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Journal articles on the topic 'Symmetric top molecules'

Author: Grafiati

Published: 4 June 2021

Last updated: 1 February 2022

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1

Chang, Zhe. "Spectra of symmetric-top molecules and the quantum-deformed-symmetric-top model." Physical Review A 46, no. 3 (August 1, 1992): 1400–1412. http://dx.doi.org/10.1103/physreva.46.1400.

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2

Mitra, Debayan, Nathaniel B. Vilas, Christian Hallas, Loïc Anderegg, Benjamin L. Augenbraun, Louis Baum, Calder Miller, Shivam Raval, and John M. Doyle. "Direct laser cooling of a symmetric top molecule." Science 369, no. 6509 (September 10, 2020): 1366–69. http://dx.doi.org/10.1126/science.abc5357.

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Ultracold polyatomic molecules have potentially wide-ranging applications in quantum simulation and computation, particle physics, and quantum chemistry. For atoms and small molecules, direct laser cooling has proven to be a powerful tool for quantum science in the ultracold regime. However, the feasibility of laser-cooling larger, nonlinear polyatomic molecules has remained unknown because of their complex structure. We laser-cooled the symmetric top molecule calcium monomethoxide (CaOCH3), reducing the temperature of ~104 molecules from 22 ± 1 millikelvin to 1.8 ± 0.7 millikelvin in one dimension and state-selectively cooling two nuclear spin isomers. These results demonstrate that the use of proper ro-vibronic transitions enables laser cooling of nonlinear molecules, thereby opening a path to efficient cooling of chiral molecules and, eventually, optical tweezer arrays of complex polyatomic species.

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3

McDowell, Robin S. "Rotational partition functions for symmetric‐top molecules." Journal of Chemical Physics 93, no. 4 (August 15, 1990): 2801–11. http://dx.doi.org/10.1063/1.458865.

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4

Wang, S. P., and M. Schwartz. "Rotational Diffusion in Prolate Symmetric top Molecules." Spectroscopy Letters 21, no. 9-10 (December 1988): 919–25. http://dx.doi.org/10.1080/00387018808082354.

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5

Wall, Michael L., Kenji Maeda, and Lincoln D. Carr. "Simulating quantum magnets with symmetric top molecules." Annalen der Physik 525, no. 10-11 (September 23, 2013): 845–65. http://dx.doi.org/10.1002/andp.201300105.

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6

Ghoshal, Sharmistha, and Pradip N. Ghosh. "Forbidden rotational transitions in symmetric top molecules." Journal of Molecular Spectroscopy 110, no. 2 (April 1985): 364–68. http://dx.doi.org/10.1016/0022-2852(85)90302-9.

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7

Jagod, Mary-Frances, and Takeshi Oka. "Inertial defects of planar symmetric top molecules." Journal of Molecular Spectroscopy 139, no. 2 (February 1990): 313–27. http://dx.doi.org/10.1016/0022-2852(90)90068-2.

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8

Wall, M. L., K. Maeda, and Lincoln D. Carr. "Realizing unconventional quantum magnetism with symmetric top molecules." New Journal of Physics 17, no. 2 (February 4, 2015): 025001. http://dx.doi.org/10.1088/1367-2630/17/2/025001.

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9

Yu, Phelan, Lawrence W. Cheuk, Ivan Kozyryev, and John M. Doyle. "A scalable quantum computing platform using symmetric-top molecules." New Journal of Physics 21, no. 9 (September 24, 2019): 093049. http://dx.doi.org/10.1088/1367-2630/ab428d.

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10

Gershnabel, E., and I. Sh Averbukh. "Deflection of rotating symmetric top molecules by inhomogeneous fields." Journal of Chemical Physics 135, no. 8 (August 28, 2011): 084307. http://dx.doi.org/10.1063/1.3626873.

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11

Anderson, Roger W. "Tracks of Symmetric Top Molecules in Hexapole Electric Fields." Journal of Physical Chemistry A 101, no. 41 (October 1997): 7664–73. http://dx.doi.org/10.1021/jp971313s.

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12

Wei, Qi, Sabre Kais, Bretislav Friedrich, and Dudley Herschbach. "Entanglement of polar symmetric top molecules as candidate qubits." Journal of Chemical Physics 135, no. 15 (October 17, 2011): 154102. http://dx.doi.org/10.1063/1.3649949.

