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Journal articles on the topic 'Rydberg atoms and molecules'

Author: Grafiati

Published: 3 June 2025

Last updated: 31 July 2025

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1

Hollerith, Simon, Johannes Zeiher, Jun Rui, et al. "Quantum gas microscopy of Rydberg macrodimers." Science 364, no. 6441 (2019): 664–67. http://dx.doi.org/10.1126/science.aaw4150.

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The subnanoscale size of typical diatomic molecules hinders direct optical access to their constituents. Rydberg macrodimers—bound states of two highly excited Rydberg atoms—feature interatomic distances easily exceeding optical wavelengths. We report the direct microscopic observation and detailed characterization of such molecules in a gas of ultracold rubidium atoms in an optical lattice. The bond length of about 0.7 micrometers, comparable to the size of small bacteria, matches the diagonal distance of the lattice. By exciting pairs in the initial two-dimensional atom array, we resolved mo

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2

Chiu, Ying-Nan. "Crystal-field theory for the Rydberg states of polyatomic molecules." Canadian Journal of Physics 64, no. 7 (1986): 782–95. http://dx.doi.org/10.1139/p86-140.

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The potential on a Rydberg electron due to the cluster of atoms near the center of a polyatomic molecule is expanded in powers of spherical harmonics. Nonvanishing potentials in totally symmetric irreducible representations are obtained using the crystal field of the cluster of atoms in D3h, C3v, D4v, C4v, Td, and D2d symmetries. Odd as well as the usual even powers of spherical harmonics are included up to [Formula: see text]. Spectroscopically observable differences in potentials between a planar versus a nonplanar XY3 molecule and among a square planar, pyramidal, tetrahedral, and dihedral

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3

Zeppenfeld, M. "Nondestructive detection of polar molecules via Rydberg atoms." EPL (Europhysics Letters) 118, no. 1 (2017): 13002. http://dx.doi.org/10.1209/0295-5075/118/13002.

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4

Ramswell, J. A., V. G. Stavros, Q. Hong, and H. H. Fielding. "Rydberg electron wavepacket dymanics in atoms and molecules." Philosophical Transactions of the Royal Society of London. Series A: Mathematical, Physical and Engineering Sciences 356, no. 1736 (1998): 363–76. http://dx.doi.org/10.1098/rsta.1998.0170.

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5

Jiao, Yuechun, Liping Hao, Jiabei Fan, Jingxu Bai, Jianming Zhao, and Suotang Jia. "Autoionization of Ultracold Cesium Rydberg Atom in 37D5/2 State." Photonics 9, no. 5 (2022): 352. http://dx.doi.org/10.3390/photonics9050352.

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We present the observation of an autoionization of cesium 37D5/2 Rydberg atoms in ultracold gases and analyze the autoionization mechanism. The autoionization process is investigated by varying the delay time tD and Rydberg atomic density. The dependence of ionization signals on Rydberg density shows that the Rydberg density has an effect on not only the initial ion signals but also the evolution of the Rydberg atoms. The results reveal that the initial ionization of 37D5/2 Rydberg atoms is mostly attributed to the blackbody radiation (BBR)-induced photoionization, and the BBR-induced transiti

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6

Dimitrijević, Milan S., Vladimir A. Srećković, Alaa Abo Zalam, Nikolai N. Bezuglov, and Andrey N. Klyucharev. "Dynamic Instability of Rydberg Atomic Complexes." Atoms 7, no. 1 (2019): 22. http://dx.doi.org/10.3390/atoms7010022.

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Atoms and molecules in highly excited (Rydberg) states have a number of unique characteristics due to the strong dependence of their properties on the values of principal quantum numbers. The paper discusses the results of an investigation of collisional Rydberg complexes specific features, resulting in the development of dynamic chaos and the accompanying diffusion autoionization processes. It is shown (experiment and theory) that, in subthermal low energies, the global chaotic regime that evolved in quasimolecular systems leads to significant changes in the Rydberg gases radiation/ionization

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7

Liu Yang, Shen Zhen-Jie, Wang Xin-Cheng, and Jiang Yu-Hai. "Electron/Ion Imaging Technology and Its Applications in Cold Atoms, Molecules, and Related Fields." Acta Physica Sinica 74, no. 15 (2025): 0. https://doi.org/10.7498/aps.74.20250415.

