Relevant bibliographies by topics / Solvolysis reactions

Contents

  1. Journal articles
  2. Dissertations / Theses
  3. Book chapters
  4. Conference papers
  5. Reports

Academic literature on the topic 'Solvolysis reactions'

Author: Grafiati
Published: 5 June 2025
Last updated: 1 August 2025

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Journal articles on the topic "Solvolysis reactions"

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Park, Kyoung Ho, Mi Hye Seong, Jin Burm Kyong, and Dennis N. Kevill. "Rate and Product Studies with 1-Adamantyl Chlorothioformate under Solvolytic Conditions." International Journal of Molecular Sciences 22, no. 14 (2021): 7394. http://dx.doi.org/10.3390/ijms22147394.

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A study was carried out on the solvolysis of 1-adamantyl chlorothioformate (1-AdSCOCl, 1) in hydroxylic solvents. The rate constants of the solvolysis of 1 were well correlated using the Grunwald–Winstein equation in all of the 20 solvents (R = 0.985). The solvolyses of 1 were analyzed as the following two competing reactions: the solvolysis ionization pathway through the intermediate (1-AdSCO)+ (carboxylium ion) stabilized by the loss of chloride ions due to nucleophilic solvation and the solvolysis–decomposition pathway through the intermediate 1-Ad+Cl− ion pairs (carbocation) with the loss
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Park, Kyoung-Ho, Chan Joo Rhu, Jin Burm Kyong, and Dennis N. Kevill. "The Effect of the ortho Nitro Group in the Solvolysis of Benzyl and Benzoyl Halides." International Journal of Molecular Sciences 20, no. 16 (2019): 4026. http://dx.doi.org/10.3390/ijms20164026.

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A kinetic study was carried out on the solvolysis of o-nitrobenzyl bromide (o-isomer, 1) and p-nitrobenzyl bromide (p-isomer, 3), and o-nitrobenzoyl chloride (o-isomer, 2) in a wide range of solvents under various temperatures. In all of the solvents without aqueous fluoroalcohol, the reactions of 1 were solvolyzed at a similar rate to those observed for 3, and the reaction rates of 2 were about ten times slower than those of the previously studied p-nitrobenzoyl chloride (p-isomer, 4). For solvolysis in aqueous fluoroalcohol, the reactivity of 2 was kinetically more reactive than 4. The l/m v
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D’Souza, Malcolm J., and Dennis N. Kevill. "Mechanistic studies of the solvolysis of alkanesulfonyl and arenesulfonyl halides." Beilstein Journal of Organic Chemistry 18 (January 17, 2022): 120–32. http://dx.doi.org/10.3762/bjoc.18.13.

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There have been several studies on the solvolysis mechanisms for alkanesulfonyl chlorides (RSO2Cl) and arenesulfonyl chlorides (ArSO2Cl). The earlier of these studies were reviewed a little over thirty years ago by Gordon, Maskill and Ruasse (Chem. Soc. Rev. 1989, 18, 123–151) in a contribution entitled “Sulfonyl Transfer Reactions”. The present review will emphasize more recent contributions and, in particular, the application of the extended Grunwald–Winstein equation and kinetic solvent isotope effects to the solvolysis reactions. There is also an appreciable number of reports concerning th
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Kevill, Dennis N., Byoung-Chun Park, and Jin Burm Kyong. "Evidence for general base catalysis by protic solvents in a kinetic study of alcoholyses and hydrolyses of 1-(phenoxycarbonyl)pyridinium ions under both solvolytic and non-solvolytic conditions." Collection of Czechoslovak Chemical Communications 74, no. 1 (2009): 43–55. http://dx.doi.org/10.1135/cccc2008164.

