Relevant bibliographies by topics / Supramolecular chemistry, terpyridine, self-assembly

Contents

  1. Journal articles
  2. Dissertations / Theses
  3. Books
  4. Book chapters
  5. Conference papers

Academic literature on the topic 'Supramolecular chemistry, terpyridine, self-assembly'

Author: Grafiati
Published: 4 June 2021
Last updated: 1 February 2022

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Journal articles on the topic "Supramolecular chemistry, terpyridine, self-assembly"

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Wang, Chao, Xin-Qi Hao, Ming Wang, Cunlan Guo, Bingqian Xu, Eric N. Tan, Yan-Yan Zhang, et al. "Self-assembly of giant supramolecular cubes with terpyridine ligands as vertices and metals on edges." Chem. Sci. 5, no. 3 (2014): 1221–26. http://dx.doi.org/10.1039/c3sc52965g.

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Wang, Yun-Chi, Yen-Peng Liang, Jhen-Yu Cai, Yun-Jui He, Yin-Hsuan Lee, and Yi-Tsu Chan. "Metal ion-modulated self-assembly of pseudo-suit[3]anes using crown ether-based terpyridine metalloprisms." Chemical Communications 52, no. 85 (2016): 12622–25. http://dx.doi.org/10.1039/c6cc07452a.

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Xie, Ting-Zheng, Yuchen Yao, Xinyu Sun, Kevin J. Endres, Shiying Zhu, Xiaolei Wu, Hui Li, et al. "Supramolecular arrays by the self-assembly of terpyridine-based monomers with transition metal ions." Dalton Transactions 47, no. 22 (2018): 7528–33. http://dx.doi.org/10.1039/c8dt01283k.

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Lee, Jookyeong, Eun Jung Choi, Imre Varga, Per M. Claesson, Sang-Ho Yun, and Changsik Song. "Terpyridine-functionalized stimuli-responsive microgels and their assembly through metal–ligand interactions." Polymer Chemistry 9, no. 8 (2018): 1032–39. http://dx.doi.org/10.1039/c8py00016f.

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Wang, Ming, Chao Wang, Xin-Qi Hao, Jingjing Liu, Xiaohong Li, Chenglong Xu, Alberto Lopez, et al. "Hexagon Wreaths: Self-Assembly of Discrete Supramolecular Fractal Architectures Using Multitopic Terpyridine Ligands." Journal of the American Chemical Society 136, no. 18 (April 23, 2014): 6664–71. http://dx.doi.org/10.1021/ja501417g.

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Wałęsa-Chorab, Monika, Adam Gorczyński, Damian Marcinkowski, Zbigniew Hnatejko, and Violetta Patroniak. "Supramolecular complexes of cobalt(II), manganese(II) and cadmium(II) with bis(terpyridine) ligand as novel luminescent materials." Polish Journal of Chemical Technology 15, no. 3 (September 1, 2013): 91–95. http://dx.doi.org/10.2478/pjct-2013-0052.

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Abstract Self-assembly of N6-donor bis(terpyridine) ligand L with transition metal ions: Co(II), Mn(II) and Cd(II) leads to a formation of three kinds of supramolecular complexes. In the electronic absorption and emission spectra of supramolecular complexes additional bands were observed what was ascribed to the coordination of ligand molecules to metal ions. Luminescence properties of these complexes strongly depend on the kind of metal ions and counter ions. The effective blue luminescence was observed in the case of Mn(II) and Cd(II) complexes in which all N-donor atoms of ligand molecules coordinate with the metal center
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Wang, Yanan, Longxin Chen, Ting Liu, and Duobin Chao. "Coordination-driven discrete metallo-supramolecular assembly for rapid and selective photochemical CO2 reduction in aqueous solution." Dalton Transactions 50, no. 18 (2021): 6273–80. http://dx.doi.org/10.1039/d1dt00692d.

