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Dissertations / Theses on the topic 'Rhodian'

Author: Grafiati

Published: 2 June 2025

Last updated: 31 July 2025

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1

Palucci, Benedetta. "Rhodium and Palladium Catalysed Unusual Regioselective Hydroformylation and Rhodium Catalysed Reductive Carbonylation." Doctoral thesis, Universitat Rovira i Virgili, 2020. http://hdl.handle.net/10803/670491.

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La present tesi doctoral té com a objectiu el desenvolupament de sistemes per aconseguir una regioselectivitat no convencional en l’hidroformilació d'alquens terminals. Degut a que nombroses substàncies naturals perfumades contenen un grup aldehid. Els processos d’hidroformilació, on es fan reaccionar monòxid de carboni i hidrogen amb olefines, han esdevenit mètodes inestimables per a les empreses de fragàncies per a la producció d’aquests derivats. La regioselectividad del procés, per a l’obtenció del producte lineal o ramificat, és extremadament dependent del substrat. Com a tendència genera

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2

Handwerk, Martin. "Heteroleptische Rhodium(III)-Polyolatokomplexe." Diss., lmu, 2003. http://nbn-resolving.de/urn:nbn:de:bvb:19-11351.

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3

Bearman, Philip Stephen. "Rhodium ruthenium heterobimetallic complexes." Thesis, University of Liverpool, 1995. http://ethos.bl.uk/OrderDetails.do?uin=uk.bl.ethos.295827.

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4

Simpson, Michael Charles. "Rhodium catalysed hydrocarbonylation reactions." Thesis, University of St Andrews, 1995. http://hdl.handle.net/10023/14927.

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The one step hydrohydroxymethylation which can be used to transform C[sub]n alkenes into C [sub](n+1) alcohols has been explored for functionalised alkenes. The catalyst system used for this study was generated in situ from [Rh2(OAc)4], Pet3, CO/ H2 and ethanol. The main alkene investigated was 2-propen-1-ol, because of the potential to produce 1,4-butanediol by a novel route, which it indeed does in reasonable yield. Of interest the branched chain product was not the expected 2-methyl-1,3-propanediol, but 2-methylpropan-1-ol. 1,4-butanediol and 2-methylpropan-1-ol make up the majority of the

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5

Brun, Pierre. "Réactivité d'un complexe bi nucléaire du rhodium à structure originale : animation du ligand cyclopentadienyle dans des complexes du fer." Nice, 1986. http://www.theses.fr/1986NICE4027.

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Réactivité et structure d'un complexe dinucléaire de Rh l'un des Rh portant 2 CO et 1 Cl, l'autre portant un coordinat phosphore : le bicycloaminophosphorane ; les 2 Rh étant portés par 1 Cl. Grande stabilité du pont chlore. On étudie une méthode originale d'amination du coordinat Cp par actions de NR₂ sur CpFel 1L 2X(L 1= L 2 =CO ou PR₃ ; L 1 = CO, L 2 = PR₃ ; X = Br, C1). Cette réaction est en fait complexe puisque selon la nature des ligands L, X et des anions NR2, nous avons isolé jusqu'à 5 composés différents

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6

Goswami, Niranjan. "105Rh(III) complexes with acyclic tetrathioether ligands : potential radiotherapeutic agents /." free to MU campus, to others for purchase, 1996. http://wwwlib.umi.com/cr/mo/fullcit?p9812951.

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7

Bahsine, Saïda Kugel Godefroy. "Caractérisation optique et électro-optique des cristaux photoréactifs BaTiO3 dopés Rh (BaTiO3:Rh) et BaxCa1-xTiO3 dopés rhodium." Metz : Université Metz, 2008. ftp://ftp.scd.univ-metz.fr/pub/Theses/2002/Bahsine.Saida.SMZ0232.pdf.

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8

Rathouis, Maïga Hélène Marjolet Michel. "Associations ANOPHELE-RHODAR." [S.l.] : [s.n.], 2007. http://castore.univ-nantes.fr/castore/GetOAIRef?idDoc=25606.