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The kinetics of nucleophilic substitution reactions of 1-(phenoxycarbonyl)pyridinium ions, prepared with the essentially non-nucleophilic/non-basic fluoroborate as the counterion, have been studied using up to 1.60 M methanol in acetonitrile as solvent and under solvolytic conditions in 2,2,2-trifluoroethan-1-ol (TFE) and its mixtures with water. Under the non- solvolytic conditions, the parent and three pyridine-ring-substituted derivatives were studied. Both second-order (first-order in methanol) and third-order (second-order in methanol) kinetic contributions were observed. In the solvolysi
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Bremner, JB, and KN Winzenberg. "Cyanogen-Bromide-Mediated and Methyl-Chloroformate-Mediated Synthesis of Some [3]Benzazonino[8,7,6-abc]Carbazole, [3]Benzazecino[9,8,7-abc]Carbazole, Naphth[1,8,7-def]Azonine and Naphth[1,8,7-def]Azecine Derivatives." Australian Journal of Chemistry 39, no. 1 (1986): 1. http://dx.doi.org/10.1071/ch9860001.

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Reaction of 7,8-dimethoxy-1,4,5,9,13c,13d-hexahydro-2H-indolo [3′,2′:4,5] indolo [1,7,6-aji] isoquinoline (4a) and 8,9-dimethoxy- 1,2,3,5,6,10,14c,14d-octahydro-indolo[3′,2′:3,4] naphtho [2,1,8-ija] quinolizine (4b) with cyanogen bromide in the presence of potassium carbonate afforded the elimination products 7,8-dimethoxy-1,2,3,4,5,9- hexahydro [3] benzazonino [8,7,6-abc]carbazole-3-carbonitrile (5a) and 8,9-dimethoxy-2,3,4,5,6,10-hexahydro-1H-[3] benzazecino [9,8,7-abc]carbazole-4-carbonitrile (5b) in 4% and 88% yield respectively; 7- (2-bromo)ethyl-1,2-dimethoxy-4,5,6,6a,7,12-hexahydroisoqu
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Kumaniaev, Ivan, Elena Subbotina, Maxim V. Galkin, et al. "A combination of experimental and computational methods to study the reactions during a Lignin-First approach." Pure and Applied Chemistry 92, no. 4 (2020): 631–39. http://dx.doi.org/10.1515/pac-2019-1002.

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AbstractCurrent pulping technologies only valorize the cellulosic fiber giving total yields from biomass below 50 %. Catalytic fractionation enables valorization of both cellulose, lignin, and, optionally, also the hemicellulose. The process consists of two operations occurring in one pot: (1) solvolysis to separate lignin and hemicellulose from cellulose, and (2) transition metal catalyzed reactions to depolymerize lignin and to stabilized monophenolic products. In this article, new insights into the roles of the solvolysis step as well as the operation of the transition metal catalyst are gi
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Huang, Xicai, and Andrew J. Bennet. "Kinetic evidence for the importance of solvent-separated ion pairs during the solvolyses of adamantylideneadamantyl derivatives." Canadian Journal of Chemistry 82, no. 9 (2004): 1336–40. http://dx.doi.org/10.1139/v04-101.

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The aqueous ethanolysis reactions of adamantylideneadamantyl tosylate, -bromide, and -iodide (1-OTs, 1-Br and 1-I) were monitored as a function of ionic strength. Special salt effects are observed during the solvolyses of both homoallylic halides, but not in the case of the tosylate 1-OTs. The measured α-secondary deuterium kinetic isotope effects for the solvolysis of 1-Br in 80:20 and 60:40 v/v ethanol–water mixtures at 25 °C are 1.110 ± 0.018 and 1.146 ± 0.009, respectively. The above results are consistent with the homoallylic halides reacting via a virtual transition state in which both f
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Mayr, Herbert, and Armin R. Ofial. "How to predict changes in solvolysis mechanisms." Pure and Applied Chemistry 81, no. 4 (2009): 667–83. http://dx.doi.org/10.1351/pac-con-08-08-26.