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A discrete metallo-supramolecular assembly bearing six iron(ii) centers and twelve terpyridine fragments has been developed for highly efficient and selective photochemical CO2 reduction with an organic TADF photosensitizer.
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Wang, Shih-Yu, Jyun-Yang Huang, Yen-Peng Liang, Yun-Jui He, Yu-Sheng Chen, Yi-Yang Zhan, Shuichi Hiraoka, Yi-Hung Liu, Shie-Ming Peng, and Yi-Tsu Chan. "Multicomponent Self-Assembly of Metallo-Supramolecular Macrocycles and Cages through Dynamic Heteroleptic Terpyridine Complexation." Chemistry - A European Journal 24, no. 37 (June 13, 2018): 9274–84. http://dx.doi.org/10.1002/chem.201801753.

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Veliks, Janis, Jui-Chang Tseng, Karla I. Arias, Florian Weisshar, Anthony Linden, and Jay S. Siegel. "Linear bilateral extended 2,2′:6′,2′′-terpyridine ligands, their coordination complexes and heterometallic supramolecular networks." Chem. Sci. 5, no. 11 (2014): 4317–27. http://dx.doi.org/10.1039/c4sc01025f.

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Combination of five- and six-membered rings allows creation of 2,2′:6′,2′′-terpyridine derivatives mimicking the topology of 5,5′-functionalized 2,2′-bipyridine. This molecular design led to the assembly of heterometallic supramolecular networks.
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Mansfeld, Ulrich, Andreas Winter, Martin D. Hager, Wolfgang Günther, Esra Altuntaş, and Ulrich S. Schubert. "A Homotelechelic bis-terpyridine macroligand: One-step synthesis and its metallo-supramolecular self-assembly." Journal of Polymer Science Part A: Polymer Chemistry 51, no. 9 (February 14, 2013): 2006–15. http://dx.doi.org/10.1002/pola.26586.

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Dissertations / Theses on the topic "Supramolecular chemistry, terpyridine, self-assembly"

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Eryazici, Ibrahim. "SUPRAMOLECULAR CHEMISTRY OF FUNCTIONALIZED TERPYRIDINES." University of Akron / OhioLINK, 2007. http://rave.ohiolink.edu/etdc/view?acc_num=akron1195677178.

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Zhu, Shiying. "Terpyridine-based, Coordination-driven, 2D and 3D Supramolecular Architectures." University of Akron / OhioLINK, 2017. http://rave.ohiolink.edu/etdc/view?acc_num=akron1490368620583045.

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Hong, Wei. "Temperature-Dependent Supramolecular Cages Self-Assembled By Tristerpyridine and Transition Metal Ions." University of Akron / OhioLINK, 2017. http://rave.ohiolink.edu/etdc/view?acc_num=akron1490352933805703.

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Zheng, Keqin. "Design and Construction of Metallo-Supramolecular Terpyridine Possessing Higher Order Structure." University of Akron / OhioLINK, 2013. http://rave.ohiolink.edu/etdc/view?acc_num=akron1375283764.

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Wu, Xiaolei. "COORDINATION-DRIVEN SELF-ASSEMBLY OF TERPYRIDINE-BASED SUPRAMOLECULES." University of Akron / OhioLINK, 2017. http://rave.ohiolink.edu/etdc/view?acc_num=akron1490372164176458.

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Ludlow, James M. III. "Design and Synthesis of Terpyridine based Metallo-Supramolecular Architectures." University of Akron / OhioLINK, 2015. http://rave.ohiolink.edu/etdc/view?acc_num=akron1444989836.

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Yao, Yuchen. "The Construction of Supramolecular Arrays by Coordination Driven Stepwise Self-Assembly of Terpyridine-Based Building Blocks and Transition Metal Ions (Ru2+, Fe2+, Zn2+)." University of Akron / OhioLINK, 2017. http://rave.ohiolink.edu/etdc/view?acc_num=akron1490370382150615.

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Yeung, Ching-lam Margaret, and 楊靖琳. "Design and synthesis of luminescent alkynylplatinum (II) terpyridine complexes and their function as optical probes for biomolecules and ions : from self-aggregarion, supramolecular assembly to host-guest chemistry." Thesis, The University of Hong Kong (Pokfulam, Hong Kong), 2013. http://hdl.handle.net/10722/208590.

