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Journal articles on the topic 'Sulfur-doped graphene'

Author: Grafiati

Published: 4 June 2021

Last updated: 1 February 2022

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1

Zhang, Xuesha, Pengtao Yan, Ruijun Zhang, Kang Liu, Yanyan Liu, Ting Liu, and Xiaoyu Wang. "A novel approach of binary doping sulfur and nitrogen into graphene layers for enhancing electrochemical performances of supercapacitors." Journal of Materials Chemistry A 4, no. 48 (2016): 19053–59. http://dx.doi.org/10.1039/c6ta08482f.

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In this paper, we present a novel route to prepare sulfur and nitrogen co-doped reduced graphene oxide, in which, two main procedures – the preparation of a sulfur-doped graphite intercalation compound (S-GIC) and the construction of the sulfur and nitrogen co-doped reduced graphene oxide (SN-RGO) are included.

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2

Bi, Dong Mei, Liang Qiao, Xiao Ying Hu, and Shu Jie Liu. "Geometrical and Electronic Structure Investigations of S-Doped Graphene." Advanced Materials Research 669 (March 2013): 144–48. http://dx.doi.org/10.4028/www.scientific.net/amr.669.144.

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The geometrical and electronic structures of pure graphene and S-doped graphene have been investigated using plane wave pseudopotential method with generalized gradient approximation based on the density functional theory. The local structure change, Mulliken population, density of states, and electron density difference of S-doped graphene have been calculated. It can be observed that the Fermi level shifts towards the conduction band after the doping of sulfur atom. The results also suggest that there are chemical bonds formed between the sulfur and carbon atoms, and the charges transfer from the doped sulfur atom to graphene.

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3

Gao, Hui, Hai Jie Guo, and Jing Zi Chen. "Synthesis of Sulfur-Doped Graphene from Sulfonated Polystyrene." Advanced Materials Research 941-944 (June 2014): 235–38. http://dx.doi.org/10.4028/www.scientific.net/amr.941-944.235.

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Herein, sulfonated polystyrene thin film was applied as the precursor to synthesize sulfur (S)-doped graphene via thermal annealing process. S atoms were proved to be successfully doped into the lattice of graphene sheets according to the analyses of high resolution transmission microscopy (HRTM) and the corresponding energy dispersive X-Ray spectroscopy (EDX). The high D band detected in the Raman spectrum of S-doped graphene indicates the large amount of defects was introduced into the lattice of graphene, and the in-plane crystallite sizes were calculated to be ca. 21.7 nm. Our method provides an efficient and simple approach for the synthesis of S-doped graphene, which would promote the research for graphene based devices in widespread applications.

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4

Zhu, J., H. Park, R. Podila, A. Wadehra, P. Ayala, L. Oliveira, J. He, et al. "Magnetic properties of sulfur-doped graphene." Journal of Magnetism and Magnetic Materials 401 (March 2016): 70–76. http://dx.doi.org/10.1016/j.jmmm.2015.10.012.

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5

Zhao, Bing, Daiyun Song, Yanwei Ding, Juan Wu, Zhixuan Wang, Zhiwen Chen, Yong Jiang, and Jiujun Zhang. "Ultrastable Li-ion battery anodes by encapsulating SnS nanoparticles in sulfur-doped graphene bubble films." Nanoscale 12, no. 6 (2020): 3941–49. http://dx.doi.org/10.1039/c9nr10608a.

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SnS nanoparticles are encapsulated into sulfur-doped graphene bubble film presenting a flake-graphite-like structure. The closely packed SnS@G composite shows much lower specific surface area, smaller irreversible Li⁺ consumption.

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6

Lee, Ji, Sung Kwon, Soonchul Kwon, Min Cho, Kwang Kim, Tae Han, and Seung Lee. "Tunable Electronic Properties of Nitrogen and Sulfur Doped Graphene: Density Functional Theory Approach." Nanomaterials 9, no. 2 (February 15, 2019): 268. http://dx.doi.org/10.3390/nano9020268.