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Stopped-flow and laser flash techniques have been employed to investigate the individual steps of the solvolysis reactions of benzhydryl (diarylmethyl) halides and carboxylates. In this way, absolute rate constants for the ionization (k1), recombination of the carbocation with the leaving group (k-1), and subsequent reaction with the solvent (kSolvOH) have been determined. As the stabilization of the carbocations increases, the mechanism changes from (a) SN1 reactions with irreversible ionization through (b) SN1 reactions with common-ion return and (c) SN2C+ reactions, where the intermediate c
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Ion, Ganescu, Bratulescu George, Papa Ion, Ganescu Anca, Chirigiu Liviu, and Barbu Alin. "Solvolysis of the [Cr(NCS)4(benztriazole)2]- ion in ethanol-water mixtures." Journal of Indian Chemical Society Vol. 79, Aug 2002 (2002): 649–54. https://doi.org/10.5281/zenodo.5843274.

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Faculty of Chemistry, University of Craiova, 13 A. I. Cuza Str., 1100 Craiova. Romania <em>Fax : </em>4-051-197048 Faculty of Pharmacy, University of Medicine and Pharmacy. Bdl. I. Antonescu, 94 Craiova, Romania <em>Manuscript received 5 November 2001. revised 8 March 2002. accepted 21 March 2002</em> Measuring the concentration of the free thiocyanate ion and the nontransformed [Cr(NCS)<sub>4</sub>(benztriazole)<sub>2</sub>]<sup>-</sup> ion, the rate constants of the solvolysis process have been calculated. The solvolysis includes two parallel reactions - the substitution of thiocyanate ions
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Mollin, Jiří, Pavlína Staňková, and Oldřiška Staňková. "The evidence and applications of equilibria between hydroxide and alkoxide ions in aqueous-alcoholic systems." Collection of Czechoslovak Chemical Communications 55, no. 11 (1990): 2614–23. http://dx.doi.org/10.1135/cccc19902614.

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The composition of solvolysis products of butyl bromide, acetanhydride, and benzoyl chloride has been followed aqueous alcohol in alkaline and (except for butyl bromide) also in neutral regions. The results have been used as a piece of evidence of the existence of equilibrium between hydroxide and alkoxide ions and for evaluation of the possibility of calculation of the concentration ratio of hydroxide and alkoxide ions from the concentration ratios of the products as well as for evaluation of selectivities of the solvolytic reactions for mechanistic purposes.
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Dissertations / Theses on the topic "Solvolysis reactions"

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Ussing, Bryson Richard. "Systematic examination of dynamically driven organic reactions via kinetic isotope effects." Texas A&M University, 2006. http://hdl.handle.net/1969.1/4877.

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Organic reactions are systematically examined experimentally and theoretically to determine the role dynamics plays in the outcome of the reaction. It is shown that trajectory studies are of vital importance in understanding reactions influenced by dynamical motion. This dissertation discusses how a combination of kinetic isotope effects, theoretical calculations, and quasiclassical dynamics trajectories aid in the understanding of the solvolysis of p-tolyldiazonium cation in water, the cycloadditions of cyclopentadiene with diphenylketene and dichloroketene, and the cycloaddition of 2- methyl
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Norman, S. J. "Solvent and structural effects in solvolytic reactions." Thesis, Swansea University, 1993. http://ethos.bl.uk/OrderDetails.do?uin=uk.bl.ethos.638338.

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Rate Constants for the solvolysis of standard compounds have been used as a measure of solvent polarity. The Grunwald and Winstein equation utilized <i>tert</i>-butyl chloride for the Y scale. Y<SUB>X</SUB> scales for the 1- and 2-adamantyl derivatives have been established to correlate various substrates with different leaving groups. This thesis presents Y<SUB>OMs</SUB> results for binary aqueous mixtures of acetonitrile and dioxane which are classified as dipolar aprotic solvents. Y<SUB>Cl</SUB> values have also been obtained. When compounds containing one aromatic ring such as <i>p</i>-met
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Firmino, Thiago Diamond Reis. "Reações de solvólise em fase gasosa do cátion +SiCl3: experimento e teoria." Universidade de São Paulo, 2010. http://www.teses.usp.br/teses/disponiveis/46/46132/tde-20072010-201222/.