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A number of cationic water-soluble alkynylplatinum(II) terpyridine complexes, [Pt(tpy){C≡CCH2OC6H3-(CH2OH)2-3,5}]OTf, [Pt(tBu3tpy){C≡CCH2OC6H3- (CH2OH)2-3,5}]Cl, [Pt(tpy){C≡CCH2OC6H4-(CH2OH)-4}]OTf, [Pt(tpy){C≡CC6H3- (CH2OH)2-3,5}]OTf, [Pt(tpy){C≡CC6H4-(CH2OH)-4}]OTf, [Pt(tpy)(C≡C－C≡CH)]OTf and [Pt(tpy){C≡CC6H4(CH2NMe3)-4}](OTf)2, have been synthesized. Phosphate anion derivatives of polyanionic nature, e.g. adenosine triphosphate and tyrosine-containing phosphopeptide, were employed to investigate the induced supramolecular helical assembly behaviors of several of the water-soluble platinum(II) complexes through the study of their UV-vis absorption, emission and circular dichroism (CD) spectroscopies. The extent of such induced self-aggregation properties has been shown to be dependent on the concentration of substrates and capable of screening their respective structurally similar analogues. Two of the complexes were further explored for their use as label-free detection probes for real-time monitoring of the conversion of these phosphate anion derivatives to their metabolic products catalyzed by several biologically important enzymes. Michaelis-Menten analyses have been performed to determine the kinetic parameters. Supramolecular self-assembly and disassembly behaviors of water-soluble platinum(II) complexes have also been explored for their sensing applications for biomacromolecules with quantitative analyses based on UV-vis, emission and CD spectral titration studies. Making use of the selective binding affinity of aptamers towards their target substrates, the extent of self-assembly of the platinum(II) complexes in the presence of lysozyme and thrombin, which arose from their electrostatic interactions with the negatively charged aptamers, could be modulated for the quantification of these substrates. The potential applicability of this probing strategy in real biological environment has been assessed. Other than that, CD spectroscopic studies revealed the formation of supramolecular helical assembly of the platinum(II) complexes upon electrostatic interaction with heparin. Such helical conformation of the heparin–complex mixture together with the distribution of the negatively charged functionalities on the heparin have endowed the complex with high differentiating power for screening possible interfering analogues. Insulin has also been employed as a template for inducing the self-assembly of the platinum(II) complex. Changes in negative surface charge distribution on insulin, brought about by its conformational changes upon conversion to insulin amyloid under destabilizing conditions, have resulted in different extent of induced self-assembly of the metal complex. Spectral changes of the platinum(II) complex has provided a convenient monitoring of insulin amyloid formation, with kinetic parameters determined. A number of platinum(II) complexes with nucleobase-functionalized alkynyl ligands, [Pt(tpy)(C≡CCH2-T-1)]OTf, [Pt(tBu3tpy)(C≡CCH2T-1)]OTf, [Pt(tpy)(C≡C– CH2-A-9)]OTf, [Pt(tpy)(C≡CCH2-C-1)]OTf and [Pt(tpy)(C≡CCH2-G-9)]OTf (T = thymine; A = adenine; C = cytosine; and G = guanine), and amide-functionalized terpyridine ligands, [Pt{tpy–(CONHPh)2}(C≡CPh)]PF6 and [Pt{tpy–(CONHC6H13)2} (C≡CPh)]PF6, have been synthesized. Cation-binding properties of [Pt(tpy)(C≡CCH2-T-1)]OTf have been examined using UV-vis and emission spectroscopies, and ESI-MS. Pronounced selectivity towards Hg2+ ions was obtained due to the formation of thymine–Hg2+–thymine base pair, through which the Pt… Pt interactions were turned on. Such binding mechanism has been confirmed with the use of a control complex [Pt(tBu3tpy)(C≡CCH2T-1)]OTf and resonance light-scattering experiments. Anion-binding properties of the complexes with amide-functionalized terpyridine moieties towards spherical and non-spherical anions have been examined with UV-vis and emission spectral titration studies. Drastic color changes were observed for [Pt{tpy–(CONHC6H13)2} (C≡CPh)]PF6 in acetone upon F– ion addition, which was attributed to the F– ion-induced deprotonation of the amide functionalities.
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Chemistry
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Doctor of Philosophy
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Young, Michael Christopher. "Self-Assembly of Functionalized Supramolecular Structures." Thesis, University of California, Riverside, 2014. http://pqdtopen.proquest.com/#viewpdf?dispub=3644049.