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We calculated the band structures of a variety of N- and S-doped graphenes in order to understand the effects of the N and S dopants on the graphene electronic structure using density functional theory (DFT). Band-structure analysis revealed energy band upshifting above the Fermi level compared to pristine graphene following doping with three nitrogen atoms around a mono-vacancy defect, which corresponds to p-type nature. On the other hand, the energy bands were increasingly shifted downward below the Fermi level with increasing numbers of S atoms in N/S-co-doped graphene, which results in n-type behavior. Hence, modulating the structure of graphene through N- and S-doping schemes results in the switching of “p-type” to “n-type” behavior with increasing S concentration. Mulliken population analysis indicates that the N atom doped near a mono-vacancy is negatively charged due to its higher electronegativity compared to C, whereas the S atom doped near a mono-vacancy is positively charged due to its similar electronegativity to C and its additional valence electrons. As a result, doping with N and S significantly influences the unique electronic properties of graphene. Due to their tunable band-structure properties, the resulting N- and S-doped graphenes can be used in energy and electronic-device applications. In conclusion, we expect that doping with N and S will lead to new pathways for tailoring and enhancing the electronic properties of graphene at the atomic level.

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7

Han, Jianmei, Baojuan Xi, Zhenyu Feng, Xiaojian Ma, Junhao Zhang, Shenglin Xiong, and Yitai Qian. "Sulfur–hydrazine hydrate-based chemical synthesis of sulfur@graphene composite for lithium–sulfur batteries." Inorganic Chemistry Frontiers 5, no. 4 (2018): 785–92. http://dx.doi.org/10.1039/c7qi00726d.

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A sulfur–hydrazine hydrate chemistry-based method is reported here to integrate the sulfur and N-doped reduced graphene oxide to obtain S@N-rGO composite with 76% sulfur. The as-obtained S@N-rGO composite displays a good rate capability and excellent stability.

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8

Yu, Yao, Zhijia Liao, Fanli Meng, and Zhenyu Yuan. "Theoretical and Experimental Research on Ammonia Sensing Properties of Sulfur-Doped Graphene Oxide." Chemosensors 9, no. 8 (August 11, 2021): 220. http://dx.doi.org/10.3390/chemosensors9080220.

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In this paper, gas sensing characteristics of sulfur-doped graphene oxide (S-GO) are firstly presented. The results of the sensing test revealed that, at room temperature (20 °C), S-GO has the optimal sensitivity to NH3. The S-GO gas sensor has a relatively short response and recovery time for the NH3 detection. Further, the sensing limit of ammonia at room temperature is 0.5 ppm. Theoretical models of graphene and S-doped graphene are established, and electrical properties of the graphene and S-doped graphene are calculated. The enhanced sensing performance was ascribed to the electrical properties’ improvement after the graphene was S-doped.

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9

Shahzad, Faisal, Pradip Kumar, Seunggun Yu, Seunghwan Lee, Yoon-Hyun Kim, Soon Man Hong, and Chong Min Koo. "Sulfur-doped graphene laminates for EMI shielding applications." Journal of Materials Chemistry C 3, no. 38 (2015): 9802–10. http://dx.doi.org/10.1039/c5tc02166a.

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Herein, for the first time, we demonstrate that a laminated structure of sulfur-doped reduced graphene oxide (SrGO) provides significant potential for electromagnetic interference shielding applications.

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10

Hassani, Fahimeh, Hossein Tavakol, Fariba Keshavarzipour, and Amin Javaheri. "A simple synthesis of sulfur-doped graphene using sulfur powder by chemical vapor deposition." RSC Advances 6, no. 32 (2016): 27158–63. http://dx.doi.org/10.1039/c6ra02109c.

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11

Kim, Myungjin, Jeongyeon Lee, Youngmoo Jeon, and Yuanzhe Piao. "Phosphorus-doped graphene nanosheets anchored with cerium oxide nanocrystals as effective sulfur hosts for high performance lithium–sulfur batteries." Nanoscale 11, no. 29 (2019): 13758–66. http://dx.doi.org/10.1039/c9nr03278a.

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12

Zhang, Fei-Fei, Chun-Li Wang, Gang Huang, Dong-Ming Yin, and Li-Min Wang. "Enhanced electrochemical performance by a three-dimensional interconnected porous nitrogen-doped graphene/carbonized polypyrrole composite for lithium–sulfur batteries." RSC Advances 6, no. 31 (2016): 26264–70. http://dx.doi.org/10.1039/c6ra02667b.

