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1

Khubaibullin, Ilnur. "Pyridinium Salts As Electron Traps: An Ultrafast Transient Absorption Spectroscopy Study." Bowling Green State University / OhioLINK, 2016. http://rave.ohiolink.edu/etdc/view?acc_num=bgsu1478704646450194.

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2

Alberding, Brian. "Photophysics and Excited State Electronic Communication in Quadruply Bonded Paddlewheel Complexes of Molybdenum and Tungsten." The Ohio State University, 2011. http://rave.ohiolink.edu/etdc/view?acc_num=osu1309959318.

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3

Challa, Jagannadha Reddy. "Electronic and Vibrational Dynamics of Heme Model Compounds-An Ultrafast Spectroscopic Study." Case Western Reserve University School of Graduate Studies / OhioLINK, 2007. http://rave.ohiolink.edu/etdc/view?acc_num=case1181323422.

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4

Pettersson, Rimgard Belinda. "Interligand Electron Transfer Dynamics in Ruthenium Polypyridyl Complexes for Dye Sensitized Solar Cells Determined with Femtosecond Transient IR Absorption Anisotropy." Thesis, Uppsala universitet, Fysikalisk kemi, 2016. http://urn.kb.se/resolve?urn=urn:nbn:se:uu:diva-347571.

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Interligand electron transfer (ILET) may be an essential parameter for the injection ofan electron from the dye into the semiconductor surface of a dye sensitized solar cell(DSSC). Without an efficient injection, competing recombination paths may become apparent. For the future development and design of DSSCs, with the hope of increased energy conversion efficiencies, the ILET dynamics is of great importance. For a long time, the most impressive DSSCs were sensitized with polypyridyl ruthenium dyes for which injection has shown to vary from sub-ps to ns duration. It may therefore be crucial to find
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5

DiScipio, Regina. "Light, Matter, Action: Electronic Relaxation Processes in Biomolecular Photosensitizers and in Photovoltaics." Case Western Reserve University School of Graduate Studies / OhioLINK, 2018. http://rave.ohiolink.edu/etdc/view?acc_num=case1522958286743542.

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6

Zhang, Lei. "Exploring Electron Transfer Dynamics of Novel Dye Sensitized Photocathodes : Towards Solar Cells and Solar Fuels." Doctoral thesis, Uppsala universitet, Fysikalisk kemi, 2016. http://urn.kb.se/resolve?urn=urn:nbn:se:uu:diva-302263.

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The design of dyes for NiO-based dye-sensitized solar cells (DSSCs) has drawn attention owing to their potential applications in photocatalysis and because they are indispensable for the development of tandem dye-sensitized solar cells. The understanding of the electron transfer mechanisms and dynamics is beneficial to guide further dye design and further improve the performance of photocathode in solar cells and solar fuel devices. Time-resolved spectroscopy techniques, especially femtosecond and nanosecond transient absorption spectroscopy, supply sufficient resolution to get insights into t
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7

Petersson, Jonas. "Ultrafast, Non-Equilibrium Electron Transfer Reactions of Molecular Complexes in Solution." Doctoral thesis, Uppsala universitet, Fysikalisk kemi, 2014. http://urn.kb.se/resolve?urn=urn:nbn:se:uu:diva-235461.

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Photoinduced electron transfer is a fundamentally interesting process; it occurs everywhere in the natural world. Studies on electron transfer shed light on questions about the interaction between molecules and how the dynamics of these can be utilized to steer the electron transfer processes to achieve a desired goal. The goal may be to get electrons to the electrode of a solar cell, or to make the electrons form an energy rich fuel such as hydrogen, and it may also be an input or output for molecular switches. The importance of electron transfer reactions will be highlighted in this thesis,
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8

Agathangelou, Damianos. "Anabaena Sensory Rhodopsin : effect of mutations on the ultrafast photo-isomerization dynamics." Thesis, Strasbourg, 2019. http://www.theses.fr/2019STRAE001/document.

