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Dissertations / Theses on the topic 'Supramolecular architectures'

Author: Grafiati

Published: 4 June 2021

Last updated: 26 July 2025

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1

Greenaway, Alex. "3D supramolecular architectures." Thesis, University of Nottingham, 2013. http://ethos.bl.uk/OrderDetails.do?uin=uk.bl.ethos.594870.

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The design, synthesis and crystallisation properties of molecular tectons that are capable of participating in the formation of 3D supramolecular architectures are outlined with two distinct aspects of research presented. A series of molecules which contain both hydrogen bond acceptor and donor sites is synthesised to test the scope of ligands to form porous supramolecular organic frameworks (SOFs). Two analogous tripodal tri carboxylate ligands which are able to form coordination complexes in both a convergent and a divergent mode of coordination are synthesised and their formation of complex

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2

Gerhardt, Warren William. "Towards Supramolecular Multifunctional Architectures." Diss., Georgia Institute of Technology, 2007. http://hdl.handle.net/1853/14619.

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The synthesis of new biological and polymeric supramolecular synthons and their assembly into unique supramolecular architectures is presented. These new supramolecular synthons are functionalized with ligands that compliment metallated pincer complexes. Through the use of ditopic metallated pincer complexes these supramolecular synthons can be self-assembled into infinite linear chains. The first class of supramolecular synthons synthesized were based on cyclic peptide units, by embedding a pyridyl unit into the side-chain of one of the peptide residues the cyclic structure can be coordinat

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3

Cordes, David B., and n/a. "Supramolecular transition metal architectures." University of Otago. Chemistry Department, 2005. http://adt.otago.ac.nz./public/adt-NZDU20060705.144929.

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This thesis describes the investigation of the coordination and supramolecular chemistry of three different types of pyridine-containing ligand with a selection of Ag(I), Cu(I), Cu(II) and Cd(II) salts. The ligand types are flexible and four-armed, rigid and four-armed and bent with two rigid arms. All the ligands also display the ability to form additional supramolecular interactions. Chapter one introduces supramolecular chemistry and crystal engineering and covers background on several areas of current interest in these fields. Network structures, both coordination polymers and hydrogen-bo

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4

Painting, C. L. "Metallo-assembled supramolecular architectures." Thesis, University of Warwick, 1999. http://ethos.bl.uk/OrderDetails.do?uin=uk.bl.ethos.344047.

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5

Theogarajan, Luke Satish Kumar. "Supramolecular architectures for neural prostheses." Thesis, Massachusetts Institute of Technology, 2007. http://hdl.handle.net/1721.1/40514.

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Thesis (Ph. D.)--Massachusetts Institute of Technology, Dept. of Electrical Engineering and Computer Science, 2007.<br>Includes bibliographical references (leaves 213-230).<br>Neural prosthetic devices offer a means of restoring function that have been lost due to neural damage. The first part of this thesis investigates the design of a 15-channel, low-power, fully implantable stimulator chip. The chip is powered wirelessly and receives wireless commands. The chip features a CMOS only ASK detector, a single-differential converter based on a novel feedback loop, a low-power adaptive bandwidth D

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6

Di, Stasio F. "Supramolecular architectures : properties and applications." Thesis, University College London (University of London), 2012. http://discovery.ucl.ac.uk/1350099/.

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Supramolecular architectures represent an increasingly interesting playground both in the chemistry and physics field. In fact, they give us the possibility to tailor the physical and chemical properties of conjugated systems, opening the doors to new applications. In this dissertation I will present my findings regarding different types of supramolecular structures. The first part is dedicated to the study of the optical properties of conjugated polyrotaxanes: conjugated polymers such as poly(4,4’-diphenylene vinylene) threaded through cyclodextrin macrocycles rings, that sterically impose in

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7

Gualandi, Lorenzo <1988&gt. "EPR investigation of supramolecular architectures." Doctoral thesis, Alma Mater Studiorum - Università di Bologna, 2019. http://amsdottorato.unibo.it/8774/1/Gualandi_Lorenzo_tesi.pdf.