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Enzymes are capable of exquisite selectivity in catalysis chemical reactions because of a well-evolved mechanism that binds substrates in internal active sites based on size and shape complementarity. The cavities of these enzymes are decorated with organic or inorganic groups which can promote reactivity once the substrate is non-covalently bound. Synthetic molecular hosts to date have been able to bind to substrates in a similar, biomimetic fashion, but functionalized molecular hosts are still virtually unknown.

One convenient way to prepare molecular hosts is by the self-assembly of organic coordinating ligands with suitable metal salts. The reversible dative bonds holding these cage structures together allow incorrect products to break apart and reform, favoring creation of the most thermodynamically stable product. This leads to discrete, solution phase cages that can function as cavity-containing hosts. Some of these hosts have shown efficacy as catalysts for pericyclic reactions due to favorable transition states of the bound substrates. These cages, however, fail to orient reactive functional groups into their interiors. Truly biomimetic cages will require modifying traditional self-assembled targets to incorporate these reactive functionalities.

This work explores the self-assembly of metal-organic cages displaying covalent modifications on their interior. Incorporation of unreactive and poorly reactive groups was found to have a significant impact on the outcome of the self-assembly process. Cages with endohedral alcoholic functionality were found to have different binding properties than unfunctionalized analogs. Cages with introverted alcohol groups were also exploited for their ability to self-catalyze reactions on the interior of the hosts. The metal vertices themselves could also be used as functional groups, and showed the ability to sense neutral analytes in hybrid dative/hydrogen bonded self-assemblies.

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Iden, Hassan. "From molecular tweezers to metallocavitands : self-assembly and supramolecular chemistry." Thesis, Université Laval, 2014. http://www.theses.ulaval.ca/2014/30840/30840.pdf.