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13

Chen, Kuo-Mei. "Laser-Induced Alignments of Symmetric and Asymmetric Top Molecules." Journal of the Chinese Chemical Society 48, no. 3 (June 2001): 609–12. http://dx.doi.org/10.1002/jccs.200100091.

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14

Zare, Richard N. "Photofragment angular distributions from oriented symmetric-top precursor molecules." Chemical Physics Letters 156, no. 1 (March 1989): 1–6. http://dx.doi.org/10.1016/0009-2614(89)87070-8.

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15

Plíva, Josef. "Anharmonic constants for degenerate modes of symmetric top molecules." Journal of Molecular Spectroscopy 139, no. 2 (February 1990): 278–85. http://dx.doi.org/10.1016/0022-2852(90)90065-x.

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16

Hu, Wan-Ping, Sean A. Harris, Peter W. Harland, and Leon F. Phillips. "Collisional reorientation of symmetric-top molecules in stark fields." International Journal of Quantum Chemistry 71, no. 1 (1999): 75–82. http://dx.doi.org/10.1002/(sici)1097-461x(1999)71:1<75::aid-qua8>3.0.co;2-g.

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17

Voges, K., J. Gripp, H. Hartwig, and H. Dreizler. "Analysis of Torsion in a Three-Top Molecule. Torsional Barrier and Moment of Inertia of Trimethyl Ethynyl Germane." Zeitschrift für Naturforschung A 51, no. 4 (April 1, 1996): 299–305. http://dx.doi.org/10.1515/zna-1996-0409.

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Internal rotation effects for a large number of molecules containing one or two symmetric internal rotors have been investigated using microwave spectroscopy. The high resolution of molecular beam Fourier transform microwave spectroscopy revealed now the internal rotation fine structure in the rotational spectrum of trimethyl ethynyl germane, (CH3)3GeC=CH. After assigning the rotational transition J = 1 → 0 in the vibrational and torsional ground state to the symmetry species of the molecular symmetry group G162 , the torsional barrier V3 and the rotational constant B0 could be determined to (4.5±0.2) kJ/mol and (1823.370±0.010) MHz, respectively.

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18

Garrett, W. R. "Critical binding and electron scattering by symmetric-top polar molecules." Journal of Chemical Physics 141, no. 16 (October 28, 2014): 164318. http://dx.doi.org/10.1063/1.4898730.

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19

Ziegler, L. D., Y. C. Chung, and Y. P. Zhang. "Resonance rotational hyper‐Raman scattering intensities of symmetric top molecules." Journal of Chemical Physics 87, no. 8 (October 15, 1987): 4498–509. http://dx.doi.org/10.1063/1.452863.

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20

Ernesti, A., and H. J. Korsch. "On rotational rainbow structures for initially excited symmetric top molecules." Journal of Physics B: Atomic, Molecular and Optical Physics 26, no. 22 (November 28, 1993): 4257–68. http://dx.doi.org/10.1088/0953-4075/26/22/028.

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21

Weida, Miles J., and Charles S. Parmenter. "Aligning symmetric and asymmetric top molecules via single photon excitation." Journal of Chemical Physics 107, no. 18 (November 8, 1997): 7138–47. http://dx.doi.org/10.1063/1.474955.

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22

Schalk, Oliver, and Paul Hockett. "Rotational dephasing of symmetric top molecules: Analytic expressions and applications." Chemical Physics Letters 517, no. 4-6 (December 2011): 237–41. http://dx.doi.org/10.1016/j.cplett.2011.10.046.

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23

Urban, Š., D. Papoušek, and M. Garcia Hernandez. "Effective Hamiltonian for degenerate vibrational states in symmetric top molecules." Journal of Molecular Spectroscopy 124, no. 2 (August 1987): 272–84. http://dx.doi.org/10.1016/0022-2852(87)90141-x.

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24

Watson, James K. G. "Quadratic Herman-Wallis factors for symmetric- and asymmetric-top molecules." Journal of Molecular Spectroscopy 153, no. 1-2 (May 1992): 211–24. http://dx.doi.org/10.1016/0022-2852(92)90470-9.