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The always increasing complexity of supramolecular systems requires not only new and efficient synthetic approaches but also the development of analytical methods capable of measuring the molecular scale phenomena exhibited by supramolecular assemblies. EPR spectroscopy, a magnetic resonance spectroscopic technique, has proven to be a useful tool for the investigation of supramolecular systems. My Ph.D. was devoted to the application EPR spectroscopy to the investigation of several supramolecular architectures. Among them, the investigation of an important non-covalent interaction, analogu

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8

Pritchard, Victoria Emily. "Metallo-supramolecular assemblies as functional architectures." Thesis, University of Leeds, 2016. http://etheses.whiterose.ac.uk/13394/.

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This thesis concerns the rational design of supramolecular metal-complexes and assemblies through combination of tripodal ligands and geometrically directing metallotectons. The aim of this work is to impart functionality into the resultant complexes, with a view towards applications exploiting the inherent luminescent emission of the systems. The metallotectons discussed in this thesis all derive from low-spin d6 metal centres, with incorporation of ancillary ligands designed to retain and modulate the resultant luminescent emission leading to high-fidelity control over the emissive outcome.

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9

El, Gemayel Mirella. "Graphene based supramolecular architectures and devices." Phd thesis, Université de Strasbourg, 2014. http://tel.archives-ouvertes.fr/tel-01070648.

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This thesis demonstrates that graphene produced by liquid-phase exfoliation can be co-deposited with a polymerie semiconductor for the fabrication of thin film field-effect transistors. The introduction of graphene to the n-type polymeric matrix enhances not only the electrical characteristics of the devices, but also the ambipolar behavior and the hole transport in particular. This provides a prospective pathway for the application of graphene composites for logic circuits.The same approach of blending was adopted to enhance the electrical characteristics of an amorphous p-type polymer semico

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10

Felloni, Marina. "Supramolecular architectures of transition metal dipicolinates." Thesis, University of Nottingham, 2003. http://ethos.bl.uk/OrderDetails.do?uin=uk.bl.ethos.289497.

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11

Lee, Sang-Hun. "Supramolecular architectures : macrocycles, catenanes and polyrotaxanes /." Diss., This resource online, 1996. http://scholar.lib.vt.edu/theses/available/etd-08232007-112703/.

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12

Henkelis, James John. "Supramolecular architectures with functionalised host ligands." Thesis, University of Leeds, 2014. http://etheses.whiterose.ac.uk/6910/.

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This thesis concerns the rational design and controlled self-assembly of supramolecular architectures for application in areas such as molecular recognition. The research focuses on the cyclotriveratrylene family of molecular hosts, where their incorporation into both polyhedral and polymeric assemblies bestows hosting ability to the complexes isolated. A novel pyridine-N-oxide ligand library has been prepared and the first examples of formal coordination polymers of the lanthanide(III) cations are subsequently reported. Their self assembly was extended to the transition metals and a variety o

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13

Barnett, Sarah Ann. "Supramolecular architectures constructed using angular bipyridyl ligands." Thesis, University of Nottingham, 2003. http://ethos.bl.uk/OrderDetails.do?uin=uk.bl.ethos.273181.

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14

Hamblin, Jacqueline. "The incorporation of supramolecular architectures into polymers." Thesis, University of Warwick, 2001. http://ethos.bl.uk/OrderDetails.do?uin=uk.bl.ethos.369634.

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15

PICCI, GIACOMO. "Novel Supramolecular Architectures based on weak interactions." Doctoral thesis, Università degli Studi di Cagliari, 2020. http://hdl.handle.net/11584/284397.

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This thesis reports the synthesis and the studies of a new series of Supramolecular architectures enable to function as selective anion receptors, efficient transmembrane transporters, and as Low Molecular Weight Gelators (LMWGs). A novel family of bis-selenoureas receptors were synthesised and their affinity towards different anion species were tested by means 1H-NMR titrations in DMSO-d6. A novel family of amide-based receptor were reported. Specifically, the role of the halogen substituents on the anion binding properties and on the activity as anion transporters of a series of isophthal

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16

SARKAR, RAJARSHI. "Design and Synthesis of Heteroleptic and Heterometallic Metallo-Supramolecular Terpyridine Architectures." University of Akron / OhioLINK, 2015. http://rave.ohiolink.edu/etdc/view?acc_num=akron1444660678.