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Íons polihalogenados de Si, X3Si+ (X = F, Cl), são fragmentos facilmente gerados em espectrometria de massas por ionização eletrônica de compostos de silício polihalogenados. Estes cátions possuem um elevado caráter eletrofílico e desempenham um papel importante como intermediários em processos de corrosão auxiliados por plasma utilizados na fabricação de dispositivos em microeletrônica. Esta dissertação apresenta um estudo sobre a reatividade dos íons +SiCl3, em fase gasosa, perante uma série de substratos neutros simples como água, alcoóis, amônia, aminas e algumas bases doadoras de elétron
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Zeng, Xiaofeng. "Mechanisms for Solvolytic Elimination and Substitution Reactions Involving Short-lived Carbocation Intermediates." Doctoral thesis, Uppsala University, Organic Chemistry, 2002. http://urn.kb.se/resolve?urn=urn:nbn:se:uu:diva-2565.

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<p>Solvolysis reactions of a range of tertiary substrates in largely aqueous solvents were studied in such respects as β-deuterium kinetic isotope effects, linear free energy relationships and stereochemistry.</p><p>Solvolysis of the fluorene derivatives 9-methyl–9-(2´-X-2´-propyl)fluorene (<b>1-X,</b> X = Cl, Br, OOCCF<sub>3</sub>) involves a very short-lived carbocation intermediate. The fraction of alkene is increased by addition of general bases, which can be expressed by a Brφnsted parameter β = 0.07. The kinetic deuterium isotope effects vary with solvent composition in a way which is no
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Ebdon, D. N. "A mechanistic study of the solvolyis reactions of selected phosphoryl chlorides and p-anisoyl chloride." Thesis, Swansea University, 1999. http://ethos.bl.uk/OrderDetails.do?uin=uk.bl.ethos.636761.

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Throughout the 1990's several investigators have used a mechanistic theory based upon third order kinetics to explain the rates of the reactions of several substrates in aqueous mixtures of protic (e.g. methanol) an aprotic (e.g. acetone) solvents. Such substrates investigated have included <I>p</I>-nitrobenzoyl chloride and <I>p</I>-nitrobenzenesulfonyl chloride. Reactions of these substrates in aqueous alcohols yield two products; an acid (RCO<SUB>2</SUB>H and RSO<SUB>3</SUB>H) and an ester (RCO<SUB>2</SUB>R and RSO<SUB>3</SUB>R). Measurements of the relative amounts of the products obtained
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Bouxin, Florent. "Solvolyse des lignines : production de synthons aromatiques de faibles masses." Thesis, Reims, 2011. http://www.theses.fr/2011REIMS004/document.

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Les lignines ne sont pas suffisamment considérées dans les procédés de bioraffinerie. Pourtant, elles sont une source abondante de synthons aromatiques, et éléments essentiels de la rentabilité de transformation des lignocelluloses. A ce jour, les perspectives de production de synthons à partir des lignines se heurtent aux réactions de condensations des lignines, limitant leurs conversions en produits de faibles masses. Cette étude nous a permis de cerner les conditions propices à l’hydrolyse et/ou aux condensations grâce à l’étude de différentes lignines modèles soumises aux conditions d’acid
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Quteishat, Laith. "Contribution à la synthèse totale de la céphalotaxine." Thesis, Paris 11, 2013. http://www.theses.fr/2013PA114846/document.