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9

Régent, Damien [Verfasser], and Bernhard [Akademischer Betreuer] Breit. "Rhodium-catalyzed intra- and intermolecular alkene hydroacylation = Rhodium-katalisierte Intra- und Intermolecular Alken Hydroacylation." Freiburg : Universität, 2014. http://d-nb.info/1115813811/34.

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10

Jongsma, Tjeerd. "Polymer-bound rhodium hydroformylation catalysts." [S.l. : [Groningen : s.n.] ; University of Groningen] [Host], 2008. http://irs.ub.rug.nl/ppn/.

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11

Unsworth, W. P. "Rhodium(II) catalysed Oxyamination Reactions." Thesis, University of Oxford, 2009. http://ethos.bl.uk/OrderDetails.do?uin=uk.bl.ethos.526154.

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12

Buck, Richard Tony. "Rhodium carbenoids in asymmetric synthesis." Thesis, University of Exeter, 1999. http://ethos.bl.uk/OrderDetails.do?uin=uk.bl.ethos.267219.

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13

Taylor, R. J. "Intramolecular rhodium carbenoid insertion reactions." Thesis, Imperial College London, 1988. http://hdl.handle.net/10044/1/47272.

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14

Doyle, Kevin James. "Rhodium carbenoid route to oxazoles." Thesis, Loughborough University, 1994. https://dspace.lboro.ac.uk/2134/33073.

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This thesis describes investigations by the author into the preparation of the oxazole heterocyclic system, by the use of rhodium carbenoid methodology. Chapter 1 is a review of the literature on the formation of oxazoles, by the reaction between diazocarbonyl compounds and nitrites. The various conditions that have been employed in the reaction are detailed, as well as developments into the understanding of its mechanism. Chapter 2 reports the study into the preparation of 4-functionalised oxazoles. A series of 4- benzenesulfonyloxazoles, oxazole-4-phosphates and oxazole-4-carbonitriles were

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15

Rode, Edward James. "Rhodium-zeolite hydroformylation of propylene." Diss., Virginia Polytechnic Institute and State University, 1985. http://hdl.handle.net/10919/71252.

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The purpose of this research was to characterize the rhodium exchanged NaX and NaY zeolites as propylene hydroformylation catalysts. Catalytic activity was measured in a differential bed reactor. Flow in situ infrared spectroscopy was used to probe the coordination chemistry of the zeolite modified rhodium carbonyls. The catalytic activity of rhodium zeolites at atmospheric pressure and between 100-150ºC was measured. The rate of n-butyraldehyde production was approximately 5x10⁻³ moles/g- Rh hr at 150°C. Regioselectivity was dependent upon pretreatment. Precarbonylation with carbon monoxide,

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16

Sapmaz, Selma. "Rhodium (I) catalysed intermolecular hydroacylation." Thesis, University of Bath, 2003. https://ethos.bl.uk/OrderDetails.do?uin=uk.bl.ethos.275828.

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17

Hargrave, Jonathan David. "Applications of Rhodiun-Catalysed 1,4-Addition Reactions in Organic Synthesis." Thesis, University of Bath, 2009. http://ethos.bl.uk/OrderDetails.do?uin=uk.bl.ethos.505705.

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18

Galvão, Rozana de Medeiros Sousa, and 92-99126-3410. "Diversidade genética de isolados de Botryosphaeria rhodina produtores de jasmonatos." Universidade Federal do Amazonas, 2008. http://tede.ufam.edu.br/handle/tede/5871.

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19

Schaak, Andreas. "Musterbildung in der heterogenen Katalyse auf Rhodiumoberflächen." [S.l. : s.n.], 1999. http://deposit.ddb.de/cgi-bin/dokserv?idn=958254540.

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20

Hinz, Monika. "Numerische Simulation der Musterbildung in der heterogenen Katalyse auf der Rh(110)-Oberfläche." [S.l. : s.n.], 2003. http://deposit.ddb.de/cgi-bin/dokserv?idn=971232393.