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17

Wessendorf, Florian. "Supramolecular fullerene-porphyrin architectures = Supramolekulare Fulleren-Porphyrin-Architekturen." kostenfrei, 2010. http://d-nb.info/1000613593/34.

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18

Smith, Michelle M. "Supramolecular reagents for the construction of predictable architectures." Diss., Manhattan, Kan. : Kansas State University, 2008. http://hdl.handle.net/2097/708.

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19

Barker, Philip. "The introduction of supramolecular architectures into macromolecular arrays." Thesis, University of Warwick, 2002. http://ethos.bl.uk/OrderDetails.do?uin=uk.bl.ethos.250967.

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20

Ciesielski, Artur. "Supramolecular nanochemistry : from self-assembly to responsive architectures." Strasbourg, 2010. http://www.theses.fr/2010STRA6087.

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La chimie supramoléculaire est l'une des innovations les plus importantes dans les dernières décennies concernant les domaines de la chimie inorganique, organiques et bio-chimie. La chimie supramoléculaire repose sur l'utilisation des interactions non-covalentes pour auto-assembler, avec une précision sous-nanométrique, des entités chimiques en forme de matériaux avec des propriétés chimiques et physiques pré-programmés: la chimie supramoléculaire ainsi est la clé pour les nanosciences et la nanotechnologie. La chimie supramoléculaire offre un excellent contrôle sur le processus d'auto-assembl

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21

Chan, Yi-Tsu. "Design and Construction of Metallo-Supramolecular Terpyridine Architectures." University of Akron / OhioLINK, 2010. http://rave.ohiolink.edu/etdc/view?acc_num=akron1285698309.

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22

Abourahma, Heba. "Structural diversity in metal-organic nanoscale supramolecular architectures." [Tampa, Fla.] : University of South Florida, 2004. http://purl.fcla.edu/fcla/etd/SFE0000336.

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23

Baroncini, Massimo <1979&gt. "Design, Synthesis and Characterization of new Supramolecular Architectures." Doctoral thesis, Alma Mater Studiorum - Università di Bologna, 2010. http://amsdottorato.unibo.it/2943/1/Baroncini_Massimo_Tesi.pdf.

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24

Baroncini, Massimo <1979&gt. "Design, Synthesis and Characterization of new Supramolecular Architectures." Doctoral thesis, Alma Mater Studiorum - Università di Bologna, 2010. http://amsdottorato.unibo.it/2943/.

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25

Marchini, Marianna <1989&gt. "Photoactive Molecules in Supramolecular Architectures and Photoredox Reactions." Doctoral thesis, Alma Mater Studiorum - Università di Bologna, 2017. http://amsdottorato.unibo.it/8014/7/PhD%20Thesis%20Marianna%20Marchini.pdf.

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My PhD reasearch activity was mainly focused on two different fields: the study of the formation of supramolecular architectures and the investigation of the photophysical behaviour of different photocatalysts in organic reactions. The first supramolecular system shown in this thesis derives from a shapepersistent molecule, featuring four bipyridinium units, that upon reduction undergoes intermolecular pimerization because of the rigid architecture of the molecule. The same tetramer, with non-methylated bipyridium units, is able to form a supramolecular architecture upon complexation with fou

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26

Bunce, Siona. "Supramolecular helical arrays of highly defined topgraphy." Thesis, University of Warwick, 2001. http://ethos.bl.uk/OrderDetails.do?uin=uk.bl.ethos.247419.

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27

Xu, Fei. "Assembly and characterization of supramolecular architectures for biosensor applications." [S.l.] : [s.n.], 2005. http://deposit.ddb.de/cgi-bin/dokserv?idn=975967894.