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Ce mémoire décrit la synthèse d’hôtes organiques et organométalliques contenant des motifs riches en électrons, particulièrement le tétrathiafulvalène (TTF), pour la complexation supramoléculaire de fullerènes C60 et C70. Le chapitre 1 est une revue de la littérature qui présente les notions de cavitant, de métallocavitant et des hôtes supramoléculaires. Le chapitre 2 présente les méthodes de caractérisation utilisées dans ce travail. Le chapitre 3 est consacré à une nouvelle méthode de synthèse de pinces moléculaires et des récepteurs tripodaux contenant l’unité riche en électrons (TTF). Les pinces triazoles ont été préparées par chimie « clic » entre l'azoture -TTF et des dérivés benzéniques disubstitués en position 1 et 3 par un acétylène. La réaction de l'azoture-TTF et des 1,3, 5-benzènes trisubstitués a donné des récepteurs tripodaux. L'affinité des hôtes avec les fullerènes C60 et C70 a été étudiée par la méthode optique spectroscopique UV-vis dans quatre solvants différents. La constante d’association la plus élevée a été calculée pour l’hôte 4 dans le chlorobenzène. Cependant, le récepteur tripodal n'a pas montré une affinité importante envers les fullerènes. Le chapitre 4 est consacré à la synthèse des nouveaux metallocavitands de zirconium TTF- Zr3 préparés par la méthode d’agrégation. Un seul hôte a été isolé et caractérisé par la méthode spectroscopique. Dans ce chapitre, nous présentons l'étude des interactions supramoléculaires avec les fullerènes en surveillant la réponse UV-vis à l’addition d’une quantité croissante de fullerènes à la solution contenant l’hôte. Le chapitre 5 décrit la synthèse de nouveaux metallocavitants de Zr3 à partir de la réaction de dichlorure de zirconocène sur l'acide carboxylique. Quatre metallocavitants de Zr3 ont été préparés. Les structures cristallographiques, les propriétés photophysiques et leurs utilisations potentielles en tant que matériaux émissifs bleus ont été présentées. Le chapitre 6 est séparé en trois sections. La première section décrit la synthèse et l’affinité de metallocavitant de tantale (V) avec les fullerènes. La deuxième section illustre la tentative de synthèse d’une librairie de Zr3 en utilisant la réaction de couplage croisée. Enfin, la dernière section présente la synthèse du nouveau metallocavitant de Ta3Carbox obtenu par la méthode d’agrégation à partir de la réaction de Cp*TaMe4 avec de l'acide 4 - iodobenzoïque. La structure est étudiée par rayons X.
This thesis described the synthesis of organic and organometallic hosts containing electron rich units in particularly tetrathiafulvalene (TFF) to bind fullerenes C60 and C70. Chapter two illustrates the different analysis techniques used in this thesis. Chapter three described new method for the synthesis of tweezers-like TTF and tripodal TTF molecules in addition to their binding affinity towards fullerenes C60 and C70. The tweezers-like TTF were prepared by click chemistry from azide-TTF and 1,3 substituted benzene. Similarly, the reaction of azide-TTF and 1,3, 5 substituted benzene yielded the tripodal-TTF receptor. The affinity toward fullerenes C60 and C70 were studied in four different solvents. The highest binding constant was calculated for host 4 in chlorobenzene toward fullerene C70. Moreover, solvent dependant behavior was observed with the studied host. However, the tripodal receptor did not showed significant affintity towards fullerenes. Chapter four described the synthesis of new TTF-Zr3 metallocavitand by coordination method; two hosts were isolated and characterized. In this chapter we present the binding study toward fullerenes by monitoring the UV-vis response to increasing amount of fullerenes added to the solution of the host. Chapter five described the synthesis of new Zr3 metallocavitand in one pot reaction from the reaction of zirconocene dichloride with carboxylic acid in aqueous media. Four Zr3 metallocavitand were prepared and the crystallography was presented in addition to the photophysical properties and their potential uses as blue emissive materials. The last chapter is separated into three sections. The first section described our early work on tantalum (V) metallocavitand in addition to their hosting capability toward fullerenes. The second section illustrate the tentative has been committed to the design and synthesis of Zr3 library using cross-coupling reaction in addition to the synthesis of extended Zr3-cinnamate metallocavitand. Lastly, the last section illustrates the synthesis of new Ta3-Carbox achieved by aggregation method from reaction of Cp*TaMe4 with 4-iodobenzoic acid. The single X-ray structure revealed a new structure with trimetallic core comparable to the core observed for tantalum metallocavitand.
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Books on the topic "Supramolecular chemistry, terpyridine, self-assembly"

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1937-, Larsson Kåre, ed. Inorganic and organic 3D-nets: From supramolecular chemistry and self assembly to crystal engineering. New York: Elsevier, 2005.

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(Editor), J. P. Sauvage, and M. W. Hosseini (Editor), eds. Comprehensive Supramolecular Chemistry : Templating, Self-Assembly and Self-Organization (Comprehensive Supramolecular Chemistry). Pergamon, 1996.

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Lindoy, L. F., and I. M. Atkinson. Self-Assembly in Supramolecular Systems (Monographs in Supramolecular Chemistry). Royal Society of Chemistry, 2001.

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Frédéric, Fages, and Araki K, eds. Low molecular mass gelators: Design, self-assembly, function. Berlin: Springer, 2005.

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Frederic, Fages, and Araki K, eds. Low molecular mass gelators: Design, self-assembly, function. Berlin: Springer, 2005.