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ASR, est une protéine photo réceptrice qui lie la base protonée de la rétine de Schiff dans deux conformations de l'état fondamental. La protéine particulière consiste en un système modèle dans lequel I'effet de l'environnement protéique sur la dynamique d'isomérisation des deux isomères peut être étudié. Dans cette thèse, une étude approfondie sur les protéines mutées ponctuellement est présentée, où la variable est l'environnement protéique. Les résultats montrent des différences significatives entre les durées de vie des états excités des deux isomères et les durées de vie plus courtes ou p
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9

Tannert, Sebastian [Verfasser], Beate [Akademischer Betreuer] Röder, Jörg [Akademischer Betreuer] Enderlein, and Karsten [Akademischer Betreuer] Heyne. "Energy and electron transfer in porphyrin-phthalocyanin-porphyrin heterotrimers : a study by transient absorption spectroscopy, fluorescence upconversion, and time correlated single photon counting / Sebastian Tannert. Gutachter: Beate Röder ; Jörg Enderlein ; Karsten Heyne." Berlin : Humboldt Universität zu Berlin, Mathematisch-Naturwissenschaftliche Fakultät I, 2013. http://d-nb.info/1044973366/34.

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10

Wirth, Adrian. "Attosecond transient absorption spectroscopy." Diss., lmu, 2011. http://nbn-resolving.de/urn:nbn:de:bvb:19-140120.

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11

Hageman, Stephen James. "Complex Attosecond Transient-absorption Spectroscopy." The Ohio State University, 2021. http://rave.ohiolink.edu/etdc/view?acc_num=osu1608050018545904.

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12

Durrant, James Robert. "Transient absorption spectroscopy of photosystem two." Thesis, Imperial College London, 1991. http://hdl.handle.net/10044/1/11455.

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13

Yang, Min-Chieh. "Electronic spectroscopy of transient molecules /." The Ohio State University, 1998. http://rave.ohiolink.edu/etdc/view?acc_num=osu1487949508372826.

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14

Simpson, Emma. "Attosecond transient absorption spectroscopy in atomic species." Thesis, Imperial College London, 2016. http://hdl.handle.net/10044/1/44970.

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When high intensity laser light is focused into a gaseous target, high energy photons can be produced through the strongly nonlinear effect of high order harmonic generation. For a 30 fs, 800 nm or 1400 nm wavelength laser pulse, the result is a train of attosecond pulses produced at odd harmonic frequencies of the driving laser field, spanning energy ranges into the 100s eV. These attosecond pulses can access timescales characteristic to the movement of electrons in atoms, and by exploiting their properties as an ultrafast probe, electron dynamics in evolving atomic systems can be observed. T
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15

Stringer, M. R. "Laser-induced transient absorption spectroscopy of phthalocyanine dyes." Thesis, Open University, 1985. http://ethos.bl.uk/OrderDetails.do?uin=uk.bl.ethos.354989.

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16

Wirth, Adrian [Verfasser], and Ferenc [Akademischer Betreuer] Krausz. "Attosecond transient absorption spectroscopy / Adrian Wirth. Betreuer: Ferenc Krausz." München : Universitätsbibliothek der Ludwig-Maximilians-Universität, 2011. http://d-nb.info/1019930233/34.

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17

Elliott, Nicola Louise. "High resolution electronic spectroscopy of transient species." Thesis, University of Bristol, 2007. http://ethos.bl.uk/OrderDetails.do?uin=uk.bl.ethos.443268.

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18

Elks, John Marcus Francis. "High resolution electronic spectroscopy of transient species." Thesis, University of Bristol, 2001. http://ethos.bl.uk/OrderDetails.do?uin=uk.bl.ethos.390790.