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13

Luo, Zhimin, Dongliang Yang, Guangqin Qi, Jingzhi Shang, Huanping Yang, Yanlong Wang, Lihui Yuwen, Ting Yu, Wei Huang, and Lianhui Wang. "Microwave-assisted solvothermal preparation of nitrogen and sulfur co-doped reduced graphene oxide and graphene quantum dots hybrids for highly efficient oxygen reduction." J. Mater. Chem. A 2, no. 48 (2014): 20605–11. http://dx.doi.org/10.1039/c4ta05096g.

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14

Zhang, Ben-Xing, Hui Gao, and Xiao-Long Li. "Synthesis and optical properties of nitrogen and sulfur co-doped graphene quantum dots." New J. Chem. 38, no. 9 (2014): 4615–21. http://dx.doi.org/10.1039/c4nj00965g.

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15

Wang, Chao, Kai Su, Wang Wan, Hua Guo, Henghui Zhou, Jitao Chen, Xinxiang Zhang, and Yunhui Huang. "High sulfur loading composite wrapped by 3D nitrogen-doped graphene as a cathode material for lithium–sulfur batteries." J. Mater. Chem. A 2, no. 14 (2014): 5018–23. http://dx.doi.org/10.1039/c3ta14921h.

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16

Liu, Zhixuan, Jie Li, Jingwei Xiang, Shuai Cheng, Hao Wu, Na Zhang, Lixia Yuan, et al. "Hierarchical nitrogen-doped porous graphene/reduced fluorographene/sulfur hybrids for high-performance lithium–sulfur batteries." Physical Chemistry Chemical Physics 19, no. 3 (2017): 2567–73. http://dx.doi.org/10.1039/c6cp07650e.

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17

Jiang, Yong, Yanwei Ding, Fang Chen, Zhixuan Wang, Yi Xu, Shoushuang Huang, Zhiwen Chen, Bing Zhao, and Jiujun Zhang. "Structural phase transformation from SnS2/reduced graphene oxide to SnS/sulfur-doped graphene and its lithium storage properties." Nanoscale 12, no. 3 (2020): 1697–706. http://dx.doi.org/10.1039/c9nr08075a.

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Structural phase transition from SnS₂/reduced graphene oxide (SnS₂/rGO) to SnS/sulfur-doped graphene (SnS/S-GNS) is demonstrated by both molecular simulation and experimental observations.

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18

Yu, Mingpeng, Junsheng Ma, Hongquan Song, Aiji Wang, Fuyang Tian, Yinshu Wang, Hong Qiu, and Rongming Wang. "Atomic layer deposited TiO2on a nitrogen-doped graphene/sulfur electrode for high performance lithium–sulfur batteries." Energy & Environmental Science 9, no. 4 (2016): 1495–503. http://dx.doi.org/10.1039/c5ee03902a.

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A nitrogen-doped graphene/sulfur composite was further modified with atomic layers of TiO₂and used as the cathode of lithium–sulfur batteries, exhibiting superior cycling stability, good rate capability and high coulombic efficiency.

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19

Ding, Kui, Yakun Bu, Qin Liu, Tengfei Li, Kai Meng, and Yaobing Wang. "Ternary-layered nitrogen-doped graphene/sulfur/ polyaniline nanoarchitecture for the high-performance of lithium–sulfur batteries." Journal of Materials Chemistry A 3, no. 15 (2015): 8022–27. http://dx.doi.org/10.1039/c5ta01195g.

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20

Li, Fei, Lang Sun, Yi Luo, Ming Li, Yongjie Xu, Guanghui Hu, Xinyu Li, and Liang Wang. "Effect of thiophene S on the enhanced ORR electrocatalytic performance of sulfur-doped graphene quantum dot/reduced graphene oxide nanocomposites." RSC Advances 8, no. 35 (2018): 19635–41. http://dx.doi.org/10.1039/c8ra02040j.

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21

Gu, Yuxing, Zhigang Chen, Juanjuan Tang, Wei Xiao, Xuhui Mao, Hua Zhu, and Dihua Wang. "Sulfur doped reduced graphene oxides with enhanced catalytic activity for oxygen reduction via molten salt redox-sulfidation." Physical Chemistry Chemical Physics 18, no. 48 (2016): 32653–57. http://dx.doi.org/10.1039/c6cp06818a.

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A facile redox-sulfidation reaction between sulfate containing molten carbonates and reduced graphene oxides (rGOs) was used to prepare sulfur and sulfur–cobalt co-doped rGOs with enhanced electrocatalytic activity.

