbespecifikprotese påvirker kinetik i nedre ekstremiteter hos mennesker med en transtibial-amputation. Metode: Kinetisk data blev indsamlet ved løbetests, med begge proteser, med et motion capture system og kraftplader i et klinisk ganganalyse lab i Göteborg, Sverige. Deltagere(n=2) udførte løbetests i selvvalgt hastighed, iført refleksive markører. Vertikal GRF, fod progressions vinkel, adducerende/abducerende hofte- og knæmoment udvalgt til videre databehandling. Resultat: Forskelle i hofte- og knæ adduktions moment og fod progressions vinkel blev observeret mellem de to protesetyper. Momenterne var mindre, når deltagerne løb med den løbespecifikke protese. Forskelle på den amputerede side og den kontralaterale side noteredes ved alle parametre uanset protesetype. Den kontralaterale side havde forøgede værdier sammenlignet med den amputerede side. Konklusion: Grundet forsøgets størrelse kan vi ikke konkludere, at individer med unilateral amputation i nedre ekstremitet absorberer belastning bedre, når de løber med en løbespecifikprotese fremfor en dagligdagsprotese.Aim: The aim of this study was to investigate how running with a daily-use prosthesis and a running specific prosthesis affects kinetics in the lower extremities when it comes to people with a transtibial amputation. Method: Kinetic data was collected through running tests, using both type of prosthesis, with a motion capture system and force plates in a clinical gait lab in Gothenburg, Sweden. Participants (n=2) executed the running tests in a self-selected speed, while wearing reflective markers. Vertical ground reaction force, foot progression angle, hip- and knee moment were selected for data processing. Results: Differences in hip- and knee adduction moment and foot progression angle were observed between the two types of prostheses. Moments were smaller when participants ran with running-specific prosthesis. Dissimilarity for the amputated side and the contralateral side were noted for all parameters regardless of type of prosthesis. The contralateral side had increased values compared to the amputated side. Conclusion: Because of the sample size we cannot conclude that individuals with a unilateral lower body amputation absorb load more efficiently when running with a running-specific prosthesis rather than a daily-use prosthesis.
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Lapinski, Felicia. "Experimental studies at CERN-nTOF of the 230Th(n,f) reaction." Thesis, Uppsala universitet, Tillämpad kärnfysik, 2020. http://urn.kb.se/resolve?urn=urn:nbn:se:uu:diva-417867.
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This work investigates the feasibility to perform an experiment at CERN n_TOF to study the fission cross section and fission fragment angular distribution (FFAD) of the 230Th(n,f) reaction. An analysis of fission fragment energy losses in the experimental target resulted in a choice of target thickness of 0.1 µm (100 µg/cm2 ), which yields good transmission out of the target at up to 45° emission angles from the target normal. A detection setup using ten PPAC detectors with nine thorium targets interleaved in between them was investigated, where the detectors and targets were tilted 45° with respect to the neutron beam. This makes it possible to measure all emission angles needed with respect to the neutron beam in order to determine the FFAD. For the experimental area EAR2 at n_TOF, a prediction of the count rate in the experiment resulted in low statistical uncertainties after a few weeks of beam time, which indicates that an experiment like this is feasible.Detta projekt undersöker genomförbarheten av ett experiment vid CERN n_TOF för att mäta tvärsnittet och fördelningen av emissionsvinklar av fissionsfragment (FFAD) från 230Th(n,f)-reaktionen. En analys av energiförlusterna av fissionsfragment inuti torium-provet resulterade i en optimal provtjocklek på 0.1 µm (100 µg/cm2 ), vilket medför att fissionsfragment som emitteras i vinklar upp till 45° från provets normal har hög sannolikhet att transmitteras ut ur provet. En detektionsuppställning med tio PPAC-detektorer med nio toriumprov mellan dem undersöktes, där detektorerna och proven antogs vara snedställda med 45° från neutronstrålens riktning. Detta möjliggör detektion av fissionsfragment i alla vinklar som är nödvändiga för att kunna mäta hela FFAD. För experimentanläggningen EAR2 vid n_TOF, resulterade en uppskattning av antalet detekterade fissionsevent per sekund i låga mätosäkerheter efter ett par veckor av mättid, vilket antyder att experimentet är görbart.
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Salamon, Lino. "Transmission and capture cross section measurements by the time-of-flight technique for validation of pile-oscillation experiments in the Minerve reactor." Thesis, Aix-Marseille, 2018. http://www.theses.fr/2018AIXM0312/document.
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Ce travail présente l'étude de faisabilité des mesures de transmission avec des échantillons MINERVE à l'installation de temps de vol GELINA. L'idée principale était de définir des procédures pour analyser les résultats des mesures de transmission réalisées avec des échantillons cylindriques ne répondant pas à la géométrie de transmission idéale. La capacité d'extraire des résultats fiables a été démontrée sur l'exemple des échantillons MINERVE enrichis en argent. De plus, des mesures de transmission et de capture avec des disques standards d'argent naturel ont été effectuées pour améliorer les paramètres de résonance pour 107Ag et 109Ag. Les principales étapes de ce travail sont la réduction des données brutes (taux de comptage) pour produire des spectres de transmission et de rendement de capture, puis l'analyse des spectres avec le code d'analyse de forme des résonances REFITThis work presents the feasibility study of transmission measurements with the MINERVE samples at time-of-flight facility GELINA. The main idea was to define procedures to analyse results of transmission measurements using cylindrical samples which do not fulfil the ideal transmission geometry. Capability of extracting reliable results was demonstrated on the example of MINERVE samples enriched in silver. In addition, transmission and capture measurements with standard discs of natural silver were performed to improve the resonance parameters for 107Ag and 109Ag. The main steps in this work are the data reduction of measured count rate spectra to produce final transmission and capture yield spectra and the spectra analysis with the resonance shape analysis code REFIT
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Benabderrahmane, Mohamed Lotfi. "Measurement of the K 0 inclusive cross section in pion-induced reactions at 1.15 GeV,c." [S.l. : s.n.], 2007. http://nbn-resolving.de/urn:nbn:de:bsz:16-opus-73321.
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