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28

Tanh, Jeazet Harold Brice. "Metallo-supramolecular Architectures based on Multifunctional N-Donor Ligands." Doctoral thesis, Saechsische Landesbibliothek- Staats- und Universitaetsbibliothek Dresden, 2010. http://nbn-resolving.de/urn:nbn:de:bsz:14-qucosa-39665.

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Self-assembly processes were used to construct supramolecular architectures based on metal-ligand interactions. The structures formed strongly depend on the used metal ion, the ligand type, the chosen counter ion and solvent as well as on the experimental conditions. The focus of the studies was the design of multifunctional N-donor ligands and the characterization of their complexing and structural properties. This work was divided into three distinct main parts: The bis(2-pyridylimine), the bis(2-hydroxyaryl) imine and the tripodal imine / amine ligand approach. In the first part a series o

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29

Vickers, Matthew S. "Anion sensing and templated assembly if interpenetrated supramolecular architectures." Thesis, University of Oxford, 2006. http://ethos.bl.uk/OrderDetails.do?uin=uk.bl.ethos.442984.

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30

Dolomanov, Oleg V. "Crystal engineering of supramolecular architectures using poly-pyridyl ligands." Thesis, University of Nottingham, 2004. http://ethos.bl.uk/OrderDetails.do?uin=uk.bl.ethos.408452.

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31

Shan, Ning. "Supramolecular architectures of organic solids : synthesis, characterisation and prediction." Thesis, University of Cambridge, 2003. http://ethos.bl.uk/OrderDetails.do?uin=uk.bl.ethos.620074.

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32

Elbatal, Hany. "Terpyridine-Based Metallo-Supramolecular Architectures: From Structure to Function." University of Akron / OhioLINK, 2013. http://rave.ohiolink.edu/etdc/view?acc_num=akron1384367887.

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33

Ludlow, James M. III. "Design and Synthesis of Terpyridine based Metallo-Supramolecular Architectures." University of Akron / OhioLINK, 2015. http://rave.ohiolink.edu/etdc/view?acc_num=akron1444989836.

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34

Zhu, Shiying. "Terpyridine-based, Coordination-driven, 2D and 3D Supramolecular Architectures." University of Akron / OhioLINK, 2017. http://rave.ohiolink.edu/etdc/view?acc_num=akron1490368620583045.

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35

Perone, Rosaria Carmela <1985&gt. "Synthesis and Supramolecular Architectures of Lipophilic Derivatives of Guanine." Doctoral thesis, Alma Mater Studiorum - Università di Bologna, 2012. http://amsdottorato.unibo.it/4543/1/Perone_Rosaria_tesi.pdf.

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Self-assembly relies on the association of pre-programmed building blocks through non-covalent interactions to give complex supramolecular architectures. Previous studies provided evidence for the unique self-assembly properties of semi-synthetic lipophilic guanosine derivatives which can sequestrate ions from an aqueous phase, carry them into an organic phase where they promote the generation of well-defined supramolecular assemblies. In the presence of cations lipophilic guanosines form columnar aggregates while in their absence they generate supramolecular ribbons. The aim of this thesis h

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36

Perone, Rosaria Carmela <1985&gt. "Synthesis and Supramolecular Architectures of Lipophilic Derivatives of Guanine." Doctoral thesis, Alma Mater Studiorum - Università di Bologna, 2012. http://amsdottorato.unibo.it/4543/.

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Self-assembly relies on the association of pre-programmed building blocks through non-covalent interactions to give complex supramolecular architectures. Previous studies provided evidence for the unique self-assembly properties of semi-synthetic lipophilic guanosine derivatives which can sequestrate ions from an aqueous phase, carry them into an organic phase where they promote the generation of well-defined supramolecular assemblies. In the presence of cations lipophilic guanosines form columnar aggregates while in their absence they generate supramolecular ribbons. The aim of this thesis h

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37

Mohebbi, Elaheh. "Surface supported supramolecular architectures: an experimental and modeling study." Doctoral thesis, Università degli studi di Padova, 2019. http://hdl.handle.net/11577/3427304.