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19

Yang, Lei. "Hole Transport Materials for Solid-State Mesoscopic Solar Cells." Doctoral thesis, Uppsala universitet, Fysikalisk kemi, 2014. http://urn.kb.se/resolve?urn=urn:nbn:se:uu:diva-232271.

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The solid-state mesoscopic solar cells (sMSCs) have been developed as a promising alternative technology to the conventional photovoltaics. However, the device performance suffers from the low hole-mobilities and the incomplete pore filling of the hole transport materials (HTMs) into the mesoporous electrodes. A variety of HTMs and different preparation methods have been studied to overcome these limitations. There are two types of sMSCs included in this doctoral thesis, namely solid-state dye-sensitized solar cells (sDSCs) and organometallic halide perovskite based solar cells. Two different
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20

Bosman, Gurthwin Wendell. "Transient absorption spectroscopy of metal complexes : dithizonatophenylmercury(II) and derivatives." Thesis, Stellenbosch : Stellenbosch University, 2012. http://hdl.handle.net/10019.1/71913.

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Thesis (PhD)--Stellenbosch University, 2012.<br>ENGLISH ABSTRACT: The availability of laser systems capable of generating ultrashort optical pulses in the visible spectral range have made it possible to study molecular species with a temporal resolution in the order of intra-molecular dynamics which previously were not accessible. Henceforth, in this study a popular pump-probe technique called ultrafast transient absorption spectroscopy (UTAS) is employed to study the initial photochromic reaction of metal complex, dithizonatophenylmercury (II) (DPM) under various conditions. These condit
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21

Polshakov, Dmitrii A. "Ultrafast spectroscopy and dynamics of nitrenes and carbenes." The Ohio State University, 2005. http://rave.ohiolink.edu/etdc/view?acc_num=osu1130968887.

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22

Pearson, Jonathan. "Electronic spectroscopy of the transient species HNO and SnF." Thesis, University of Bristol, 1996. http://ethos.bl.uk/OrderDetails.do?uin=uk.bl.ethos.319048.

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23

Menting, Raoul. "Light-induced energy and charge transfer processes in artificial photosynthetic systems." Doctoral thesis, Humboldt-Universität zu Berlin, Mathematisch-Naturwissenschaftliche Fakultät I, 2013. http://dx.doi.org/10.18452/16656.

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Der Gegenstand der vorliegenden Arbeit ist die Untersuchung von photoinduzierten Energietransferprozessen (EET) und Elektronentransferprozessen (ET) in Modellsystemen, die als potentiell geeignet für eine Nutzung in der artifiziellen Photosynthese angesehen werden. Den beiden wesentlichen Zugängen zur Architektur artifizieller Photosynthese-Systeme entsprechend wurden vergleichend kovalente und sich selbst organisierende Systeme untersucht. In beiden Zugängen wurden ähnliche chemische Komponenten als optisch aktive Moleküle eingesetzt, insbesondere Phthalocyanine mit einem Silizium-Zentralatom
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24

Torche, Fayçal. "Contribution à l'étude des électrons solvatés dans l’eau et les alcools et des processus radiolytiques dans les carbonates organiques par radiolyse impulsionnelle picoseconde." Thesis, Paris 11, 2012. http://www.theses.fr/2012PA112132/document.

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Le travail présenté dans cette thèse, s’inscrit dans le domaine d'étude de l'interaction des rayonnements ionisants avec les liquides polaires. Bénéficiant de l’accélérateur d'électrons picoseconde ELYSE, les études ont été menées en utilisant les techniques de la radiolyse impulsionnelle associées à la spectrophotométrie d’absorption résolue en temps dans le domaine de la picoseconde. Ce travail est réparti sur deux chapitres distincts. Le premier aborde l’étude la variation temporelle du rendement radiolytique de l’électron solvaté dans l'eau et les alcools simples. Grâce au système de détec
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25

Chan, Mau Hing. "Photothermal deflection spectroscopy of novel electronic materials." HKBU Institutional Repository, 1996. http://repository.hkbu.edu.hk/etd_ra/66.