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21

Šušnjar, Nevena. "Towards rhodium and iridium oxo complexes." [S.l.] : [s.n.], 2006. http://deposit.ddb.de/cgi-bin/dokserv?idn=979943604.

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22

Pater, Boke Chan de. "Terpyridine complexes of rhodium (I, III)." [S.l. : Amsterdam : s.n.] ; Universiteit van Amsterdam [Host], 2003. http://dare.uva.nl/document/70850.

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23

Rutherford, Marcus William. "A study of rhodium doped zeolites." Thesis, University of Liverpool, 1994. http://ethos.bl.uk/OrderDetails.do?uin=uk.bl.ethos.240774.

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24

Duckett, Simon Benedict. "Silicon-hydride activation at cyclopentadienyl-rhodium." Thesis, University of York, 1989. http://ethos.bl.uk/OrderDetails.do?uin=uk.bl.ethos.329690.

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25

Rengakos, Antonios. "Apollonios Rhodios und die antike Homererklärung." München : C.H. Beck, 1994. http://books.google.com/books?id=XC1gAAAAMAAJ.

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26

Randell-Sly, Helen Elizabeth. "Rhodium catalysed intermolecular chelation controlled hydroacylation." Thesis, University of Bath, 2006. https://ethos.bl.uk/OrderDetails.do?uin=uk.bl.ethos.442159.

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27

Randrianalimanana, Claire. "Recherche d'une induction asymétrique pour la réaction d'hydroformylation catalysée par des complexes dinucléaires du rhodium (I)." Toulouse, INPT, 1987. http://www.theses.fr/1987INPT035G.

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En premier lieu, nous avons examiné le comportement des ligands diphosine classiques Ph2 P (CH2)n PPh2 vis à vis du complexe dinucléaire du rhodium Rh2 (u-S-tBu)2 (CO)4 au cours de la réaction d'hydroformylation de l'hexène-1. Si n+2, des espèces mononucléaires sont formées. Pour n+3, 4 les complexes dinucléaires où le ligand est en pont entre les deux atomes de rhodium sont sélectivement obtenus. Ceux-ci présentent une activité catalytique basse pression importante. Cette étude nous a permis d'aborder l'hydrofromylation asymétrique du styrène en utilisant ces mêmes complexes dinucléaires du r

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28

Cicoira, Fabio. "Electron beam induced deposition of rhodium nanostructures /." [S.l.] : [s.n.], 2002. http://library.epfl.ch/theses/?nr=2528.

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29

Wathier, Matthew James. "Mechanistic investigations of rhodium-catalyzed alkyne hydrothiolation." Thesis, University of British Columbia, 2016. http://hdl.handle.net/2429/59308.

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Herein, thorough mechanistic investigations into alkyne hydrothiolation catalyzed by [Tp*RhI(PPh₃)₂] (Tp* = tris(3,5-dimethylpyrazolyl)borate) are reported. The mechanism is shown to proceed through an intermediate [Tp*RhIIIH(SR)] complex (R = alkyl, aryl). Alkyne migratory insertion is shown to occur chemoselectively into the Rh-SR bond, despite the availability of a Rh-H bond, to produce a rhodathiacyclobutene intermediate. The regioselectivity of product formation is revealed to be the result of a competition between 1,2 and 2,1 migratory insertion of the alkyne to produce regioisomeric rho

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30

Oke, Okemona Efe. "Heterobinocular alkyl complexes of rhodium and iridium." Thesis, National Library of Canada = Bibliothèque nationale du Canada, 1999. http://www.collectionscanada.ca/obj/s4/f2/dsk1/tape7/PQDD_0019/NQ46898.pdf.

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31

Berg, Michel van den. "Rhodium-catalyzed asymmetric hydrogenation using phosphoramidite ligands." [S.l. : [Groningen : s.n.] ; University Library Groningen] [Host], 2006. http://irs.ub.rug.nl/ppn/291254144.