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With the continuous advancement and maturation of laser cooling techniques for atoms and molecules and full-dimensional electron and ion imaging technology, the application of momentum imaging techniques to investigate the characteristic properties of cold atoms and collision dynamics has emerged as a burgeoning research direction. This progress has driven the development of a series of high-resolution electron and ion detection devices, leading to innovative breakthroughs in fields such as cold molecule reactions, Rydberg atoms, nuclear decay, photoionization of Bose-Einstein condensates (BEC

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8

Desfrançois, C., H. Abdoul-Carime, N. Khelifa, and J. P. Schermann. "From1rto1r2Potentials: Electron Exchange between Rydberg Atoms and Polar Molecules." Physical Review Letters 73, no. 18 (1994): 2436–39. http://dx.doi.org/10.1103/physrevlett.73.2436.

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9

Fu, Yijiao, and Jinhui Wu. "One-Step Implementation of Collective Anti-Blockade in a Rydberg Ring." Photonics 10, no. 10 (2023): 1172. http://dx.doi.org/10.3390/photonics10101172.

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In contrast to Rydberg blockade, Rydberg anti-blockade allows multiple atoms to be simultaneously excited in the presence of significant nonlocal interactions and can lead to distinct phenomena and applications. This inspires us to examine here general conditions, numerical verifications, and realistic restrictions regarding the collective anti-blockade excitations of N Rydberg atoms equally arranged along a ring. We find that by adjusting the detuning of a pump field to compensate for nonlocal interactions between one atom and all others, it is viable to realize resonant excitations of N atom

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10

Saakyan, Sergey, Nikita Morozov, Vladimir Sautenkov, and Boris B. Zelener. "Rydberg Interaction-Induced Distortion of the Autler–Townes Spectra in Cold Lithium Atoms." Atoms 11, no. 4 (2023): 73. http://dx.doi.org/10.3390/atoms11040073.

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In this article, effects of the strong long-range interaction of Rydberg atoms on the Autler–Townes splitting spectrum are investigated. Preliminary results are obtained for various excitation times and Rydberg atom densities. The 2S1/2 and 2P1/2 levels of lithium-7 are coupled with strong laser field and probed by another laser via excitation into a 70S Rydberg level. Interactions between Rydberg atoms excited by the probe beam lead to the broadening of the Autler–Townes spectra. At high concentrations of Rydberg atoms, a suppression of the excitation of the Autler–Townes peak at red detuning

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11

Malbrunot, C., T. Wolz, L. Nowak, and D. Comparat. "Simulation of antihydrogen deexcitation in neutral atom traps for improved trapping and cooling." Journal of Physics B: Atomic, Molecular and Optical Physics 55, no. 4 (2022): 044003. http://dx.doi.org/10.1088/1361-6455/ac5188.

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Abstract We present results of simulations highlighting the performance of a cooling mechanism in a magnetic trap tailored for excited Rydberg atoms (or molecules) with high magnetic moment. Unlike previous work, the cooling is achieved through fast stimulated decay of inter-manifold transitions which optimizes the scheme. This mechanism is relevant to experiments with trapped antihydrogen atoms for which the trapping fraction is currently low. We find several-fold enhancements of the number of atoms trapped in the configurations probed.

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12

Wang, L. J., M. King, and T. J. Morgan. "Fast Rydberg hydrogen atom collisions with neutral atoms and molecules." Journal of Physics B: Atomic and Molecular Physics 19, no. 18 (1986): L623—L628. http://dx.doi.org/10.1088/0022-3700/19/18/006.

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13

Shirai, Toshizo, and Hiroki Nakamura. "Ionization of Rydberg atoms in thermal collisions with polar molecules." Physical Review A 36, no. 9 (1987): 4290–97. http://dx.doi.org/10.1103/physreva.36.4290.

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14

Hammer, N. I., F. Gao, R. M. Pagni, and R. N. Compton. "Charge transfer reactions between chiral Rydberg atoms and chiral molecules." Journal of Chemical Physics 117, no. 9 (2002): 4299–305. http://dx.doi.org/10.1063/1.1496760.

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15

Even, U. "Decay dynamics of high Rydberg states in atoms and molecules." Philosophical Transactions of the Royal Society of London. Series A: Mathematical, Physical and Engineering Sciences 355, no. 1729 (1997): 1539–50. http://dx.doi.org/10.1098/rsta.1997.0075.