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Depuis plus de 40 ans des chimistes se sont intéressés à l’extraction, à l’activité biologique et à la synthèse de l’homoharringtonine (HHT), un ester naturel de la céphalotaxine, qui est un puissant antileucémique utilisé pour le traitement des leucémies résistantes aux inhibiteurs de tyrosine kinase. Ces alcaloïdes sont extraits de Cephalotaxus, des conifères originaires du sud de la Chine à croissance extrêmement lente et menacés d’extinction. Leur synthèse est donc nécessaire. L’homoharringtonine utilisée en thérapeutique est obtenue à partir de (-)-céphalotaxine d’origine naturelle, par g
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Chamseddine, Yssam. "Sondes mecanistiques chirales et/ou regioselectivement deuteriees : application a l'etude de quelques processus de substitution nucleophile." Paris 6, 1988. http://www.theses.fr/1988PA066133.

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Moumaneix, Lilian. "De l’élaboration de matériaux graphéniques tridimensionnels dopés à l’azote : vers des catalyseurs pour l’électroréduction de l’oxygène sans platine." Electronic Thesis or Diss., Université de Lorraine, 2020. http://www.theses.fr/2020LORR0081.

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Le stockage de l’énergie sous la forme de dihydrogène suscite un intérêt grandissant dans la communauté scientifique et les industries du secteur de l’énergie et du transport. Les piles à combustible à membrane échangeuse de protons (PEMFC) permettent de convertir ce gaz en électricité sans rejets nocifs, à des températures peu élevées. Les catalyseurs actuels sont majoritairement constitués de nanoparticules de platine, déposées sur un matériau carboné microporeux. Or, ce métal noble est source de problèmes environnementaux et sociétaux, et son approvisionnement est soumis à des tensions et a
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Chang, Chih-Wei, and 張志偉. "Studies on the Solvolysis Reactions of Highly Hindered Benzhydryl and 9-Fluorenyl Substrates." Thesis, 1998. http://ndltd.ncl.edu.tw/handle/12571597271252574433.

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碩士<br>國立臺灣大學<br>化學系<br>86<br>In chapter 1, we use 2-naphthyl-2-adamantyl p-nitrobenzoate to measure the solvolysis rate constant and to show the necessary that develop the YxBnX scales. In chapter 2 and chapter 3，we use Grundwald-Winstein equation correlation analysis ortho-methyl substituted of benzhydryl and 9-aryl-9-fluorenyl substrates. For benzhydryl substrates，we can know the different effect by means of solvolysis when the increase of ortho-methyl group. The log k value of 9-
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Book chapters on the topic "Solvolysis reactions"

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Zingaro, R. A. "From Solvolysis of the As-N or the As-P Bond." In Inorganic Reactions and Methods. John Wiley & Sons, Inc., 2007. http://dx.doi.org/10.1002/9780470145197.ch105.

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Zingaro, R. A. "From Solvolyses of Arsenic Compounds." In Inorganic Reactions and Methods. John Wiley & Sons, Inc., 2007. http://dx.doi.org/10.1002/9780470145197.ch104.

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Gallego, Mar Gómez, and Miguel A. Sierra. "Level 3 - Case 35 Solvolysis of Vinyl Iodonium Salts." In Organic Reaction Mechanisms. Springer Berlin Heidelberg, 2004. http://dx.doi.org/10.1007/978-3-642-18788-9_35.

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Gallego, Mar Gómez, and Miguel A. Sierra. "Level 3 - Case 40 Solvolysis of 8-Deltacyclyl Brosylates." In Organic Reaction Mechanisms. Springer Berlin Heidelberg, 2004. http://dx.doi.org/10.1007/978-3-642-18788-9_40.

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Zingaro, R. A. "O-Sb Bonds by Solvolytic Reactions." In Inorganic Reactions and Methods. John Wiley & Sons, Inc., 2007. http://dx.doi.org/10.1002/9780470145197.ch114.

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Gallego, Mar Gómez, and Miguel A. Sierra. "Level 1 — Case 9 Solvolysis of Electron-Deficient Norbornyl Triflates." In Organic Reaction Mechanisms. Springer Berlin Heidelberg, 2004. http://dx.doi.org/10.1007/978-3-642-18788-9_9.