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Fages, Frederic. Low Molecular Mass Gelators : Design, Self-Assembly, Function (Topics in Current Chemistry) (Topics in Current Chemistry). Springer, 2005.

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M, Rotello Vincent, and Thayumanavan Sankaran, eds. Molecular recognition and polymers: Control of polymer structure and self-assembly. Hoboken, N.J: Wiley, 2008.

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Lin, Nian, and Sebastian Stepanow. Designing low-dimensional nanostructures at surfaces by supramolecular chemistry. Edited by A. V. Narlikar and Y. Y. Fu. Oxford University Press, 2017. http://dx.doi.org/10.1093/oxfordhb/9780199533046.013.10.

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This article describes the use of supramolecular chemistry to design low-dimensional nanostructures at surfaces. In particular, it discusses the design strategies of two types of low-dimensional supramolecular nanostructures: structures stabilized by hydrogen bonds and structures stabilized by metal-ligand co-ordination interactions. After providing an overview of hydrogen-bond systems such as 0D discrete clusters, 1D chains, and 2D open networks and close-packed arrays, the article considers metal-co-ordination systems. It also presents experimental results showing that both hydrogen bonds and metal co-ordination offer protocols to achieve unique nanostructured systems on 2D surfaces or interfaces. Noting that the conventional 3D supramolecular self-assembly has generated a vast number of nanostructures revealing high complexity and functionality, the article suggests that 2D approaches can be applied to substrates with different symmetries as well as physical and chemical properties.
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Book chapters on the topic "Supramolecular chemistry, terpyridine, self-assembly"

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Ashton, Peter R., Richard A. Bissell, Douglas Philp, Neil Spencer, and J. Fraser Stoddart. "Self-Assembly in Chemical Systems." In Supramolecular Chemistry, 1–16. Dordrecht: Springer Netherlands, 1992. http://dx.doi.org/10.1007/978-94-011-2492-8_1.

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Cantrill, S. J., M. C. T. Fyfe, F. M. Raymo, and J. F. Stoddart. "Probing Self-Assembly by NMR." In NMR in Supramolecular Chemistry, 1–18. Dordrecht: Springer Netherlands, 1999. http://dx.doi.org/10.1007/978-94-011-4615-9_1.

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Grotzfeld, R. M., N. R. Branda, C. Valdes, and J. Rebek. "Control of Self-Assembly by Acid-Base Chemistry." In Supramolecular Stereochemistry, 195–97. Dordrecht: Springer Netherlands, 1995. http://dx.doi.org/10.1007/978-94-011-0353-4_24.

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Williams, A. F., C. Piguet, and R. F. Carina. "Following the Self-Assembly Process in Solution." In Transition Metals in Supramolecular Chemistry, 409–23. Dordrecht: Springer Netherlands, 1994. http://dx.doi.org/10.1007/978-94-015-8380-0_22.

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Fredericks, John R., and Andrew D. Hamilton. "Metal Template Control of Self-Assembly in Supramolecular Chemistry." In Perspectives in Supramolecular Chemistry, 1–39. Chichester, UK: John Wiley & Sons, Ltd., 2007. http://dx.doi.org/10.1002/9780470511473.ch1.

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Lin, Xiankun, Zhiguang Wu, and Qiang He. "Controlled Molecular Assembly Toward Self-propelled Micro-/Nanomotors." In Supramolecular Chemistry of Biomimetic Systems, 259–81. Singapore: Springer Singapore, 2017. http://dx.doi.org/10.1007/978-981-10-6059-5_11.

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Saalfrank, Rolf W., and Bernhard Demleitner. "Ligand and Metal Control of Self-Assembly in Supramolecular Chemistry." In Perspectives in Supramolecular Chemistry, 1–51. Chichester, UK: John Wiley & Sons, Ltd., 2007. http://dx.doi.org/10.1002/9780470511510.ch1.