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16

Wahiddin, M. R. B., B. M. Garraway, and R. K. Bullough. "Squeezing with Rydberg Atoms." Journal of Modern Optics 34, no. 6-7 (1987): 1007–20. http://dx.doi.org/10.1080/09500348714550901.

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17

Tretyakov, Denis B., Vasily M. Entin, Ilya I. Beterov, et al. "Two-Photon Laser Excitation of Rb Rydberg Atoms in the Magneto-Optical Trap and Vapor Cell." Photonics 10, no. 11 (2023): 1201. http://dx.doi.org/10.3390/photonics10111201.

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We present our experimental results of two-photon laser excitation 5S1/2→5P3/2→nS1/2 of Rb atoms to Rydberg nS1/2 states with a homemade 480 nm laser in the second excitation step. In an experiment with cold Rb atoms, we excited the 42S1/2 state and detected Rydberg atoms with a selective-field-ionization (SFI) detector that provides single-atom resolution. The resonance line shapes well agreed with numerical simulations in a three-level theoretical model. We also studied the multiatom spectra of Rydberg excitation of mesoscopic atom ensembles which are of interest to quantum information proce

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18

Wu, Meimei, Xin Bao, Shuxian Yu, et al. "Electromagnetically Induced Transparency Spectra of 6Li Rydberg Atoms." Photonics 10, no. 12 (2023): 1367. http://dx.doi.org/10.3390/photonics10121367.

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Rydberg atoms possess highly excited valence electrons that are far away from atomic cations. Compared with ground states, Rydberg states are excited states with a high principal quantum number n that exhibit large electric dipole moments and have a variety of applications in quantum information processing. In this communication, we report the measurement of the 6Li Rydberg excitation spectrum by ladder-type electromagnetically induced transparency (EIT) in a vapor cell. The 2p→ns/nd EIT spectra were recorded by sweeping the frequency of an ultraviolet Rydberg pumping laser while keeping the p

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19

Austin, Publishing Group. "Microwave Radiation in the Environment and Its Impact on the State of Living Organisms." Austin Journal of Infectious Diseases 10, no. 3 (2023): 1089. https://doi.org/10.26420/AustinJInfectDis.2023.1089.

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In the early 1990s [1], we proposed a new agent of the impact of geocosmos on a set of processes in the lower atmosphere and biosphere - the microwave radiation of the earth's ionosphere, emitted by all its atoms, molecules and their ions when high-energy (Rydberg) states are excited by photo- and secondary electrons mainly during solar flares and geomagnetic storms. 

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20

Kalamarides, A., C. W. Walter, B. G. Zollars, K. A. Smith, and F. B. Dunning. "Associative ionization in collisions of K(nd) Rydberg atoms with molecules." Journal of Chemical Physics 87, no. 7 (1987): 4238–39. http://dx.doi.org/10.1063/1.452880.

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21

Scheuing, Trevor, and Jesús Pérez-Ríos. "Quasi-Static Lineshape Theory for Rydberg Excitations in High-Density Media." Atoms 11, no. 6 (2023): 95. http://dx.doi.org/10.3390/atoms11060095.

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This work presents a theoretical approach for lineshapes of Rydberg excitations in high-density media. In particular, we introduce the quasi-static lineshape theory, leading to a methodic and general approach, and its validity is studied. Next, using 84Sr as a prototypical scenario, we discuss the role of the thermal atoms and core–perturber interactions, generally disregarded in Rydberg physics. Finally, we present a characterization of the role of Rydberg–core perturber interactions based on the density and principal quantum number that, beyond affecting the lineshape, could potentially appl

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22

Belov, A. A., A. P. Kazantsev, D. V. Khveshchenko, and V. L. Pokrovsky. "Rydberg atoms in crossed fields." Journal of Physics B: Atomic and Molecular Physics 18, no. 24 (1985): 4683–97. http://dx.doi.org/10.1088/0022-3700/18/24/013.

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23

Qiao, Chang, та Wenxian Zhang. "Spontaneous decay-induced quantum dynamics in Rydberg-blockaded Λ-type atoms". Journal of Physics B: Atomic, Molecular and Optical Physics 54, № 20 (2021): 205501. http://dx.doi.org/10.1088/1361-6455/ac2d81.