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32

Haaren, Richard Johannes van. "Palladium and rhodium allyl complexes in catalysis." [S.l. : Amsterdam : s.n.] ; Universiteit van Amsterdam [Host], 2002. http://dare.uva.nl/document/64738.

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33

Hoogervorst, Wilhelmus Johannes. "Isophthalaldimine compounds of palladium, platinum and rhodium." [S.l. : Amsterdam : s.n.] ; Universiteit van Amsterdam [Host], 2003. http://dare.uva.nl/document/69284.

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34

Douglas, Thomas Mark. "Chemistry of cationic rhodium alkyl phosphine complexes." Thesis, University of Oxford, 2009. http://ethos.bl.uk/OrderDetails.do?uin=uk.bl.ethos.504386.

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35

Miu, Wah-sing, and 苗華昇. "The electrodeposition of rhodium by pulse current." Thesis, The University of Hong Kong (Pokfulam, Hong Kong), 1985. http://hub.hku.hk/bib/B31207030.

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36

Harding, Duncan A. J. "Fluoro-complexes of ruthenium, iridium and rhodium." Thesis, University of Leicester, 2005. http://ethos.bl.uk/OrderDetails.do?uin=uk.bl.ethos.431985.

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37

Winter, Nicholas John. "Homogeneous rhodium catalysed hydrocarbonylation reactions of alkenes." Thesis, Durham University, 1991. http://etheses.dur.ac.uk/6194/.

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The conversion of ethene, carbon monoxide and water to propanoic acid by the catalytic action of various rhodium species, was investigated by infra-red spectroscopy and autoclave batch reactions. Utilisation of a high pressure infra-red cell and a Fourier Transform infra-red spectrometry enabled study of the spectra of the catalytic systems at temperatures up to 180ºC, and at pressures of 10 -150 bar. The batch autoclave reactions enable rates, yield and selectivities to be determined with the aid of Gas Chromatography and Mass Spectroscopy. Rhodium halides were used as precursors and the effe

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38

Shaw, J. M. "Oxygenation at rhodium centres and related studies." Thesis, University of Exeter, 1986. http://ethos.bl.uk/OrderDetails.do?uin=uk.bl.ethos.374943.

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39

Hasnip, Sarah Katherine. "Iridium and rhodium hydrides : the parahydrogen perspective." Thesis, University of York, 2000. http://ethos.bl.uk/OrderDetails.do?uin=uk.bl.ethos.341484.

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40

Belt, S. T. "Intermediates and mechanisms in organo-rhodium photochemistry." Thesis, University of York, 1988. http://ethos.bl.uk/OrderDetails.do?uin=uk.bl.ethos.234935.

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41

Kaye, Philip Ian. "Silane, vinylsilane and vinylketone complexes of Rhodium." Thesis, University of York, 1998. http://ethos.bl.uk/OrderDetails.do?uin=uk.bl.ethos.265457.

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42

Jones, Zoe Amanda. "A study of rhodium catalysed homogeneous hydrogenation." Thesis, University of Cambridge, 2005. http://ethos.bl.uk/OrderDetails.do?uin=uk.bl.ethos.615269.

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43

Blagbrough, Tamzin C. "Alkene hydrogenation catalysed by dinuclear rhodium complexes." Thesis, Kingston University, 1990. http://eprints.kingston.ac.uk/20533/.

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The work reported in this thesis is concerned with two separated but related studies. The first involved examination of hydrogenation reactions of alkenes, dienes and alkynes using (Rh[sub]2C1(CO)[sub]2(dppm)[sub]2JBPh[sub]4 as a catalyst. Kinetic studies have been performed on the reaction of hexene. The system only well-behaved in the presence of a base, R[sub]3N, where a rst order dependance on both catalyst and hydrogen concentations observed. The order with respect to alkene is of the Michaelis-Menton type. This behaviour suggests that the active catalyst is a neutral monohydride generate

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44

Epton, Jeremy W. "Alkene hydroformylation catalysed by dinuclear rhodium complexes." Thesis, Kingston University, 1990. http://eprints.kingston.ac.uk/20536/.