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26

Asakura, Hiroyuki. "Study of X-ray Absorption Spectroscopy of Heavy Elements and Transient Chemical Species." 京都大学 (Kyoto University), 2015. http://hdl.handle.net/2433/198946.

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27

Hassan, Karim H. "Absorption and laser induced fluorescence spectra of some aromatic molecules." Thesis, University of Reading, 1990. http://ethos.bl.uk/OrderDetails.do?uin=uk.bl.ethos.278083.

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28

Colley, Christopher S. "Time-resolved infrared spectroscopy of organic and biological transient species." Thesis, Nottingham Trent University, 2001. http://ethos.bl.uk/OrderDetails.do?uin=uk.bl.ethos.367318.

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29

Newman, Stuart Michael. "Electronic spectroscopy of molecules of atmospheric interest using sensitive absorption techniques." Thesis, University of Bristol, 2000. http://ethos.bl.uk/OrderDetails.do?uin=uk.bl.ethos.322613.

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30

Megerle, Uwe. "Photoinduced molecular dynamics in increasingly complex systems: From ultrafast transient absorption spectroscopy to nanoscopic models." Diss., lmu, 2011. http://nbn-resolving.de/urn:nbn:de:bvb:19-130444.

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31

Briand, Julien. "Ultrafast isomerization and vibrational coherence of biomimetic photoswitches : experimental investigation by femtosecond transient absorption spectroscopy." Strasbourg, 2009. http://www.theses.fr/2009STRA6261.

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Ce travail concerne une nouvelle famille de photo-commutateurs basés sur la structure alkylée d’Indanylidene-Pyrroline (NAIP), supposée reproduire, selon les résultats d’études théoriques, l’isomérisation du rétinal dans la rhodopsine. Ce travail de doctorat rapporte l’étude expérimentale de l’isomérisation ultra-rapide cette famille de molécules. Tout d’abord, ce travail a nécessité la réalisation d’un montage expérimental de spectroscopie d’absorption résolue en temps qui, grâce à une résolution temporelle suffisante et une large couverture spectrale, permet de suivre l’évolution temporelle
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32

Osawa, Koji. "Reaction Dynamics in Designer Fluids Studied by Ultrafast Transient Absorption Spectroscopy: Supercritical Water and Ionic Liquids." 京都大学 (Kyoto University), 2013. http://hdl.handle.net/2433/175134.

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33

Husek, Jakub. "Elucidating Surface Charge Carrier Dynamics of Functional Materials By Femtosecond Transient Extreme Ultraviolet Reflection-Absorption Spectroscopy." The Ohio State University, 2019. http://rave.ohiolink.edu/etdc/view?acc_num=osu1553099994360381.

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34

Liao, Chen-Ting, and Arvinder Sandhu. "XUV Transient Absorption Spectroscopy: Probing Laser-Perturbed Dipole Polarization in Single Atom, Macroscopic, and Molecular Regimes." MDPI AG, 2017. http://hdl.handle.net/10150/624358.

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We employ an extreme ultraviolet (XUV) pulse to impulsively excite dipole polarization in atoms or molecules, which corresponds to coherently prepared superposition of excited states. A delayed near infrared (NIR) pulse then perturbs the fast evolving polarization, and the resultant absorbance change is monitored in dilute helium, dense helium, and sulfur hexafluoride (SF6) molecules. We observe and quantify the time-dependence of various transient phenomena in helium atoms, including laser-induced phase (LIP), time-varying (AC) Stark shift, quantum path interference, and laser-induced continu
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35

Ekvall, Karin. "Time resolved laser spectroscopy." Doctoral thesis, KTH, Physics, 2000. http://urn.kb.se/resolve?urn=urn:nbn:se:kth:diva-3063.