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Abstract Strongly Rydberg-blockaded two-level atoms form a Rydberg superatom which is excited only to a collective symmetrical Dicke state. However, emerging often in the alkali-earth atoms, spontaneous decay from the Rydberg state to an additional pooling state renders the ensemble no longer a closed superatom. Herein we present a computationally efficient model to characterize the interaction between a fully Rydberg-blockaded ensemble of N Λ-type three-level atoms and a strong probe light field in a coherent state. The model enables us to achieve a decomposition of the coupled dynamics in th

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24

Ye, Gen-Sheng, Biao Xu, Feng-Yuan Kuang, et al. "Wheeler’s delayed-choice experiment based on Rydberg atoms." Journal of Physics B: Atomic, Molecular and Optical Physics 55, no. 4 (2022): 044002. http://dx.doi.org/10.1088/1361-6455/ac505e.

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Abstract The delayed choice gedanken-experiment initially proposed by J A Wheeler reveals the nontrivial features of wave–particle duality in quantum world, that is, the choice of whether to observe the particle/wave character of a quantum system at a delayed time can affect its evolution history. In this work, the Wheeler’s delayed-choice experiment is conducted and tested in a new regime based on a Rydberg-ground level atomic Mach–Zehnder interferometer with optical coherent manipulation. Our quantum system exhibits an excellent single-excitation of the collective atomic state due to the Ryd

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25

Distante, Emanuele, Auxiliadora Padrón-Brito, Matteo Cristiani, David Paredes-Barato, and Riedmatten Hugues de. "Storage Enhanced Nonlinearities in a Cold Atomic Rydberg Ensemble." Physical Review Letters 117 (September 26, 2016): 113001. https://doi.org/10.5281/zenodo.815848.

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The combination of electromagnetically induced transparency with the nonlinear interaction between Rydberg atoms provides an effective interaction between photons. In this Letter, we investigate the storage of optical pulses as collective Rydberg atomic excitations in a cold atomic ensemble. By measuring the dynamics of the stored Rydberg polaritons, we experimentally demonstrate that storing a probe pulse as Rydberg polaritons strongly enhances the Rydberg mediated interaction compared to the slow propagation case. We show that the process is characterized by two time scales. At short storage

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26

Oliver, Brian J., and C. R. Stroud. "Bell’s inequalities for Rydberg atoms." Journal of the Optical Society of America B 4, no. 9 (1987): 1426. http://dx.doi.org/10.1364/josab.4.001426.

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27

Xu, Peng, and Ming-Sheng Zhan. "Ultrafast interaction between Rydberg atoms." Nature Photonics 16, no. 10 (2022): 673–74. http://dx.doi.org/10.1038/s41566-022-01074-z.

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28

Hickman, Albert P. "Collisional phenomena involving rydberg atoms." International Journal of Quantum Chemistry 24, S17 (2009): 65–76. http://dx.doi.org/10.1002/qua.560240808.

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29

Glukhov, I. L., A. A. Kamenski, and V. D. Ovsyannikov. "Interaction of blackbody radiation with rubidium and caesium atoms in small-angular-momentum Rydberg states." Quantum Electronics 52, no. 6 (2022): 570–76. http://dx.doi.org/10.1070/qel18059.

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Abstract We examine the possibilities of refining an asymptotic description and quantitative calculations of the effects induced by thermal blackbody radiation (BBR) of the environment on the Rydberg states of atoms. Numerical values are calculated and asymptotic expressions are proposed for simplified estimates of natural lifetimes and threshold photoionisation cross sections for Rydberg states of rubidium and caesium atoms with large values of the principal quantum number, n ≥ 20, and small orbital momenta, l = 0, 1, 2, 3. Based on analytical expressions, we present numerical estimates for t

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30

Lundin, Joergen, and Leif Holmlid. "Electron excitation energy transfer from highly excited cesium atoms forming high Rydberg state atoms and molecules." Journal of Physical Chemistry 95, no. 3 (1991): 1029–34. http://dx.doi.org/10.1021/j100156a003.

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31

Bai, Jiandong, Xin Wang, Xiaokai Hou, Wenyuan Liu, and Junmin Wang. "Angle-Dependent Magic Optical Trap for the 6S1/2↔nP3/2 Rydberg Transition of Cesium Atoms." Photonics 9, no. 5 (2022): 303. http://dx.doi.org/10.3390/photonics9050303.