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45

Ferris, Leigh. "Rhodium carboxylates as catalysts for carbenoid transformations." Thesis, Loughborough University, 1996. https://dspace.lboro.ac.uk/2134/32620.

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Chapter One reviews the literature, discussing the application of metallocarbenoids in asymmetric synthesis. This introduction is mainly concerned with asymmetric carbon-carbon and carbon-heteroatom bond forming reactions and pays particular attention to the levels of stereoselectivity that have been achieved. Chapter Two discusses the use of novel homochiral rhodium(II) carboxylates to effect asymmetric induction in a range of carbenoid transformations. The preparation of these novel rhodium(II) carboxylates is discussed, together with their application in asymmetric catalysis. The work prese

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46

Roscioni, Otello Maria. "A computational study of supported rhodium catalysts." Thesis, University of Southampton, 2010. https://eprints.soton.ac.uk/191339/.

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In this work, density functional theory (DFT) was used to obtain microscopic structures of heterogeneous catalysts based on rhodium supported on a metal oxide (-Al2O3). Two different methodologies were used. The first methodology uses a periodic model and a plane-wave basis set to solve the Schrödinger equation in the framework of Bloch’s theorem. The optimised structures of RhI(CO)2/ -Al2O3 species obtained at this level of theory have bond lengths in agreement with experimental EXAFS determinations. The weighted linear combination of Rh K-edge XANES spectra computed using the three most domi

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47

Baiden, Joseph Eshun. "The structure of uranium-palladium-rhodium alloys." Thesis, University of Surrey, 1985. http://epubs.surrey.ac.uk/847229/.

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The structure and phases of alloys of uranium and two of the light platinum metals, Pd and Rh have been studied. Using X-ray diffraction, metallography and electron microscopy, the phase diagram of the noble metal-rich end of the ternary system, U-Pd-Rh has been established. Portions of the binary systems, U-Pd and U-Rh have also been studied and the Pd-Rh phase diagram re-established. The structure of the solid phases which are stable at 1050°C, 1150°C and 1250°C have been determined. A thermodynamic calculation of the isothermal sections of the ternary U-Pd-Rh system at 1350°

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48

Schnitzer, Jill. "Liquid phase hydroformylation by zeolite supported rhodium." Thesis, Virginia Tech, 1985. http://hdl.handle.net/10919/45732.

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The purpose of this research was to directly compare the behavior of zeolites containing rhodium with that of homogeneous rhodium species as catalysts for liquid phase hydroformylation of 1-hexene in order to study the effects of zeolite immobilization. NaX zeolite was cation exchanged with several rhodium salts and used as hydroformylation catalysts at 50°C and 125°C in the presence of: triphenylphosphine (PPh₃), dimethylphenylphosphine (PMe₂Ph), and the poison for zeolite surface and solution rhodium: triphenylmethylmercaptan (Ph₃CSH). The results of these experiments were compared with thos

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49

LaLama, Matthew. "Rhodium-Catalyzed Decomposition of Carbohydrate Diazo Esters." Youngstown State University / OhioLINK, 2018. http://rave.ohiolink.edu/etdc/view?acc_num=ysu1532881612843223.

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50

Zhu, Kechen, and Kechen Zhu. "Chemical and Microbial Processes for Rhodium Recovery." Thesis, The University of Arizona, 2017. http://hdl.handle.net/10150/625349.

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This is the first report that demonstrates the ability of anaerobic methanogenic granular sludge to reduce Rh(III) to Rh(0). Recovery of rhodium(Rh) during anaerobic incubations under abiotic and biotic condition with different electron donors was studied. H2 and formate reduced Rh(III) to Rh(0) nanoparticles(NPs) in the absence of microorganisms. However, the presence of microorganism was crucial for Rh(III) reduction with ethanol. Results of X-ray powder diffraction (XRD) and transmission electron microscopy (TEM) confirmed the formation of Rh(0) NPs and indicated the localization and morpho

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