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22

Kuzhandaivel, Hemalatha, Sornalatha Manickam, Suresh Kannan Balasingam, Manik Clinton Franklin, Hee-Je Kim, and Karthick Sivalingam Nallathambi. "Sulfur and nitrogen-doped graphene quantum dots/PANI nanocomposites for supercapacitors." New Journal of Chemistry 45, no. 8 (2021): 4101–10. http://dx.doi.org/10.1039/d1nj00038a.

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23

Wu, Ping, Hai-Yan Hu, Ning Xie, Chen Wang, Fan Wu, Ming Pan, Hua-Fei Li, et al. "A N-doped graphene–cobalt nickel sulfide aerogel as a sulfur host for lithium–sulfur batteries." RSC Advances 9, no. 55 (2019): 32247–57. http://dx.doi.org/10.1039/c9ra05202j.

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Herein, three-dimensional (3D) N-doped reduced graphene oxide (N-rGO) nanosheets were decorated with a uniform distribution of Co–Ni–S (CNS) nanoparticles to form the CNS/N-rGO composite as a sulfur host material for lithium–sulfur batteries.

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24

Lu, Zhiwei, Yujuan Chen, Zhaoen Liu, Aoqi Li, Dong Sun, and Kelei Zhuo. "Nitrogen and sulfur co-doped graphene aerogel for high performance supercapacitors." RSC Advances 8, no. 34 (2018): 18966–71. http://dx.doi.org/10.1039/c8ra01715h.

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25

Hao, Yong, Xifei Li, Xueliang Sun, and Chunlei Wang. "Nitrogen-doped graphene nanosheets/sulfur composite as lithium–sulfur batteries cathode." Materials Science and Engineering: B 213 (November 2016): 83–89. http://dx.doi.org/10.1016/j.mseb.2016.04.009.

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26

Zhao, Yan, Zagipa Bakenova, Yongguang Zhang, Huifen Peng, Hongxian Xie, and Zhumabay Bakenov. "High performance sulfur/nitrogen-doped graphene cathode for lithium/sulfur batteries." Ionics 21, no. 7 (February 10, 2015): 1925–30. http://dx.doi.org/10.1007/s11581-015-1376-4.

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27

Yan, Huimin, Meng Cheng, Benhe Zhong, and Yanxiao Chen. "Three-dimensional nitrogen-doped graphene/sulfur composite for lithium-sulfur battery." Ionics 22, no. 11 (May 26, 2016): 1999–2006. http://dx.doi.org/10.1007/s11581-016-1739-5.

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28

Niu, Shuzhang, Wei Lv, Chen Zhang, Fangfei Li, Linkai Tang, Yanbing He, Baohua Li, Quan-Hong Yang, and Feiyu Kang. "A carbon sandwich electrode with graphene filling coated by N-doped porous carbon layers for lithium–sulfur batteries." Journal of Materials Chemistry A 3, no. 40 (2015): 20218–24. http://dx.doi.org/10.1039/c5ta05324b.

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A sheet-like carbon sandwich, which contains a graphene layer as the conductive filling with N-doped porous carbon layers uniformly coated on both sides, is designed as a sulfur reservoir for lithium–sulfur batteries.

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29

Ngoc Anh, Nguyen Thi, Pei-Yi Chang, and Ruey-An Doong. "Sulfur-doped graphene quantum dot-based paper sensor for highly sensitive and selective detection of 4-nitrophenol in contaminated water and wastewater." RSC Advances 9, no. 46 (2019): 26588–97. http://dx.doi.org/10.1039/c9ra04414k.

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30

Liu, Fanfan, Xiaolong Cheng, Rui Xu, Ying Wu, Yu Jiang, and Yan Yu. "Binding Sulfur-Doped Nb2O5Hollow Nanospheres on Sulfur-Doped Graphene Networks for Highly Reversible Sodium Storage." Advanced Functional Materials 28, no. 18 (March 8, 2018): 1800394. http://dx.doi.org/10.1002/adfm.201800394.

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31

Struzzi, C., H. Sezen, M. Amati, L. Gregoratti, N. Reckinger, J. F. Colomer, R. Snyders, C. Bittencourt, and M. Scardamaglia. "Fluorine and sulfur simultaneously co-doped suspended graphene." Applied Surface Science 422 (November 2017): 104–10. http://dx.doi.org/10.1016/j.apsusc.2017.05.258.