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Constable, E. C. "Metal-Ions: A Self-Assembly Motif in Supramolecular Oligomers." In Transition Metals in Supramolecular Chemistry, 81–99. Dordrecht: Springer Netherlands, 1994. http://dx.doi.org/10.1007/978-94-015-8380-0_4.

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Kim, Kimoon. "Self-Assembly of Interlocked Structures with Cucurbituril, Metal Ions and Metal Complexes." In Perspectives in Supramolecular Chemistry, 371–402. Chichester, UK: John Wiley & Sons, Ltd., 2007. http://dx.doi.org/10.1002/9780470511510.ch8.

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Yang, Yong, and Chuan-Feng Chen. "Hydrogen Bonding-Mediated Self-assembly of Aromatic Supramolecular Duplexes." In Lecture Notes in Chemistry, 115–36. Berlin, Heidelberg: Springer Berlin Heidelberg, 2015. http://dx.doi.org/10.1007/978-3-662-45756-6_4.

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Conference papers on the topic "Supramolecular chemistry, terpyridine, self-assembly"

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Romero, María J., Luis M. González-Barcia, Manuel R. Bermejo, M. Isabel Fernández, and Esther Gómez-Fórneas. "Supramolecular self-assembly of a symmetric imine ligand functionalized with a dansyl fluorophore moiety." In The 20th International Electronic Conference on Synthetic Organic Chemistry. Basel, Switzerland: MDPI, 2016. http://dx.doi.org/10.3390/ecsoc-20-d002.

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Bruck, Hugh A., Alan L. Gershon, and Satyandra K. Gupta. "Enhancement of Mechanical Engineering Curriculum to Introduce Manufacturing Techniques and Principles for Bio-Inspired Product Development." In ASME 2004 International Mechanical Engineering Congress and Exposition. ASMEDC, 2004. http://dx.doi.org/10.1115/imece2004-60584.

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Bio-inspired products and devices take their inspiration from nature [Gold00]. Current mechanical engineering curricula do not cover manufacturing techniques and principles needed to develop such products and devices. We have been enhancing the mechanical engineering undergraduate curriculum by integrating recent advances in the manufacturing of bio-inspired products and devices through the following activities: 1. Insert a new sequence of instructional materials on bio-inspired concepts into the mechanical engineering curriculum. 2. Disseminate the materials developed for the new modules and course notes through a dedicated web site. As a result of the curriculum enhancement, a new generation of mechanical engineers will acquire the knowledge necessary to develop products and conduct research for a wide variety of applications utilizing bio-inspired concepts. The project (1) integrates emerging manufacturing technologies based on biological principles into the Mechanical Engineering curriculum, (2) utilizes multi-media technology for disseminating course content, and (3) trains graduate students and faculty participating in its implementation in an emerging technology and thereby contribute to faculty development. Specifically, curriculum is being developed that discusses the following manufacturing technologies and principles: 1. Concurrent Fabrication and Assembly: Manufacturing techniques and principles, such as solid freeform fabrication, compliant mechanisms, and multi-stage molding, that can eliminate the manufacturing and assembly of individual components as is the case for almost all natural systems. 2. Self Assembly: Principles for manufacturing a variety of products from a few building blocks using bio-inspired techniques such as templating and supramolecular chemistry. 3. Functionally Graded Materials: Bio-inspired development of new products through the gradual variation of material properties at multiple length scales through manufacturing processes such as sputtering and powder processing. The curriculum development effort makes two significant contributions to mechanical engineering education: (a) integration of a new research on bio-inspired products and devices into the mechanical engineering curriculum through new courses and revision of existing courses, (b) development of new instructional material for mechanical engineering education based on bio-inspired concepts. There are also broader impacts in the following areas: (a) undergraduate students who might not otherwise puruse studies in mechanical engineering will be attracted to the multidisciplinary area of bio-inspired products, (b) dissemination of the curriculum enhancement through conference presentations, a workshop, and dedicated web site, and (c) a biologically-oriented pedagogical approach to mechanical engineering education that ensures broader access to the knowledge needed to enhance the interest and skills of future engineers and researchers educated through this research program.
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