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The existence of an anisotropic tensor part of atomic states with an angular momentum greater than 1/2 causes their dynamic polarizabilities to be very sensitive to the polarization direction of the laser field. Therefore, the magic wavelength of the transition between two atomic states also depends on the polarization angle between the quantized axis and the polarization vector. We perform a calculation of the magic conditions of the 6S1/2↔nP3/2 (n = 50–90) Rydberg transition of cesium atoms by introducing an auxiliary electric diople transition connected to the target Rydberg state and a low

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32

Seiler, Christian, Stephen D. Hogan, and Frédéric Merkt. "Dynamical Processes in Rydberg-Stark Deceleration and Trapping of Atoms and Molecules." CHIMIA International Journal for Chemistry 66, no. 4 (2012): 208–11. http://dx.doi.org/10.2533/chimia.2012.208.

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33

Schachenmayer, J., I. Lesanovsky, A. Micheli, and A. J. Daley. "Dynamical crystal creation with polar molecules or Rydberg atoms in optical lattices." New Journal of Physics 13, no. 5 (2011): 059503. http://dx.doi.org/10.1088/1367-2630/13/5/059503.

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34

Michel, L. "Rydberg states of atoms and molecules. Basic group theoretical and topological analysis." Physics Reports 341, no. 1-6 (2001): 173–264. http://dx.doi.org/10.1016/s0370-1573(00)00090-9.

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35

Schachenmayer, J., I. Lesanovsky, A. Micheli, and A. J. Daley. "Dynamical crystal creation with polar molecules or Rydberg atoms in optical lattices." New Journal of Physics 12, no. 10 (2010): 103044. http://dx.doi.org/10.1088/1367-2630/12/10/103044.

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36

Gong, Shunsheng, Bingmo Liu, Jiamin Wang, Sihong Gu, Zuoyao Dai, and Baiwen Li. "Ionization properties in the collision of Rydberg Cs atoms with CCl4 molecules." Science in China Series A: Mathematics 41, no. 7 (1998): 779–84. http://dx.doi.org/10.1007/bf02901961.

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37

Ovsiannikov, Vitaly D., Vitaly G. Palchikov, and Igor L. Glukhov. "Microwave Field Metrology Based on Rydberg States of Alkali-Metal Atoms." Photonics 9, no. 9 (2022): 635. http://dx.doi.org/10.3390/photonics9090635.

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The high-precision determination of microwave radiation parameters may be based on measurements of the spectral characteristics of radiation transitions between the Rydberg states of atoms. Frequencies and matrix elements are calculated for dipole transitions from even-parity nS1/2 and nD5/2 to odd-parity n′P3/2 and n′F7/2 (where n′ = n, n ± 1, n ± 2) for the Rydberg states of alkali-metal atoms. The matrix elements determine the splitting of Rydberg-state energy levels in the field of a resonance microwave (μw) radiation, which results in the splitting of the resonance in electromagnetic indu

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38

Duspayev, Alisher, Ryan Cardman, and Georg Raithel. "Dynamic Polarizability of the 85Rb 5D3/2-State in 1064 nm Light." Atoms 10, no. 4 (2022): 117. http://dx.doi.org/10.3390/atoms10040117.

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We report a measurement of the dynamic (ac) scalar polarizability of the 5D3/2 state in 85Rb atoms at a laser wavelength of 1064 nm. Contrary to a recent measurement in Phys. Rev. A 104, 063304 (2021), the experiments are performed in a low-intensity regime in which the ac shift is less than the 5D3/2 state’s hyperfine structure, as utilized in numerous experiments with cold, trapped atoms. The extracted ac polarizability is α5D3/2=−499±59 a.u., within the uncertainty of the aforementioned previous result. The calibration of the 1064 nm light intensity, performed by analyzing light shifts of t

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39

Mu, Wei-Lin, Xiao-Xuan Li, and Xiao-Qiang Shao. "Cooling neutral atoms into maximal entanglement in the Rydberg blockade regime." Optics Letters 47, no. 17 (2022): 4491. http://dx.doi.org/10.1364/ol.471591.