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32

Islam, Md Monirul, Chandrasekar M. Subramaniyam, Taslima Akhter, Shaikh Nayeem Faisal, Andrew I. Minett, Hua Kun Liu, Konstantin Konstantinov, and Shi Xue Dou. "Three dimensional cellular architecture of sulfur doped graphene: self-standing electrode for flexible supercapacitors, lithium ion and sodium ion batteries." Journal of Materials Chemistry A 5, no. 11 (2017): 5290–302. http://dx.doi.org/10.1039/c6ta10933k.

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33

Guo, Jianqiang, Weimiao Wang, Yue Li, Jiafeng Liang, Qiaosi Zhu, Jiongli Li, and Xudong Wang. "Room-temperature synthesis of water-dispersible sulfur-doped reduced graphene oxide without stabilizers." RSC Advances 10, no. 44 (2020): 26460–66. http://dx.doi.org/10.1039/d0ra04838k.

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34

Li, Hui, Hai Ping He, and Zhi Zhen Ye. "Preparation of Doped Graphene Quantum Dots with Bright and Excitation-Independent Blue Fluorescence." Advanced Materials Research 950 (June 2014): 44–47. http://dx.doi.org/10.4028/www.scientific.net/amr.950.44.

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Highly bright-fluorescent N (nitrogen), S (sulfur) co-doped graphene quantum dots (GQDs) were synthesized through an modified hydrothermal method. The doped GQDs are smaller than 10 nm in size in average and stable in aqueous solution. Unlike many reports on graphene oxide (GO), the as-synthesized doped GQDs exhibit bright blue photoluminescence (PL) emission and the emission wavelength is excitation-independent. The intriguling results indicate that GQDs may have great potential in the optic and optoelectronic applications.

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35

Kim, Jae-Hong, Aravindaraj G. Kannan, Hyun-Sik Woo, Dae-Gun Jin, Wonkeun Kim, Kyounghan Ryu, and Dong-Won Kim. "A bi-functional metal-free catalyst composed of dual-doped graphene and mesoporous carbon for rechargeable lithium–oxygen batteries." Journal of Materials Chemistry A 3, no. 36 (2015): 18456–65. http://dx.doi.org/10.1039/c5ta05334j.

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36

Xiao, Lili, Jiao Yin, Yingchun Li, Qunhui Yuan, Hangjia Shen, Guangzhi Hu, and Wei Gan. "Facile one-pot synthesis and application of nitrogen and sulfur-doped activated graphene in simultaneous electrochemical determination of hydroquinone and catechol." Analyst 141, no. 19 (2016): 5555–62. http://dx.doi.org/10.1039/c6an00812g.

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37

Cheng, Xu, Ren Na, Xiaxia Wang, Nan Xia, Zhongqiang Shan, and Jianhua Tian. "Si nanoparticles embedded in 3D carbon framework constructed by sulfur-doped carbon fibers and graphene for anode in lithium-ion battery." Inorganic Chemistry Frontiers 6, no. 8 (2019): 1996–2003. http://dx.doi.org/10.1039/c9qi00488b.

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38

Xu, Chenyu, Qing Han, Yang Zhao, Lixia Wang, Yang Li, and Liangti Qu. "Sulfur-doped graphitic carbon nitride decorated with graphene quantum dots for an efficient metal-free electrocatalyst." Journal of Materials Chemistry A 3, no. 5 (2015): 1841–46. http://dx.doi.org/10.1039/c4ta06149g.

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39

Qiao, Xiaochang, Jutao Jin, Hongbo Fan, Yingwei Li, and Shijun Liao. "In situ growth of cobalt sulfide hollow nanospheres embedded in nitrogen and sulfur co-doped graphene nanoholes as a highly active electrocatalyst for oxygen reduction and evolution." Journal of Materials Chemistry A 5, no. 24 (2017): 12354–60. http://dx.doi.org/10.1039/c7ta00993c.

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40

Wang, Weixue, Xiangxue Wang, Jinlu Xing, Qiaobin Gong, Huihui Wang, Jianjun Wang, Zhe Chen, Yuejie Ai, and Xiangke Wang. "Multi-heteroatom doped graphene-like carbon nanospheres with 3D inverse opal structure: a promising bisphenol-A remediation material." Environmental Science: Nano 6, no. 3 (2019): 809–19. http://dx.doi.org/10.1039/c8en01196f.