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L’auto-organizzazione di molecole organiche su superfici solide è uno degli approcci più diffusi per la creazione di architetture supramolecolari supportate di dimensioni controllate e con proprietà innovative. L’uso combinato di differenti interazioni di natura non covalente adsorbato–adsorbato e adsorbato–substrato consente infatti la modulazione dell’associazione di specie distinte in modo quasi altrettanto accurato che nei sistemi biologici, fonte primaria di ispirazione per ciò che può essere realizzato artificialmente. Il consenso sull’uso d’interazioni intermolecolari estese non covalen

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38

Robertson, Craig Collumbine. "Building complex systems based on simple molecular architectures." Thesis, University of St Andrews, 2011. http://hdl.handle.net/10023/2573.

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Over the past twenty years molecules capable of templating their own synthesis, so called self–replicating molecules have gained prominence in the literature. We show herein that mixing the reagents for replicating molecules can produce a network of self–replicators which coexist and that the networks can be instructed by the addition of preformed template upon initiation of the reaction. Whilst self–replicating molecules offer the simplest form of replication, nature has evolved to utilise not minimal self–replication but reciprocal replication where one strand templates the formation of not

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39

Scott, Benjamin M. T. "From small molecules to nano-scale architectures - a supramolecular approach." Diss., Manhattan, Kan. : Kansas State University, 2008. http://hdl.handle.net/2097/612.

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40

Palma, Matteo. "Supramolecular architectures on surfaces : self-organization and nanoscale electronic properties." Université Louis Pasteur (Strasbourg) (1971-2008), 2007. http://www.theses.fr/2007STR13212.

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La création de matériaux multifonctionnels en ayant recours à l’auto-assemblage de molécules spécifiques est d’un grand intérêt dans le domaine des nanotechnologies. Dans ce contexte un réel effort a été produit afin d’obtenir le contrôle total de l’auto-organisation de molécules π-conjuguées ; ceci dans le but de créer des architectures supramoléculaires anisotropes et de créer des nano-objets électriquement actifs. Il est en effet connu que l’ordre, à un niveau supramoléculaire, affecte de façon importante les propriétés électroniques d’assemblages moléculaires. Dans ce travail de thèse nous

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41

Tessarolo, J. "Design and synthesis of metallo-supramolecular architectures towards advanced materials." Doctoral thesis, Università degli studi di Padova, 2017. http://hdl.handle.net/11577/3422402.

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Self-assembly is a key step to obtain functional supramolecular objects towards complex matter. With self-assembly of metal ions and well-designed polytopic ligands is possible to access a particular class of supramolecular functional materials: metal-organic polygons and polyhedra endowed with confined space, and functional properties deriving from the building blocks. Herein, firstly is presented a system that in solution self-assembles in a collection of Cu(II) based boxes: a rhomboid and a triangle in dynamic equilibrium. This system is a small constitutional dynamic library (CDL). The des

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42

Riddell, Imogen Anne. "Construction and application of new supramolecular architectures using subcomponent self-assembly." Thesis, University of Cambridge, 2013. http://ethos.bl.uk/OrderDetails.do?uin=uk.bl.ethos.648239.

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43

Pike, Sarah Jane. "Dynamic platinum(II)- based metallosupramolecular architectures." Thesis, University of Edinburgh, 2012. http://hdl.handle.net/1842/7942.

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Over the past two decades, transitions metals have been extensively employed towards the construction (using coordination driven assembly) and operation (using reversible metal-ligand switching motifs) of supramolecular architectures. This Thesis details the investigation of an array of dynamic platinum(II)-based metallosupramolecular architectures and includes a series of model studies on switchable platinum(II) coordination modes. Chapter Two describes the synthesis and study of a series of prototype noninterlocked molecular machines. The inherent dynamics of intramolecular metalligand subst

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44

Schilter, David. "Synthesis and DNA-binding of Metallocyclic Architectures." Thesis, The University of Sydney, 2009. http://hdl.handle.net/2123/5317.