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25

Chang-Yuan, Chen, Sun Guo-Hua, Wang Xiao-Hua, Sun Dong-Sheng, You Yuan, Lu Fa-Lin, and Dong Shi-Hai. "Exact solutions to Stark effect of rigid symmetric-top molecules." Acta Physica Sinica 70, no. 18 (2021): 180301. http://dx.doi.org/10.7498/aps.70.20210214.

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26

Brom, Alrik J. van den, T. Peter Rakitzis, and Maurice H. M. Janssen. "Molecular frame properties from photodissociation of laboratory-oriented symmetric top and chiral molecules." Physica Scripta 73, no. 1 (December 22, 2005): C83—C88. http://dx.doi.org/10.1088/0031-8949/73/1/n15.

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27

Zhang, H., F. Billard, X. Yu, O. Faucher, and B. Lavorel. "Dissipation dynamics of field-free molecular alignment for symmetric-top molecules: Ethane (C2H6)." Journal of Chemical Physics 148, no. 12 (March 28, 2018): 124303. http://dx.doi.org/10.1063/1.5019356.

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28

Papoušek, Dušan. "Forbidden transitions in molecular vibrational-rotational spectroscopy." Collection of Czechoslovak Chemical Communications 54, no. 10 (1989): 2555–630. http://dx.doi.org/10.1135/cccc19892555.

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A review is given of the forbidden ( more precisely: perturbation allowed) transistions between molecular vibrational-rotational states including transistions which are induced by the electric dipole and quadrupole moments and the magnetic dipole moment. The basic theory of these transistions is outlined starting with the overall symmetry selection rules, followed by the discussion of the spin statistics isomers, approximate selection rules for the usual vibrational-rotational transistions, and forbidden transistions induced by the electric quadrupole and magnetic dipole moments. Forbidden transistions due to the vibrationally and rotationally induced electric dipole moments are the discussed in detail for symmetric top and spherical top molecules with the emphasis on the physical nature of the various phenomena leading to these transistions. A summary is also given of the most important experimental work on the forbidden transistions in diatomic molecules and polar as well as nonpolar polyatomics.

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29

Brooks, Philip R., Peter W. Harland, Leon F. Phillips, and Howard S. Carman. "Collision dynamics of alkali-metal atoms with oriented symmetric-top molecules." Journal of Physical Chemistry 96, no. 4 (February 1992): 1557–61. http://dx.doi.org/10.1021/j100183a014.

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30

Burrows, B. L., M. Cohen, and T. Feldmann. "Stark energy levels of symmetric-top molecules: an elementary algebraic treatment." Journal of Physics B: Atomic, Molecular and Optical Physics 28, no. 19 (October 14, 1995): 4249–57. http://dx.doi.org/10.1088/0953-4075/28/19/010.

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31

Déjardin, J. L. "Nonlinear harmonic components of the electric polarization of symmetric-top molecules." Journal of Chemical Physics 117, no. 4 (July 22, 2002): 1750–58. http://dx.doi.org/10.1063/1.1488578.

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32

Coffey, W. T., and Y. P. Kalmykov. "The langevin equation for the dipole vector of symmetric top molecules." Journal of Molecular Liquids 49 (September 1991): 79–85. http://dx.doi.org/10.1016/0167-7322(91)80066-d.

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33

Levine, R. D., and R. B. Bernstein. "Rotational state dependence of the reactivity of oriented symmetric top molecules." Chemical Physics Letters 132, no. 1 (November 1986): 11–15. http://dx.doi.org/10.1016/0009-2614(86)80685-6.

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34

Storozhev, A. V., and M. L. Strekalov. "Rotational energy relaxation of symmetric top molecules by collisions with atoms." Chemical Physics 200, no. 1-2 (November 1995): 125–35. http://dx.doi.org/10.1016/0301-0104(95)00226-e.

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35

Ho, P. J., D. Starodub, D. K. Saldin, V. L. Shneerson, A. Ourmazd, and R. Santra. "Molecular structure determination from x-ray scattering patterns of laser-aligned symmetric-top molecules." Journal of Chemical Physics 131, no. 13 (October 7, 2009): 131101. http://dx.doi.org/10.1063/1.3245404.

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36

Jang, Joonkyung, and Kook Joe Shin. "Extended diffusion theory of reorientation of symmetric top molecules with internal rotation." Journal of Chemical Physics 106, no. 17 (May 1997): 6813–19. http://dx.doi.org/10.1063/1.473708.