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41

Duraivel, Malarkodi, Saravanan Nagappan, B. Balamuralitharan, S. Selvam, S. N. Karthick, K. Prabakar, Chang-Sik Ha, and Hee-Je Kim. "Superior one-pot synthesis of a doped graphene oxide electrode for a high power density supercapacitor." New Journal of Chemistry 42, no. 13 (2018): 11093–101. http://dx.doi.org/10.1039/c8nj01672k.

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42

Higgins, D. C., F. M. Hassan, M. H. Seo, J. Y. Choi, M. A. Hoque, D. U. Lee, and Z. Chen. "Shape-controlled octahedral cobalt disulfide nanoparticles supported on nitrogen and sulfur-doped graphene/carbon nanotube composites for oxygen reduction in acidic electrolyte." Journal of Materials Chemistry A 3, no. 12 (2015): 6340–50. http://dx.doi.org/10.1039/c4ta06667g.

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43

Tian, Zhengshan, Jitao Li, Gangyi Zhu, Junfeng Lu, Yueyue Wang, Zengliang Shi, and Chunxiang Xu. "Facile synthesis of highly conductive sulfur-doped reduced graphene oxide sheets." Physical Chemistry Chemical Physics 18, no. 2 (2016): 1125–30. http://dx.doi.org/10.1039/c5cp05475c.

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44

Geng, Dongsheng, Ni-Ni Ding, T. S. Andy Hor, Sheau Wei Chien, Zhaolin Liu, and Yun Zong. "Cobalt sulfide nanoparticles impregnated nitrogen and sulfur co-doped graphene as bifunctional catalyst for rechargeable Zn–air batteries." RSC Advances 5, no. 10 (2015): 7280–84. http://dx.doi.org/10.1039/c4ra13404d.

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45

Zhou, Jinhao, Zegao Wang, Yuanfu Chen, Jingbo Liu, Binjie Zheng, Wanli Zhang, and Yanrong Li. "Growth and properties of large-area sulfur-doped graphene films." Journal of Materials Chemistry C 5, no. 31 (2017): 7944–49. http://dx.doi.org/10.1039/c7tc00447h.

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46

Zheng, Penglun, Zhengfei Dai, Yu Zhang, Khang Ngoc Dinh, Yun Zheng, Haosen Fan, Jun Yang, et al. "Scalable synthesis of SnS2/S-doped graphene composites for superior Li/Na-ion batteries." Nanoscale 9, no. 39 (2017): 14820–25. http://dx.doi.org/10.1039/c7nr06044k.

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47

Lojka, Michal, Ondřej Jankovský, David Sedmidubský, Vlastimil Mazánek, Daniel Bouša, Martin Pumera, Stanislava Matějková, and Zdeněk Sofer. "Synthesis and properties of phosphorus and sulfur co-doped graphene." New Journal of Chemistry 42, no. 19 (2018): 16093–102. http://dx.doi.org/10.1039/c8nj03321h.

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48

Vinayan, B. P., Thomas Diemant, R. Jürgen Behm, and S. Ramaprabhu. "Iron encapsulated nitrogen and sulfur co-doped few layer graphene as a non-precious ORR catalyst for PEMFC application." RSC Advances 5, no. 81 (2015): 66494–501. http://dx.doi.org/10.1039/c5ra09030j.

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49

Kotal, Moumita, Hyunjun Kim, Sandipan Roy, and Il-Kwon Oh. "Sulfur and nitrogen co-doped holey graphene aerogel for structurally resilient solid-state supercapacitors under high compressions." Journal of Materials Chemistry A 5, no. 33 (2017): 17253–66. http://dx.doi.org/10.1039/c7ta05237e.

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50

Li, Xuecheng, Guanlun Guo, Ning Qin, Zhao Deng, Zhouguang Lu, Dong Shen, Xu Zhao, Yu Li, Bao-Lian Su, and Hong-En Wang. "SnS2/TiO2 nanohybrids chemically bonded on nitrogen-doped graphene for lithium–sulfur batteries: synergy of vacancy defects and heterostructures." Nanoscale 10, no. 33 (2018): 15505–12. http://dx.doi.org/10.1039/c8nr04661a.

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