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We propose a cooling scheme to prepare stationary entanglement of neutral atoms in the Rydberg blockade regime by the combination of periodically collective laser pumping and dissipation. In each cycle, the controlled unitary dynamics process can selectively pump atoms away from the nontarget state while keeping the target state unchanged. The subsequent dissipative process redistributes the populations of ground states through the engineered spontaneous emission. After a number of cycles, the system will eventually be stabilized into the desired steady state, independent of the initial state.

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40

Batra, K., V. Prasad, and M. Mohan. "Collisional excitation of Na-Rydberg atoms." European Physical Journal D 20, no. 2 (2002): 191–98. http://dx.doi.org/10.1140/epjd/e2002-00134-y.

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41

Jones, Matthew PA, Luis Gustavo Marcassa, and James Shaffer. "Special issue on cold Rydberg atoms." Journal of Physics B: Atomic, Molecular and Optical Physics 48, no. 18 (2015): 180201. http://dx.doi.org/10.1088/0953-4075/48/18/180201.

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42

Oks, E., and T. Uzer. "Rydberg atoms as sensitive magnetic probes." Journal of Physics B: Atomic, Molecular and Optical Physics 33, no. 12 (2000): 2207–18. http://dx.doi.org/10.1088/0953-4075/33/12/304.

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43

Parzynski, R., M. Sobczak, and A. Wójcik. "Photoionization artifacts from model Rydberg atoms." Journal of Physics B: Atomic, Molecular and Optical Physics 34, no. 18 (2001): 3629–39. http://dx.doi.org/10.1088/0953-4075/34/18/302.

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44

Fregenal, D., M. Førre, E. Horsdal, C. Fisker, and N. A. Kjær. "Transient intrashell resonances in Rydberg atoms." Journal of Physics B: Atomic, Molecular and Optical Physics 41, no. 10 (2008): 105003. http://dx.doi.org/10.1088/0953-4075/41/10/105003.

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45

Schlosser, Malte, Daniel Ohl de Mello, Dominik Schäffner, Tilman Preuschoff, Lars Kohfahl, and Gerhard Birkl. "Assembled arrays of Rydberg-interacting atoms." Journal of Physics B: Atomic, Molecular and Optical Physics 53, no. 14 (2020): 144001. http://dx.doi.org/10.1088/1361-6455/ab8b46.

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46

Li, Jiachen, Ye Jin, Neil Qiang Su, and Weitao Yang. "Combining localized orbital scaling correction and Bethe–Salpeter equation for accurate excitation energies." Journal of Chemical Physics 156, no. 15 (2022): 154101. http://dx.doi.org/10.1063/5.0087498.

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We applied localized orbital scaling correction (LOSC) in Bethe–Salpeter equation (BSE) to predict accurate excitation energies for molecules. LOSC systematically eliminates the delocalization error in the density functional approximation and is capable of approximating quasiparticle (QP) energies with accuracy similar to or better than GW Green’s function approach and with much less computational cost. The QP energies from LOSC, instead of commonly used G0 W0 and ev GW, are directly used in BSE. We show that the BSE/LOSC approach greatly outperforms the commonly used BSE/ G0 W0 approach for p

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47

Belyayev, Yu E., A. V. Dem'yanenko, and A. A. Puretzky. "Formation and Luminescence of Molybdenum Atoms After UV Multiphoton Excitation of Gas Phase Mo(CO)6." Laser Chemistry 12, no. 3-4 (1992): 223–29. http://dx.doi.org/10.1155/lc.12.223.

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The delayed luminescence of Mo atoms was observed in XeCl laser excitation of Mo(CO)6 gas. The observed luminescence was explained by production of Mo Rydberg atoms under UV laser excitation of Mo(CO)6.

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48

Camus, P. "Correlation effects in double Rydberg atoms." Physica Scripta T51 (January 1, 1994): 20–27. http://dx.doi.org/10.1088/0031-8949/1994/t51/003.

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49

Gallagher, T. F. "Time domain spectroscopy of Rydberg atoms." Physica Scripta 76, no. 4 (2007): C145—C149. http://dx.doi.org/10.1088/0031-8949/76/4/n07.

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50

Deiglmayr, Johannes. "Long-range interactions between Rydberg atoms." Physica Scripta 91, no. 10 (2016): 104007. http://dx.doi.org/10.1088/0031-8949/91/10/104007.

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