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Henderson, Richard A. "Catalysed substitution reactions." In The Mechanisms of Reactions at Transition Metal Sites. Oxford University Press, 1993. http://dx.doi.org/10.1093/hesc/9780198557463.003.0006.

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This chapter shows how the rates of substitution reactions at a variety of metal sites can be accelerated by base, acid, or electron transfer. It mentions Werner-type complexes of cobalt(III), chromium(III), ruthenium(III), rhodium (III), and iridium(III), which are the most extensively studied system showing base catalysis. What generated interest in these reactions was the apparent anomaly in the reaction of hydroxide that appears to be an exception to the general rule that the rate of substitution at cobalt(III) complexes show the characteristics of a dissociative mechanism. In addition, re
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Richard, John P., Tina L. Amyes, Maria M. Toteva, and Yutaka Tsuji. "Dynamics for the reactions of ion pair intermediates of solvolysis." In Advances in Physical Organic Chemistry. Elsevier, 2004. http://dx.doi.org/10.1016/s0065-3160(04)39001-5.

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Okuyama, Tadashi, and Howard Maskill. "Rearrangement Reactions involving Polar Molecules and Ions." In Organic Chemistry. Oxford University Press, 2013. http://dx.doi.org/10.1093/hesc/9780199693276.003.0022.

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This chapter focuses on the [1,2] sigmatropic rearrangements. It shows how 1,2-shifts in carbenium ion intermediates in solvolytic reactions, for example, can be considered as [1,2] sigmatropic rearrangements, and (consequently) related to concerted sigmatropic rearrangements of nonpolar compounds. The MO description of these simple 1,2-shifts in carbenium ions can be extended to describe the rearrangement steps in more complicated multistep heterolytic reactions. The chapter also details the catalysed rearrangement of carbonyl compounds involving 1,2-shifts, then investigates the 1,2-shifts f
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Jolivet, Jean-Pierre. "Water and Metal Cations in Solution." In Metal Oxide Nanostructures Chemistry. Oxford University Press, 2019. http://dx.doi.org/10.1093/oso/9780190928117.003.0005.

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Water has an exceptional ability to dissolve minerals. It is safe and chemically stable, and it remains liquid over a wide temperature range. Thus, it is the best solvent and reaction medium for both laboratory and industrial purposes. Water is able to dissolve ionic and ionocovalent solids because of the high polarity of the molecule (dipole moment μ = 1.84 Debye) as well as the high dielectric constant of the liquid (ε = 78.5 at 25°C). This high polarity allows water to exhibit a strong solvating power: that is, the ability to fix onto ions as a result of electrical dipolar interactions. Wat
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Conference papers on the topic "Solvolysis reactions"

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Singh, Anil Kr. "Kinetics Investigation of Solvent Polarity on Reaction Rate for Solvolysis of Ethyl Caprylate Ester in Binary Solvent System." In 2021 10th International Conference on System Modeling & Advancement in Research Trends (SMART). IEEE, 2021. http://dx.doi.org/10.1109/smart52563.2021.9676306.

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Reports on the topic "Solvolysis reactions"

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Braun, Andre M. Enhanced Oxidation and Solvolysis Reactions in Chemically Inert Microheterogeneous Systems. Defense Technical Information Center, 1986. http://dx.doi.org/10.21236/ada191248.

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Braun, Andre M. Enhanced Oxidation and Solvolysis Reactions in Chemically Inert Microheterogeneous Systems. Defense Technical Information Center, 1985. http://dx.doi.org/10.21236/ada191250.

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Braun, Andre M. Enhanced Oxidation and Solvolysis Reactions in Chemically Inert Microheterogeneous Systems. Defense Technical Information Center, 1987. http://dx.doi.org/10.21236/ada191251.

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Braun, Andre M. Enhanced Oxidation and Solvolysis Reactions in Chemically Inert Microheterogeneous Systems. Defense Technical Information Center, 1987. http://dx.doi.org/10.21236/ada191252.

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