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36

Bîrzǎ, Petre A. "Development of a cw-cavity ring down spectrometer and electronic spectroscopy of transient species /." Basel : [s.n.], 2004. http://edoc.unibas.ch/diss/DissB_6934.

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37

Krebs, Nils [Verfasser], and Eberhard [Akademischer Betreuer] Riedle. "New insights for femtosecond spectroscopy : from transient absorption to 2-dimensional spectroscopy in the UV spectral domain / Nils Krebs. Betreuer: Eberhard Riedle." München : Universitätsbibliothek der Ludwig-Maximilians-Universität, 2013. http://d-nb.info/1045152978/34.

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38

Harris, Stephanie. "Investigating photo-induced bond breaking and making in solution phase aromatic molecules via ultrafast transient absorption spectroscopy." Thesis, University of Bristol, 2015. http://ethos.bl.uk/OrderDetails.do?uin=uk.bl.ethos.682337.

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This thesis details ultrafast absorption spectroscopy studies of photo-induced processes in solution phase aromatic molecules. Application of this technique to the systems detailed below, using both a broadband infrared (IR) and/or ultraviolet (UV)/visible probe, has allowed the key species created directly by photo-excitation and subsequent processes to be identified as well as their transient behaviour to be followed. Kinetic and mechanistic information on the process or reaction is obtained, adding to both the understanding of the underlying photo-physics that drive the process in addition
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39

Barnard, David Thomas. "EXCITED STATE DYNAMICS AND CHARGE REDISTRIBUTION OF EXTREMOPHILE DNA PHOTOLYASE AND FLAVIN COFACTORS." Diss., Temple University Libraries, 2018. http://cdm16002.contentdm.oclc.org/cdm/ref/collection/p245801coll10/id/597264.

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Chemistry<br>Ph.D.<br>Repair mechanisms for damaged DNA are essential for the proliferation of nearly all forms of life. Although DNA is quite robust, the vital information-storing molecule can often be damaged from environmental exposures such as ultra-violet (UV) light. Exposure to UV light can result in various types of mutagens creating structural damages. One specific type of UV-induced damage is the creation of a cyclobutylpyrimidine dimer (CPD). This specific type of lesion can be efficiently repaired by the flavoenzyme DNA photolyase (PL). DNA photolyase is an ancient protein found acr
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40

Bell, Steven Ernest John. "Transient electronic and resonance Raman spectroscopy of some photoexcited transition metal and metal-carbene complexes." Thesis, Queen's University Belfast, 1986. http://ethos.bl.uk/OrderDetails.do?uin=uk.bl.ethos.317048.

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41

Lin, Na. "Theoretical Studies on Electronic and Vibrationally Resolved Multi-Photon Absorption and Dichroism." Doctoral thesis, Stockholm : Skolan för bioteknologi, Kungliga Tekniska högskolan, 2009. http://urn.kb.se/resolve?urn=urn:nbn:se:kth:diva-10212.

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42

Pauszek, Raymond Francis. "Excited state charge redistribution and dynamics of flavins, flavorproteins, and their cofactors." Diss., Temple University Libraries, 2013. http://cdm16002.contentdm.oclc.org/cdm/ref/collection/p245801coll10/id/245456.

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Chemistry<br>Ph.D.<br>The excited state electronic structures of several biologically important chromophores were studied by Stark spectroscopy. The extent of charge redistribution upon excitation to the lowest excited states of the oxidized and semiquinone forms of flavin adenine dinucleotide (FAD) bound to the light activated DNA repair enzyme DNA photolyase have been studied previously by this technique. This work focuses on the catalytically active form, the two-electron reduced anion. To facilitate analysis of this experiment, the Stark spectra of a simple flavin derivative that is solubl
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43

Hare, Patrick Michael. "Excuted state dynamics in DNA base monomers: the effects of solvent and chemical modification in ultrafast internal conversion." The Ohio State University, 2007. http://rave.ohiolink.edu/etdc/view?acc_num=osu1166623261.