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37

Hsieh, H. C., and W. C. Ermler. "Numerical and analytical representations of Eulerian angle matrices for symmetric top molecules." Computer Physics Communications 66, no. 2-3 (September 1991): 266–70. http://dx.doi.org/10.1016/0010-4655(91)90075-v.

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38

Maergoiz, A. I., and J. Troe. "Weak‐ and strong‐field Stark energy levels of symmetric top dipolar molecules." Journal of Chemical Physics 99, no. 5 (September 1993): 3218–23. http://dx.doi.org/10.1063/1.465130.

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39

Koput, J. "Quasi-symmetric top molecule approach to the rotational-vibrational problem of CH3XY molecules: Application to CH3OD." Journal of Molecular Spectroscopy 111, no. 2 (June 1985): 440–50. http://dx.doi.org/10.1016/0022-2852(85)90018-9.

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40

Ni, C. K., and G. W. Flynn. "Correlation between molecular recoil and molecular orientation in collisions of symmetric top molecules with hot hydrogen atoms." Chemical Physics Letters 193, no. 1-3 (May 1992): 69–76. http://dx.doi.org/10.1016/0009-2614(92)85684-3.

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41

Meyer, Henning. "Determination of alignment parameters for symmetric top molecules using nonresonant two-photon absorption." Chemical Physics Letters 230, no. 6 (December 1994): 510–18. http://dx.doi.org/10.1016/0009-2614(94)01195-8.

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42

Ortigoso, Juan, and Rafael Escribano. "Convergence properties of a pertubative treatment for Coriolis coupling in symmetric top molecules." Journal of Molecular Spectroscopy 148, no. 1 (July 1991): 136–48. http://dx.doi.org/10.1016/0022-2852(91)90043-a.

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43

Sakimoto, Kazuhiro. "On the capture rate constant of collisions between ions and symmetric-top molecules." Chemical Physics Letters 116, no. 1 (April 1985): 86–88. http://dx.doi.org/10.1016/0009-2614(85)80131-7.

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44

Graner, G. "About Hot Bands and PAPE Bands in Spectra of C3v Symmetric Top Molecules." Journal of Molecular Spectroscopy 161, no. 1 (September 1993): 58–79. http://dx.doi.org/10.1006/jmsp.1993.1216.

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45

El Hilali, A., Ch Wenger, V. Boudon, and M. Loëte. "C3v Top Data System (C3vTDS) software for spectrum simulation of XY3Z symmetric-top molecules using the group chain." Journal of Quantitative Spectroscopy and Radiative Transfer 111, no. 9 (June 2010): 1305–15. http://dx.doi.org/10.1016/j.jqsrt.2010.01.012.

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46

Luo, Sizuo, Wenhui Hu, Jiaqi Yu, Ruihan Zhu, Lanhai He, Xiaokai Li, Pan Ma, et al. "Rotational Dynamics of Quantum State-Selected Symmetric-Top Molecules in Nonresonant Femtosecond Laser Fields." Journal of Physical Chemistry A 121, no. 4 (January 23, 2017): 777–83. http://dx.doi.org/10.1021/acs.jpca.6b11209.

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47

Turulski, Jan, Jan Niedzielski, and Barbara Pezler. "Transition-state theory treatment of capture collisions between ions and symmetric top dipolar molecules." Journal of the Chemical Society, Faraday Transactions 90, no. 20 (1994): 3061. http://dx.doi.org/10.1039/ft9949003061.

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48

Härtelt, Marko, and Bretislav Friedrich. "Directional states of symmetric-top molecules produced by combined static and radiative electric fields." Journal of Chemical Physics 128, no. 22 (June 14, 2008): 224313. http://dx.doi.org/10.1063/1.2929850.

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49

Ji-xin, Cheng, Wang Xiao-gang, Lin Hai, and Zhu Qing-shi. "Symmetry Reduction and Rotational Re-quantization of Symmetric Top Molecules at Local Mode Limit." Chinese Physics Letters 14, no. 9 (September 1997): 656–59. http://dx.doi.org/10.1088/0256-307x/14/9/005.

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50

Koput, J. "Characteristic patterns in microwave spectra of quasi-symmetric top molecules of the WH3XYZ type." Journal of Molecular Spectroscopy 118, no. 2 (August 1986): 448–58. http://dx.doi.org/10.1016/0022-2852(86)90181-5.

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