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A new family of cationic N-heterocyclic ligand derivatives was prepared and characterised. Among these compounds are halide salts of the dications [Y(spacer)Y]2+, each of which comprise two N heterocyclic donor groups (Y = 4,4′-bipy, pyz, apyz, apym) linked by a conformationally flexible spacer such as (CH2)n, α,α′-xylylene, 2,6-lutidylene or thiabicyclo[3.3.1]nonane-2,6 diyl. The diquaternary halide salts were converted to NO3- and PF6- salts, and interaction of these bridging ligands with labile palladium(II) and platinum(II) precursors afforded several multinuclear complexes. Bis(4,4′-bipyr

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Schilter, David. "Synthesis and DNA-binding of Metallocyclic Architectures." University of Sydney, 2009. http://hdl.handle.net/2123/5317.

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PhD<br>A new family of cationic N-heterocyclic ligand derivatives was prepared and characterised. Among these compounds are halide salts of the dications [Y(spacer)Y]2+, each of which comprise two N heterocyclic donor groups (Y = 4,4′-bipy, pyz, apyz, apym) linked by a conformationally flexible spacer such as (CH2)n, α,α′-xylylene, 2,6-lutidylene or thiabicyclo[3.3.1]nonane-2,6 diyl. The diquaternary halide salts were converted to NO3- and PF6- salts, and interaction of these bridging ligands with labile palladium(II) and platinum(II) precursors afforded several multinuclear complexes. Bis(4,4

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46

Deng, Shining. "Synthesis of supramolecular architectures using P n -ligands as building blocks." kostenfrei, 2007. http://www.opus-bayern.de/uni-regensburg/volltexte/2008/809/.

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47

Beck, John Benjamin. "Using the Metal-Ligand Interaction to Construct Complex Supramolecular Polymer Architectures." Case Western Reserve University School of Graduate Studies / OhioLINK, 2005. http://rave.ohiolink.edu/etdc/view?acc_num=case1112815582.

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48

Pandoli, Omar <1977&gt. "Supramolecular hybrid organic-inorganic multicomponent architectures in solution and on surface." Doctoral thesis, Alma Mater Studiorum - Università di Bologna, 2008. http://amsdottorato.unibo.it/1068/1/Tesi_Pandoli_Omar.pdf.

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Supramolecular architectures can be built-up from a single molecular component (building block) to obtain a complex of organic or inorganic interactions creating a new emergent condensed phase of matter, such as gels, liquid crystals and solid crystal. Further the generation of multicomponent supramolecular hybrid architecture, a mix of organic and inorganic components, increases the complexity of the condensed aggregate with functional properties useful for important areas of research, like material science, medicine and nanotechnology. One may design a molecule storing a recognition p

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Pandoli, Omar <1977&gt. "Supramolecular hybrid organic-inorganic multicomponent architectures in solution and on surface." Doctoral thesis, Alma Mater Studiorum - Università di Bologna, 2008. http://amsdottorato.unibo.it/1068/.

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Supramolecular architectures can be built-up from a single molecular component (building block) to obtain a complex of organic or inorganic interactions creating a new emergent condensed phase of matter, such as gels, liquid crystals and solid crystal. Further the generation of multicomponent supramolecular hybrid architecture, a mix of organic and inorganic components, increases the complexity of the condensed aggregate with functional properties useful for important areas of research, like material science, medicine and nanotechnology. One may design a molecule storing a recognition p

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50

Savage, Rebecca. "Self-assembled supramolecular π-π architectures : Low-dimensional structures for organic electronics". Strasbourg, 2010. https://publication-theses.unistra.fr/restreint/theses_doctorat/2010/SAVAGE_Rebecca_2010.pdf.

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Contrairement à l'électronique conventionnelle basée sur des matériaux inorganiques, dans le domaine de l'électronique organique, des matériaux organiques à la base de carbone, tel que des polymères ou des petites molécules, sont utilisées comme composants actifs. Le niveau de sophistication de la synthèse chimique moderne permet de produire des composés organiques possédant des propriétés pré-déterminées, faits sur mesure pour des applications spécifiques. En plus, ces matériaux peuvent être utilisés pour créer des architectures moléculaires ascendantes ("bottom-up") en utilisant des techniqu

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