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44

Kanal, Florian [Verfasser], Tobias [Gutachter] Brixner, and Patrick [Gutachter] Nürnberger. "Femtosecond Transient Absorption Spectroscopy – Technical Improvements and Applications to Ultrafast Molecular Phenomena / Florian Kanal. Gutachter: Tobias Brixner ; Patrick Nürnberger." Würzburg : Universität Würzburg, 2015. http://d-nb.info/1111125368/34.

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45

Pawlowska, Zuzanna. "The photophysics of pyridinium betaines studied by ultrafast transient absorption spectroscopy : focus on the photoinduced intramolecular charge transfer process." Thesis, Lille 1, 2011. http://www.theses.fr/2011LIL10029/document.

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Ce travail concerne la photophysique en solution de la Pyridinium betaine, 2-Pyridin-1-yl-1H-benzimidazole (SBPa), et de deux dérivés substitués par des groupes mono- ou bi-thiophéniques. Il repose sur un ensemble de mesures par spectroscopies stationnaires et par absorption résolue en temps, complétées par des calculs PCM-(TD)DFT. Les données d’absorption/émission et de TDDFT révèlent pour SBPa une transition de transfert de charge intramoléculaire S0→S2(CT) intense et fortement solvatochromique, accompagnée d’une considérable variation de moment dipolaire, et une transition d’émission S1→S0
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46

Lewis, Kristin A. "Development of a dual-wavelength photoacoustic instrument for measurement of light absorption and scattering by aerosol and gases." abstract and full text PDF (free order & download UNR users only), 2007. http://0-gateway.proquest.com.innopac.library.unr.edu/openurl?url_ver=Z39.88-2004&rft_val_fmt=info:ofi/fmt:kev:mtx:dissertation&res_dat=xri:pqdiss&rft_dat=xri:pqdiss:3258842.

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47

Singh, Asmita. "Illuminating the ultrafast excited state dynamics of protein-bound carotenoids in plants." Diss., University of Pretoria, 2017. http://hdl.handle.net/2263/63170.

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Global energy demands have escalated over the past few decades, creating a necessity for alternative energy sources. Solar technologies inspired by the primary solar energy storing process known on earth, photosynthesis, have subsequently gained popularity. The natural photosynthetic apparatus comprises a network of membrane-bound pigment-protein complexes, with the main plant light-harvesting complex (LHCII) consisting of chlorophyll (Chl) and carotenoid (Car) pigments. Electronic excitation energy transfer (ET) of the harvested energy takes place amongst these pigments on ultrafast timescale
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48

Blancon, Jean-Christophe. "Optical absorption and electronic properties of individual carbon nanotubes." Thesis, Lyon 1, 2013. http://www.theses.fr/2013LYO10164/document.

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Au cours de ce travail de thèse à caractère expérimental, nous nous sommes attachés à mesurer les spectres absolus de section efficace d’absorption de nanotubes de carbone individuels placés dans différents environnements. Pour ce faire, nous avons développé un dispositif expérimental basé sur la technique de spectroscopie à modulation spatiale qui permet d’accéder de manière directe à la section efficace d’absorption de nano-objets individuels. Cette méthode ne requière aucun a priori sur les propriétés des nanotubes, et très important nous affranchit des effets d’ensemble. Ainsi, nous avons
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49

Robertson, John Michael. "Nonlinear optical properties of absorbing molecular systems." Thesis, University of Essex, 2002. http://ethos.bl.uk/OrderDetails.do?uin=uk.bl.ethos.390961.

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50

Dickson, Nicole M. "Solute/Solvent Interactions And Excited State Photophysics Of 1,4-Diphenyl-1,3-Butadiene And 1,4-Diphenyl-1,3-Cyclopentadiene." The Ohio State University, 2008. http://rave.ohiolink.edu/etdc/view?acc_num=osu1206119352.

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